We introduce a local radiative heat-pumping effect between two bodies in a many-body system, obtained by periodically modulating both the temperature and the position of an intermediate object using an external source of energy. We show that the magnitude and the sign of energy flow can be tuned by changing the oscillation amplitude and dephasing of the two parameters. This many-body effect paves the way for an efficient and active control of heat fluxes at the nanoscale.
We propose using a phonon pumping mechanism to transfer heat from a cold to a hot body using a propagating modulation of the medium connecting the two bodies. This phonon pump can cool nanomechanical systems without the need for active feedback. We compute the lowest temperature that this refrigerator can achieve.
A mechanism of electron-mediated pumping of heat in the absence of net charge transfer is proposed. It may be realized in charge-neutral electron systems, such as graphene, coupled to an external electric potential. The flow of heat in this pumping cycle is not accompanied by a buildup of voltage along the system, which offers advantages over traditional thermoelectric cooling setups. Efficiency of heat pumping and magnitude of heat flux are studied in the hydrodynamic regime for weak disorder. In a pristine system, even for an infinitesimal pumping potential the heat flux remains finite. In p…
A `toy model' - aimed at capturing the essential physics - is presented that jointly describes spin-polarized hot electron transport and spin pumping driven by local heating. These two processes both contribute to spin-current generation in laser-excited magnetic heterostructures. The model is used to compare the two contributions directly. The spin-polarized hot electron current is modeled as one generation of hot electrons with a spin-dependent excitation and relaxation scheme. Upon decay, the excess energy of the hot electrons is transferred to a thermalized electron bath. The elevated elec…
We study the heat transport due to phonons in nanomechanical structures using a phase space representation of non-equilibrium Green's functions. This representation accounts for the atomic degrees of freedom making it particularly suited for the description of small (molecular) junctions systems. We show that for the steady state limit our formalism correctly recovers the heuristic Landauer-like heat conductance for a quantum coherent molecular system coupled to thermal reservoirs. We find general expressions for the non-stationary heat current due to an external periodic drive. In both cases …
It is shown that the presence of discrete symmetries in Floquet systems connected to metallic reservoirs imprints a definite parity on the charge and heat pumping as a function of the reservoir's chemical potential, $μ$. In particular, when particle-hole symmetry (PHS) holds, the pumping of charge (heat) is an odd (even) function of $μ$. Whereas, if only the product of PHS and parity symmetry is present, pumping of charge (heat) is even (odd) in $μ$. Our results also extend to the presence of other unitary symmetries and provide a simple criterion for reversing (or maintaining) the direction o…
A general formalism for calculating the Radiative Heat Transfer in many body systems with anisotropic component is presented. Our scheme extends the theory of radiative heat transfer in isotropic many body systems to anisotropic cases. In addition, the radiative heating of the particles by the thermal bath is taken into account in our formula. It is shown that the radiative heat exchange (HE) between anisotropic particles and their radiative cooling/heating (RCH) could be enhanced several order of magnitude than that of isotropic particles. Furthermore, we demonstrate that both the HE and RCH …
Spin pumping consists in the injection of spin currents into a non-magnetic material due to the precession of an adjacent ferromagnet. In addition to the pumping of spin the precession always leads to pumping of heat, but in the presence of spin-orbital entanglement it also leads to a charge current. We investigate the pumping of charge, spin and heat in a device where a superconductor and a quantum spin Hall insulator are in proximity contact with a ferromagnetic insulator. We show that the device supports two robust operation regimes arising from topological effects. In one regime, the pumpe…
We consider transport properties of a two dimensional topological insulator in a double quantum point contact geometry in presence of a time-dependent external field. In the proposed setup an external gate is placed above a single constriction and it couples only with electrons belonging to the top edge. This asymmetric configuration and the presence of an ac signal allow for a quantum pumping mechanism, which, in turn, can generate finite heat and charge currents in an unbiased device configuration. A microscopic model for the coupling with the external time-dependent gate potential is develo…
Majorana zero modes are non-Abelian quasiparticles that emerge on the edges of topological phases of superconductors. Evidence of their presence has been reported in transport measurements on engineered superconducting-based nanostructures. In this manuscript we identify signatures of a topologically protected dynamical manipulation of Majorana zero modes via continuous transport measurement during the manipulation. Specifically, we show that, in a two-terminal geometry, the heat pumped across the terminals at low temperature and voltage bias is characterized by a universal value. We show that…
Facultad de Ciencias Exactas, Ingeniería y Agrimensura, Universidad Nacional de Rosario（罗萨里奥国立大学精确科学、工程与测量学院）；Instituto de Física Rosario (CONICET)（罗萨里奥物理研究所（CONICET））；Centro Atómico Bariloche（巴里洛切原子中心）；Instituto de Nanociencia y Nanotecnología CONICET-CNEA（CONICET-CNEA纳米科学与纳米技术研究所）；Instituto Balseiro（巴尔塞罗研究所）
