Measurements of the quenching factor for sodium recoils in a 5 cm diameter NaI(Tl) crystal at room temperature have been made at a dedicated neutron facility at the University of Sheffield. The crystal has been exposed to 2.45 MeV mono-energetic neutrons generated by a Sodern GENIE 16 neutron generator, yielding nuclear recoils of energies between 10 and 100 keVnr. A cylindrical BC501A detector has been used to tag neutrons that scatter off sodium nuclei in the crystal. Cuts on pulse shape and time of flight have been performed on pulses recorded by an Acqiris DC265 digitiser with a 2 ns sampling time. Measured quenching factors of Na nuclei range from 19% to 26% in good agreement with other experiments, and a value of 25.2 \pm 6.4% has been determined for 10 keV sodium recoils. From pulse shape analysis, the mean times of pulses from electron and nuclear recoils have been compared down to 2 keVee. The experimental results are compared to those predicted by Lindhard theory, simulated by the SRIM Monte Carlo code, and a preliminary curve calculated by Prof. Akira Hitachi.
We have performed measurements of sodium nuclear recoils in NaI:Tl crystals, following scattering by neutrons produced in a $^{7}$Li(p,n)$^{7}$Be reaction. Understanding the light output from such recoils, which is reduced relative to electrons of equivalent energy by the quenching factor, is critical to interpret dark matter experiments that search for nuclear scattering interactions. We have developed a spectrum-fitting methodology to extract the quenching factor from our measurements, and report quenching factors for nuclear recoil energies between 36 and 401 keV. Our results agree with oth…
We analyzed the response of NaI(Tl) to low energy nuclear recoils in the experiment that is reported on here. Such detectors have been used recently to search for evidence of dark matter in the form of weakly interacting massive particles (WIMPs). Understanding the response of these detectors to low energy nuclear recoils is crucial in these searches. We have measured nuclear recoils and associated quenching factors (QF) for sodium recoils in the energy range of 8 keV - 48 keV. The results are characterized by a decrease in QF as the recoil energy decreases. The measured values are significant…
Scintillation crystals are commonly used for direct detection of weakly interacting massive particles (WIMPs), which are suitable candidates for a particle dark matter. It is well known that the scintillation light yields are different for electron recoil and nuclear recoil. To calibrate the energies of WIMP-induced nuclear recoil signals, the quenching factor (QF) needs to be measured, which is the light yield ratio of the nuclear recoil to electron recoil. Measurements of the QFs for Na and I recoils in a small (2 cm x 2 cm x 1.5 cm) NaI(Tl) crystal are performed with 2.43-MeV mono-energetic…
We present preliminary results of measurements of the quenching factor for Na recoils in NaI(Tl) at room temperature, made at a dedicated neutron facility at the University of Sheffield. Measurements have been performed with a 2.45 MeV mono-energetic neutron generator in the energy range from 10 keV to 100 keV nuclear recoil energy. A BC501A liquid scintillator detector was used to tag neutrons. Cuts on pulse-shape discrimination from the BC501A liquid scintillator detector and neutron time-of-flight were performed on pulses recorded by a digitizer with a 2 ns sampling time. Measured quenching…
There is considerable experimental effort dedicated to the directional detection of particle dark matter. Gaseous mu-TPC detectors present the privileged features of being able to reconstruct the track and the energy of the recoil nucleus following the interaction. A precise measurement of the recoil energy is a key point for the directional search strategy. Quenching has to be taken into account, i.e. only a certain fraction of the recoil energy is deposited in the ionization channel. Measurements of the ionization quenching factor for different gas mixture at room temperature have been made …
The dark matter interpretation of the DAMA modulation signal depends on the NaI(Tl) scintillation efficiency of nuclear recoils. Previous measurements for Na recoils have large discrepancies, especially in the DAMA/LIBRA modulation energy region. We report a quenching effect measurement of Na recoils in NaI(Tl) from 3keV$_{\text{nr}}$ to 52keV$_{\text{nr}}$, covering the whole DAMA/LIBRA energy region for light WIMP interpretations. By using a low-energy, pulsed neutron beam, a double time-of-flight technique, and pulse-shape discrimination methods, we obtained the most accurate measurement of…
A new experimental evaluation of the quenching factor for nuclear recoils in NaI[Tl] is described. Systematics affecting previous measurements are addressed by careful characterization of the emission spectrum of the neutron source, use of a small scintillator coupled to an ultra-bialkali high quantum efficiency photomultiplier, and evaluation of non-linearities in the electron recoil response via Compton scattering. A trend towards a rapidly diminishing quenching factor with decreasing sodium recoil energy is revealed. Additionally, no evidence for crystal lattice channeling of low-energy rec…
