Cross-correlation signals are recorded from fluorescence photons scattered in free space off a trapped ion structure. The analysis of the signal allows for unambiguously revealing the spatial frequency, thus the distance, as well as the spatial alignment of the ions. For the case of two ions we obtain from the cross-correlations a spatial frequency $f_\text{spatial}=1490 \pm 2_{stat.}\pm 8_{syst.}\,\text{rad}^{-1}$, where the statistical uncertainty improves with the integrated number of correlation events as $N^{-0.51\pm0.06}$. We independently determine the spatial frequency to be $1494\pm 11\,\text{rad}^{-1}$, proving excellent agreement. Expanding our method to the case of three ions, we demonstrate its functionality for two-dimensional arrays of emitters of indistinguishable photons, serving as a model system to yield structural information where direct imaging techniques fail.
Resonance fluorescence of a single trapped ion is spectrally analyzed using a heterodyne technique. Motional sidebands due to the oscillation of the ion in the harmonic trap potential are observed in the fluorescence spectrum. From the width of the sidebands the cooling rate is obtained and found to be in agreement with the theoretical prediction.
Efficient collection of fluorescence from trapped ions is crucial for quantum optics and quantum computing applications, specifically, for qubit state detection and in generating single photons for ion-photon and remote ion entanglement. In a typical setup, only a few per cent of ion fluorescence is intercepted by the aperture of the imaging optics. We employ a simple metallic spherical mirror integrated with a linear Paul ion trap to achieve photon collection efficiency of at least 10% from a single Ba$^+$ ion. An aspheric corrector is used to reduce the aberrations caused by the mirror and a…
We experimentally investigate the resonance fluorescence spectrum of single 171Yb and 172Yb ions which are laser cooled to the Lamb-Dicke regime in a radiofrequency trap. While the fluorescence scattering of 172Yb is continuous, the 171Yb fluorescence is interrupted by quantum jumps because a nonvanishing rate of spontaneous transitions leads to electron shelving in the metastable hyperfine sublevel 2D3/2(F=2). The average duration of the resulting dark periods can be varied by changing the intensity of a repumping laser field. Optical heterodyne detection is employed to analyze the fluorescen…
We investigate theoretically the spectrum of resonance fluorescence of a harmonically trapped atom, whose internal transitions are $Λ$--shaped and driven at two-photon resonance by a pair of lasers, which cool the center--of--mass motion. For this configuration, photons are scattered only due to the mechanical effects of the quantum interaction between light and atom. We study the spectrum of emission in the final stage of laser--cooling, when the atomic center-of-mass dynamics is quantum mechanical and the size of the wave packet is much smaller than the laser wavelength (Lamb--Dicke limit). …
We theoretically study the occurrence of quantum jumps in the resonance fluorescence of a trapped atom. Here, the atom is laser cooled in a configuration of level such that the occurrence of a quantum jump is associated to a change of the vibrational center-of-mass motion by one phonon. The statistics of the occurrence of the dark fluorescence period is studied as a function of the physical parameters and the corresponding features in the spectrum of resonance fluorescence are identified. We discuss the information which can be extracted on the atomic motion from the observation of a quantum j…
Integration of fiber optics may play a critical role in the development of quantum information processors based on trapped ions and atoms by enabling scalable collection and delivery of light and coupling trapped ions to optical microcavities. We trap 24Mg+ ions in a surface-electrode Paul trap that includes an integrated optical fiber for detecting 280-nm fluorescence photons. The collection numerical aperture is 0.37 and total collection efficiency is 2.1 %. The ion can be positioned between 80 \mum and 100 \mum from the tip of the fiber by use of an adjustable rf-pseudopotential.
