We present the responses of a NaI(Tl) crystal in terms of the light yield and pulse shape characteristics of nuclear recoil events at two different temperatures: 22 C (room temperature) and -35 C (low temperature). The light yield is measured using 59.54 keV gamma-rays using a 241Am source relative to the mean charge of single photoelectrons. At the low temperature, we measure a 4.7 +/- 1.3% increase in the light yield compared to that at room temperature. A significantly increased decay time is also observed at the low temperature. The responses to nuclear recoil events are measured using neutrons from a 252Cf source and compared to those to electron recoil events. The measured pulse shape discrimination (PSD) power of the NaI(Tl) crystal at the low temperature is found to be improved in the entire energy range studied because of the increased light yield and the different scintillation characteristics. We also find an approximately 9% increased quenching factor of alpha-induced events, which is the light yield ratio of alpha recoil to electron recoil, at the low temperature. This supports the possibility of an increased quenching factor of the nuclear recoil events that are known to have similar processes of dark matter interaction. The increased light yield and the improved PSD power of nuclear recoil events enhance the sensitivity for dark matter detection via dark matter-nuclei interactions.
Using a narrow band positron beam, the response of a large high-resolution NaI(Tl) crystal to an incident positron beam was measured. It was found that nuclear interactions cause the appearance of additional peaks in the low energy tail of the deposited energy spectrum.
Scintillation characteristics of a thallium doped sodium iodide (NaI(Tl)) crystal with a dimension of 0.6 x 0.6 x 2 cm3 are studied by attaching a silicon photomultiplier (SiPM) direct to the crystal over a temperature range from 93 to 300 K. The scintillation light output and decay time are measured by irradiating 59.54 keV gamma-rays from a 241Am source. We observed approximately 20% increase in light yield at 230K compared to that at the room temperature. At this condition, the NaI(Tl) crystal coupled with the SiPM can be a good candidate for future dark matter search detector.
Thallium-doped sodium iodide (NaI(Tl)) crystals are widely used in radiation detection applications, from gamma-ray spectroscopy to particle dark matter searches. However, if the crystal is exposed to relative humidity of even a few percent, its light emission degrades, making the crystal impractical as a detector. Surrounding the crystal with organic scintillators not only protects the surface of the crystal from humid air but also offers a new capability to tag backgrounds such as external gamma rays and surface contaminations. We developed a detector that is constructed by fully encasing a …
KIMS-NaI is a direct detection experiment searching for Weakly Interacting Massive Particles (WIMP) via their scattering off of nuclei in a NaI(Tl) crystal. The KIMS-NaI collaboration has carried out tests of six crystals in the Yangyang underground laboratory in order to develope low-background NaI(Tl) crystals. Studies of internal backgrounds crystals have been performed with the goal of reducing backgrounds levels to 1 dru at 2 keV. Pulse shape discrimination (PSD) capabilities were also investigated for distinguishing between WIMP nuclear recoil signals and electron recoil backgrounds. The…
The annual modulation of scintillation event rate observed by the DAMA/LIBRA experiment has been a long-standing controversy in the quest of the direct detection of dark matter. The effort to definitively confirm or refute the annual modulation has turned out to be challenging due to the lack of NaI(Tl) crystals with high enough radio-purity. Most recently, we successfully grew a 6-kg ingot free from contamination during growth, from which a 3.4-kg crystal scintillator was made. The $^{39}$K concentration in the final crystal is estimated to be 4.3$\pm$0.2~ppb, unprecedented for NaI(Tl) crysta…
Among the direct search experiments for WIMP dark matter, the DAMA experiment observed an annual modulation signal interpreted as WIMP interactions with 9.2$σ$ significance. However, this result is contradictory with other direct search experiments reporting null signals in the same parameter space allowed by the DAMA observation, necessitating clarification of the origin of the modulation signal observed using the NaI(Tl) crystals of the DAMA experiment independently. Here, we report the first results of NaI(Tl) crystal measurement at the Yangyang Underground Laboratory to grow ultra-low-back…
