Photon Statistics of Filtered Resonance Fluorescence
Catherine L. Phillips, Alistair J. Brash, Dara P. S. McCutcheon, Jake Iles-Smith, Edmund Clarke, Benjamin Royall, Maurice S. Skolnick, A. Mark Fox, Ahsan Nazir
备注：
Main manuscript 7 pages with 4 figures, supplementary material of 4 pages
Spectral filtering of resonance fluorescence is widely employed to improve single photon purity and indistinguishability by removing unwanted backgrounds. For filter bandwidths approaching the emitter linewidth, complex behaviour is predicted due to preferential transmission of components with differing photon statistics. We probe this regime using a Purcell-enhanced quantum dot in both weak and strong excitation limits, finding excellent agreement with an extended sensor theory model. By changing only the filter width, the photon statistics can be transformed between antibunched, bunched, or Poissonian. Our results verify that strong antibunching and a sub-natural linewidth cannot simultaneously be observed, providing new insight into the nature of coherent scattering.
The broadband parametric fluorescence pulse (probe light) with center frequency resonant on 87Rb D1 line was injected into a cold atomic ensemble with coherent light (control light). Due to the low gain in the parametric down conversion process, the probe light was in a highly bunched photon-pair state. By switching off the control light, the probe light within the electromagnetically induced transparency window was mapped on the atoms. When the control light was switched on, the probe light was retrieved and frequency filtered storage was confirmed from the superbunching effect and an increas…
Signatures of inter-sideband coherence in the resonance fluorescence spectrum of an acoustically-modulated quantum dot
Institute of Theoretical Physics, Wrocław University of Science and Technology（弗罗茨瓦夫科技大学理论物理研究所）；Institute of Physics, University of Münster（明斯特大学物理研究所）
Multi-photon emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multi-level atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has remained a challenge due to the small oscillator strengths involved. Here we present a study of two-photon resonance fluorescence at microwave frequencies, using a superconducting, ladder-type artificial atom, a transmon, strongly coupled to a waveguide. We drive the two-photon transition between the ground and second-excited state at increasingly high powers a…
A simple calculation method for photon statistics of frequency-filtered fields is proposed. This method, based on eigenvalue decompositions of superoperators, allows us to study effects on the photon statistics of spectral filtering by various types of filters, such as Gaussian and rectangular filters as well as Lorentzian filters, which is not possible by conventional approaches. As an example, this method is applied to a simulation of quantum dot single-photon emitters, where we found the efficient choice of the filter types to have pure single photons depends on the excitation conditions i.…
We investigate the continuous quantum measurement of a superconducting qubit undergoing fluorescence. The fluorescence of the qubit is detected via a phase-preserving heterodyne measurement, giving the fluorescence quadrature signals as two continuous qubit readout results. By using the stochastic path integral approach to the measurement physics, we derive most likely paths between boundary conditions on the state, and compute approximate time correlation functions between all stochastic variables via diagrammatic perturbation theory. We focus on paths that increase in energy during the conti…
We report high time-resolution measurements of photon statistics from pairs of dye molecules coupled by fluorescence resonance energy transfer (FRET). In addition to quantum-optical photon antibunching, we observe photon bunching on a timescale of several nanoseconds. We show by numerical simulation that configuration fluctuations in the coupled fluorophore system could account for minor deviations of our data from predictions of basic Forster theory. With further characterization we believe that FRET photon statistics could provide a unique tool for studying DNA mechanics on timescales from 1…
This proposal investigates the photon-statistics of light emitted by a statistical ensemble of cold atoms excited by the near-field of an optical nanofiber tip. Dipole-dipole interactions of atoms at such short distance from each other suppress the simultaneous emission of more than one photon and lead to antibunching of photons. We consider a mean atom number on the order of one and deal with a poissonian mixture of one and two atoms including dipole-dipole interactions and collective decay. Time tracks of the atomic states are simulated in quantum Monte Carlo simulations from which the $g^{(…
We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of $(20.7\pm0.8)~\%$ per linear polarization basis. This yields an overall extraction efficiency of $(41.4\pm1.5)~\%$ in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical…
