Rocky asteroids and planets display nucleosynthetic isotope variations that are attributed to the heterogeneous distribution of stardust from different stellar sources in the solar protoplanetary disk. Here we report new high precision palladium isotope data for six iron meteorite groups, which display smaller nucleosynthetic isotope variations than the more refractory neighbouring elements. Based on this observation we present a new model in which thermal destruction of interstellar medium dust results in an enrichment of s-process dominated stardust in regions closer to the Sun. We propose that stardust is depleted in volatile elements due to incomplete condensation of these elements into dust around asymptotic giant branch (AGB) stars. This led to the smaller nucleosynthetic variations for Pd reported here and the lack of such variations for more volatile elements. The smaller magnitude variations measured in heavier refractory elements suggest that material from high-metallicity AGB stars dominated stardust in the Solar System. These stars produce less heavy s-process elements compared to the bulk Solar System composition.
Analyses of primitive meteorites and cometary samples have shown that the solar nebula must have experienced a phase of large-scale outward transport of small refractory grains as well as homogenization of initially spatially heterogeneous short-lived isotopes. The stable oxygen isotopes, however, were able to remain spatially heterogenous at the $\sim$ 6% level. One promising mechanism for achieving these disparate goals is the mixing and transport associated with a marginally gravitationally unstable (MGU) disk, a likely cause of FU Orionis events in young low-mass stars. Several new sets of…
We use new experiments and a theoretical analysis of the results to show that the isotopic fractionation associated with laser-heating aerodynamic levitation experiments is consistent with the velocity of flowing gas as the primary control on the fractionation. The new Fe and Mg isotope data are well explained where the gas is treated as a low-viscosity fluid that flows around the molten spheres with high Reynolds numbers and minimal drag. A relationship between the ratio of headwind velocity to thermal velocity and saturation is obtained on the basis of this analysis. The recognition that it …
The oxygen isotope fractionation scenario, which has been developed to explain the oxygen isotope anomaly in the solar system materials, predicts that CO gas is depleted in 18O in protoplanetary disks, where segregation between solids and gas inside disks had already occurred. Based on ALMA observations, we report the first detection of HC18O+(4-3) in a Class II protoplanetary disk (TW Hya). This detection allows us to explore the oxygen isotope fractionation of CO in the TW Hya disk from optically thin HCO+ isotopologues as a proxy of optically thicker CO isotopologues. Using the H13CO+(4-3) …
Planetary systems are thought to be born in protoplanetary disks. Isotope ratios are a powerful tool for investigating the material origin and evolution from molecular clouds to planetary systems via protoplanetary disks. However, it is challenging to measure the isotope (isotopologue) ratios, especially in protoplanetary disks, because the emission lines of major species are saturated. We developed a new method to overcome these challenges by using optically thin line wings induced by thermal broadening. As a first application of the method, we analyzed two carbon monoxide isotopologue lines,…
Observations of different molecular lines in protoplanetary disks provide valuable information on the gas kinematics, as well as constraints on the radial density and temperature structure of the gas. With ALMA we have detected H13CO+ (J=4-3) and HC15N (J=4-3) in the HD97048 protoplanetary disk for the first time. We compare these new detections to the ringed continuum mm-dust emission and the spatially resolved CO (J=3-2) and HCO+ (J=4-3) emission. The radial distributions of the H13CO+ and HC15N emission show hints of ringed sub-structure whereas, the optically thick tracers, CO and HCO+, do…
Short-lived radioisotopes (SLRI) such as $^{60}$Fe and $^{26}$Al were likely injected into the solar nebula in a spatially and temporally heterogeneous manner. Marginally gravitationally unstable (MGU) disks, of the type required to form gas giant planets, are capable of rapid homogenization of isotopic heterogeneity as well as of rapid radial transport of dust grains and gases throughout a protoplanetary disk. Two different types of new models of a MGU disk in orbit around a solar-mass protostar are presented. The first set has variations in the number of terms in the spherical harmonic solut…