Limits on the cross section for weakly interacting massive particles (WIMPs) scattering off nucleons in the NaI(Tl) detectors at the Yangyang Underground Laboratory are obtained with a 2967.4 kg*day data exposure. Nuclei recoiling are identified by the pulse shape of scintillating photon signals. Data are consistent with no nuclear recoil hypothesis, and 90% confidence level upper limits are set. These limits partially exclude the DAMA/LIBRA region of WIMP-sodium interaction with the same NaI(Tl) target detector. This 90% confidence level upper limit on WIMP-nucleon spin-independent cross sect…
Testing the DAMA/LIBRA annual modulation result independently of dark matter particle and halo models has been a challenge for twenty years. Using the same target material, NaI(Tl), is required and presently two experiments, ANAIS-112 and COSINE-100, are running for such a goal. A precise knowledge of the detector response to nuclear recoils is mandatory because this is the most likely channel to find the dark matter signal. The light produced by nuclear recoils is quenched with respect to that produced by electrons by a factor that has to be measured experimentally. However, current quenching…
A thorough understanding of the background sources is mandatory in any experiment searching for rare events. The ANAIS (Annual Modulation with NaI(Tl) Scintillators) experiment aims at the confirmation of the DAMA/LIBRA signal at the Canfranc Underground Laboratory (LSC). Two NaI(Tl) crystals of 12.5 kg each produced by Alpha Spectra have been taking data since December 2012. The complete background model of these detectors and more precisely in the region of interest will be described. Preliminary background analysis of a new 12.5 kg crystal received at Canfranc in March 2015 will be presente…
NaI(Tl) crystals are used as particle detectors in a variety of rare-event search experiments because of their superb light-emission quality. The crystal light yield is generally high, above 10 photoelectrons per keV, and its emission spectrum is peaked around 400 nm, which matches well to the sensitive region of bialkali photocathode photomultiplier tubes. However, since NaI(Tl) crystals are hygroscopic, a sophisticated method of encapsulation has to be applied that prevents moisture from chemically attacking the crystal and thereby degrading the emission. In addition, operation with low ener…
The COSINE-100 experiment has been operating with 106 kg of low-background NaI(Tl) detectors to test the results from the DAMA/LIBRA experiment, which claims to have observed dark matter. However, since the background of the NaI(Tl) crystals used in the COSINE-100 experiment is 2-3 times higher than that in the DAMA detectors, no conclusion regarding the claimed observation from the DAMA/LIBRA experiment could be reached. Therefore, we plan to upgrade the current COSINE-100 experiment to the next phase, COSINE-200, by using ultra-low background NaI(Tl) detectors. The basic principle was alread…
Scintillating NaI(Tl) crystals are used for various rare decay experiments, such as dark matter searches. The hygroscopicity of NaI(Tl) crystal makes the construction of crystal detectors in these experiments challenging and requires a tight encapsulation to prevent from air contact. More importantly, in a low radioactivity measurement, identification of external radiations and surface contamination is crucial to characterize the origin of total crystal radioactivities. Studies for NaI(Tl) crystal encapsulation with active organic scintillator vetoes have been performed to mitigate the above-m…
Upgrade of NaI(Tl) crystal encapsulation for the NEON experiment
Seoul National University（首尔大学）；Institute for Basic Science (IBS)（韩国基础科学研究院）；University of Science and Technology (UST)（科学技术联合大学院大学）；Korea Atomic Energy Research Institute（韩国原子能研究所）；Chung-Ang University（中央大学）
