Anomalous metals are observed in numerous experiments on disordered two-dimensional systems proximate to superconductivity. A characteristic feature of an anomalous metal is that its low temperature conductivity has a weakly temperature dependent value, significantly higher than that of a disordered Fermi liquid. We propose a dynamical mean-field model of an anomalous metal: interacting electrons similar in structure to that of the well-studied universal Hamiltonian of mesoscopic metallic grains, but with independent random interactions between pairs of sites, involving Cooper pair hopping and spin exchange. We find evidence for critical anomalous phases or points between a superconducting phase and a disordered Fermi liquid phase in this model. Our results are obtained by a renormalization group analysis in a weak coupling limit, and a complementary solution at large $M$ when the spin symmetry is generalized to USp($M$). The large $M$ limit describes the anomalous metal by fractionalization of the electron into spinons, holons, and doublons, with these partons forming critical non-Fermi liquids in the Sachdev-Ye-Kitaev class. We compute the low temperature conductivity in the large $M$ limit, and find temperature-independent values moderately enhanced from that in the disordered metal.
We propose a theory for quasi-two-dimensional transition metal dichalcogenides that provides a unified microscopic picture of the charge density wave (CDW) and superconducting phases. We show, based on the electron-phonon coupling and Fermi surface topology, that a CDW order parameter with six-fold symmetry and nodes (f-wave) gives a consistent description of the available experimental data. The elementary excitations in the CDW phase are Dirac electrons. The superconducting state has its origin on the attractive interaction mediated by phonons. The theory predicts strong deviations from Fermi…
We report high-temperature (300-1120 K) magnetization data of Fe and Fe3O4 nanoparticles embedded in multi-walled carbon nanotubes. The magnetic impurity concerntations are precisely determined by both high-energy synchrotron x-ray diffractometer and inductively coupled plasma mass spectrometer. We unambiguously show that the magnetic moments of Fe and Fe3O4 nanoparticles are enhanced by a factor of about 3 compared with what they would be expected to have for free (unembedded) magnetic nanoparticles. The magnetization enhancement factor is nearly independent of the applied magnetic field but …
Competing orders in condensed matter give rise to the emergence of fascinating, new phenomena. Here, we investigate the competition between superconductivity and charge density wave in the context of layered-metallic compounds, transition metal dichalcogenides, in which the superconducting state is usually suppressed by the charge density wave. We show, using real-space self-consistent Bogoliubov-de Gennes calculations and momentum-space calculations involving density-functional theory and dynamical mean-field theory, that there is a surprising reappearance of superconductivity in the presence…
We report magnetic and calorimetric measurements down to T = 1 mK on the canonical heavy-electron metal YbRh2Si2. The data reveal the development of nuclear antiferromagnetic order slightly above 2 mK. The latter weakens the primary electronic antiferromagnetism, thereby paving the way for heavy-electron superconductivity below Tc = 2 mK. Our results demonstrate that superconductivity driven by quantum criticality is a general phenomenon.
We compare predictions of the mean-field theory of superconductivity for nearly antiferromagnetic and nearly ferromagnetic metals in two dimensions. The calculations are based on a parametrization of the effective interaction arising from the exchange of magnetic fluctuations. The Eliashberg equations for the transition temperature are solved including the full momentum dependence of the self-energy. The results show that for comparable parameters d-wave singlet pairing in nearly antiferromagnetic metals is generally much stronger than p-wave triplet pairing in nearly ferromagnetic metals in q…
The electronic structure of Bi2Sr2-xRxCuOy(R=La, Eu) near the (pi,0) point of the first Brillouin zone was studied by means of angle-resolved photoemission spectroscopy (ARPES). The temperature T* above which the pseudogap structure in the ARPES spectrum disappears was found to have an R dependence that is opposite to that ofthe superconducting transition temperature Tc. This indicates that the pseudogap state is competing with high-Tc superconductivity, and the large Tc suppression observed with increasing the out-of-plane disorder is due to the stabilization of the pseudogap state.
