The surface $^{210}$Pb is one of the main background sources for dark-matter-search experiments using NaI(Tl) crystals, and its spectral features associated with the beta-decay events for energies less than 60 keV depends on the depth distribution of $^{210}$Pb in the surface of an NaI(Tl) crystal. Therefore, we must understand the profile of surface $^{210}$Pb to precisely model the background measurement in the low-energy region for the low-background experiment using NaI(Tl) crystals. We estimate the depth profile of the surface $^{210}$Pb contamination by modeling the measured spectrum of the alpha emission from the decay of $^{210}$Po at the decay sequence of the surface $^{210}$Pb contamination that is obtained using an $^{222}$Rn-contaminated crystal. In order to describe the energy spectra of the surface contamination we perform a log-likelihood fit of the measured data to a sum of Geant4 Mote Carlo simulations, weighted by an exponential curve as a function of the surface depth. The low- and high-energy events from the beta decay of surface $^{210}$Pb are also modeled to improve the depth profile for shallow depths. We simulate the energy spectra from beta decays of $^{210}$Pb that are exponentially distributed in the surface by following two exponential functions where the mean-depth coefficients are free parameters in the data fitting; we observed that the energy spectra are in good agreement with the measured data.
Scintillating NaI(Tl) crystals are used for various rare decay experiments, such as dark matter searches. The hygroscopicity of NaI(Tl) crystal makes the construction of crystal detectors in these experiments challenging and requires a tight encapsulation to prevent from air contact. More importantly, in a low radioactivity measurement, identification of external radiations and surface contamination is crucial to characterize the origin of total crystal radioactivities. Studies for NaI(Tl) crystal encapsulation with active organic scintillator vetoes have been performed to mitigate the above-m…
We have developed ultra-low-background NaI(Tl) crystals to reproduce the DAMA results with the ultimate goal of achieving purity levels that are comparable to or better than those of the DAMA/LIBRA crystals. Even though the achieved background level does not approach that of DAMA/LIBRA, it is crucial to have a quantitative understanding of the backgrounds. We have studied background simulations toward a deeper understanding of the backgrounds and developed background models for a 9.16-kg NaI(Tl) crystal used in the test arrangement. In this paper we describe the contributions of background sou…
Among the direct search experiments for WIMP dark matter, the DAMA experiment observed an annual modulation signal interpreted as WIMP interactions with 9.2$σ$ significance. However, this result is contradictory with other direct search experiments reporting null signals in the same parameter space allowed by the DAMA observation, necessitating clarification of the origin of the modulation signal observed using the NaI(Tl) crystals of the DAMA experiment independently. Here, we report the first results of NaI(Tl) crystal measurement at the Yangyang Underground Laboratory to grow ultra-low-back…
The Korea Invisible Mass Search (KIMS) collaboration has developed low-background NaI(Tl) crystals that are suitable for the direct detection of WIMP dark matter. With experience built on the KIMS-CsI programs, the KIMS-NaI experiment will consist of a 200~kg NaI(Tl) crystal array surrounded by layers of shielding structures and will be operated at the Yangyang underground laboratory. The goal is to provide an unambiguous test of the DAMA/LIBRA's annual modulation signature. Measurements of six prototype crystals show progress in the reduction of internal contaminations of radioisotopes. Based…
The COSINE-100 dark matter search experiment is an array of NaI(Tl) crystal detectors located in the Yangyang Underground Laboratory (Y2L). To understand measured backgrounds in the NaI(Tl) crystals we have performed Monte Carlo simulations using the Geant4 toolkit and developed background models for each crystal that consider contributions from both internal and external sources, including cosmogenic nuclides. The background models are based on comparisons of measurement data with Monte Carlo simulations that are guided by a campaign of material assays and are used to evaluate backgrounds and…