We investigate a hypothesis that energy accumulation and the subsequent release in NaI(Tl) may lead to pulse-like events in the few-keV energy regime, a phenomenon suggested by the crystal manufacturing company Saint-Gobain, who provided the crystals for DAMA-LIBRA. While we observed delayed long-lasting light emission in a 3" NaI(Tl) crystal after exposing it to UV light, the delayed light consists primarily of single photons that are uncorrelated with each other. We also observe delayed light emission in NaI(Tl) following gamma radiation and large ionization events like cosmic-ray muons. We …
We report on the response of a high light-output NaI(Tl) crystal to nuclear recoils induced by neutrons from an Am-Be source and compare the results with the response to electron recoils produced by Compton scattered 662 keV $γ$-rays from a $^{137}$Cs source. The measured pulse-shape discrimination (PSD) power of the NaI(Tl) crystal is found to be significantly improved because of the high light output of the NaI(Tl) detector. We quantify the PSD power with a quality factor and estimate the sensitivity to the interaction rate for weakly interacting massive particles (WIMPs) with nucleons, and …
Scintillating NaI(Tl) crystals are widely used in a large variety of experimental applications. However, for the use as Dark Matter (DM) detectors, such crystals demand a high level of radio-purity, not achievable by means of standard industrial techniques. One of the main difficulties comes from the presence of potassium that always accompanies sodium in alkali halides. On the other hand, the arguable DM detection by DAMA experiment using NaI(Tl) scintillating crystals requires a reliable verification able to either confirm the existence of DM or rule out the DAMA claim. Ultra-low radioactivi…
We present new results on the radiopurity of a 3.4-kg NaI(Tl) crystal scintillator operated in the SABRE proof-of-principle detector setup. The amount of potassium contamination, determined by the direct counting of radioactive $^{40}$K, is found to be $2.2\pm1.5$ ppb, lowest ever achieved for NaI(Tl) crystals. With the active veto, the average background rate in the crystal in the 1-6 keV energy region-of-interest (ROI) is $1.20\pm0.05$ counts/day/kg/keV, which is a breakthrough since the DAMA/LIBRA experiment. Our background model indicates that the rate is dominated by $^{210}$Pb and that a…
The dark matter search project by means of ultra high purity NaI(Tl) scintillator is now underdevelopment. An array of large volume NaI(Tl) detectors whose volume is 12.7 cm$ϕ\times$12.7 cm is applied to search for dark matter signal. To remove radioactive impurities in NaI(Tl) crystal is one of the most important task to find small number of dark matter signals. We have developed high purity NaI(Tl) crystal which contains small amounts of radioactive impurities, $<4$ ppb of $^{nat}$K, 0.3 ppt of Th chain, 58 $μ$Bq/kg of $^{226}$Ra and 30 $μ$Bq/kg of $^{210}$Pb. Future prospects to search for …
Thin and large area NaI(Tl) scintillator to search for WIMPs dark matter was developed. The performance of thin and wide area NaI(Tl) showed good enough to search for dark matter. The energy threshold was as low as 2keV and the energy resolution was about 24% in FWHM at 60keV.
A new experimental evaluation of the quenching factor for nuclear recoils in NaI[Tl] is described. Systematics affecting previous measurements are addressed by careful characterization of the emission spectrum of the neutron source, use of a small scintillator coupled to an ultra-bialkali high quantum efficiency photomultiplier, and evaluation of non-linearities in the electron recoil response via Compton scattering. A trend towards a rapidly diminishing quenching factor with decreasing sodium recoil energy is revealed. Additionally, no evidence for crystal lattice channeling of low-energy rec…
The R&D project COSINUS (Cryogenic Observatory for SIgnatures seen in Next-generation Underground Searches) aims to develop a cryogenic scintillating calorimeter using NaI as target crystal for direct darkmatter search. Dark matter particles interacting with the detector material generate both a phonon signal and scintillation light. While the phonon signal provides a precise determination of the deposited energy, the simultaneously measured scintillation light allows for a particle identification on an event-by-event basis, a powerful tool to study material-dependent interactions, and to supp…
