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arXiv 1901.00575cond-mat.mes-hall
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应变MoS2高次谐波带内和带间激发的协同演化

Cooperative evolution of intraband and interband excitations for high harmonic generation in strained MoS2

Meng-Xue Guan, Chao Lian, Shi-Qi Hu, Hang Liu, Sheng-Jie Zhang, Jin Zhang, Sheng Meng

摘要:

调制二维(2D)材料的电子结构代表了一个令人兴奋的途径,定制其光电性能。在这里,我们确定了应变引起的,带内和带间激发的合作效应,有助于高次谐波产生(HHG)在原型二硫属化物二硫化钼单层。我们发现,除了主要的带内贡献,带间电流也是不可或缺的调制高次谐波。由于平坦的带色散和Berry曲率增强了带间和带内动力学,HHG产率随压缩应变线性增加。能带结构可以通过监测应变引起的HHG谱的演化来以高可靠性检索,这表明应变不仅提供了额外的旋钮来控制固体中的HHG,而且标志着一种完全理解潜在微观机制的方式。

英文摘要:

Modulating electronic structure of two-dimensional (2D) materials represents an exciting avenue for tailoring their optoelectronic properties. Here, we identify a strain-induced, cooperative effect of intraband and interband excitations contributing to high harmonic generation (HHG) in prototype dichalcogenide MoS2 monolayer. We find that besides the dominant intraband contributions, interband current is also indispensable in modulating HHG. The HHG yields increase linearly with the compressive strain since flatter band dispersion and Berry curvature enhance both interband and intraband dynamics. Band structure can be retrieved with high reliability by monitoring the strain-induced evolution of HHG spectra, suggesting that strain not only provides an additional knob to control HHG in solids, but also marks a way towards a complete understanding of underlying microscopic mechanisms.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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