Antiferromagnetic insulators can become active spintronics components by controlling and detecting their dynamics via spin currents in adjacent metals. This cross-talk occurs via spin-transfer and spin-pumping, phenomena that have been predicted to be as strong in antiferromagnets as in ferromagnets. Here, we demonstrate that a temperature gradient drives a significant heat flow from magnons in antiferromagnetic insulators to electrons in adjacent normal metals. The same coefficients as in the spin-transfer and spin-pumping processes also determine the thermal conductance. However, in contrast…
The control of heat flow is a formidable challenge due to lack of good thermal insulators. Promising new oppor-tunities for heat flow control were recently theoretically discovered for radiative heat flow in near field, where large heat flow contrasts may be achieved by tuning electronic excitations on surfaces. Here we show experi-mentally that the phase transition of VO2 entails a change of surface polariton states that significantly affects radiative heat transfer in near field. In all cases the Derjaguin approximation correctly predicted radiative heat transfer in near field, but it undere…
We study the effects of the coupling between magnetization dynamics and the electronic degrees of freedom in a heterostructure of a metallic nanomagnet with dynamic magnetization coupled with a superconductor containing a steady spin-splitting field. We predict how this system exhibits a non-linear spin torque, which can be driven either with a temperature difference or a voltage across the interface. We generalize this notion to arbitrary magnetization precession by deriving a Keldysh action for the interface, describing the coupled charge, heat and spin transport in the presence of a precess…
Applying adiabatic, cyclic two parameter modulations we investigate quantum heat transfer across an anharmonic molecular junction contacted with two heat baths. We demonstrate that the pumped heat typically exhibits a Berry phase effect in providing an additional geometric contribution to heat flux. Remarkably, a robust fractional quantized geometric phonon response is identified as well. The presence of this geometric phase contribution in turn causes a breakdown of the fluctuation theorem of the Gallavotti-Cohen type for quantum heat transfer. This can be restored only if (i) the geometric p…
We investigate the radiative heat transport along a Su-Schrieffer-Heeger chain of InSb nanoparticles. We show that in the topological non-trivial phase, the edge modes dominate the radiative heat transport despite their strong localization at the edges of the finite chain due to a long-range coupling of the first and last particle. We further discuss the scaling laws of the heat transfer with respect to the chain length for the longitudinal and transversal band- and edge modes and conclude that both type of modes obey the same scaling law.
We study the near-field radiative energy transfer between graphene and an amorphous SiO$_2$ substrate. In comparison with the existing theories of near-field radiative heat transfer our theory takes into account that the free carriers in graphene are moving relative to the substrate with a drift velocity $v$. In this case the heat flux is determined by both thermal and quantum fluctuations. We find that quantum fluctuations give an important contribution to the radiative energy transfer for low temperatures and high electric field (large drift velocities). For nonsuspended graphene the near-fi…
We present a general framework for studying strongly coupled radiative and conductive heat transfer between arbitrarily shaped bodies separated by sub-wavelength distances. Our formulation is based on a macroscopic approach that couples our recent fluctuating volume--current (FVC) method of near-field heat transfer to the more well known Fourier conduction transport equation. We apply our technique to consider heat exchange between aluminum-zinc oxide nanorods and show that the presence of bulk plasmon resonances can result in extremely large radiative heat transfer rates (roughly twenty times…
Owing to its two dimensional electronic structure, graphene exhibits many unique properties. One of them is a wave vector and temperature dependent plasmon in the infrared range. Theory predicts that due to these plasmons, graphene can be used as a universal material to enhance nanoscale radiative heat exchange for any dielectric substrate. Here we report on radiative heat transfer experiments between SiC and a SiO2 sphere which have non matching phonon polariton frequencies, and thus only weakly exchange heat in near field. We observed that the heat flux contribution of graphene epitaxially g…
We study the near-field radiative heat transfer between two twisted finite-size polar dielectric nanoparticle gratings. Differently from previous studies of the same configuration, we do not rely on any approximated effective medium theory to describe the gratings. By the full many-body radiative heat transfer theory we are able to investigate how the size, distance and relative orientation between the gratings influence the radiative heat flux. By changing the twisting angle $θ$, we show a significant oscillation of the thermal conductance $G(θ)$, due to the size effect for gratings of both s…
We analyze the coupling between conduction and radiative heat transfer in near-field regime between two coaxial cylinders separated by a vacuum gap. By solving the heat transport equation in the steady-state regime between metals or polar materials we highlight a flux saturation mechanism for the radiative transfer even without non-local effect. In the case of polar materials this saturation occurs in the separation distances range of 1 to 10 nm which can be experimentally explored.