Among the direct search experiments for weakly interacting massive particle (WIMP) dark matter, the DAMA experiment observed an annual modulation signal interpreted as WIMP interactions with a significance of 9.2$σ$. Recently, Jonathan Davis claimed that the DAMA modulation may be interpreted on the basis of the neutron scattering events induced by the muons and neutrinos together. We tried to simulate the neutron backgrounds at the Gran Sasso and Yangyang laboratory with and without the polyethylene shielding to quantify the effects of the ambient neutrons on the direct detection experiments …
The Korea Invisible Mass Search (KIMS) collaboration has developed low-background NaI(Tl) crystals that are suitable for the direct detection of WIMP dark matter. With experience built on the KIMS-CsI programs, the KIMS-NaI experiment will consist of a 200~kg NaI(Tl) crystal array surrounded by layers of shielding structures and will be operated at the Yangyang underground laboratory. The goal is to provide an unambiguous test of the DAMA/LIBRA's annual modulation signature. Measurements of six prototype crystals show progress in the reduction of internal contaminations of radioisotopes. Based…
The cosmogenic production of long-lived radioactive isotopes in materials is an hazard for experiments demanding ultra-low background conditions. Although NaI(Tl) scintillators have been used in this context for a long time, very few activation data were available. We present results from two 12.5 kg NaI(Tl) detectors, developed within the ANAIS project and installed at the Canfranc Underground Laboratory. The prompt data taking starting made possible a reliable quantification of production of some I, Te and Na isotopes with half-lives larger than ten days. Initial activities underground were …
We have developed ultra-low-background NaI(Tl) crystals to reproduce the DAMA results with the ultimate goal of achieving purity levels that are comparable to or better than those of the DAMA/LIBRA crystals. Even though the achieved background level does not approach that of DAMA/LIBRA, it is crucial to have a quantitative understanding of the backgrounds. We have studied background simulations toward a deeper understanding of the backgrounds and developed background models for a 9.16-kg NaI(Tl) crystal used in the test arrangement. In this paper we describe the contributions of background sou…
Preventing quart-NaI adhesion in Bridgman growth using ammonium iodide
Kyungpook National University（庆北国立大学）；Center for High Energy Physics, Kyungpook National University（庆北国立大学高能物理中心）；Abdul Wali Khan University Mardan（马尔丹阿卜杜勒瓦利汗大学）；Institute for Basic Science (IBS)（基础科学研究院）；Damavan Imaging（达马万成像）
We report the measurement of muons and muon-induced phosphorescence in DM-Ice17, a NaI(Tl) direct detection dark matter experiment at the South Pole. Muon interactions in the crystal are identified by their observed pulse shape and large energy depositions. The measured muon rate in DM-Ice17 is 2.93 +/- 0.04 muons/crystal/day with a modulation amplitude of 12.3 +/- 1.7%, consistent with expectation. Following muon interactions, we observe long-lived phosphorescence in the NaI(Tl) crystals with a decay time of 5.5 +/- 0.5 s. The prompt energy deposited by a muon is correlated to the amount of d…
NaI(Tl) large crystals are applied in the search for galactic dark matter particles through their elastic scattering off the target nuclei in the detector by measuring the scintillation signal produced. However, energies deposited in the form of nuclear recoils are small, which added to the low efficiency to convert that energy into scintillation, makes that events at or very near the energy threshold, attributed either to radioactive backgrounds or to spurious noise (non-bulk NaI(Tl) scintillation events), can compromise the sensitivity goals of such an experiment. DAMA/LIBRA experiment, usin…
The annual modulation signal observed by the DAMA experiment is a long-standing question in the community of dark matter direct detection. This necessitates an independent verification of its existence using the same detection technique. The COSINE-100 experiment has been operating with 106~kg of low-background NaI(Tl) detectors providing interesting checks on the DAMA signal. However, due to higher backgrounds in the NaI(Tl) crystals used in COSINE-100 relative to those used for DAMA, it was difficult to reach final conclusions. Since the start of COSINE-100 data taking in 2016, we also have …