Testing the DAMA/LIBRA annual modulation result independently of dark matter particle and halo models has been a challenge for twenty years. Using the same target material, NaI(Tl), is required and presently two experiments, ANAIS-112 and COSINE-100, are running for such a goal. A precise knowledge of the detector response to nuclear recoils is mandatory because this is the most likely channel to find the dark matter signal. The light produced by nuclear recoils is quenched with respect to that produced by electrons by a factor that has to be measured experimentally. However, current quenching…
The COSINE-100 experiment has been operating with 106 kg of low-background NaI(Tl) detectors to test the results from the DAMA/LIBRA experiment, which claims to have observed dark matter. However, since the background of the NaI(Tl) crystals used in the COSINE-100 experiment is 2-3 times higher than that in the DAMA detectors, no conclusion regarding the claimed observation from the DAMA/LIBRA experiment could be reached. Therefore, we plan to upgrade the current COSINE-100 experiment to the next phase, COSINE-200, by using ultra-low background NaI(Tl) detectors. The basic principle was alread…
We investigate a hypothesis that energy accumulation and the subsequent release in NaI(Tl) may lead to pulse-like events in the few-keV energy regime, a phenomenon suggested by the crystal manufacturing company Saint-Gobain, who provided the crystals for DAMA-LIBRA. While we observed delayed long-lasting light emission in a 3" NaI(Tl) crystal after exposing it to UV light, the delayed light consists primarily of single photons that are uncorrelated with each other. We also observe delayed light emission in NaI(Tl) following gamma radiation and large ionization events like cosmic-ray muons. We …
We report on the response of a high light-output NaI(Tl) crystal to nuclear recoils induced by neutrons from an Am-Be source and compare the results with the response to electron recoils produced by Compton scattered 662 keV $γ$-rays from a $^{137}$Cs source. The measured pulse-shape discrimination (PSD) power of the NaI(Tl) crystal is found to be significantly improved because of the high light output of the NaI(Tl) detector. We quantify the PSD power with a quality factor and estimate the sensitivity to the interaction rate for weakly interacting massive particles (WIMPs) with nucleons, and …
Scintillating NaI(Tl) crystals are widely used in a large variety of experimental applications. However, for the use as Dark Matter (DM) detectors, such crystals demand a high level of radio-purity, not achievable by means of standard industrial techniques. One of the main difficulties comes from the presence of potassium that always accompanies sodium in alkali halides. On the other hand, the arguable DM detection by DAMA experiment using NaI(Tl) scintillating crystals requires a reliable verification able to either confirm the existence of DM or rule out the DAMA claim. Ultra-low radioactivi…
Using a narrow band positron beam, the response of a large high-resolution NaI(Tl) crystal to an incident positron beam was measured. It was found that nuclear interactions cause the appearance of additional peaks in the low energy tail of the deposited energy spectrum.
Scintillation characteristics of a thallium doped sodium iodide (NaI(Tl)) crystal with a dimension of 0.6 x 0.6 x 2 cm3 are studied by attaching a silicon photomultiplier (SiPM) direct to the crystal over a temperature range from 93 to 300 K. The scintillation light output and decay time are measured by irradiating 59.54 keV gamma-rays from a 241Am source. We observed approximately 20% increase in light yield at 230K compared to that at the room temperature. At this condition, the NaI(Tl) crystal coupled with the SiPM can be a good candidate for future dark matter search detector.