H$_2^{18}$O in the terrestrial planet-forming regions of protoplanetary disks
Vassar College（瓦萨学院）；Jet Propulsion Laboratory, California Institute of Technology（加州理工学院喷气推进实验室）；Division of Geological and Planetary Sciences, California Institute of Technology（加州理工学院地质与行星科学系）；Department of Astronomy, University of Wisconsin-Madison（威斯康星大学麦迪逊分校天文学系）；Center for Astrophysics, Harvard & Smithsonian（哈佛-史密森尼天体物理中心）；Department of Physics, Texas State University（德克萨斯州立大学物理系）；Weber State University（韦伯州立大学）；Department of Astronomy, University of Michigan（密歇根大学天文学系）；Astrophysics & Space Institute, Schmidt Sciences（施密特科学天体物理学与空间研究所）；Department of Physics and Astronomy, University of Exeter（埃克塞特大学物理与天文系）；Department of Astronomy, University of Maryland（马里兰大学天文学系）
We discuss the current state of knowledge of terrestrial planet formation from the aspects of different planet formation models and isotopic data from 182Hf-182W, U-Pb, lithophile-siderophile elements, 48Ca/44Ca isotope samples from planetary building blocks, 36Ar/38Ar, 20Ne/22Ne, 36Ar/22Ne isotope ratios in Venus' and Earth's atmospheres, the expected solar 3He abundance in Earth's deep mantle and Earth's D/H sea water ratios that shed light on the accretion time of the early protoplanets. Accretion scenarios that can explain the different isotope ratios, including a Moon-forming event after …
Meteorites contain relict decay products of short-lived radionuclides that were present in the protoplanetary disk when asteroids and planets formed. Several studies reported a high abundance of 60Fe (t1/2=2.62+/-0.04 Myr) in chondrites (60Fe/56Fe~6*10-7), suggesting that planetary materials incorporated fresh products of stellar nucleosynthesis ejected by one or several massive stars that exploded in the vicinity of the newborn Sun. We measured 58Fe/54Fe and 60Ni/58Ni isotope ratios in whole rocks and constituents of differentiated achondrites (ureilites, aubrites, HEDs, and angrites), unequi…
The presence or absence of variations in the mass-independent abundances of Si isotopes in bulk meteorites provides important clues concerning the evolution of the early solar system. No Si isotopic anomalies have been found within the level of analytical precision of 15 ppm in 29Si/28Si across a wide range of inner solar system materials, including terrestrial basalts, chondrites, and achondrites. A possible exception is the angrites, which may exhibit small excesses of 29Si. However, the general absence of anomalies suggests that primitive meteorites and differentiated planetesimals formed i…
Isotope anomalies among planetary bodies provide key constraints on planetary genetics and the Solar System's dynamical evolution. However, to unlock the full potential of these anomalies for constraining the processing, mixing, and transport of material in the disk it is essential to identify the main components responsible for producing planetary-scale isotope variations, and to investigate how they relate to the isotopic heterogeneity inherited from the Solar System's parental molecular cloud. To address these issues we measured the Ti and Sr isotopic compositions of Ca,Al-rich inclusions (…
Chondrites are the likely building blocks of Earth, and identifying the group of chondrite that best represents Earth is a key to resolving the state of the early Earth. The origin of chondrites, however, remains controversial partly because of their puzzling major element compositions, some exhibiting depletion in Al, Ca, and Mg. Based on a new thermochemical evolution model of protoplanetary disks, we show that planetesimals with depletion patterns similar to ordinary and enstatite chondrites can originate at 1-2 AU just outside where enstatite evaporates. Around the "evaporation front" of e…
An understanding of the abundance and distribution of water vapor in the innermost region of protoplanetary disks is key to understanding the origin of habitable worlds and planetary systems. Past observations have shown H2O to be abundant and a major carrier of elemental oxygen in disk surface layers that lie within the inner few au of the disk. The combination of high abundance and strong radiative transitions leads to emission lines that are optically thick across the infrared spectral range. Its rarer isotopologue H2-18O traces deeper into this layer and will trace the full content of the …