The observation of flat energy bands in transition metal dichalcogenide bilayers such as twisted WSe${}_2$ makes those materials interesting prospects for reproducing the behavior observed in graphene-based systems. We use an effective Hubbard model providing a description of twisted WSe${}_2$ to explore the presence of superconductivity, which was previously reported in experiments. Using both the variational cluster approximation and cluster dynamical mean-field theory, we predict the existence of chiral supercondictivity of type $d\pm id$ that can be tuned by the twist angle and by the appl…
The proposed high-spin superconductivity in the half-Heusler compounds changes the landscape of superconductivity research. While superconducting instability is possible only in systems with quantum mechanically coherent quasiparticles, it has not been verified for any proposed high-spin Fermi surfaces. Here we report an observation of anomalous Shubnikov-de Haas effect in half-Heusler YPtBi, which is compatible with a coherent $j=3/2$ Fermi surface. The quantum oscillation (QO) signal in cubic YPtBi manifests extreme anisotropy upon rotation of the magnetic field from [100] to [110] crystallo…
Strange metallicity encompasses high magnetic field-induced superconductivity in UTe2
Charles University, Faculty of Mathematics and Physics（查理大学数学物理学院）；Hochfeld-Magnetlabor Dresden (HLD-EMFL), Helmholtz-Zentrum Dresden-Rossendorf（德累斯顿强磁场实验室（HLD-EMFL），德累斯顿罗森多夫亥姆霍兹中心）；Cavendish Laboratory, University of Cambridge（剑桥大学卡文迪许实验室）
We use scanning tunneling microscopy to investigate Bi2Sr2Ca2Cu3O10+δ trilayer cuprates from the optimally doped to overdoped regime. We find that the two distinct superconducting gaps from the inner and outer CuO2 planes both decrease rapidly with doping, in sharp contrast to the nearly constant Tc. Spectroscopic imaging reveals the absence of quasiparticle interference in the antinodal region of overdoped samples, showing an opposite trend to that in single- and double-layer compounds. We propose that the existence of two types of inequivalent CuO2 planes and the intricate interaction betwee…
We show that Floquet chiral topological superconductivity arises naturally in Josephson junctions made of magnetic topological insulator-superconductor sandwich structures. The Josephson phase modulation associated with an applied bias voltage across the junction drives the system into the anomalous Floquet chiral topological superconductor hosting chiral Majorana edge modes in the quasienergy spectrum, with the bulk Floquet bands carrying zero Chern numbers. The bias voltage acts as a tuning parameter enabling novel dynamical topological quantum phase transitions driving the system into a myr…
In the iron-based superconductors, understanding the relation between superconductivity and electronic structure upon doping is crucial for exploring the pairing mechanism. Recently it was found that in iron selenide (FeSe), enhanced superconductivity (Tc over 40K) can be achieved via electron doping, with the Fermi surface only comprising M-centered electron pockets. Here by utilizing surface potassium dosing, scanning tunneling microscopy/spectroscopy (STM/STS) and angle-resolved photoemission spectroscopy (ARPES), we studied the electronic structure and superconductivity of (Li0.8Fe0.2OH)Fe…
We consider a strongly spin-orbit-coupled metal, one of whose Fermi surfaces is close to a Lifshitz (topological) transition. Via a renormalization group analysis of the square-lattice Hubbard model with strong Rashba spin-orbit coupling, we show that such a metal is generically unstable to the formation of mixed-parity superconductivity with a helical triplet component.
Compelling evidence for band-type conductivity and even bulk superconductivity below $T\_{\text{c}}\approx 8$ K has been found in $^{69,71}$Ga-NMR experiments in crystalline ordered, giant Ga$\_{84}$ cluster-compounds. This material appears to represent the first realization of a theoretical model proposed by Friedel in 1992 for superconductivity in ordered arrays of weakly coupled, identical metal nanoparticles.
We investigate the behavior of weak ferromagnetic metals close to the ferromagnetic critical point. We show that in the limit of small magnetic moment the low temperature metallic phase is rigorously described by a local ferromagnetic Fermi liquid that has a momentum-independent self-energy. Whereas, non-Fermi liquid features develop at higher temperatures. Furthermore, we find that an instability towards s-wave superconductivity is possible when the exchange splitting is comparable to the superconducting gap.