A qubit can relax by fluorescence, which prompts the release of a photon into its electromagnetic environment. By counting the emitted photons, discrete quantum jumps of the qubit state can be observed. The succession of states occupied by the qubit in a single experiment, its quantum trajectory, depends in fact on the kind of detector. How are the quantum trajectories modified if one measures continuously the amplitude of the fluorescence field instead? Using a superconducting parametric amplifier, we have performed heterodyne detection of the fluorescence of a superconducting qubit. For each…
We discuss the statistics of emission of photons by a single atom or ion illuminated by a laser beam at the frequency of quasi-resonance between two energy levels, a situation that corresponds to real experiments. We extend this to the case of two laser beams resonant with the energy differences between two excited levels and the ground state (three level atom in V-configuration). We use a novel approach of this type of problem by considering Kolmogorov equation for the probability distribution of the atomic state which takes into account first the deterministic evolution of this state under t…
We show how to calculate the first- and second-order statistics of the scattered fields for an arbitrary intensity coherent state light field interacting with a two-level system in a waveguide geometry. Specifically, we calculate the resonance fluorescence from the qubit, using input-output formalism. We derive the transmission and reflection coefficients, and illustrate the bunching and anti-bunching of light that is scattered in the forward and backward directions, respectively. Our results agree with previous calculations on one- and two-photon scattering as well as those that are based on …
Mandel Q-parameter, which is determined from single event photon statistics, provides an alternative to differentiate single-molecule with fluorescence detection. In this work, by using the Q-parameter of the sample fluorescence compared to that of an ideal double-molecule system with the same average photon number, we present a novel and fast approach for identifying single molecules based on single event photon statistics analyses, compared with commonly used two-time correlation measurements. The error estimates for critical values of photon statistics are also presented for single-molecule…
Photon correlations are investigated for a single laser-excited ion trapped in front of a mirror. Varying the relative distance between the ion and the mirror, photon correlation statistics can be tuned smoothly from an antibunching minimum to a bunching-like maximum. Our analysis concerns the non-Markovian regime of the ion-mirror interaction and reveals the field establishment in a half-cavity interferometer.
Number state filtering in coherent states leads to sub-Poissonian photon statistics. These states are more suitable for phase estimation when compared with the coherent states. Nonclassicality of these states is quantified in terms of the negativity of the Wigner function and the entanglement potential. Filtering of the vacuum from a coherent state is almost like the photon-addition. However, filtering makes the state more resilient against dissipation than photon-addition. Vacuum state filtered coherent states perform better than the photon-added coherent states for a two-way quantum key dist…
Photon correlations in the emission of a resonantly driven quantum dot are investigated, accounting for the influence of the solid-state phonon environment. An analytical expression is derived for the second-order fluorescence intensity correlation function, from which regimes of correlated and uncorrelated photon emission are predicted as the driving field is varied. Experiments to investigate this effect would provide valuable insight into quantum dot carrier-phonon dynamics and are feasible with current technology.
We demonstrate a robust fiber-optics-based fluorescence detector, fully integrated on an atom chip, which detects single atoms propagating in a guide with 66% efficiency. We characterize the detector performance and the atom flux by analyzing the photon statistics. Near-perfect photon antibunching proves that single atoms are detected, and allows us to study the second-order intensity correlation function of the fluorescence over three orders of magnitude in atomic density.
In quantum physics, measurement results are random but their statistics can be predicted assuming some knowledge about the system in the past. Additional knowledge from a future measurement deeply changes the statistics in the present and leads to purely quantum features. In particular conditioned average outcomes of a weak measurement, so-called weak values, were shown to go beyond the conventional range, give a way to directly measure complex quantities, and can be used to enhance the sensitivity of quantum meters. Recently, these concepts have been considered in the general case of open qua…
We studied intensity fluctuations of a single photon source relying on the pulsed excitation of the fluorescence of a single molecule at room temperature. We directly measured the Mandel parameter Q(T) over 4 orders of magnitude of observation timescale T, by recording every photocount. On timescale of a few excitation periods, subpoissonian statistics is clearly observed and the probablility of two-photons events is 10 times smaller than Poissonian pulses. On longer times, blinking in the fluorescence, due to the molecular triplet state, produces an excess of noise.