We present a theory to describe the fluctuations of nonequilibrium radiative heat transfer between two bodies both in far and near-field regime. As predicted by the blackbody theory, in far field, we show that the variance of radiative heat flux is of the same order of magnitude as its mean value. However, in near-field regime we demonstrate that the presence of surface polaritons makes this variance more than one order of magnitude larger than the mean flux. We further show that the correlation time of heat flux in this regime is comparable to the relaxation time of heat carriers in each medi…
Radiative heat transfer between bodies is often dominated by a narrow resonance in the transmission, e.~g. due to a cavity mode or a surface excitation. However, this resonant character is not visible in the average heat current. Here, we show that the noise spectrum of heat current can serve as a direct probe of the heat-carrying excitations. Namely, the resonant mode produces a sharp peak in the noise spectrum with a width related to the mode lifetime. We demonstrate that heat transfer in realistic superconducting circuits or between two-dimensional metals can realize our predictions.
In this Letter a N-body theory for the radiative heat exchange in thermally non equilibrated discrete systems of finite size objects is presented. We report strong exaltation effects of heat flux which can be explained only by taking into account the presence of many body interactions. Our theory extends the standard Polder and van Hove stochastic formalism used to evaluate heat exchanges between two objects isolated from their environment to a collection of objects in mutual interaction. It gives a natural theoretical framework to investigate the photon heat transport properties of complex sy…
We study the radiative heat transfer between two semi-infinite half-spaces, bounded by conductive surfaces in contact with vacuum. This setup is interpreted as a four-terminal mesoscopic transport problem. The slabs and interfaces are viewed as bosonic reservoirs, coupled perfectly to a scattering center consisting of the two interfaces and vacuum. Using Rytov's fluctuational electrodynamics and assuming Kirchhoff's circuital law, we calculate the heat flow in each bath. This allows for explicit evaluation of a conductance matrix, from which one readily verifies Büttiker symmetry. Thus, radiat…
We describe how adiabatically rocked quantum electron ratchets can act as heat pumps. In general, ratchets may be described as non-equilibrium systems in which directed particle motion is generated using spatial or temporal asymmetry. In a rocked ratchet, which may also be described as a non-linear rectifier, an asymmetric potential is tilted symmetrically and periodically. The potential deforms differently during each half-cycle, producing a net current of particles when averaged over a full period of rocking. Recently it was found that in the quantum regime, where tunnelling contributes to t…
The radiative heat transfer between two dielectrics can be strongly enhanced in the near field in the presence of surface phonon-polariton resonances. Nevertheless, the spectral mismatch between the surface modes supported by two dissimilar materials is responsible for a dramatic reduction of the radiative heat flux they exchange. In the present paper we study how the presence of a graphene sheet, deposited on the material supporting the surface wave of lowest frequency, allows to widely tune the radiative heat transfer, producing an amplification factor going up to one order of magnitude. By …
Lindbladian approach for many-qubit thermal machines: enhancing the performance with geometric heat pumping by interaction
Facultad de Ciencias Exactas, Ingeniería y Agrimensura, Universidad Nacional de Rosario（罗萨里奥国立大学精确科学、工程与测量学院）；Instituto de Física Rosario (CONICET)（罗萨里奥物理研究所（阿根廷国家科学研究委员会））；Departamento de Sólidos Cuánticos y Sistemas Desordenados, Centro Atómico Bariloche, Instituto de Nanociencia y Nanotecnología CONICET-CNEA and Instituto Balseiro（巴里洛切原子中心量子固体与无序系统系，纳米科学与技术研究所（阿根廷国家科学研究委员会-阿根廷国家原子能委员会）和巴尔塞罗研究所）
The transport of heat mediated by thermal photons in hyperbolic multilayer metamaterials is studied using the fluctuational electrodynamics theory. We demonstrate that in comparison to bulk materials the flux inside layered hyperbolic materials can be transported at much longer distances, making these media very promising for thermal management and for near-field energy harvesting.