We investigate the temporal dynamics of Doppler cooling of an initially hot single trapped atom in the weak binding regime using a semiclassical approach. We develop an analytical model for the simplest case of a single vibrational mode for a harmonic trap, and show how this model allows us to estimate the initial energy of the trapped particle by observing the fluorescence rate during the cooling process. The experimental implementation of this temperature measurement provides a way to measure atom heating rates by observing the temperature rise in the absence of cooling. This method is techn…
This review presents the Laser-Induced Fluorescence Spectroscopy (LIFS) of trapped gas-phase molecular ions. A brief description of the theory and experimental approaches involved in fluorescence spectroscopy, together with state-of-the-art LIFS experiments employing ion traps, is presented. Quadrupole ion traps are commonly used for spatial confinement of ions. One of the main challenges involved in such experiments is poor Signal-to-Noise Ratio (SNR) arising due to weak gas-phase fluorescence emission, high background noise, and small solid angle for the fluorescence collection optics. The e…
Isolation of a single atomic particle and monitoring its resonance fluorescence is a powerful tool for studies of quantum effects in radiation-matter interaction. Here we present observations of quantum dynamics of an isolated neutral atom stored in a magneto-optical trap. By means of photon correlations in the atom's resonance fluorescence we demonstrate the well-known phenomenon of photon antibunching which corresponds to transient Rabi oscillations in the atom. Through polarization-sensitive photon correlations we show a novel example of resolved quantum fluctuations: spontaneous magnetic o…
Trapped, laser-cooled ions produce intense fluorescence. Detecting this fluorescence enables efficient measurement of quantum state of qubits based on trapped atoms. It is desirable to collect a large fraction of the photons to make the detection faster and more reliable. Additionally, efficient fluorescence collection can improve speed and fidelity of remote ion entanglement and quantum gates. Here we show a novel ion trap design that incorporates metallic spherical mirror as the integral part of the trap itself, being its RF electrode. The mirror geometry enables up to 35% solid angle collec…
We study the formation and destabilization of dark states in a single trapped 88Sr+ ion caused by the cooling and repumping laser fields required for Doppler cooling and fluorescence detection of the ion. By numerically solving the time-dependent density matrix equations for the eight-level system consisting of the sublevels of the 5s 2S1/2, 5p 2P1/2, and 4d 2D3/2 states, we analyze the different types of dark states and how to prevent them in order to maximize the scattering rate, which is crucial for both the cooling and the detection of the ion. The influence of the laser linewidths and ion…
We report on the first demonstration of fluorescence detection using single-photon avalanche photodiodes (SPADs) monolithically integrated with a microfabricated surface ion trap. The SPADs are positioned below the trapping positions of the ions, and designed to detect 370 nm photons emitted from single $^{174}$Yb$^+$ and $^{171}$Yb$^+$ ions. We achieve an ion/no-ion detection fidelity for $^{174}$Yb$^+$ of 0.99 with an average detection window of 7.7(1) ms. We report a dark count rate as low as 1.2 kHz at room temperature operation. The fidelity is limited by laser scatter, dark counts, and h…
In this paper we present a method to measure transient fluorescent dynamics with single trapped ions in a Paul trap. We use $^{40}$Ca$^+$ ions which exhibit a $Λ$-type three-level system and measure the characteristic optical pumping times between the ground $S_{1/2}$ and the meta-stable $D_{3/2}$ levels. We prepare one of these states, then pump it to the opposite via the excited $P_{1/2}$ state. By measuring the scattered photons of the ion, we retrieve transient curves of the atomic fluorescence. These curves provide fundamental information about the atomic system, such as branching fractio…
We demonstrate simple and robust methods for Doppler cooling and obtaining high fluorescence from trapped 43Ca+ ions at a magnetic field of 146 Gauss. This field gives access to a magnetic-field-independent "atomic clock" qubit transition within the ground level hyperfine structure of the ion, but also causes the complex internal structure of the 64 states relevant to Doppler cooling to be spread over many times the atomic transition line-width. Using a time-dependent optical Bloch equation simulation of the system we develop a simple scheme to Doppler-cool the ion on a two-photon dark resonan…
Photon correlations are investigated for a single laser-excited ion trapped in front of a mirror. Varying the relative distance between the ion and the mirror, photon correlation statistics can be tuned smoothly from an antibunching minimum to a bunching-like maximum. Our analysis concerns the non-Markovian regime of the ion-mirror interaction and reveals the field establishment in a half-cavity interferometer.