This article reports the measurement of the ionization quenching factor in germanium for nuclear recoil energies between 0.4 and 6.3 keV$_{nr}$. Precise knowledge of this factor in this energy range is relevant for coherent elastic neutrino-nucleus scattering and low mass dark matter searches with germanium-based detectors. Nuclear recoils were produced in a thin high-purity germanium target with a very low energy threshold via irradiation with monoenergetic neutron beams. The energy dependence of the ionization quenching factor was directly measured via kinematically constrained coincidences …
We present a model of the ionization efficiency, or quenching factor, for low-energy nuclear recoils, based on a solution to Lindhard integral equation with binding energy and apply it to the calculation of the relative scintillation efficiency and charge yield for nuclear recoils in noble liquid detectors. The quenching model incorporates a constant average binding energy together with an electronic stopping power proportional to the ion velocity, and is an essential input in an analysis of charge recombination processes to predict the ionization and scintillation yields. Our results are comp…
We examine a recent measurement of the quenching factor (QF) in germanium at 80 K, noticing a number of inconsistencies capable of affecting a claimed agreement with Lindhard's ion-stopping formalism in the sub-keV nuclear recoil energy regime. Namely, an underestimated uncertainty in the energy scale and a missing correction for a large instrumental non-linearity in this scale able to severely distort the QF behavior at low energy, favoring reduced values. The discussion is expanded to inspect the impact of QF model selection on a study of neutrino electromagnetic properties using CE$ν$NS dat…
The scintillation mechanism in NaI:Tl crystals produces different pulse shapes that are dependent on the incoming particle type. The time distribution of scintillation light from nuclear recoil events decays faster than for electron recoil events and this difference can be categorised using various Pulse Shape Discrimination (PSD) techniques. In this study, we measured nuclear and electron recoils in a NaI:Tl crystal, with electron equivalent energies between 2 and 40 keV. We report on a new PSD approach, based on an event-type likelihood; this outperforms the charge-weighted mean-time, which …
Organic liquid scintillators are used in a wide variety of applications in experimental nuclear and particle physics. Boron-loaded scintillators are particularly useful for detecting neutron captures, due to the high thermal neutron capture cross section of $^{10}$B. These scintillators are commonly used in neutron detectors, including the DarkSide-50 neutron veto, where the neutron may produce a signal when it scatters off protons in the scintillator or when it captures on $^{10}$B. Reconstructing the energy of these recoils is complicated by scintillation quenching. Understanding how nuclear…
We employ an $^{88}$Y/Be photoneutron source to derive the quenching factor for neutron-induced nuclear recoils in germanium, probing recoil energies from a few hundred eV$_{nr}$ to 8.5keV$_{nr}$. A comprehensive Monte Carlo simulation of our setup is compared to experimental data employing a Lindhard model with a free electronic energy loss $k$ and an adiabatic correction for sub-keV$_{nr}$ nuclear recoils. The best fit $k=0.179\pm 0.001$ obtained using a Monte Carlo Markov Chain (MCMC) ensemble sampler is in good agreement with previous measurements, confirming the adequacy of the Lindhard m…
We present the responses of a NaI(Tl) crystal in terms of the light yield and pulse shape characteristics of nuclear recoil events at two different temperatures: 22 C (room temperature) and -35 C (low temperature). The light yield is measured using 59.54 keV gamma-rays using a 241Am source relative to the mean charge of single photoelectrons. At the low temperature, we measure a 4.7 +/- 1.3% increase in the light yield compared to that at room temperature. A significantly increased decay time is also observed at the low temperature. The responses to nuclear recoil events are measured using neu…
We report on the response of a high light-output NaI(Tl) crystal to nuclear recoils induced by neutrons from an Am-Be source and compare the results with the response to electron recoils produced by Compton scattered 662 keV $γ$-rays from a $^{137}$Cs source. The measured pulse-shape discrimination (PSD) power of the NaI(Tl) crystal is found to be significantly improved because of the high light output of the NaI(Tl) detector. We quantify the PSD power with a quality factor and estimate the sensitivity to the interaction rate for weakly interacting massive particles (WIMPs) with nucleons, and …
Linear alkylbenzene has been recently used as the solvent of liquid scintillator by several neutrino experiments. The energy quenching effect of a linear alkylbenzene based liquid scintillator is studied in this paper with a 14 MeV D-T compact neutron generator, to improve the energy non-linearity modelling of this kind of detectors. The recoiled proton in the liquid scintillator has a kinetic energy ranging from 0.5 MeV to 13 MeV. The data is used to extract the parameters of the Birk's law, an empirical model to describe the energy quenching effect of the liquid scintillator.