Injection of material from a core-collapse supernova into the solar system's already-formed disk is one proposed mechanism for producing the short-lived radionuclides, such as 26Al and 41Ca, inferred from isotopic studies of meteorites to have existed in the solar nebula. This hypothesis has recently been challenged on the basis that the injection of enough supernova material to match the meteoritic abundances of 26Al and 41Ca would produce large, measureable, and unobserved collateral effects on oxygen isotopes. Here we calculate again the shifts in oxygen isotopes due to injection of superno…
Isotopic ratios provide a powerful tool for understanding the origins of materials, including the volatile and refractory matter within solar system bodies. Recent high sensitivity observations of molecular isotopologues, in particular with ALMA, have brought us new information on isotopic ratios of hydrogen, carbon, nitrogen and oxygen in star and planet forming regions as well as the solar system objects. Solar system exploration missions, such as Rosetta and Cassini, have given us further new insights. Meanwhile, the recent development of sophisticated models for isotope chemistry including…
Oxygen Isotopic Compositions of Chondrules as Probes of Solar Protoplanetary Disk Formation
Japan Agency for Marine-Earth Science and Technology（日本海洋地球科学技术局）；Kochi Institute for Core Sample Research, EMS, Japan Agency for Marine-Earth Science and Technology（日本海洋地球科学技术局高知岩心研究所以及EMS）；Marine Core Research Institute, Kochi University（高知大学海洋岩心研究所）；Department of Earth and Planetary Sciences, Institute of Science Tokyo（东京科学大学地球与行星科学系）
Organic matter and hydrous silicates are intimately mixed in the matrix of chondrites and in-situ determination of their individual D/H ratios is therefore challenging. Nevertheless, the D/H ratio of each pure component in this mixture should yield a comprehensible signature of the origin and evolution of water and organic matter in our solar system. We measured hydrogen isotope ratios of organic and hydrous silicates in the matrices of two carbonaceous chondrites (Orgueil CI1 and Renazzo CR2) and one unequilibrated ordinary chondrite (Semarkona, LL3.0). A novel protocol was adopted, involving…
The fundamentally different isotopic compositions of non-carbonaceous (NC) and carbonaceous (CC) meteorites reveal the presence of two distinct reservoirs in the solar protoplanetary disk that were likely separated by Jupiter. However, the extent of material exchange between these reservoirs, and how this affected the composition of the inner disk are not known. Here we show that NC meteorites display broadly correlated isotopic variations for Mo, Ti, Cr, and Ni, indicating the addition of isotopically distinct material to the inner disk. The added material resembles bulk CC meteorites and Ca-…
X-ray emission in young stellar objects (YSOs) is orders of magnitude more intense than in main sequence stars1,2, suggestive of cosmic ray irradiation of surrounding accretion disks. Protoplanetary disk irradiation has been detected around YSOs by HERSCHEL3. In our solar system, short-lived 10Be (half-life = 1.39 My4), which cannot be produced by stellar nucleosynthesis, was discovered in the oldest solar system solids, the calcium-aluminium-rich inclusions (CAIs)5. The high 10Be abundance, as well as detection of other irradiation tracers6,7, suggest 10Be likely originates from cosmic ray ir…
When planetesimals grow via collisions in a turbulent disk, stirring through density fluctuation caused by turbulence effectively increases the relative velocities between planetesimals, which suppresses the onset of runaway growth. We investigate the onset of runaway growth in a turbulent disk through simulations that calculate the mass and velocity evolution of planetesimals. When planetesimals are small, the average relative velocity between planetesimals, $v_{\rm r}$, is much greater than their surface escape velocity, $v_{\rm esc}$, so that runaway growth does not occur. As planetesimals …
Chondrules formed by the melting of dust aggregates in the solar protoplanetary disk and as such provide unique insights into how solid material was transported and mixed within the disk. Here we show that chondrules from enstatite and ordinary chondrites show only small 50Ti variations and scatter closely around the 50Ti composition of their host chondrites. By contrast, chondrules from carbonaceous chondrites have highly variable 50Ti compositions, which, relative to the terrestrial standard, range from the small 50Ti deficits measured for enstatite and ordinary chondrite chondrules to the l…