We investigate a single laser driven atom trapped in a non-harmonic potential. We present the performance of ground-state laser cooling and Doppler cooling and the signatures of the center-of-mass motion in the power spectrum of the scattered light. In order to illustrate the results we provide two explicit examples for the confining potential: the infinite square well and the Morse potential.
Based on the multi-level model, we have calculated light shifts for Zeeman states of hyperfine levels of cesium (Cs) 6S1/2 ground state and 6P3/2 excited state.The magic-wavelength linearly-polarized optical dipole trap (ODT) for Cs 6S1/2 F=4, mF=+4 - 6P3/2 F'=5, mF=+5 transition is experimentally constructed and characterized by using the laser-induced fluorescence spectra of trapped single Cs atoms. The magic wavelength is 937.7 nm which produces almost the same light shift for 6S1/2 F=4, mF=+4 ground state and 6P3/2 F'=5, mF=+5 excited state with linearly-polarized ODT laser beam. Compared …
We report measurements of an intensity-field correlation function of the resonance fluorescence of a single trapped Ba+ ion. Detection of a photon prepares the atom in its ground state and we observe its subsequent evolution under interaction with a laser field of well defined phase. We record the regression of the resonance fluorescence source field. This provides a direct measurement of the field of the radiating dipole of a single atom and exhibits its strong non-classical behavior. In the experimental setup an interference measurement is conditioned on a fluorescence photon detection. The …
We observe quantum interference of photons emitted by two continuously laser-excited single ions, independently trapped in distinct vacuum vessels. High contrast two-photon interference is observed in two experiments with different ion species, calcium and barium. Our experimental findings are quantitatively reproduced by Bloch equation calculations. In particular, we show that the coherence of the individual resonance fluorescence light field is determined from the observed interference.
We propose a method for scaling trapped ions for large-scale quantum computation and communication based on a probabilistic ion-photon mapping. Deterministic quantum gates between remotely located trapped ions can be achieved through detection of spontaneously-emitted photons, accompanied by the local Coulomb interaction between neighboring ions. We discuss gate speeds and tolerance to experimental noise for different probabilistic entanglement schemes.
Resonance fluorescence of laser-driven highly charged ions is studied in the relativistic regime by solving the time-dependent master equation in a multi-level model. Our ab initio approach based on the Dirac equation allows for investigating highly relativistic ions, and, consequently, provides a sensitive means to test correlated relativistic dynamics, bound-state quantum electrodynamic phenomena and nuclear effects by applying coherent light with x-ray frequencies. Atomic dipole or multipole moments may be determined to unprecedented accuracy by measuring the interference-narrowed fluoresce…
We describe the optimal realization of entangling quantum gates for trapped ions mediated by a dissipative bus mode. With suitably shaped control pulses one can substantially decrease ion-phonon entanglement while maintaining the mediated interaction.
We collect the fluorescence from two trapped atomic ions, and measure quantum interference between photons emitted from the ions. The interference of two photons is a crucial component of schemes to entangle atomic qubits based on a photonic coupling. The ability to preserve the generated entanglement and to repeat the experiment with the same ions is necessary to implement entangling quantum gates between atomic qubits, and allows the implementation of protocols to efficiently scale to larger numbers of atomic qubits.
The theory of interactions between lasers and cold trapped ions as it pertains to the design of Cirac-Zoller quantum computers is discussed. The mean positions of the trapped ions, the eigenvalues and eigenmodes of the ions' oscillations, the magnitude of the Rabi frequencies for both allowed and forbidden internal transitions of the ions and the validity criterion for the required Hamiltonian are calculated. Energy level data for a variety of ion species is also presented.
Trapped ion hardware has made significant progress recently and is now one of the leading platforms for quantum computing. To construct two-qubit gates in trapped ions, experimental manipulation approaches for ion chains are becoming increasingly prevalent. Given the restricted control technology, how implementing high-fidelity quantum gate operations is crucial. Many works in current pulse design optimization focus on ion-phonon and effective ion-ion coupling while ignoring the higher-order expansion impacts of these two terms brought on by experiment defects. This paper proposed a novel robu…
By means of the Ising terms generated by Coulomb interaction between ions and the magnetic field gradient, we carry out teleportation with insurance with trapped ions. We show the feasibility and the favorable feature of our scheme by comparing with the recently achieved teleportation experiments with trapped ions.
