arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 1908.06450cond-mat.str-elcond-mat.mtrl-sci
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近场LaCrO3 LaFeO3体系的异常磁行为和复杂磁结构

Anomalous magnetic behavior and complex magnetic structure of proximate LaCrO3 LaFeO3 system

Brajesh Tiwari, Ambesh Dixit, M. S. Ramachandra Rao

摘要:

研究了多功能LaCrO_3-LaFeO_3体系的复合磁性。磁性测量证实存在竞争复杂的磁有序对温度,顺磁性铁磁过渡在300 K,其次是反铁磁(AFM)过渡近250 K叠加在亚铁磁相。弱亚铁磁有序的发生归因于两个AFM LaCrO 3-LaFeO 3亚晶格之间的竞争复杂的相互作用。低温AFM有序性也得到了温度依赖性拉曼测量的证实,其中700 cm-1拉曼活性模的强度比显示出明显的增强与降低温度。磁矩在LaCrO 3-LaFeO 6的非饱和性质表明,在250 K至300 K高达5 T的磁场之间,AFM有序与亚铁磁有序结合占主导地位。构建了LaCrO_3-LaFeO_3复合磁结构,强调了室温附近的亚稳磁相和低温反铁磁态。

英文摘要:

We investigated complex magnetic properties of multifunctional LaCrO3-LaFeO3 system. The magnetic measurements substantiate the presence of competing complex magnetic ordering against temperature, showing paramagnetic to ferrimagnetic transition at 300 K, followed by antiferromagnetic (AFM) transition near 250 K superimposed on ferrimagnetic phase. The onset of weak ferrimagnetic ordering is attributed to the competing complex interaction between two AFM LaCrO3-LaFeO3 sublattices. The low-temperature AFM ordering is also substantiated by temperature-dependent Raman measurements, where the intensity ratio of 700 cm-1 Raman active mode showed the clear enhancement with lowering the temperature. The non-saturating nature of magnetic moments in LaCrO3-LaFeO6 suggests the predominating AFM ordering in conjunction with ferrimagnetic ordering between 250 K to 300 K up to 5 T magnetic field. A complex magnetic structure of LaCrO3-LaFeO3 is constructed, emphasizing the metastable magnetic phase near room temperature and low temperature antiferromagnetic state.

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