Proximity to a Mott insulating phase is likely to be an important physical ingredient of a theory that aims to describe high-temperature superconductivity in the cuprates. Quantum cluster methods are well suited to describe the Mott phase. Hence, as a step towards a quantitative theory of the competition between antiferromagnetism (AFM) and d-wave superconductivity (SC) in the cuprates, we use Cellular Dynamical Mean Field Theory to compute zero temperature properties of the two-dimensional square lattice Hubbard model. The d-wave order parameter is found to scale like the superexchange coupli…
This article reviews recent results of magnetotransport and magnetization measurements performed on highly oriented pyrolitic graphite (HOPG) and single crystalline Kish graphite samples. Both metal-insulator and insulator-metal transitions driven by magnetic field applied perpendicular to the basal planes of graphite were found and discussed in the light of relevant theories. The results provide evidence for the existence of localized superconducting domains in HOPG even at room temperature, as well as an interplay between superconducting and ferromagnetic correlations. We also present experi…
Monovalent metals contain half filled band (HFB) of s-electrons. Emphasizing importance of Coulomb repulsions in HFB in 2D and 1D monovalent systems we sketched a theory (2018) for ambient temperature granular superconductivity reported by Thapa and Pandey (2018) in Au-Ag nanostructures (updated by Thapa et al., 2019). Sharpening our theory, we suggest that \textit{Coulomb repulsions in certain structurally perturbed regions (atomic clusters, stacking faults, grain boundaries etc.) create nanoscale reservoirs of singlet electron pairs}. These low dimensional patches are hybridized to a backgro…
When a Mott metal-insulator transition is inhibited by a small amount of disorder in the layered dichalcogenide 1T-TaS$_2$, an inhomogeneous superconducting state arises below T=2.1 K, and coexists with a nearly-commensurate charge-density-wave. By angle-resolved photoelectron spectroscopy (ARPES) we show that it emerges from a bad metal state with strongly damped quasiparticles. Superconductivity is almost entirely suppressed by an external magnetic field of 0.1 T.
Using the theory of the high temperature superconductivity based on the idea of the fermion condensation quantum phase transition (FCQPT), we show that neither the d-wave pairing symmetry, nor the pseudogap phenomenon, nor the presence of the Cu-O_2 planes are of decisive importance for the existence of the high-T_c superconductivity. We analyze recent experimental data on this type of superconductivity in different materials and show that these facts can be understood within the theory of superconductivity based on FCQPT. The latter can be considered as a universal cause of the high-T_c super…
We study the renormalization of the quasiparticle properties in weak ferromagnetic metals, due to spin fluctuations, away from the quantum critical point for small magnetic moment. We explain the origin of the s-wave superconducting instability in the ferromagnetic phase and find that the vertex corrections are small and Migdal's theorem is satisfied away from the quantum critical point.
The interdependence of antiferromagnetism and superconductivity in the Bechgaard salts series of organic conductors is examined in the light of the anomalous temperature dependence of the nuclear spin-lattice relaxation rate. We apply the renormalization group approach to the electron gas model to show that the crossover from antiferromagnetism to superconductivity along with the anomalous nuclear relaxation rate of the Bechgaard salts can be well described within a unified microscopic framework. For sizable nesting deviations of the Fermi surface, scaling theory reveals how pairing correlatio…
High-resolution x-ray diffraction measurements reveal an unusually strong response of the lattice to superconductivity in Ba[Fe(1-x)Cox]2As2. The orthorhombic distortion of the lattice is suppressed and, for Co-doping near x = 0.063, the orthorhombic structure evolves smoothly back to a tetragonal structure. We propose that the coupling between orthorhombicity and superconductivity is indirect and arises due to the magneto-elastic coupling, in the form of emergent nematic order, and the strong competition between magnetism and superconductivity.