We have experimentally observed the dynamics of a single polariton and two polaritons in a two-ion chain. By driving two trapped ions at a motional blue-sideband transition, we realize the anti-Jaynes-Cummings-Hubbard model. When a single polariton exists in a trapped-ion chain, the polariton hops between the ion sites. On the other hand, when there are single polaritons at each ion site, the hopping of the polaritons is suppressed because of the polariton-polariton interaction induced by the nonlinearity of the anti-Jaynes-Cummings interaction, thereby realizing the blockade of polariton hopp…
A new approach for reconstructing the vibrational quantum state of a trapped ion is proposed. The method rests upon the current ability of manipulating the trapped ion state and on the possibility of effectively measuring the scalar product of the two vibrational cofactors of a vibronic entangled state. The experimental feasibility of the method is briefly discussed.
There has been much interest in developing methods for transferring quantum information. We discuss a way to transfer quantum information between two trapped ions through a wire. The motion of a trapped ion induces oscillating charges in the trap electrodes. By sending this current to the electrodes of a nearby second trap, the motions of ions in the two traps are coupled. We investigate the electrostatics of a set-up where two separately trapped ions are coupled through an electrically floating wire. We also discuss experimental issues, including possible sources of decoherence.
In this tutorial we review the basic building blocks of Quantum Information Processing with cold trapped atomic-ions. We mainly focus on methods to implement single-qubit rotations and two-qubit entangling gates, which form a universal set of quantum gates. Different ion qubit choices and their respective gate implementations are described.
We propose a novel scheme to implement a quantum controlled phase gate for trapped ions in thermal motion with one standing wave laser pulse. Instead of applying the rotating wave approximation this scheme makes use of the counter-rotating terms of operators. We also demonstrate that the same scheme can be used to generate maximally entangled states of $N$ trapped ions by a single laser pulse.
Motivated by the challenge of identifying intruder ions in a cold ion crystal, we investigate calorimetry from emitted fluorescence light. Under continuous Doppler cooling, the ion crystal reaches a temperature equilibrium with a fixed level of fluorescence intensity and any change in the motional energy of the crystal results in a modification of this intensity. We theoretically determine the fluorescence rate of an ion crystal as a function of the temperature, assuming that laser light is scattered along a two-level electronic transition, which couples to the crystal's vibrations via the mec…
We demonstrate an optical method for detecting the mechanical oscillations of an atom with single-phonon sensitivity. The measurement signal results from the interference between the light scattered by a single trapped atomic ion and that of its mirror image. The motion of the atom modulates the interference path length and hence the photon detection rate. We detect the oscillations of the atom in the Doppler cooling limit and reconstruct average trajectories in phase space. We demonstrate single-phonon sensitivity near the ground state of motion after EIT cooling. These results could be appli…
We propose and demonstrate a scalable scheme for the simultaneous determination of internal and motional states in trapped ions with single-site resolution. The scheme is applied to the study of polaritonic excitations in the Jaynes- Cummings Hubbard model with trapped ions, in which the internal and motional states of the ions are strongly correlated. We observe quantum phase transitions of polaritonic excitations in two ions by directly evaluating their variances per ion site. Our work establishes an essential technological method for large-scale quantum simulations of polaritonic systems.
There are several known schemes for entangling trapped ion quantum bits for large-scale quantum computation. Most are based on an interaction between the ions and external optical fields, coupling internal qubit states of trapped-ions to their Coulomb-coupled motion. In this paper, we examine the sensitivity of these motional gate schemes to phase fluctuations introduced through noisy external control fields, and suggest techniques to suppress the resulting phase decoherence.
The decoherence in trapped ion induced by coupling the ion to the engineered reservoir is studied in this paper. The engineered reservoir is simulated by random variations in the trap frequency, and the trapped ion is treated as a two-level system driven by a far off-resonant plane wave laser field. The dependence of the decoherence rate on the amplitude of the superposition state is given.