We present the first search for a dark matter annual modulation signal in the Southern Hemisphere conducted with NaI(Tl) detectors, performed by the DM-Ice17 experiment. Nuclear recoils from dark matter interactions are expected to yield an annually modulated signal independent of location within the Earth's hemispheres. DM-Ice17, the first step in the DM-Ice experimental program, consists of 17 kg of NaI(Tl) located at the South Pole under 2200 m.w.e. overburden of Antarctic glacial ice. Taken over 3.6 years for a total exposure of 60.8 kg yr, DM-Ice17 data are consistent with no modulation i…
A high purity and large volume NaI(Tl) scintillator was developed to search for cosmic dark matter. The required densities of radioactive impurities (RIs) such as U-chain, Th-chain are less than a few ppt to establish high sensitivity to dark matter. The impurity of RIs were effectively reduced by selecting raw materials of crucible and by performing chemical reduction of lead ion in NaI raw powder. The impurity of $^{226}$Ra was reduced less than 100 $μ$Bq/kg in NaI(Tl) crystal. It should be remarked that the impurity of $^{210}$Pb, which is difficult to reduce, is effectively reduced by chem…
A dark matter search project needs and extremely low background radiation detector since the expected event rate of dark matter is less than a few events in one year in one tonne of the detector mass. The authors developed a highly radiopure NaI(Tl) crystal to search for dark matter. The best combination of the purification methods was developed, resulting $^{\mathrm{nat}}$K and $^{210}$Pb were less than 20 ppb and 5.7 $μ$Bq/kg, respectively. The authors will construct a large volume detector system with high-purity NaI(Tl) crystals. The design and the performance of the prototype detector mod…
We report on a measurement of the neutron detection efficiency in NaI crystals in the Crystal Ball detector obtained from a study of single p0 photoproduction on deuterium using the tagged photon beam at the Mainz Microtron. The results were obtained up to a neutron energy of 400 MeV. They are compared to previous measurements made more than 15 years ago at the pion beam at the BNL AGS.
Scintillation crystals are commonly used for direct detection of weakly interacting massive particles (WIMPs), which are suitable candidates for a particle dark matter. It is well known that the scintillation light yields are different for electron recoil and nuclear recoil. To calibrate the energies of WIMP-induced nuclear recoil signals, the quenching factor (QF) needs to be measured, which is the light yield ratio of the nuclear recoil to electron recoil. Measurements of the QFs for Na and I recoils in a small (2 cm x 2 cm x 1.5 cm) NaI(Tl) crystal are performed with 2.43-MeV mono-energetic…
Scintillators play an important role in radiation detection and imaging. Thallium-doped cesium iodide (CsI:Tl) and sodium iodide (NaI:Tl) are two of the major scintillators that have been used for many applications for many decades. In this paper we will present an improved scintillation performance of Bridgman method grown CsI(Tl) and NaI(Tl) crystals developed by Xtallized Intelligence, Inc. (XI, Inc.) and we will compare the performance with commercially available CsI:Tl and NaI:Tl. In a preliminary testing using MicroFJ-60035-TSV silicon photomultipliers (ON Semiconductor), the newly devel…
The surface $^{210}$Pb is one of the main background sources for dark-matter-search experiments using NaI(Tl) crystals, and its spectral features associated with the beta-decay events for energies less than 60 keV depends on the depth distribution of $^{210}$Pb in the surface of an NaI(Tl) crystal. Therefore, we must understand the profile of surface $^{210}$Pb to precisely model the background measurement in the low-energy region for the low-background experiment using NaI(Tl) crystals. We estimate the depth profile of the surface $^{210}$Pb contamination by modeling the measured spectrum of …
At present the results in the field of direct dark matter search are in tension: the positive claim of DAMA/LIBRA versus null results from other experiments. However, the comparison of the results of different experiments involves model dependencies, in particular because of the different target materials in use. The COSINUS R&D project aims to operate NaI as a cryogenic calorimeter. Such a detector would not only allow for a direct comparison to DAMA/LIBRA, but would also provide a low(er) nuclear recoil threshold and particle discrimination.