Thallium-doped sodium iodide (NaI(Tl)) crystals are widely used in radiation detection applications, from gamma-ray spectroscopy to particle dark matter searches. However, if the crystal is exposed to relative humidity of even a few percent, its light emission degrades, making the crystal impractical as a detector. Surrounding the crystal with organic scintillators not only protects the surface of the crystal from humid air but also offers a new capability to tag backgrounds such as external gamma rays and surface contaminations. We developed a detector that is constructed by fully encasing a …
The annual modulation of scintillation event rate observed by the DAMA/LIBRA experiment has been a long-standing controversy in the quest of the direct detection of dark matter. The effort to definitively confirm or refute the annual modulation has turned out to be challenging due to the lack of NaI(Tl) crystals with high enough radio-purity. Most recently, we successfully grew a 6-kg ingot free from contamination during growth, from which a 3.4-kg crystal scintillator was made. The $^{39}$K concentration in the final crystal is estimated to be 4.3$\pm$0.2~ppb, unprecedented for NaI(Tl) crysta…
KIMS-NaI is a direct detection experiment searching for Weakly Interacting Massive Particles (WIMP) via their scattering off of nuclei in a NaI(Tl) crystal. The KIMS-NaI collaboration has carried out tests of six crystals in the Yangyang underground laboratory in order to develope low-background NaI(Tl) crystals. Studies of internal backgrounds crystals have been performed with the goal of reducing backgrounds levels to 1 dru at 2 keV. Pulse shape discrimination (PSD) capabilities were also investigated for distinguishing between WIMP nuclear recoil signals and electron recoil backgrounds. The…
Preventing quart-NaI adhesion in Bridgman growth using ammonium iodide
Kyungpook National University（庆北国立大学）；Center for High Energy Physics, Kyungpook National University（庆北国立大学高能物理中心）；Abdul Wali Khan University Mardan（马尔丹阿卜杜勒瓦利汗大学）；Institute for Basic Science (IBS)（基础科学研究院）；Damavan Imaging（达马万成像）
We report the measurement of muons and muon-induced phosphorescence in DM-Ice17, a NaI(Tl) direct detection dark matter experiment at the South Pole. Muon interactions in the crystal are identified by their observed pulse shape and large energy depositions. The measured muon rate in DM-Ice17 is 2.93 +/- 0.04 muons/crystal/day with a modulation amplitude of 12.3 +/- 1.7%, consistent with expectation. Following muon interactions, we observe long-lived phosphorescence in the NaI(Tl) crystals with a decay time of 5.5 +/- 0.5 s. The prompt energy deposited by a muon is correlated to the amount of d…
NaI(Tl) large crystals are applied in the search for galactic dark matter particles through their elastic scattering off the target nuclei in the detector by measuring the scintillation signal produced. However, energies deposited in the form of nuclear recoils are small, which added to the low efficiency to convert that energy into scintillation, makes that events at or very near the energy threshold, attributed either to radioactive backgrounds or to spurious noise (non-bulk NaI(Tl) scintillation events), can compromise the sensitivity goals of such an experiment. DAMA/LIBRA experiment, usin…
The annual modulation signal observed by the DAMA experiment is a long-standing question in the community of dark matter direct detection. This necessitates an independent verification of its existence using the same detection technique. The COSINE-100 experiment has been operating with 106~kg of low-background NaI(Tl) detectors providing interesting checks on the DAMA signal. However, due to higher backgrounds in the NaI(Tl) crystals used in COSINE-100 relative to those used for DAMA, it was difficult to reach final conclusions. Since the start of COSINE-100 data taking in 2016, we also have …
NaI(Tl) crystals are used as particle detectors in a variety of rare-event search experiments because of their superb light-emission quality. The crystal light yield is generally high, above 10 photoelectrons per keV, and its emission spectrum is peaked around 400 nm, which matches well to the sensitive region of bialkali photocathode photomultiplier tubes. However, since NaI(Tl) crystals are hygroscopic, a sophisticated method of encapsulation has to be applied that prevents moisture from chemically attacking the crystal and thereby degrading the emission. In addition, operation with low ener…