Unusual properties of strongly correlated liquid observed in the high-$T_c$ superconductors and heavy-fermion (HF) metals are determined by quantum phase transitions taking place at their critical points. Therefore, direct experimental studies of these transitions and critical points are of crucial importance for understanding the physics of high-$T_c$ superconductors and HF metals. In case of high-$T_c$ superconductors such direct experimental studies are absent since at low temperatures corresponding critical points are occupied by the superconductivity. Recent experimental data on the behav…
We report $^{115}$In nuclear-quadrupole-resonance (NQR) measurements of the pressure($P$)-induced superconductor CeRhIn$_5$ in the antiferromagnetic (AF) and superconducting (SC) states. In the AF region, the internal field $H_{int}$ at the In site is substantially reduced from $H_{int}=1.75$ kOe at P=0 to 0.39 kOe at $P=1.23$ GPa, while the Néel temperature slightly changes with increasing $P$. This suggests that either the size in the ordered moment $M_{Q}(P)$ or the angle $θ(P)$ between the direction of $M_{Q}(P)$ and the tetragonal $c$ axis is extrapolated to zero at $P^*=1.6 \pm 0.1$ GPa …
A possibility of high, room-temperature superconductivity was predicted for metallic hydrogen in the 1960s. However, metallization and superconductivity of hydrogen are yet to be unambiguously demonstrated in the laboratory and may require pressures as high as 5 million atmospheres. Rare earth based "superhydrides" such as LaH10 can be considered a close approximation of metallic hydrogen even though they form at moderately lower pressures. In superhydrides the predominance of H-H metallic bonds and high superconducting transition temperatures bear the hallmarks of metallic hydrogen. Still, ex…
We use electrical transport, magnetoresistance, and heat capacity measurements on high quality single crystals of the recently discovered superconducting Type-II Dirac semi-metal PdTe$_2$, to probe the nature of it's superconducting phase. The magnitude of the electronic heat capacity anomaly at $T_c$, the low temperature exponential $T$ dependence of the heat capacity, and a conventional $H - T$ phase diagram establish that the superconductivity in PdTe$_2$ is conventional in nature despite the presence of a topologically non-trivial Fermi surface band which contributes to the electrical cond…
Here we report the observation of bulk superconductivity in single crystals of the two-dimensional kagome metal KV$_3$Sb$_5$. Magnetic susceptibility, resistivity, and heat capacity measurements reveal superconductivity below $T_c = 0.93$K, and density functional theory (DFT) calculations further characterize the normal state as a $\mathbb{Z}_2$ topological metal. Our results demonstrate that the recent observation of superconductivity within the related kagome metal CsV$_3$Sb$_5$ is likely a common feature across the AV$_3$Sb$_5$ (A: K, Rb, Cs) family of compounds and establish them as a rich…
We report bulk superconductivity at 2.5K in LaO0.5F0.5BiSe2 compound through the DC magnetic susceptibility and electrical resistivity measurements. The synthesized LaO0.5F0.5BiSe2 compound is crystallized in tetragonal structure with space group P4/nmm and Reitveld refined lattice parameters are a= 4.15(1)A and c=14.02(2)A. The lower critical field of Hc1= 40Oe, at temperature 2K is estimated through the low field magnetization measurements. The LaO0.5F0.5BiSe2 compound showed metallic normal state electrical resistivity with residual resistivity value of 1.35mΩ-cm. The compound is type-II su…
In this paper we address the question of coexistence of superconductivity and ferromagnetism in the high temperature superconductor RuSr$_2$GdCu$_2$O$_{8-δ}$. Using a field theoretical approach we study a one-fermion effective model of a ferromagnetic superconductor in which the quasiparticles responsible for the ferromagnetism form the Cooper pairs as well. We discuss the physical features which are different in this model and the standard BCS model and consider their experimental consequences.
In this review, we present a comprehensive overview of superconductivity in electron-doped metal nitride halides $M$N$X$ ($M$ = Ti, Zr, Hf; $X$ = Cl, Br, I) with layered crystal structure and two-dimensional electronic states. The parent compounds are band insulators with no discernible long-range ordered state. Upon doping tiny amount of electrons, superconductivity emerges with several anomalous features beyond the conventional electron-phonon mechanism, which stimulate theoretical investigations. We will discuss experimental and theoretical results reported thus far and compare the electron…
We have studied the charge dynamics of Sr-doped La2CuO4 at hole concentration p =0.07. We observed a clear indication of the competition between two new characteristic collective modes of the Wigner lattice orders suggested earlier: one corresponds to a Tc =15 K superconductivity and the other to Tc =30 K. Our results naturally explain the recent observation of metallic transport in extremely low (1%) Sr-doped La2CuO4 and establish a novel insulator to metal transition mechanismand superconductivity in the two-dimensional Wigner lattice ground state. We suggest that the fluctuations of the rel…
Significant manifestation of interplay of superconductivity and charge density wave, spin density wave or magnetism is dome-like variation in superconducting critical temperature (Tc) for cuprate, iron-based and heavy Fermion superconductors. Overall behavior is that the ordered temperature is gradually suppressed and the Tc is enhanced under external control parameters. Many phenomena like pesudogap, quantum critical point and strange metal emerge in the different doping range. Exploring dome-shaped Tc in new superconductors is of importance to detect emergent effects. Here, we report that th…
We study the emergence of multiband superconductivity with $s$- and $d-$wave symmetry on the background of spin density wave (SDW). We show that the SDW coherence factors renormalize the momentum dependence of the superconducting (SC) gap, yielding a SC state with an \emph{unconventional} s-wave symmetry. Interband Cooper pair scattering stabilizes superconductivity in both symmetries. With increasing SDW order, the s-wave state is more strongly suppressed than the d-wave state. Our results are universally applicable to two-dimensional systems with a commensurate SDW.