Testing the DAMA/LIBRA annual modulation result independently of dark matter particle and halo models has been a challenge for twenty years. Using the same target material, NaI(Tl), is required and presently two experiments, ANAIS-112 and COSINE-100, are running for such a goal. A precise knowledge of the detector response to nuclear recoils is mandatory because this is the most likely channel to find the dark matter signal. The light produced by nuclear recoils is quenched with respect to that produced by electrons by a factor that has to be measured experimentally. However, current quenching…
The scintillation yields of ZnWO$_4$ crystals change depending on the incident direction of particles. This property can be used as a direction-sensitive dark matter detector. So, we investigated the ZnWO$_4$ light yields ratio of neutron-induced nuclear recoils to gamma-ray induced electron recoils(quenching factor). Two surfaces almost perpendicular to the crystal axis of ZnWO$_4$ were irradiated with a quasi-monochromatic neutron beam of 0.885MeV, and the quenching factors of both surfaces for the oxygen-nucleus recoil in the ZnWO$_4$ crystal were measured. The obtained quenching factors of…
The organic liquid scintillator used in the LVD experiment (INFN Gran Sasso National Laboratory) has been exposed to an Am-Be neutron source to measure the light response function for neutron energies in the region from about 4 to 11 MeV. A full Monte Carlo simulation, incorporating the detector response, is used to generate neutron scattering spectra which are matched to the observed ones to determine the quenching factors. The obtained light output response is well described by the semi-empirical Birks model. The results, consistent with those obtained by other authors using similar hydrocar…
Dark matter particles scattering off some target nuclei are expected to deposit very small energies in form of nuclear recoils (below 100 keV). Because of the low scintillation efficiency for nuclear recoils vs. electron recoils, in most of the scintillating targets considered in the search for dark matter, the region below 10 keVee concentrates most of the expected dark matter signal. For this reason, very low energy threshold (at or below 2 keVee) and very low background are required. This is the case of the ANAIS (Annual modulation with NaI Scintillators) experiment. A good knowledge of the…
KIMS-NaI is a direct detection experiment searching for Weakly Interacting Massive Particles (WIMP) via their scattering off of nuclei in a NaI(Tl) crystal. The KIMS-NaI collaboration has carried out tests of six crystals in the Yangyang underground laboratory in order to develope low-background NaI(Tl) crystals. Studies of internal backgrounds crystals have been performed with the goal of reducing backgrounds levels to 1 dru at 2 keV. Pulse shape discrimination (PSD) capabilities were also investigated for distinguishing between WIMP nuclear recoil signals and electron recoil backgrounds. The…
We study the basic integral equation in Lindhard's theory describing the energy given to atomic motion by nuclear recoils in a pure material when the atomic binding energy is taken into account. The numerical solution, which depends only on the slope of the velocity-proportional electronic stopping power and the binding energy, leads to an estimation of the ionization efficiency which is in good agreement with the available experimental measurements for Si and Ge. In this model, the quenching factor for nuclear recoils features a cut-off at an energy equal to twice the assumed binding energy. …
In order to test the capabilities of Barium Fluoride (BaF2) Crystal for dark matter direct detection, nuclear recoils are studied with mono-energetic neutron beam. The energy spectra of nuclear recoils, quenching factors for elastic scattering neutrons and discrimination capability between neutron inelastic scattering events and γ events are obtained for various recoil energies of the F content in BaF2.