Crossovers between Time-Bin and Energy-Time Entanglement in Homodyned Resonance Fluorescence
Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）；Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；University of Chinese Academy of Sciences（中国科学院大学）
Motivated by recent experiments on photon statistics from individual dye pairs planted on biomolecules and coupled by fluorescence resonance energy transfer (FRET), we show here that the FRET dynamics can be modelled by Gaussian random processes with colored noise. Using Monte-Carlo numerical simulations, the photon intensity correlations from the FRET pairs are calculated, and are turned out to be very close to those observed in experiment. The proposed stochastic description of FRET is consistent with existing theories for microscopic dynamics of the biomolecule that carries the FRET coupled…
Cross-correlation signals are recorded from fluorescence photons scattered in free space off a trapped ion structure. The analysis of the signal allows for unambiguously revealing the spatial frequency, thus the distance, as well as the spatial alignment of the ions. For the case of two ions we obtain from the cross-correlations a spatial frequency $f_\text{spatial}=1490 \pm 2_{stat.}\pm 8_{syst.}\,\text{rad}^{-1}$, where the statistical uncertainty improves with the integrated number of correlation events as $N^{-0.51\pm0.06}$. We independently determine the spatial frequency to be $1494\pm 1…
Emission from a resonantly excited quantum emitter is a fascinating research topic within quantum optics and a useful source for different types of quantum light fields. The resonance spectrum consists of a single spectral line below saturation of a quantum emitter which develops into a triplet at powers above saturation of the emitter. The spectral properties of the triplet strongly depends on pump power and detuning of the excitation laser. The three closely spaced photon channels from the resonance fluorescence have different photon statistical signatures. We present a detailed photon-stati…
Resonance fluorescence arises from the interaction of an optical field with a two-level system and has played a fundamental role in the development of quantum optics and its applications. Despite its conceptual simplicity it entails a wide range of intriguing phenomena, such as the Mollow-triplet emission spectrum and coherent photon emission. One fundamental aspect of resonance fluorescence, reduced quantum fluctuations in the single photon stream from an atom in free space, was predicted more than 30 years ago. However, the requirement to operate in the weak excitation regime, together with …
We theoretically study the occurrence of quantum jumps in the resonance fluorescence of a trapped atom. Here, the atom is laser cooled in a configuration of level such that the occurrence of a quantum jump is associated to a change of the vibrational center-of-mass motion by one phonon. The statistics of the occurrence of the dark fluorescence period is studied as a function of the physical parameters and the corresponding features in the spectrum of resonance fluorescence are identified. We discuss the information which can be extracted on the atomic motion from the observation of a quantum j…
Resonance fluorescence---the light emitted when exciting resonantly a two-level system---is a popular quantum source as it seems to inherit its spectral properties from the driving laser and its statistical properties from the two-level system, thus providing a subnatural-linewidth single-photon source. However, these two qualities do not actually coexist in resonance fluorescence, since an optical target detecting these antibunched photons will either be spectrally broad itself and not benefit from the spectrally narrow source, or match spectrally with the source but in this case the antibunc…
It is shown that spectrally resolved photon-statistics measurements of the resonance fluorescence from realistic semiconductor quantum-dot systems allow for high contrast identification of the two-photon strong-coupling states. Using a microscopic theory, the second-rung resonance is analyzed and optimum excitation conditions are determined. The computed photon-statistics spectrum displays gigantic, experimentally robust resonances at the energetic positions of the second-rung emission.
We experimentally demonstrate quantum enhanced resolution in confocal fluorescence microscopy exploiting the non-classical photon statistics of single nitrogen-vacancy colour centres in diamond. By developing a general model of super-resolution based on the direct sampling of the kth-order autocorrelation function of the photoluminescence signal, we show the possibility, in some cases, to resolve in principle arbitrarily close emitting centers.
We calculate the one- and two-photon scattering matrices of a pair of collocated non-identical two-level atoms coupled to a waveguide. We show that by proper choice of a two-photon input, the background fluorescence by the atoms may be completely quenched, as a result of quantum interference, and that when the atoms' detuning is smaller than their linewidths, extremely narrow fluorescence features emerge. Furthermore, the system emits a two-photon bound state which can display spatial oscillations/quantum beats, and can be tuned from bunched to anti-bunched statistics as the total photon energ…
n a recent experiment, we reported the time-domain intensity noise measurement of a single photon source relying on single molecule fluorescence control. In this article we present data processing, starting from photocount timestamps. The theoretical analytical expression of the time-dependent Mandel parameter Q(T) of an intermittent single photon source is derived from ON<->OFF dynamics . Finally, source intensity noise analysis using the Mandel parameter is quantitatively compared to the usual approach relying on the time autocorrelation function, both methods yielding the same molecular dyn…
