Frictional interfaces are abundant in natural and engineering systems, and predicting their behavior still poses challenges of prime scientific and technological importance. At the heart of these challenges lies the inherent coupling between the interfacial constitutive relation -- the macroscopic friction law -- and the bulk elasticity of the bodies that form the frictional interface. In this feature paper, we discuss the generic properties of the macroscopic friction law and the many ways in which its coupling to bulk elasticity gives rise to rich spatiotemporal frictional dynamics. We first present the widely used rate-and-state friction constitutive framework, discuss its power and limitations, and propose extensions that are supported by experimental data. We then discuss how bulk elasticity couples different parts of the interface, and how the range and nature of this interaction are affected by the system's geometry. Finally, in light of the coupling between interfacial and bulk physics, we discuss basic phenomena in spatially-extended frictional systems, including the stability of homogeneous sliding, the onset of sliding motion and a wide variety of propagating frictional modes (e.g. rupture fronts, healing fronts and slip pulses). Overall, the results presented and discussed in this feature paper highlight the inseparable roles played by interfacial and bulk physics in spatially-extended frictional systems.
Sliding along frictional interfaces separating dissimilar elastic materials is qualitatively different from sliding along interfaces separating identical materials due to the existence of an elastodynamic coupling between interfacial slip and normal stress perturbations in the former case. This bimaterial coupling has important implications for the dynamics of frictional interfaces, including their stability and rupture propagation along them. We show that while this bimaterial coupling is a monotonically increasing function of the bimaterial contrast, when it is coupled to interfacial shear s…
We present single contact friction experiments between a glassy polymer and smooth silica substrates grafted with alkylsilane layers of different coverage densities and morphologies. This allows us to adjust the polymer/substrate interaction strength. We find that, when going from weak to strong interaction, the response of the interfacial junction where shear localizes evolves from that of a highly viscous threshold fluid to that of a plastically deformed glassy solid. This we analyse as resulting from an interaction-induced ``interfacial glass transition'' helped by pressure.
Hypothesis Saponins are natural surfactants which can provide highly viscoelastic interfaces. This property can be used to quantify precisely the effect of interfacial dilatational elasticity on the various rheological properties of bulk emulsions. Experiments We measured the interfacial dilatational elasticity of adsorption layers from four saponins (Quillaja, Escin, Berry, Tea) adsorbed on hexadecane-water and sunflower oil-water interfaces. In parallel, the rheological properties under steady and oscillatory shear deformations were measured for bulk emulsions, stabilized by the same saponin…
We propose an elasto-plastic inspired friction model which incorporates interfacial stiffness. Steady state sliding friction is characterized by a generic nonmonotonic behavior, including both velocity weakening and strengthening branches. In 1D and upon the application of sideway loading, we demonstrate the existence of transient cracklike fronts whose velocity is independent of sound speed, which we propose to be analogous to the recently discovered slow interfacial rupture fronts. Most importantly, the properties of these transient inhomogeneously loaded fronts are determined by steady stat…
We measure the elastic and dissipative responses of a multicontact interface, formed between the rough surfaces of two contacting macroscopic solids, submitted to a biased oscillating shear force. We evidence that beyond a linear viscoelastic regime, observed at low shear amplitude, the interface response exhibits a dissipative component which corresponds to the onset of frictional dissipation. The latter regime exists whereas the tangential force applied, far from the nominal static threshold, does not provoke any sliding. This result, akin to that of Mindlin for a single contact, leads us to…
We study an elasticity model for compressed protein monolayers or particle rafts at a liquid interface. Based on the microscopic view of hard-core particles with soft shells, a bead-spring model is formulated and analyzed in terms of continuum elasticity theory. The theory can be applied, for example, to hydrophobin-coated air-water interfaces or, more generally, to liquid interfaces coated with an adsorbed monolayer of interacting hard-core particles. We derive constitutive relations for such particle rafts and describe the buckling of compressed planar liquid interfaces as well as their appa…