We study LiFeP, LiFeAs and NaFeAs in their paramagnetic metallic phase including dynamical electronic correlations within a density functional theory + slave-spin mean-field framework. The three compounds are found to lie next to the crossover between a normal and a Hund's metal, where a region of enhanced electronic compressibility that may boost superconductivity is systematically present in this type of systems. We find that LiFeP lies in the normal metallic regime, LiFeAs at the crossover, and NaFeAs is in the Hund's metal regime, which possibly explains the different experimental trends f…
In quantum materials, electrons that have strong correlations tend to localize, leading to quantum spins as the building blocks for low-energy physics. When strongly correlated electrons coexist with more weakly-correlated conduction electrons, multiple channels of effective interactions develop and compete with each other. The competition creates quantum fluctuations having a large spectral weight, with the associated entropies reaching significant fractions of $R\ln 2$ per electron. Advancing a framework to understand how the fluctuating local moments influence unconventional superconductivi…
Departing from the assumption that pairing is induced by an retarded external 'bosonic glue', we reformulate the Bardeen-Cooper-Schrieffer theory of superconductivity as a scaling theory. Conventional superconductors correspond with the asymptotically free case but the theory can be effortlessly generalized to handle quantum critical metals. We find that superconducting Tc's are strongly enhanced in the latter when retardation is strong while the coupling is weak. It appears that this simple scaling theory does account quite well for superconducting properties near quantum critical points.
Some of the highest-transition-temperature superconductors across various materials classes exhibit linear-in-temperature `strange metal' or `Planckian' electrical resistivities in their normal state. It is thus believed by many that this behavior holds the key to unlock the secrets of high-temperature superconductivity. However, these materials typically display complex phase diagrams governed by various competing energy scales, making an unambiguous identification of the physics at play difficult. Here we use electrical resistivity measurements into the micro-Kelvin regime to discover superc…
Superconductivity in low carrier density metals challenges the conventional electron-phonon theory due to the absence of retardation required to overcome Coulomb repulsion. In quantum critical polar metals, the Coulomb repulsion is heavily screened, while the critical transverse optic phonons decouple from the electron charge. In the resulting vacuum, the residual interactions between quasiparticles are carried by energy fluctuations of the polar medium, resembling the gravitational interactions of a dark matter universe. Here we demonstrate that pairing inevitably emerges from "gravitational'…
We have synthesized a novel europium bismuth sulfofluoride, Eu3Bi2S4F4, by solid-state reactions in sealed evacuated quartz ampoules. The compound crystallizes in a tetragonal lattice (space group I4/mmm, a = 4.0771(1) A, c = 32.4330(6) A, and Z = 2), in which CaF2-type Eu3F4 layers and NaCl-like BiS2 bilayers stack alternately along the crystallographic c axis. There are two crystallographically distinct Eu sites, Eu(1) and Eu(2) at the Wyckoff positions 4e and 2a, respectively. Our bond-valence-sum calculation, based on the refined structural data, indicates that Eu(1) is essentially divalen…
Many unconventional superconductors exhibit a common set of anomalous charge transport properties that characterize them as `strange metals', which provides hope that there is single theory that describes them. However, model-independent connections between the strange metal and superconductivity have remained elusive. In this letter, we show that the Hall effect of the unconventional superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$ contains an anomalous contribution arising from the correlations within the strange metal. This term has a distinctive dependence on magnetic field, which allows us to…
The nature of superconductivity in newly discovered Kagome materials, $\text{AV}_3\text{Sb}_5$ (A=K, Rb, Cs), has been a subject of intense debate. Recent experiments suggest the presence of orbital current order on top of the charge density wave (CDW) and superconductivity. Since the orbital current order breaks time-reversal symmetry, it may fundamentally affect possible superconducting states. In this work, we investigate the mutual influence between the orbital current order and superconductivity in Kagome metal with characteristic van Hove singularity (vHS). By explicitly deriving the Lan…
The emergence of superconductivity in unconventional superconductors usually accompanies the normal-state phases of pseudogap, strange metal and Fermi liquid. It indicates these phases are strongly related to the superconducting state and should be dominated by yet unclear mechanism of superconductivity. Here, we propose a microscopic theory that, according to the coupling between localized and extended states, the pairing electrons which leap on and off a localized state result in superconducting instability. Two distinguishable pairing gaps are observed in these states, one dominates the sup…
We argue that a single-band itinerant electron model with short-range interactions, proposed by Karchev et al. (cond-mat/9911489) and investigated further by Jackiewicz et al. (cond-mat/0302449), cannot describe the coexistence of superconducting and ferromagnetic order.