Limits on the cross section for weakly interacting massive particles (WIMPs) scattering off nucleons in the NaI(Tl) detectors at the Yangyang Underground Laboratory are obtained with a 2967.4 kg*day data exposure. Nuclei recoiling are identified by the pulse shape of scintillating photon signals. Data are consistent with no nuclear recoil hypothesis, and 90% confidence level upper limits are set. These limits partially exclude the DAMA/LIBRA region of WIMP-sodium interaction with the same NaI(Tl) target detector. This 90% confidence level upper limit on WIMP-nucleon spin-independent cross sect…
Background: Organic scintillators are widely used for neutron detection in both basic nuclear physics and applications. While the proton light yield of organic scintillators has been extensively studied, measurements of the light yield from neutron interactions with carbon nuclei are scarce. Purpose: Demonstrate a new approach for the simultaneous measurement of the proton and carbon light yield of organic scintillators. Provide new carbon light yield data for the EJ-309 liquid and EJ-204 plastic organic scintillators. Method: A 33~MeV $^{2}$H$^{+}$ beam from the 88-Inch Cyclotron at Lawrence …
Anisotropic scintillators can offer a unique possibility to exploit the so-called directionality approach in order to investigate the presence of those Dark Matter (DM) candidates inducing nuclear recoils. In fact, their use can overcome the difficulty of detecting extremely short nuclear recoil traces. In this paper we present recent measurements performed on the anisotropic response of a ZnWO$_4$ crystal scintillator to nuclear recoils, in the framework of the ADAMO project. The anisotropic features of the ZnWO$_4$ crystal scintillators were initially measured with $α$ particles; those resul…
We have studied channeling effects in a Cesium Iodide (CsI) crystal that is similar in composition to the ones being used in a search for Weakly Interacting Massive Particles (WIMPs) dark matter candidates, and measured its energy-dependent quenching factor, the relative scintillation yield for electron and nuclear recoils. The experimental results are reproduced with a GEANT4 simulation that includes a model of the scintillation efficiency as a function of electronic stopping power. We present the measured and simulated quenching factors and the estimated effects of channeling.
The importance is emphasized of taking into account the channeling along the low index crystallographic axes and planes of a part of low-energy (1-10 keV) recoil ions in measurements of their parameters with crystal scintillators of the type of NaI(Tl) etc. Because the nucleus stopping power in channels is low as compared with electronic stopping power, the light yield of the scintillator must be, accordingly, higher in the given case than that for ions having higher energy (tens keV and more), which lose most part of their energy via nuclear collisions outside channels. Hence, in particular, …
In recent decades, inorganic crystals have been widely used in dark matter direct search experiments. To contribute to the understanding of the capabilities of $CsI(Na)$ and $CaF_{2}(Eu)$ crystals, a mono-energetic neutron beam is utilized to study the properties of nuclear recoils, which are expected to be similar to signals of dark matter direct detection. The quenching factor of nuclear recoils in $CsI(Na)$ and $CaF_{2}(Eu)$, as well as an improved discrimination factor between nuclear recoils and $γ$ backgrounds in $CsI(Na)$, are reported.