Scintillation crystals are commonly used for direct detection of weakly interacting massive particles (WIMPs), which are suitable candidates for a particle dark matter. It is well known that the scintillation light yields are different for electron recoil and nuclear recoil. To calibrate the energies of WIMP-induced nuclear recoil signals, the quenching factor (QF) needs to be measured, which is the light yield ratio of the nuclear recoil to electron recoil. Measurements of the QFs for Na and I recoils in a small (2 cm x 2 cm x 1.5 cm) NaI(Tl) crystal are performed with 2.43-MeV mono-energetic…
Scintillators play an important role in radiation detection and imaging. Thallium-doped cesium iodide (CsI:Tl) and sodium iodide (NaI:Tl) are two of the major scintillators that have been used for many applications for many decades. In this paper we will present an improved scintillation performance of Bridgman method grown CsI(Tl) and NaI(Tl) crystals developed by Xtallized Intelligence, Inc. (XI, Inc.) and we will compare the performance with commercially available CsI:Tl and NaI:Tl. In a preliminary testing using MicroFJ-60035-TSV silicon photomultipliers (ON Semiconductor), the newly devel…
We present new results on the radiopurity of a 3.4-kg NaI(Tl) crystal scintillator operated in the SABRE proof-of-principle detector setup. The amount of potassium contamination, determined by the direct counting of radioactive $^{40}$K, is found to be $2.2\pm1.5$ ppb, lowest ever achieved for NaI(Tl) crystals. With the active veto, the average background rate in the crystal in the 1-6 keV energy region-of-interest (ROI) is $1.20\pm0.05$ counts/day/kg/keV, which is a breakthrough since the DAMA/LIBRA experiment. Our background model indicates that the rate is dominated by $^{210}$Pb and that a…
Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low $^{39}$K contamination of 4.3$\pm$0.2 ppb as determined by mass spectrometry. We mea…
Limits on the cross section for weakly interacting massive particles (WIMPs) scattering off nucleons in the NaI(Tl) detectors at the Yangyang Underground Laboratory are obtained with a 2967.4 kg*day data exposure. Nuclei recoiling are identified by the pulse shape of scintillating photon signals. Data are consistent with no nuclear recoil hypothesis, and 90% confidence level upper limits are set. These limits partially exclude the DAMA/LIBRA region of WIMP-sodium interaction with the same NaI(Tl) target detector. This 90% confidence level upper limit on WIMP-nucleon spin-independent cross sect…
Very large thallium doped sodium iodide crystals operated underground and in very low background environment in the context of a dark matter search experiment have been used to determine scintillation components in the tens of ms range in the light pulse induced by different interacting particles: gammas/muons and alphas.
PICOLON (Pure Inorganic Crystal Observatory for LOw-energy Neutr(al)ino) aims to search for cosmic dark matter by high purity NaI(Tl) scintillator. We developed extremely pure NaI(Tl) crystal by hybrid purification method. The recent result of $^{210}$Pb in our NaI(Tl) is less than 5.7 $μ$Bq/kg. We will report the test experiment in the low-background measurement at Kamioka Underground Laboratory. The sensitivity for annual modulating signals and finding dark matter particles will be discussed.
The ANAIS (Annual modulation with NaI(Tl) Scintillators) experiment aims at the confirmation of the DAMA/LIBRA positive annual modulation signal using the same target and technique at the Canfranc Underground Laboratory (LSC). A first step, named ANAIS-25 (two 12.5 kg NaI(Tl) modules) taking data from December 2012 to February 2015, provided interesting outcomes: very high light collection efficiency, that could allow to lower the analysis energy threshold down to the level of 1 keVee, and a good understanding of the different background components, in particular the cosmogenic activated isoto…
We present the responses of a NaI(Tl) crystal in terms of the light yield and pulse shape characteristics of nuclear recoil events at two different temperatures: 22 C (room temperature) and -35 C (low temperature). The light yield is measured using 59.54 keV gamma-rays using a 241Am source relative to the mean charge of single photoelectrons. At the low temperature, we measure a 4.7 +/- 1.3% increase in the light yield compared to that at room temperature. A significantly increased decay time is also observed at the low temperature. The responses to nuclear recoil events are measured using neu…