A "continuous measurement" Quantum Zeno Effect (QZE) in the context of trapped ions is predicted. We describe the physical system and study its exact time evolution showing the appearance of Zeno Phenomena. New indicators for the occurrence of QZE in oscillatory systems are proposed and carefully discussed.
Coherent operations constitutive for the implementation of single and multi-qubit quantum gates with trapped ions are demonstrated that are robust against variations in experimental parameters and intrinsically indeterministic system parameters. In particular, pulses developed using optimal control theory are demonstrated for the first time with trapped ions. Their performance as a function of error parameters is systematically investigated and compared to composite pulses.
We propose a scheme to implement quantum phase gate for two $Λ$ ions trapped in optical cavity. It is shown that quantum phase gate can be implemented by applying a laser addressing to a single ions in strongly detuned optical cavity. We further demonstrate that geometric quantum phase gate can be implemented by introducing a auxiliary ground state.
We show how NOON states may be generated in ion traps. We use the individual interaction of light with each of two vibrational modes of the ion to entangle them. This allows us to generate NOON states with N=8.
Applying a magnetic field gradient to a trapped ion allows long-wavelength microwave radiation to produce a mechanical force on the ion's motion when internal transitions are driven. We demonstrate such a coupling using a single trapped \Yb{171}~ion, and use it to produce entanglement between the spin and motional state, an essential step towards using such a field gradient to implement multi-qubit operations.
We propose an architecture and methodology for large-scale quantum simulations using hyperfine states of trapped-ions in an arbitrary-layout microtrap array with laserless interactions. An ion is trapped at each site, and the electrode structure provides for the application of single and pairwise evolution operators using only locally created microwave and radio-frequency fields. The avoidance of short-lived atomic levels during evolution effectively eliminates errors due to spontaneous scattering; this may allow scaling of quantum simulators based on trapped ions to much larger systems than c…
Trapped-ion quantum information processors store information in atomic ions maintained in position in free space via electric fields. Quantum logic is enacted via manipulation of the ions' internal and shared motional quantum states using optical and microwave signals. While trapped ions show great promise for quantum-enhanced computation, sensing, and communication, materials research is needed to design traps that allow for improved performance by means of integration of system components, including optics and electronics for ion-qubit control, while minimizing the near-ubiquitous electric-f…
A protocol is provided to reconstruct the Wigner function for the motional state of a trapped ion via fluorescence detection on another ion in the same trap. This "sympathetic tomography" of a dark ion without optical transitions suitable for state measurements is based on the mapping of its motional state onto one of the collective modes of the ion pair. The quantum state of this vibrational eigenmode is subsequently measured through sideband excitation of the bright ion. Physical processes to implement the desired state transfer and read-out are derived, and the accomplishment of the scheme …
We demonstrate tunable spin-spin couplings between trapped atomic ions, mediated by laser forces on multiple transverse collective modes of motion. A $σ_x σ_x$-type Ising interaction is realized between quantum bits stored in the ground hyperfine clock states of Yb ions. We demonstrate entangling gates and tailor the spin-spin couplings with two and three trapped ions. The use of closely-spaced transverse modes provides a new class of interactions relevant to quantum computing and simulation with large collections of ions in a single crystal.
We propose a scheme to perform basic gates of quantum computing and prepare entangled states in a system with cold trapped ions located in a single mode optical cavity. General quantum computing can be made with both motional state of the trapped ion and cavity state being qubits. We can also generate different kinds of entangled states in such a system without state reduction, and can transfer quantum states from the ion in one trap to the ion in another trap. Experimental requirement for achieving our scheme is discussed.
We propose to use a large cloud of cold trapped ions as a medium for quantum optics and quantum information experiments. Contrary to most recent realizations of qubit manipulation based on a small number of trapped and cooled ions, we study the case of traps containing a macroscopic number of ions. We consider in particular the implementation of a quantum memory for quantum information stored in continuous variables and study the impact of the relevant physical parameters on the expected performances of the system.
A k-quantum nonlinear Jaynes-Cummings model for two trapped ions interacting with laser beams resonant to k-th red side-band of center-of-mass mode, far from Lamb-Dicke regime, has been obtained. The exact analytic solution showed the existence of quantum collapses and revivals of the occupation of two atoms.