The ZnWO$_4$ is an anisotropic crystal scintillator; for its peculiar characteristics, it is a very promising detector to exploit the so-called directionality approach in the investigation of those Dark Matter (DM) candidates inducing nuclear recoils. Recently, in the framework of the ADAMO project, an R\&D to develop high quality and ultra-radiopure ZnWO$_4$ crystal scintillators has been carried out. In the present paper the measurements to study the anisotropic response of a ZnWO$_4$ to $α$ particles and to nuclear recoils induced by neutron scattering are reported. Monochromatic neutrons h…
Scintillation response of cryogenic CsI to few-keV and sub-keV nuclear recoils
University of Chicago（芝加哥大学）；Donostia International Physics Center (DIPC)（多诺西亚国际物理中心）；Ikerbasque, Basque Foundation for Science（伊克尔巴斯基克，巴斯克科学基金会）；Instituto de Física Corpuscular, CSIC & Universitat de València（粒子物理研究所，西班牙国家科学研究委员会与瓦伦西亚大学）
The Korea Invisible Mass Search (KIMS) collaboration has developed low-background NaI(Tl) crystals that are suitable for the direct detection of WIMP dark matter. With experience built on the KIMS-CsI programs, the KIMS-NaI experiment will consist of a 200~kg NaI(Tl) crystal array surrounded by layers of shielding structures and will be operated at the Yangyang underground laboratory. The goal is to provide an unambiguous test of the DAMA/LIBRA's annual modulation signature. Measurements of six prototype crystals show progress in the reduction of internal contaminations of radioisotopes. Based…
Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low $^{39}$K contamination of 4.3$\pm$0.2 ppb as determined by mass spectrometry. We mea…
The low-energy monochromatic neutron emission from an Y-88/Be source can be exploited to mimic the few keVnr nuclear recoils expected from low-mass Weakly Interacting Massive Particles (WIMPs) and coherent scattering of neutrinos off nuclei. Using this source, a ~<10% quenching factor is measured for sodium recoils below 24 keVnr in NaI[Tl]. This is considerably smaller than the 30% typically adopted in the interpretation of the DAMA/LIBRA dark matter experiment, resulting in a marked increase of its tension with other searches, under the standard set of phenomenological assumptions. The metho…
There is a long standing debate about whether or not the annual modulation signal reported by the DAMA/LIBRA collaboration is induced by Weakly Interacting Massive Particles~(WIMP) in the galaxy's dark matter halo scattering from nuclides in their NaI(Tl) crystal target/detector. This is because regions of WIMP-mass vs. WIMP-nucleon cross-section parameter space that can accommodate the DAMA/LIBRA-phase1 modulation signal in the context of the standard WIMP dark matter galactic halo and isospin-conserving~(canonical), spin-independent~(SI) WIMP-nucleon interactions have been excluded by many o…
Liquid argon is used as active medium in a variety of neutrino and Dark Matter experiments thanks to its excellent properties of charge yield and transport and as a scintillator. Liquid argon scintillation photons are emitted in a narrow band of 10~nm centered around 127 nm and with a characteristic time profile made by two components originated by the decay of the lowest lying singlet and triplet state of the excimer Ar$_2^*$ to the dissociative ground state. A model is proposed which takes into account the quenching of the long lived triplet states through the self-interaction with other tri…
Radionuclide Identification Devices (RIDs) or Backpack Radiation Detection Systems (BRDs) are often equipped with NaI(Tl) detectors. We demonstrate that such instruments could be provided with reasonable thermal- and fast-neutron sensitivity by means of an improved and sophisticated processing of the digitized detector signals: Fast neutrons produce nuclear recoils in the scintillation crystal. Corresponding signals are detectible and can be distinguished from that of electronic interactions by pulse-shape discrimination (PSD) techniques as used in experiments searching for weakly interacting …
In order to measure energy and fluence of neutron fields, with energy ranging from 8 keV to 1 MeV, a new primary standard is being developed at the IRSN (Institute for Radioprotection and Nuclear Safety). This project, micro-TPC (Micro Time Projection Chamber), carried out in collaboration with the LPSC, is based on the nucleus recoil detector principle. The measurement strategy requires track reconstruction of recoiling nuclei down to a few keV, which can be achieved with a low pressure gaseous detector using a micro-pattern gaseous detector. A gas mixture, mainly isobutane, is used as a n-p …
The $α$-particle light response of liquid scintillators based on linear alkylbenzene (LAB) has been measured with three different experimental approaches. In the first approach, $α$-particles were produced in the scintillator via $^{12}$C($n$,$α$)$^9$Be reactions. In the second approach, the scintillator was loaded with 2% of $^{\mathrm{nat}}$Sm providing an $α$-emitter, $^{147}$Sm, as an internal source. In the third approach, a scintillator flask was deployed into the water-filled SNO+ detector and the radioactive contaminants $^{222}$Rn, $^{218}$Po and $^{214}$Po provided the $α$-particle s…
NaI(Tl) large crystals are applied in the search for galactic dark matter particles through their elastic scattering off the target nuclei in the detector by measuring the scintillation signal produced. However, energies deposited in the form of nuclear recoils are small, which added to the low efficiency to convert that energy into scintillation, makes that events at or very near the energy threshold, attributed either to radioactive backgrounds or to spurious noise (non-bulk NaI(Tl) scintillation events), can compromise the sensitivity goals of such an experiment. DAMA/LIBRA experiment, usin…