The cosmogenic production of long-lived radioactive isotopes in materials is an hazard for experiments demanding ultra-low background conditions. Although NaI(Tl) scintillators have been used in this context for a long time, very few activation data were available. We present results from two 12.5 kg NaI(Tl) detectors, developed within the ANAIS project and installed at the Canfranc Underground Laboratory. The prompt data taking starting made possible a reliable quantification of production of some I, Te and Na isotopes with half-lives larger than ten days. Initial activities underground were …
Upgrade of NaI(Tl) crystal encapsulation for the NEON experiment
Seoul National University（首尔大学）；Institute for Basic Science (IBS)（韩国基础科学研究院）；University of Science and Technology (UST)（科学技术联合大学院大学）；Korea Atomic Energy Research Institute（韩国原子能研究所）；Chung-Ang University（中央大学）
We demonstrate the linearity and stability of a gamma-ray scintillation detector comprised of a NaI(Tl) crystal and a scientific-grade CMOS camera. After calibration, this detector exhibits excellent linearity more than three decades of activity levels. Because the detector is not counting pulses, no dead-time correction is required. When high activity sources are brought into close proximity to the NaI crystal, several minutes are required for the scintillation to achieve a steady state. On longer time scales, we measure drifts of a few percent over several days. These instabilities have impo…
In this paper results of scintillation properties measurements of pure and Ce3+-doped strontium fluoride crystals are presented. We measure light output, scintillation decay time profile and temperature stability of light output. X-ray excited luminescence outputs corrected for spectral response of monochromator and photomultiplier for pure SrF2 and SrF2-0.3 mol.% Ce3+ are approximately 95% and 115% of NaI-Tl emission output, respectively. A photopeak with a 10% full width at half maximum is observed at approximately 84% the light output of a NaI-Tl crystal after correction for spectral respon…
We report on a measurement of the neutron detection efficiency in NaI crystals in the Crystal Ball detector obtained from a study of single p0 photoproduction on deuterium using the tagged photon beam at the Mainz Microtron. The results were obtained up to a neutron energy of 400 MeV. They are compared to previous measurements made more than 15 years ago at the pion beam at the BNL AGS.
Measurements of the quenching factor for sodium recoils in a 5 cm diameter NaI(Tl) crystal at room temperature have been made at a dedicated neutron facility at the University of Sheffield. The crystal has been exposed to 2.45 MeV mono-energetic neutrons generated by a Sodern GENIE 16 neutron generator, yielding nuclear recoils of energies between 10 and 100 keVnr. A cylindrical BC501A detector has been used to tag neutrons that scatter off sodium nuclei in the crystal. Cuts on pulse shape and time of flight have been performed on pulses recorded by an Acqiris DC265 digitiser with a 2 ns sampl…
We have performed measurements of sodium nuclear recoils in NaI:Tl crystals, following scattering by neutrons produced in a $^{7}$Li(p,n)$^{7}$Be reaction. Understanding the light output from such recoils, which is reduced relative to electrons of equivalent energy by the quenching factor, is critical to interpret dark matter experiments that search for nuclear scattering interactions. We have developed a spectrum-fitting methodology to extract the quenching factor from our measurements, and report quenching factors for nuclear recoil energies between 36 and 401 keV. Our results agree with oth…
A new experimental evaluation of the quenching factor for nuclear recoils in NaI[Tl] is described. Systematics affecting previous measurements are addressed by careful characterization of the emission spectrum of the neutron source, use of a small scintillator coupled to an ultra-bialkali high quantum efficiency photomultiplier, and evaluation of non-linearities in the electron recoil response via Compton scattering. A trend towards a rapidly diminishing quenching factor with decreasing sodium recoil energy is revealed. Additionally, no evidence for crystal lattice channeling of low-energy rec…
ANAIS (Annual modulation with NaI Scintillators) is a project aiming to set up at the new facilities of the Canfranc Underground Laboratory (LSC), a large scale NaI(Tl) experiment in order to explore the DAMA/LIBRA annual modulation positive result using the same target and technique. Two 12.5 kg each NaI(Tl) crystals provided by Alpha Spectra took data at the LSC in the ANAIS-25 set-up. The comparison of the background model for the ANAIS-25 prototypes with the experimental results is presented. ANAIS crystal radiopurity goals have been achieved for Th-232 and U-238 chains, but a Pb-210 conta…