An increase of static friction during stationary contacts of two solids due to interfacial chemical bonding has been reported in multiple experiments. However, the physics underlying such frictional aging is still not fully understood because it involves multiple physical and chemical effects coupled with each other, making direct interpretation of experimental results difficult. Here, we develop a multiphysics chemical aging model that combines contact mechanics, mechanochemistry, and interfacial chemical reaction kinetics. Our model predicts that aging is proportional to normal loads in a lo…
The dynamics of frictional interfaces play an important role in many physical systems spanning a broad range of scales. It is well-known that frictional interfaces separating two dissimilar materials couple interfacial slip and normal stress variations, a coupling that has major implications on their stability, failure mechanism and rupture directionality. In contrast, interfaces separating identical materials are traditionally assumed not to feature such a coupling due to symmetry considerations. We show, combining theory and experiments, that interfaces which separate bodies made of macrosco…
We study the collective behaviour of a close packed monolayer of non-Brownian particles at a fluid-liquid interface. Such a particle raft forms a two-dimensional elastic solid and can support anisotropic stresses and strains, e.g. it buckles in uniaxial compression and cracks in tension. We characterise this solid in terms of a Young's modulus and Poisson ratio derived from simple theoretical considerations and show the validity of these estimates by using an experimental buckling assay to deduce the Young's modulus.
Permeability heterogeneity and bulk linear elasticity of displaced clay suspensions determine interfacial pattern morphologies in Hele-Shaw experiments
We study the peeling process of a thin viscoelastic tape from a rigid substrate. Two different boundary conditions are considered at the interface between the tape and the substrate: stuck adhesion, and relative sliding in the presence of frictional shear stress. In the case of perfectly sticking interfaces, we found that the viscoelastic peeling behavior resembles the classical Kendall behavior of elastic tapes, with the elastic modulus given by the tape high-frequency viscoelastic modulus. Including the effect of frictional sliding, which occurs at the interface adjacent to the peeling front…
The failure of frictional interfaces and the spatiotemporal structures that accompany it are central to a wide range of geophysical, physical and engineering systems. Recent geophysical and laboratory observations indicated that interfacial failure can be mediated by slow slip rupture phenomena which are distinct from ordinary, earthquake-like, fast rupture. These discoveries have influenced the way we think about frictional motion, yet the nature and properties of slow rupture are not completely understood. We show that slow rupture is an intrinsic and robust property of simple non-monotonic …
Classically, the quantity of contact area $A_R$ between two bodies is considered a proxy for the force of friction. However, bond density across the interface - quality of contact - is also relevant, and contemporary debate often centers around the relative importance of these two factors. In this work, we demonstrate that a third factor, often overlooked, plays a significant role in static frictional strength: the distribution of contact. We perform static friction measurements, $μ$, on three pairs of solid blocks while imaging the contact plane. By using linear regression on hundreds of imag…
Stiff scales adorn the exterior surfaces of fishes, snakes, and many reptiles. They provide protection from external piercing attacks and control over global deformation behavior to aid locomotion, slithering, and swimming across a wide range of environmental condition. In this letter, we investigate the dynamic behavior of biomimetic scale substrates for further understanding the origins of the nonlinearity that involve various aspect of scales interaction, sliding kinematics, interfacial friction, and their combination. Particularly, we study the vibrational characteristics through an analyt…
The onset of frictional instabilities, e.g. earthquakes nucleation, is intimately related to velocity-weakening friction, in which the frictional resistance of interfaces decreases with increasing slip velocity. While this frictional response has been studied extensively, less attention has been given to steady-state velocity-strengthening friction, in spite of its potential importance for various aspects of frictional phenomena such as the propagation speed of interfacial rupture fronts and the amount of stored energy released by them. In this note we suggest that a crossover from steady-stat…