Isotope abundance ratios play an important role in astronomy and planetary sciences, providing insights in the origin and evolution of the Solar System, interstellar chemistry, and stellar nucleosynthesis. In contrast to deuterium/hydrogen ratios, carbon isotope ratios are found to be roughly constant (~89) in the Solar System, but do vary on galactic scales with 12C/13C~68 in the current local interstellar medium. In molecular clouds and protoplanetary disks, 12CO/13CO isotopologue ratios can be altered by ice and gas partitioning, low-temperature isotopic ion exchange reactions, and isotope-…
Carbonaceous asteroids represent the principal source of water in the inner Solar System and might correspond to the main contributors for the delivery of water to Earth. Hydrogen isotopes in water-bearing primitive meteorites, e.g. carbonaceous chondrites, constitute a unique tool for deciphering the sources of water reservoirs at the time of asteroid formation. However, fine-scale isotopic measurements are required to unravel the effects of parent body processes on the pre-accretion isotopic distributions. Here we report in situ micrometer-scale analyses of hydrogen isotopes in six CM-type c…
The meteorite sample Erg Chech (EC) 002 is the oldest felsic igneous rock from the Solar System analysed to date and provides a unique opportunity to study the formation of felsic crusts on differentiated protoplanets immediately after metal-silicate equilibration or core formation. The extinct 53Mn-53Cr chronometer provides chronological constraints on the formation of EC 002 by applying the isochron approach using chromite, metal-silicate-sulphide and whole-rock fractions as well as "leachates" obtained by sequential digestion of a bulk sample. Assuming a chondritic evolution of its parent b…
We use N-body simulations of star cluster evolution to explore the hypothesis that short-lived radioactive isotopes found in meteorites, such as 26-Al, were delivered to the Sun's protoplanetary disc from a supernova at the epoch of Solar System formation. We cover a range of star cluster formation parameter space and model both clusters with primordial substructure, and those with smooth profiles. We also adopt different initial virial ratios - from cool, collapsing clusters to warm, expanding associations. In each cluster we place the same stellar population; the clusters each have 2100 star…
The isotopic heterogeneity of the Solar System shown by meteorite analyses is more pronounced for its earliest objects, the Calcium-Aluminum-rich Inclusions (CAIs). This suggests that it was inherited from spatial variations in different stardust populations in the protosolar cloud. We model the formation of the solar protoplanetary disk following its collapse and find that the solid-weighted standard deviation of different nucleosynthetic contributions in the disk is reduced by one order of magnitude compared to the protosolar cloud, whose successive isotopic signatures are fossilized by CAIs…
Using very high resolution (lambda / Dlambda ~ 95000) 4.7 micron fundamental and 2.3 micron overtone ro-vibrational CO absorption spectra obtained with the CRIRES infrared spectrometer on the Very Large Telescope (VLT), we report detections of four CO isotopologues -- C16O, 13CO, C18O and the rare species, C17O -- in the circumstellar environment of two young protostars, VV CrA and Reipurth 50. We argue that the observed CO absorption lines probe a protoplanetary disk in VV CrA, and a protostellar envelope in Reipurth 50. All CO line profiles are spectrally resolved, permitting direct calculat…
Systematic variations in 54Cr/52Cr ratios between meteorite classes (Qin et al., 2010a; Trinquier et al., 2007) point to large scale spatial and/or temporal isotopic heterogeneity in the solar protoplanetary disk. Two explanations for these variations have been proposed, with important implications for the formation of the Solar System: heterogeneous seeding of the disk with dust from a supernova, or energetic-particle irradiation of dust in the disk. The key to differentiating between them is identification of the carrier(s) of the 54Cr anomalies. Here we report the results of our recent Nano…
Late infall of molecular cloud material reshaped the outer Solar System
Centre for Star and Planet Formation, Globe Institute, University of Copenhagen（哥本哈根大学环球学院恒星与行星形成中心）；School of Earth Sciences, University of Bristol（布里斯托大学地球科学学院）