The importance is emphasized of taking into account the channeling along the low index crystallographic axes and planes of a part of low-energy (1-10 keV) recoil ions in measurements of their parameters with crystal scintillators of the type of NaI(Tl) etc. Because the nucleus stopping power in channels is low as compared with electronic stopping power, the light yield of the scintillator must be, accordingly, higher in the given case than that for ions having higher energy (tens keV and more), which lose most part of their energy via nuclear collisions outside channels. Hence, in particular, …
A thorough understanding of the background sources is mandatory in any experiment searching for rare events. The ANAIS (Annual Modulation with NaI(Tl) Scintillators) experiment aims at the confirmation of the DAMA/LIBRA signal at the Canfranc Underground Laboratory (LSC). Two NaI(Tl) crystals of 12.5 kg each produced by Alpha Spectra have been taking data since December 2012. The complete background model of these detectors and more precisely in the region of interest will be described. Preliminary background analysis of a new 12.5 kg crystal received at Canfranc in March 2015 will be presente…
The scintillation mechanism in NaI:Tl crystals produces different pulse shapes that are dependent on the incoming particle type. The time distribution of scintillation light from nuclear recoil events decays faster than for electron recoil events and this difference can be categorised using various Pulse Shape Discrimination (PSD) techniques. In this study, we measured nuclear and electron recoils in a NaI:Tl crystal, with electron equivalent energies between 2 and 40 keV. We report on a new PSD approach, based on an event-type likelihood; this outperforms the charge-weighted mean-time, which …
The production of long-lived radioactive isotopes in materials due to the exposure to cosmic rays on Earth surface can be an hazard for experiments demanding ultra-low background conditions, typically performed deep underground. Production rates of cosmogenic isotopes in all the materials present in the experimental set-up, as well as the corresponding cosmic rays exposure history, must be both well known in order to assess the relevance of this effect in the achievable sensitivity of a given experiment. Although NaI(Tl) scintillators are being used in experiments aiming at the direct detectio…
Application of NaI(Tl) detectors in the search for galactic dark matter particles through their elastic scattering off the target nuclei is well motivated because of the long standing DAMA/LIBRA highly significant positive result on annual modulation, still requiring confirmation. For such a goal, it is mandatory to reach very low threshold in energy (at or below the keV level), very low radioactive background (at a few counts/keV/kg/day), and high detection mass (at or above the 100 kg scale). One of the most relevant technical issues is the optimization of the crystal intrinsic scintillation…
Among the direct search experiments for weakly interacting massive particle (WIMP) dark matter, the DAMA experiment observed an annual modulation signal interpreted as WIMP interactions with a significance of 9.2$σ$. Recently, Jonathan Davis claimed that the DAMA modulation may be interpreted on the basis of the neutron scattering events induced by the muons and neutrinos together. We tried to simulate the neutron backgrounds at the Gran Sasso and Yangyang laboratory with and without the polyethylene shielding to quantify the effects of the ambient neutrons on the direct detection experiments …
Development and Initial Performance of an Upgraded NaI(Tl) Crystal Encapsulation for COSINE-100U
Kyungpook National University（庆北国立大学）；Chung-Ang University（中央大学）；Institute for Basic Science（基础科学研究院）；University of Science and Technology（科学技术大学）；Seoul National University（首尔国立大学）；Jeju National University（济州国立大学）；Carnegie Mellon University（卡内基梅隆大学）
ANAIS (Annual modulation with NAI Scintillators) experiment aims to look for dark matter annual modulation with 250 kg of ultrapure NaI(Tl) scintillators at the Canfranc Underground Laboratory (LSC), in order to confirm the DAMA/LIBRA positive signal in a model-independent way. The detector will consist in an array of close-packed single modules, each of them coupled to two high efficiency Hamamatsu photomultipliers. Two 12.5 kg each NaI(Tl) crystals provided by Alpha Spectra are currently taking data at the LSC. These modules have shown an outstanding light collection efficiency (12-16 phe/ke…