We study the 2D linear stability analysis of a deformable solid of a finite height $H$, steadily sliding on top of a rigid solid within a generic rate-and-state friction type constitutive framework, fully accounting for elastodynamic effects. We derive the linear stability spectrum, quantifying the interplay between stabilization related to the frictional constitutive law and destabilization related both to the elastodynamic bi-material coupling between normal stress variations and interfacial slip, and to finite size effects. The stabilizing effects related to the frictional constitutive law …
The morphology of an elastic strip subject to vertical compressive stress on a frictional rigid substrate is investigated by a combination of theory and experiment. We find a rich variety of morphologies, which -when the bending elasticity dominates over the effect of gravity- are classified into three distinct types of states: pinned, partially slipped, and completely slipped, depending on the magnitude of the vertical strain and coefficient of static friction. We develop a theory of elastica under mixed clamped-hinged boundary conditions combined with the Coulomb-Amontons friction law, and f…
Biomimetic scale-covered substrates provide geometric tailorability via scale orientation, spacing and also interfacial properties of contact in various deformation modes. No work has investigated the effect of friction in twisting deformation of biomimetic scale-covered beams. In this work, we investigate the frictional effects in the biomimetic scale-covered structure by developing an analytical model verified by the finite element simulations. In this model, we consider dry (Coulomb) friction between rigid scales surfaces, and the substrate as the linear elastic rectangular beam. The obtain…
We report on the frictional properties of a single contact between a glassy polymer lens and a flat silica substrate covered either by a disordered or by a self-assembled alkylsilane monolayer. We find that, in contrast to common belief, the Amontons proportionality between frictional and normal stresses does not hold. Besides, we observe that the velocity dependence of the sliding stress is strongly sensitive to the structure of the silane layer. Analysis of the frictional rheology observed on both disordered and self-assembled monolayers suggests that dissipation is controlled by the plastic…
The physical mechanism of elasticity of liquid surfaces coated with colloidal particles is proposed. It is suggested that particles are separated by water clearings and the capillary interaction between them is negligible. The case is treated when the colloidal layer is deformed normally to its surface. The elasticity arises as an interfacial effect. The effective Young modulus of a surface depends on the interfacial tension, equilibrium contact angle, radius of colloidal particles and their surface density. For the nanometrically scaled particles the line tension becomes essential and has an …
We construct a generic coarse-grained dynamics of a thin inflexible planar layer of polar-ordered suspension of active particles, that is frictionally coupled to an embedding isotropic passive fluid medium with a friction coefficient $Γ$. Being controlled by $Γ$, our model provides a unified framework to describe the long wavelength behaviour of a variety of thin polar-ordered systems, ranging from {\em wet} to {\em dry} active matters and free standing active films. Investigations of the linear instabilities around a chosen orientationally ordered uniform reference state reveal generic moving…
The failure of the population of micro-junctions forming the frictional interface between two solids is central to fields ranging from biomechanics to seismology. This failure is mediated by the propagation along the interface of various types of rupture fronts, covering a wide range of velocities. Among them are so-called slow fronts, which are recently discovered fronts much slower than the materials' sound speeds. Despite intense modelling activity, the mechanisms underlying slow fronts remain elusive. Here, we introduce a multi-scale model capable of reproducing both the transition from fa…
A Landau-de Gennes model that integrates the nematic quadrupolar tensor order parameter and complex smectic-A order parameters is used to simulate the two-dimensional growth of an initially homogeneous smectic-A spherulite in an isotropic matrix. These simulations are performed in the shape-dynamic (nano-scale) regime of growth under two material conditions: isotropic nematic elasticity and equal splay-bend nematic elasticity. A comparison of the growth kinetics, spherulite morphology, interfacial/bulk energy landscapes between both cases is made showing that equal nematic splay-bend elasticit…