Recently there is a flourishing and notable interest in the crystalline scintillator material sodium iodide (NaI) as target for direct dark matter searches. This is mainly driven by the long-reigning contradicting situation in the dark matter sector: the positive evidence for the detection of a dark matter modulation signal claimed by the DAMA/LIBRA collaboration is (under so-called standard assumptions) inconsistent with the null-results reported by most of the other direct dark matter experiments. We present the results of a first prototype detector using a new experimental approach in compa…
The highly radiopure NaI(Tl) was developed to search for particle candidates of dark matter. The optimized methods were combined to reduce various radioactive impurities. The $^{40}$K was effectively reduced by the re-crystallization method. The progenies of the decay chains of uranium and thorium were reduced by appropriate resins. The concentration of natural potassium in NaI(Tl) crystal was reduced down to 20 ppb. Concentrations of alpha-ray emitters were successfully reduced by appropriate selection of resin. The present concentration of thorium series and 226Ra were $1.2 \pm1.4$ $μ$Bq/kg …
Development and Initial Performance of an Upgraded NaI(Tl) Crystal Encapsulation for COSINE-100U
Kyungpook National University（庆北国立大学）；Chung-Ang University（中央大学）；Institute for Basic Science（基础科学研究院）；University of Science and Technology（科学技术大学）；Seoul National University（首尔国立大学）；Jeju National University（济州国立大学）；Carnegie Mellon University（卡内基梅隆大学）
The COSINE-100 dark matter search experiment is an array of NaI(Tl) crystal detectors located in the Yangyang Underground Laboratory (Y2L). To understand measured backgrounds in the NaI(Tl) crystals we have performed Monte Carlo simulations using the Geant4 toolkit and developed background models for each crystal that consider contributions from both internal and external sources, including cosmogenic nuclides. The background models are based on comparisons of measurement data with Monte Carlo simulations that are guided by a campaign of material assays and are used to evaluate backgrounds and…
Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low $^{39}$K contamination of 4.3$\pm$0.2 ppb as determined by mass spectrometry. We mea…
We present preliminary results of measurements of the quenching factor for Na recoils in NaI(Tl) at room temperature, made at a dedicated neutron facility at the University of Sheffield. Measurements have been performed with a 2.45 MeV mono-energetic neutron generator in the energy range from 10 keV to 100 keV nuclear recoil energy. A BC501A liquid scintillator detector was used to tag neutrons. Cuts on pulse-shape discrimination from the BC501A liquid scintillator detector and neutron time-of-flight were performed on pulses recorded by a digitizer with a 2 ns sampling time. Measured quenching…
In order to test the capabilities of Barium Fluoride (BaF2) Crystal for dark matter direct detection, nuclear recoils are studied with mono-energetic neutron beam. The energy spectra of nuclear recoils, quenching factors for elastic scattering neutrons and discrimination capability between neutron inelastic scattering events and γ events are obtained for various recoil energies of the F content in BaF2.
The inorganic crystals have been widely used for dark matter direct searching for many decades. However, limited by the crystal growth technique, a lot of small crystals have to be used together for large target mass, which results in a degradation of light collection efficiency. An experiment was built up to study the degradation, and the method of soaking crystals into mineral oil to improve the efficiency as well as reduce the interface effect were proposed and validated. Good data and MC agreements were achieved in the experiment.
We demonstrate the linearity and stability of a gamma-ray scintillation detector comprised of a NaI(Tl) crystal and a scientific-grade CMOS camera. After calibration, this detector exhibits excellent linearity more than three decades of activity levels. Because the detector is not counting pulses, no dead-time correction is required. When high activity sources are brought into close proximity to the NaI crystal, several minutes are required for the scintillation to achieve a steady state. On longer time scales, we measure drifts of a few percent over several days. These instabilities have impo…
The scintillation light output of a pure and a Thallium doped Sodium Iodide (NaI) crystal under irradiation with 5.486MeV α-particles has been measured over a temperature range from 1.7K to 300K. Estimates of the decay time constant at three selected temperatures are given. For pure NaI an increase in light yield towards low temperatures could be confirmed and measured at higher precision. For NaI(Tl) below 60K an increase in light output has been found.