We study the radiative heat transfer and the van der Waals friction between graphene and an amorphous SiO$_2$ substrate. We study the surface phonon-polaritons contribution to the low-field mobility as a function of temperature and of carrier density. We find that the electric current saturate at a high electric field, in agreement with experiment. The saturation current depends weakly on the temperature, which we attribute to the "quantum" friction between the graphene carriers and the substrate optical phonons. We calculate the frictional drag between two graphene sheets caused by van der Wa…
We present a general nonequilibrium Green's function formalism for modeling heat transfer in systems characterized by linear response that establishes the formal algebraic relationships between phonon and radiative conduction, and reveals how upper bounds for the former can also be applied to the latter. We also propose an extension of this formalism to treat systems susceptible to the interplay of conductive and radiative heat transfer, which becomes relevant in atomic systems and at nanometric and smaller separations where theoretical descriptions which treat each phenomenon separately may b…
We numerically study the tuning of the radiative heat transfer between a spherical InSb nanoparticle in the vicinity of a flat SiC surface assisted by a static magnetic field. By changing the value of the applied magnetic field, the dielectric function of the nanosphere becomes anisotropic due to the excitation of magneto-plasmons. In the dipolar approximation, the plasmon resonance of the particle splits into two additional satellite resonances that shift to higher and lower frequencies as the field increases. When one of the particle resonances overlaps with the phonon-polariton frequency of…
We derive exact analytical formulas for the radiative heat transfer between parallel slabs separated by vacuum and subject to arbitrary temperature profiles. We show that, depending on the derivatives of the temperature at points close to the slab--vacuum interfaces, the flux can exhibit one of several different asymptotic low-distance ($d$) behaviors, obeying either $1/d^2$, $1/d$, or logarithmic power laws, or approaching a constant. Tailoring the temperature profile within the slabs could enable unprecedented tunability over heat exchange, leading for instance to sign-flip transitions (wher…
Radiative heat transfer between two bodies saturates at very short separation distances due to the nonlocal optical response of the materials. In this work, we show that the presence of radiative interactions with a third body or external bath can also induce a saturation of the heat transfer, even at separation distances for which the optical response of the materials is purely local. We demonstrate that this saturation mechanism is a direct consequence of a thermalization process resulting from many-body interactions in the system. This effect could have an important impact in the field of n…
Using the standard fluctuational electrodynamics framework, we analytically calculate the radiative heat current between two thin metallic layers, separated by a vacuum gap. We analyse different contributions to the heat current (travelling or evanescent waves, transverse electric or magnetic polarization) and reveal the crucial qualitative role played by the dc conductivity of the metals as compared to the speed of light. For poorly conducting metals, the heat current may be dominated by evanescent waves even when the separation between the layers greatly exceeds the thermal photon wavelength…
It is shown that the fundamental results obtained in the works by Levine, Polevoi, Rytov (1980) and Polevoi (1990), based on the fluctuation-electromagnetic theory by Levine and Rytov, adequately describe the rate of radiative heat exchange and the frictional force in a system of two parallel thick plates in relative lateral motion. A numerically calculated friction force for good metals and thin gaps turns out to be by a factor 107 higher than earlier obtained by Polevoi and increases with increasing conductivity of the metals.
We show the existence of Fano resonances in the context of near-field radiative heat transfer, which enable the strong suppression and enhancement of the spectral heat flux at specific wavelengths. This is demonstrated by making use of the plasmon-phonon coupling in a symmetric nano cavity composed by a polaritonic material coated with a metallic layer, in which each side of the cavity is kept at different temperatures. The strong hybridization of the plasmonic and phononic modes sustained by the multilayer structure is determined by the matching of their polarization. This leads to the openin…
We study a one-dimensional model of radiative heat transfer for which the effect of the electromag- netic field is only from the scalar potential and thereby ignoring the vector potential contribution. This is a valid assumption when the distances between objects are of the order of nanometers. Using Lorenz gauge, the scalar field is quantized with the canonical quantization scheme, giving rise to scalar photons. In the limit as the speed of light approaches infinity, the theory reduces to a pure Coulomb interaction governed by the Poisson equation. The model describes very well parallel plate…
The nonlinear response of electrons (holes) in doped graphene on ac pumping is considered theoretically for the frequency region above the energy relaxation rate but below the momentum and carrier-carrier scattering rates. Temporally-dependent heating of electrons by a strong ac field, which is described within the energy balance approach, leads to an effective generation of high-order harmonics. The efficiency of up-conversion of the 1 mm radiation into the third harmonic by a single-layer graphene is about 10^{-7} at pumping level ~100 kW/cm^2, room temperature, and concentration ~5 x 10^{11…
We study the effect of particles shape on the radiative heat transfer in a three-body system. It is found that the radiative heat flux between two nanoparticles in a three body system can be tuned by the shape of the third particle. In particular, we show that the heat flux is very sensitive to the particle shapes and slight mismatches of shapes results in either enhanced or suppressed heat flux.