We investigate the Green function of two-dimensional dense random packings of grains in order to discriminate between the different theories of stress transmission in granular materials. Our computer simulations allow for a detailed quantitative investigation of the dynamics which is difficult to obtain experimentally. We show that both hyperbolic and parabolic models of stress transmission fail to predict the correct stress distribution in the studied region of the parameters space. We demonstrate that the compressional and shear components of the stress compare very well with the predictions…
A MEMS-based sensing device is used to measure the normal and tangential stress fields at the base of a rough elastomer film in contact with a smooth glass cylinder in steady sliding. This geometry allows for a direct comparison between the stress profiles measured along the sliding direction and the predictions of an original \textit{exact} bidimensional model of friction. The latter assumes Amontons' friction law, which implies that in steady sliding the interfacial tangential stress is equal to the normal stress times a pressure-independent dynamic friction coefficient $μ_d$, but makes no f…
We present confocal microscopy studies of novel particle-stabilized emulsions. The novelty arises because the immiscible fluids have an accessible upper critical solution temperature. The emulsions have been created by beginning with particles dispersed in the single-fluid phase. On cooling, regions of the minority phase nucleate. While coarsening these nuclei become coated with particles due to the associated reduction in interfacial energy. The resulting emulsion is arrested, and the particle-coated interfaces have intriguing properties. Having made use of the binary-fluid phase diagram to c…
We report on the multi-contact frictional dynamics of model elastomer surfaces rubbed against bare glass slides. The surfaces consist of layers patterned with thousands spherical caps (radius of curvature 100 $μ$m) distributed both spatially and in height, regularly or randomly. Use of spherical asperities yields circular micro-contacts whose radius is a direct measure of the contact pressure distribution. In addition, optical tracking of individual contacts provides the in-plane deformations of the tangentially loaded interface, yielding the shear force distribution. We then investigate the s…
Hydrogel consists of a crosslinked polymer matrix imbibed with a solvent such as water at volume fractions that can exceed 90\%. They are important in many scientific and engineering applications due to their tunable physiochemical properties, bio-compatibility, and ultra-low friction. Their multiphase structure leads to a complex interfacial rheology, yet a detailed, microscopic understanding of hydrogel friction is still emerging. Using a custom-built tribometer, here we identify three distinct regimes of frictional behavior for polyacrylic acid (PAA), polyacrylamide (PAAm), and agarose hydr…
Microgels are soft colloidal particles constituted by cross-linked polymer networks with a high potential for applications. In particular, after adsorption at a fluid interface, interfacial tension provides two-dimensional (2D) confinement for microgel monolayers and drives the reconfiguration of the particles, enabling their deployment in foam and emulsion stabilization and in surface patterning for lithography, sensing and optical materials. However, most studies focus on systems of fluids with a high interfacial tension, e.g. alkanes/ or air/water interfaces, which imparts similar propertie…
We study the frictional behavior of both elastic and viscoelastic thin coatings bonded to a seemingly rigid substrate and sliding against a rough profile in the presence of Coulomb friction at the interface. The aim is to explore the effect of the coupling between the normal and tangential displacement fields arising from the finiteness of the material thickness and to quantify the contribution this can have on energy losses. We found that, due to normal-tangential coupling, asymmetric contacts and consequently additional friction are observed even for purely elastic layers, indeed associated …
We study the outflow dynamics and clogging phenomena of mixtures of soft, elastic low-friction spherical grains and hard frictional spheres of similar size in a quasi-two-dimensional (2D) silo with narrow orifice at the bottom. Previous work has demonstrated the crucial influence of elasticity and friction on silo discharge. We show that the addition of small amounts, even as low as 5\%, of hard grains to an ensemble of soft, low-friction grains already has significant consequences. The mixtures allow a direct comparison of the probabilities of the different types of particles to clog the orif…
Macroscopic sliding between two solids is triggered by the propagation of a micro-slip front along the frictional interface. In certain conditions, sliding is preceded by the propagation of aborted fronts, spanning only part of the contact interface. The selection of the characteristic size spanned by those so-called precursors remains poorly understood. Here, we introduce a 1D toy model of precursors between a slider and a track in which the fronts are quasi-static self-healing slip pulses. When the slider's thickness is large compared to the elastic correlation length and when the interfacia…
