Coupled electron-hole states are realized in a system consisting of a combination of an electrostatic potential barrier and ring-shaped potential well, which resembles a circular dipole. A perpendicular magnetic field induces confined states inside the Landau gaps which are mainly located at the barrier or ring. Hybridizations between the barrier and ring states are seen as anticrossings in the energy spectrum. As a consequence, the energy levels show an oscillating dependence on the electrostatic potential strength in combination with an oscillating migration of the wave functions between the barrier and ring. At the anticrossing points the quantum state consists of a mixture of electron and hole. The present system mimics closely the behavior of a relativistic dipole on gapped graphene.
We develop a general theory of the layer circular photogalvanic effect (LCPGE) in quasi two-dimensional chiral bilayers, which refers to the appearance of a polarization-dependent, out-of-plane dipole moment induced by circularly polarized light. We elucidate the geometric origin of the LCPGE as two types of interlayer coordinate shift weighted by the quantum metric tensor and the Berry curvature, respectively. As a concrete example, we calculate the LCPGE in twisted bilayer graphene, and find that it exhibits a resonance peak whose frequency can be tuned from visible to infrared as the twisti…
We study the polarization dependence of optical absorption for the modified Haldane model, which exhibits antichiral edge modes in presence of sample boundaries and has been argued to be realizable in transition metal dichalcogenides or Weyl semimetals. A rich optical phase diagram is unveiled, in which the correlations between perfect circular dichroism, pseudospin and valley polarization can be tuned independently upon varying the Fermi energy. Importantly, perfect circular dichroism and valley polarization are achieved simultaneously. This unprecedented combination of optical properties sug…
Characterizing and manipulating the circular polarization of light is central to numerous emerging technologies, including spintronics and quantum computing. Separately, monolayer tungsten disulfide (WS2) is a versatile material that has demonstrated promise in a variety of applications, including single photon emitters and valleytronics. Here, we demonstrate a method to tune the photoluminescence (PL) intensity (factor of x161), peak position (38.4meV range), circular polarization (39.4% range), and valley polarization of a Bi2Se3-WS2 2D heterostructure using a low-power laser (0.762uW) in am…
We report on a planar microwave resonator providing arbitrarily polarized oscillating magnetic fields that enable selective excitation of the electronic spins of nitrogen-vacancy (NV) centers in diamond. The polarization plane is parallel to the surface of diamond, which makes the resonator fully compatible with (111)-oriented diamond. The field distribution is spatially uniform in a circular area with a diameter of 4 mm, and a near-perfect circular polarization is achieved. We also demonstrate that the original resonance frequency of 2.8 GHz can be varied in the range of 2-3.2 GHz by introduc…
A magnetic field can generally induce circular phonon dichroism based on the formation of Landau levels of electrons. Here, we study the magnetization-induced circular phonon dichroism in transition metal dichalcogenides, without forming Landau levels. We find that, instead of the conventional deformation potential coupling, pseudogauge-type electron-phonon coupling plays an essential role in the emergence of the phenomenon. As a concrete example, a large dichroism signal is obtained in monolayer MoTe2 on a EuO substrate, even without considering Rashba spin-orbit coupling. Due to the two-dime…
In the presence of strong magnetic fields the electronic bandstructure of graphene drastically changes. The Dirac cone collapses into discrete non-equidistant Landau levels, which can be externally tuned by changing the magnetic field. In contrast to conventional materials, specific Landau levels are selectively addressable using circularly polarized light. Exploiting these unique properties, we propose the design of a tunable laser operating in the technologically promising terahertz spectral range. To uncover the many-particle physics behind the emission of light, we perform a fully quantum …
Berry curvature is analogous to magnetic field but in momentum space and is commonly present in materials with non-trivial quantum geometry. It endows Bloch electrons with transverse anomalous velocities to produce Hall-like currents even in the absence of a magnetic field. We report the direct observation of in situ tunable valley-selective Hall effect (VSHE), where inversion symmetry, and thus the geometric phase of electrons, is controllable by an out-of-plane electric field. We use high-quality bilayer graphene with an intrinsic and tunable bandgap, illuminated by circularly polarized mid-…
Graphene charge carriers behave as relativistic massless fermions, thereby exhibiting a variety of counter-intuitive behaviors. In particular, at p-n junctions, they behave as photons encountering a negative index media, therefore experiencing a peculiar refraction known as Veselago lensing. However, the way Dirac fermions flow through a Veselago lens remains largely unexplored experimentally. Here, a novel approach to create a movable and tunable circular p-n junction in graphene is proposed, using the polarized tip of a scanning gate microscope. Scanning the tip in the vicinity of a graphene…