We show that a multi-step quantum walk can be realized for a single trapped ion with interpolation between quantum and random walk achieved by randomizing the generalized Hadamard coin flip phase. The signature of the quantum walk is manifested not only in the ion's position but also its phonon number, which makes an ion trap implementation of the quantum walk feasible.
The mode-mode entanglement between trapped ions and cavity fields is investigated in the dispersive regime. We show how a simple initial preparation of Gaussian coherent states and a postselection may be used to generate motional non-local mesoscopic states (NLMS) involving ions in different traps. We also present a study of the entanglement induced by dynamical Stark-shifts considering a cluster of N-trapped ions. In this case, all entanglement is due to the dependence of the Stark-shifts on the ions' state of motion manifested as a cross-Kerr interaction between each ion and the field.
Invariant-based inverse engineering is an elegant approach to quantum control with corresponding experimental implementations that perform tasks with applications in quantum information processing such as shuttling trapped ions. We build on recent work to generalise invariant-based inverse engineering to control two coupled harmonic oscillators in any number of spatial dimensions. This may be used to perform experimentally relevant tasks such as separation of trapped ions, which is demonstrated numerically, achieving transfer fidelities of over 96% as well as low motional number excitations.
We propose a scheme for generating vibrational pair coherent states of the motion of an ion in a two-dimensional trap. In our scheme, the trapped ion is excited bichromatically by three laser beams along different directions in the X-Y plane of the ion trap. We show that if the initial vibrational state is given by a two-mode Fock state, the final steady state, indicated by the extinction of the fluorescence emitted by the ion, is a pure state. The motional state of the ion in the equilibrium realizes that of the highly-correlated pair coherent state.
Resonance fluorescence from atomic systems consists of a single spectral peak that evolves into a Mollow triplet for a strong excitation field. Photons from different peaks of the triplet show distinct photon correlation that make the fluorescence a useful light source for quantum information purpose. We characterize the fluorescence of a single optically trapped $^{87}$Rb atom that is excited resonantly at different power levels. Second-order correlation measurements reveal the single photon nature of the fluorescence concurrently with Rabi oscillations of a strongly excited atom. The asymmet…
We propose a physical implementation of time and spatial parity transformations, as well as Galilean boosts, in a trapped-ion quantum simulator. By embedding the simulated model into an enlarged simulating Hilbert space, these fundamental symmetry operations can be fully realized and measured with ion traps. We illustrate our proposal with analytical and numerical techniques of prototypical examples with state-of-the-art trapped-ion platforms. These results pave the way for the realization of time and spatial parity transformations in other models and quantum platforms.
Squeezed and rotated quadrature of an ion in a Paul trap is discussed in connection with reconstructing its quantum state using symplectic-tomography method. Marginal distributions of the quadrature for squeezed and correlated states and for nonlinear coherent states of a trapped ion are obtained and the density matrices in the Fock basis are expressed explicitly in terms of these marginal distributions.
Based on the exact conditional quantum dynamics for a two-ion system, we propose an efficient {\it single-step} scheme for coherently manipulating quantum information of two trapped cold ions by using a pair of synchronous laser pulses. Neither the auxiliary atomic level nor the Lamb-Dicke approximation are needed.
We demonstrate experimentally how the process of Stimulated Raman Adiabatic Passage (STIRAP) can be utilized for efficient coherent internal state transfer in single trapped and laser-cooled $^{40}$Ca$^+$ ions. The transfer from the D$_{3/2}$ to the D$_{5/2}$ state, is detected by a fluorescence measurement revealing the population not transfered to the D$_{5/2}$ state. A coherent population transfer efficiency at the level of 95 % in a setup allowing for the internal state detection of individual ions in a string has been obtained.
The interaction of a trapped ion with a laser beam in the strong excitation regime is analyzed. In this regime, a variety of non--classical states of motion can be prepared either by using laser pulses of well defined area, or by an adiabatic passage scheme based on the variation of the laser frequency. We show how these states can be used to investigate fundamental properties of quantum mechanics. We also study possible applications of this system to build an ion interferometer.