Digital Image Correlation is used to study the micromechanics of a multi-contact interface formed between a rough elastomer and a smooth glass surface. The in-plane elastomer deformation is monitored during the incipient sliding regime, i.e. the transition between static and sliding contact. As the shear load is increased, an annular slip region, in coexistence with a central stick region, is found to progressively invade the contact. From the interfacial displacement field, the tangential stress field can be further computed using a numerical inversion procedure. These local mechanical measur…
When a soft glassy colloidal suspension is displaced by a Newtonian fluid in a radial Hele-Shaw geometry, the pattern morphology that develops at the interface is determined by the complex rheology of the former. We had reported in an earlier work [Palak, V. R. S. Parmar, D. Saha and R. Bandyopadhyay, JCIS Open, 6 (2022) 100047] that a range of interfacial patterns can be formed by controlling the elasticity of the displaced suspension, the flow rate of the displacing fluid and the interfacial tension of the fluid pair. Interestingly, all the different morphological features can be distinguish…
Rolling of a small sphere on a solid support is governed by a non-linear friction that is akin to the Coulombic dry fiction. No motion occurs when the external field is weaker than the frictional resistance. However, with the intervention of an external noise, a viscous friction like property emerges; thus the sphere rolls with an uniform drift velocity that is proportional to the applied field. As the sphere rolls, it rocks forward and backward resulting in substantial fluctuation of displacement opposite to the net drift. The ratio of the integrated probabilities of the negative to positive …
Surface Force Apparatus (SFA) allows to accurately resolve the interfacial properties of fluids confined between extended surfaces. The accuracy of the SFA makes it an ubiquitous tool for the nanoscale mechanical characterization of soft matter systems. The SFA traditionally measures force-distance profiles through interferometry with subnanometric distance precision. However, these techniques often require a dedicated and technically demanding experimental setup, and there remains a need for versatile and simple force-distance measurement tools. Here we present a MicroMegascope based dynamic …
Hypothesis: Particle-laden fluid interfaces are the central component of many natural and engineering systems. Understanding the mechanical properties and improving the stability of such interfaces are of great practical importance. Janus particles, a special class of heterogeneous colloids, might be utilized as an effective surface-active agent to control the assembly and interfacial rheology of particle-laden fluid interfaces. Experiments: Using a custom-built interfacial stress rheometer, we explore the effect of Janus particle additives on the interfacial rheology and microscopic structure…
The use of electrophoretic forces to tune friction at material-nanoparticle-liquid interfaces with static or low frequency (0.6-50 mHz) electric fields is reported for the first time. External electric fields were employed to reposition negatively charged TiO2 or positively charged Al2O3 nanoparticles suspended in water in directions perpendicular to a planar platinum surface of a quartz crystal microbalance, which was then used to monitor frictional shear forces at the interface. Active electro-tunable control of friction has been demonstrated for both TiO2 and Al2O3 suspensions. For TiO2 sus…
The complexity of the frictional dynamics at the microscopic scale makes difficult to identify all of its controlling parameters. Indeed, experiments on sheared elastic bodies have shown that the static friction coefficient depends on loading conditions, the real area of contact along the interfaces and the confining pressure. Here we show, by means of numerical simulations of a 2D Burridge-Knopoff model with a simple local friction law, that the macroscopic friction coefficient depends non-monotonically on the bulk elasticity of the system. This occurs because elastic constants control the ge…
The intricate interaction between the deformability of a substrate and the dynamic spreading of a liquid drop on the same, under the application of an electrical voltage, has remained far from being well understood. Here, we demonstrate that electrospreading dynamics on soft substrates is dictated by the combined interplay of electrocapillarity, the wetting line friction and the viscoelastic energy dissipation at the contact line. Our results reveal that during such electro-elastocapillarity mediated spreading of a sessile drop, the contact radius evolution exhibits a universal power law in a …