A major achievement of the past decade has been the realization of macroscopic quantum systems by exploiting interactions between optical cavities and mechanical resonators. In these systems, phonons are coherently annihilated or created in exchange for photons. Similar phenomena have recently been observed through "phonon cavity" coupling -- energy exchange between modes of a single system as mediated by intrinsic material nonlinearity. To date, this has been demonstrated primarily for bulk crystalline, high-quality-factor (Q>100,000) mechanical systems operated at cryogenic temperatures. Her…
The motion of massless Dirac-electrons in graphene mimics the propagation of photons. This makes it possible to control the charge-carriers with components based on geometrical-optics and has led to proposals for an all-graphene electron-optics platform. An open question arising from the possibility of reducing the component-size to the nanometer-scale is how to access and understand the transition from optical-transport to quantum-confinement. Here we report on the realization of a circular p-n junction that can be continuously tuned from the nanometer-scale, where quantum effects are dominan…
Nonlinear optical probe of tunable surface electrons on a topological insulator
我们用超快激光脉冲实验证明了拓扑绝缘体Bi $_2$ Se $_3$的体单晶的二阶光学响应对它的表面电子是敏感的。通过进行表面掺杂依赖性测量作为光子偏振和样品取向的函数，我们表明，二次谐波产生可以同时探测表面晶体结构和表面电荷的Bi $_2$ Se $_3$。此外，我们发现，使用圆偏振光的二次谐波产生揭示了系统的时间反演对称性，并且对表面充电具有令人惊讶的鲁棒性，这使其成为拓扑表面和掩埋界面的光谱研究的有前途的工具。
Purcell enhanced and blinking free single photons from InAs/GaAs quantum dots in deterministically placed circular Bragg gratings
Julius-Maximilians-Universität Würzburg（维尔茨堡大学）；Korea Advanced Institute of Science and Technology (KAIST)（韩国科学技术院）；Johannes Kepler Universität Linz（林茨约翰内斯·开普勒大学）；Ruhr-Universität Bochum（波鸿鲁尔大学）；Paderborn University（帕德博恩大学）；Karlsruhe Institute of Technology（卡尔斯鲁厄理工学院）
Spatially indirect excitons with displaced wavefunctions of electrons and holes play a pivotal role in a large portfolio of fascinating physical phenomena and emerging optoelectronic applications, such as valleytronics, exciton spin Hall effect, excitonic integrated circuit and high-temperature superfluidity. Here, we uncover three types of spatially indirect excitons (including their phonon replicas) and their quantum-confined Stark effects in hexagonal boron nitride encapsulated bilayer WSe2, by performing electric field-tunable photoluminescence measurements. Because of different out-of-pla…
Circular polarization resolved magneto-infrared studies of multilayer epitaxial graphene (MEG) are performed using tunable quantum cascade lasers in high magnetic fields up to 17.5 T. Landau level (LL) transitions in the monolayer and bilayer graphene inclusions of MEG are resolved, and considerable electron-hole asymmetry is observed in the extracted electronic band structure. For monolayer graphene, a four-fold splitting of the $n=0$ to $n=1$ LL transition is evidenced and attributed to the lifting of the valley and spin degeneracy of the zeroth LL and the broken electron-hole symmetry. The …
We propose a tunable optical setup to engineer topologically nontrivial flat bands in twisted bilayer graphene under circularly polarized light. Using both analytical and numerical calculations, we demonstrate that nearly flat bands can be engineered at small twist angles near the magic angles of the static system. The flatness and the gaps between these bands can be tuned optically by varying laser frequency and amplitude. We study the effects of interlayer hopping variations on Floquet flat bands and find that lattice relaxation favors their formation. Furthermore, we find that, once formed,…
The unique gate-voltage dependent optical properties of graphene make it a promising electrically-tunable plasmonic material. In this work, we proposed in-situ control of the polarization of nanoantennas by combining plasmonic structures with an electrostatically tunable graphene monolayer. The tunable polarizer is designed based on an asymmetric cross nanoantenna comprising two orthogonal metallic dipoles sharing the same feed gap. Graphene monolayer is deposited on a Si/SiO2 substrate, and inserted beneath the nanoantenna. Our modelling demonstrates that as the chemical potential is incremen…
A properly strained graphene monolayer or bilayer is expected to harbour periodic pseudo-magnetic fields with high symmetry, yet to date, a convincing demonstration of such pseudo-magnetic fields has been lacking, especially for bilayer graphene. Here, we report the first definitive experimental proof for the existence of large-area, periodic pseudo-magnetic fields, as manifested by vortex lattices in commensurability with the moiré patterns of low-angle twisted bilayer graphene. The pseudo-magnetic fields are strong enough to confine the massive Dirac electrons into circularly localized pseud…
We explore the tunability of the phonon polarization in suspended uniaxially strained graphene by magneto-phonon resonances. The uniaxial strain lifts the degeneracy of the LO and TO phonons, yielding two cross-linearly polarized phonon modes and a splitting of the Raman G peak. We utilize the strong electron-phonon coupling in graphene and the off-resonant coupling to a magneto-phonon resonance to induce a gate-tunable circular phonon dichroism. This, together with the strain-induced splitting of the G peak, allows us to controllably tune the two linearly polarized G mode phonons into circula…