The quantum spin liquid candidate NaYbSe$_2$ was recently reported to exhibit a Mott transition under pressure. Superconductivity was observed in the high-pressure metallic phase, raising the question concerning its relation with the low-pressure quantum spin liquid ground state. Here we combine the density functional theory and the dynamical mean-field theory to explore the underlying mechanism of the insulator-to-metal transition and superconductivity and establish an overall picture of its electronic phases under pressure. Our results suggest that NaYbSe$_2$ is a charge-transfer insulator a…
We present a review of theoretical investigations into the Kohn-Luttinger nonphonon superconductivity mechanism in various 3D and 2D repulsive electron systems described by the Fermi-gas, Hubbard, and Shubin-Vonsovsky models. Phase diagrams of the superconducting state are considered, including regions of anomalous $s$-, $p$-, and $d$-wave pairing. The possibility of a strong increase in the superconducting transition temperature $T_c$ even for a low electron density is demonstrated by analyzing the spin-polarized case or the two-band situation. The Kohn-Luttinger theory explains or predicts s…
Conventional Hartree-Fock mean field theory is used, for the first time, to investigate the full two-dimensional t-J model. To date, all other nontrivial mean field approaches modify the Hamiltonian or violate the double occupancy constraint. Unlike conventional mean field theory, these methods do not give variational results for the t-J model. The mean field phase diagram of the t-J model predicts enhanced superconductivity at the crossover between an insulating phase at low doping and a metallic phase at moderate doping. This behavior is remarkably similar to that of high temperature superco…
We report theoretical and experimental results on the transition metal pnictide WP. The theoretical outcomes based on tight-binding calculations and density functional theory indicate that WP is a three-dimensional superconductor with an anisotropic electronic structure and nonsymmorphic symmetries. On the other hand, magnetoresistance experimental data and the analysis of superconducting fluctuations of the conductivity in external magnetic field indicate a weakly anisotropic three-dimensional superconducting phase.
We report Muon Spin Relaxation studies in weak transverse fields of the superconductivity in the metal cluster compound, Ga$\_{84}$[N(SiMe$\_{3}$)$\_{2}$]$\_{20}$-Li$\_{6}$Br$\_{2}$(thf)$\_{20}\cdot $2toluene. The temperature and field dependence of the muon spin relaxation rate and Knight shift clearly evidence type II bulk superconductivity below $T\_{\text{c}}\approx7.8$ K, with $B\_{\text{c1}}\approx 0.06$ T, $B\_{\text{c2}}\approx 0.26 $ T, $κ\sim 2$ and weak flux pinning. The data are well described by the s-wave BCS model with weak electron-phonon coupling in the clean limit. A qualitat…
The electronic structures of zig-zag and arm-chair single-walled carbon nanotubes interacting with a transitional-metal atomic nanowire of Ni have been determined. The Ni nanowire creates a large electron density of states (DOS)at the Fermi energy. The dependence of the enhanced DOS on the spin state and positioning of the transition-metal wire(inside or outside the nanotube) is studied. Preliminary estimates of the electron-phonon interaction suggest that such systems may have a superconducting transition temperature of $\sim$ 10-50 K. The signs of superconductivity seen in ``ropes'' of nanot…
Metallic ferromagnets with strongly interacting electrons often exhibit remarkable electronic phases such as ferromagnetic superconductivity, complex spin textures, and nontrivial topology. In this report, we discuss the synthesis of a layered magnetic metal NiTa$_4$Se$_8$ (or Ni$_{1/4}$TaSe$_{2}$) with a Curie temperature of 58 Kelvin. Magnetization data and \textit{ab initio} calculations indicate that the nickel atoms host uniaxial ferromagnetic order of about 0.7$μ_{B}$ per atom, while an even smaller moment is generated in the itinerant tantalum conduction electrons. Strong correlations a…