We present an overview of recent advances in the study of energy dynamics and mechanisms for energy conversion in qubit systems with special focus on realizations in superconducting quantum circuits. We briefly introduce the relevant theoretical framework to analyze heat generation, energy transport and energy conversion in these systems with and without time-dependent driving considering the effect of equilibrium and non-equilibrium environments. We analyze specific problems and mechanisms under current investigation in the context of qubit systems. These include the problem of energy dissipa…
The recent development of a scanning thermal microscope (SThM) has led to measurements of radiative heat transfer between a heated sensor and a cooled sample down to the nanometer range. This allows for comparision of the known theoretical description of radiative heat transfer, which is based on fluctuating electrodynamics, with experiment. The theory itself is a macroscopic theory, which can be expected to break down at distances much smaller than 10-8m. Against this background it seems to be reasonable to revisit the known macroscopic theory of fluctuating electrodynamics and of radiative h…
We demonstrate the existence of a shuttling effect for the radiative heat flux exchanged between two bodies separated by a vacuum gap when the chemical potential of photons or the temperature difference is modulated. We show that this modulation typically gives rise to a supplementary flux which superimposes to the flux produced by the mean gradient, enhancing the heat exchange. When the system displays a negative differential thermal resistance, however, the radiative shuttling contributes to insulate the two bodies from each other. These results pave the way for a novel strategy for an activ…
The radiative properties of most structures are intimately connected to the way in which their constituents are ordered on the nano-scale. We have proposed a new representation for radiative heat transfer formalism in many-body systems. In this representation, we explain why collective effects depend on the morphology of structures, and how the arrangement of nanoparticles and their material affects the thermal properties in many-body systems. We investigated the radiative heat transfer problem in fractal (i.e., scale invariant) structures. In order to show the effect of the structure morpholo…
In this work, we study the near-field radiative heat transfer between two suspended sheets of anisotropic 2D materials. It is found that the radiative heat transfer can be enhanced with orders-of-magnitude over the blackbody limit for nanoscale separation. The enhancement is attributed to the excitation of anisotropic and hyperbolic plasmonic modes. Meanwhile, a large thermal modulation effect, depending on the twisted angle of principal axes between the upper and bottom sheets of anisotropic 2D materials, is revealed. The near-field radiative heat transfer for different concentrations of elec…
We demonstrate in this work that the use of metasurfaces provides a viable strategy to largely tune and enhance near-field radiative heat transfer between extended structures. In particular, using a rigorous coupled wave analysis, we predict that Si-based metasurfaces featuring two-dimensional periodic arrays of holes can exhibit a room-temperature near-field radiative heat conductance much larger than any unstructured material to date. We show that this enhancement, which takes place in a broad range of separations, relies on the possibility to largely tune the properties of the surface plasm…
We present a formulation of the nanoscale radiative heat transfer (RHT) using concepts of mesoscopic physics. We introduce the analog of the Sharvin conductance using the quantum of thermal conductance. The formalism provides a convenient framework to analyse the physics of RHT at the nanoscale. Finally, we propose a RHT experiment in the regime of quantized conductance.
We present a theoretical analysis that demonstrates that the far-field radiative heat transfer between objects with dimensions smaller than the thermal wavelength can overcome the Planckian limit by orders of magnitude. We illustrate this phenomenon with micron-sized structures that can be readily fabricated and tested with existing technology. Our work shows the dramatic failure of the classical theory to predict the far-field radiative heat transfer between micro- and nano-devices.
The near-field electromagnetic interaction between nanoscale objects produces enhanced radiative heat transfer that can greatly surpass the limits established by far-field black-body radiation. Here, we present a theoretical framework to describe the temporal dynamics of the radiative heat transfer in ensembles of nanostructures, which is based on the use of an eigenmode expansion of the equations that govern this process. Using this formalism, we identify the fundamental principles that determine the thermalization of collections of nanostructures, revealing general but often unintuitive dyna…
A parametric study of Drude and Lorentz models performances in maximizing near-field radiative heat transfer between two semi-infinite planes separated by nanometric distances at room temperature is presented in this paper. Optimal parameters of these models that provide optical properties maximizing the radiative heat flux are reported and compared to real materials usually considered in similar studies, silicon carbide and heavily doped silicon in this case. Results are obtained by exact and approximate (in the extreme near-field regime and the electrostatic limit hypothesis) calculations. T…
