We show that the measured intrinsic octupole moments of $^{220}$Rn, $^{224}$Ra, and $^{226}$Ra constrain the intrinsic Schiff moments of $^{225}$Ra$^{221}$Rn, $^{223}$Rn, $^{223}$Fr, $^{225}$Ra, and $^{229}$Pa. The result is a dramatically reduced uncertainty in intrinsic Schiff moments. Direct measurements of octupole moments in odd nuclei will reduce the uncertainty even more. The only significant source of nuclear-physics error in the laboratory Schiff moments will then be the intrinsic matrix elements of the time-reversal non-invariant interaction produced by CP-violating fundamental physics. Those matrix elements are also correlated with octupole moments, but with a larger systematic uncertainty.
We examine the time-reversal-violating nuclear ``Schiff moment'' that induces electric dipole moments in atoms. After presenting a self-contained derivation of the form of the Schiff operator, we show that the distribution of Schiff strength, an important ingredient in the ground-state Schiff moment, is very different from the electric-dipole-strength distribution, with the Schiff moment receiving no strength from the giant dipole resonance in the Goldhaber-Teller model. We then present shell-model calculations in light nuclei that confirm the negligible role of the dipole resonance and show t…
An analytic, parameter-free (up to overall scale factors) solution of the Bohr Hamiltonian involving axially symmetric quadrupole and octupole deformations, as well as an infinite well potential, is obtained, after separating variables in a way reminiscent of the Variable Moment of Inertia (VMI) concept. Normalized spectra and B(EL) ratios are found to agree with experimental data for 226-Ra and 226-Th, the nuclei known to lie closest to the border between octupole deformation and octupole vibrations in the light actinide region.
Nuclear forces violating parity and time reversal invariance (${\cal P},{\cal T}$-odd) produce ${\cal P},{\cal T}$-odd nuclear moments, for example, the nuclear Schiff moment. In turn, this moment can induce the electric dipole moment in the atom. The nuclear Schiff moment is predicted to be enhanced in nuclei with static quadrupole and octupole deformation. The analogous suggestion of the enhanced contribution to the Schiff moment from the soft collective quadrupole and octupole vibrations in spherical nuclei is tested in this article in the framework of the quasiparticle random phase approxi…
The analytic quadrupole octupole axially symmetric model, which had successfully predicted 226Ra and 226Th as lying at the border between the regions of octupole deformation and octupole vibrations in the light actinides using an infinite well potential (AQOA-IW), is made applicable to a wider region of nuclei exhibiting octupole deformation, through the use of a Davidson potential (AQOA-D). Analytic expressions for energy spectra and B(E1), B(E2), B(E3) transition rates are derived. The spectra of 222-226Ra and 224,226Th are described in terms of the two parameters phi_0 (expressing the relat…
Octupole deformed shapes in neutron-rich actinides and superheavy nuclei as well as extremely deformed shapes of the N~Z light nuclei have been investigated within the framework of covariant density functional theory. We confirmed the presence of new region of octupole deformation in neutron-rich actinides with the center around Z~96, N~196 but our calculations do not predict octupole deformation in the ground states of superheavy Z~108 nuclei. As exemplified by the study of 36Ar, the nodal structure of the wavefunction of occupied single-particle orbitals in extremely deformed structures allo…
Quadrupole and octupole deformation energy surfaces, low-energy excitation spectra, and electric transition rates in eight neutron-rich isotopic chains -- Ra, Th, U, Pu, Cm, Cf, Fm, and No -- are systematically analyzed using a quadrupole-octupole collective Hamiltonian model, with parameters determined by constrained reflection-asymmetric and axially-symmetric relativistic mean-field calculations based on the PC-PK1 energy density functional. The theoretical results of low-lying negative-parity bands, odd-even staggering, average octupole deformations $\langleβ_3\rangle$, and $B(E3; 3^-_1\to …
An analytic collective model in which the relative presence of the quadrupole and octupole deformations is determined by a parameter (phi_0), while axial symmetry is obeyed, is developed. The model [to be called the analytic quadrupole octupole axially symmetric model (AQOA)] involves an infinite well potential, provides predictions for energy and B(EL) ratios which depend only on phi_0, draws the border between the regions of octupole deformation and octupole vibrations in an essentially parameter-independent way, and describes well 226-Th and 226-Ra, for which experimental energy data are sh…
Parity (P) and time reversal (T) violating nuclear forces create P, T -odd moments in expansion of the nuclear electrostatic potential. We derive expression for the nuclear electric octupole field which includes the electron screening correction (similar to the screening term in the Schiff moment). Then we calculate the Z alpha corrections to the Schiff moment which appear due to the finite nuclear size. Such corrections are important in heavy atoms with nuclear charge Z > 50. The Schiff and octupole moments induce atomic electric dipole moments (EDM) and P, T -odd interactions in molecules wh…
A systematic search for axial octupole deformation in the actinides and superheavy nuclei with proton numbers $Z=88-126$ and neutron numbers from two-proton drip line up to $N=210$ has been performed in covariant density functional theory (DFT) using four state-of-the-art covariant energy density functionals representing different model classes. The nuclei in the $Z\sim 96, N\sim 196$ region of octupole deformation have been investigated in detail and the systematic uncertainties in the description of their observables have been quantified. Similar region of octupole deformation exists also in…
The interplay between quadrupole and octupole degrees of freedom is discussed in a series of neutron-rich actinides and superheavy nuclei with $92 \le$ Z $\le 110$ and $186 \le$ N $\le 202$. In addition to the static Hartree-Fock-Bogoliubov approach, dynamical beyond-mean-field correlations are taken into account via both parity restoration and symmetry-conserving Generator Coordinate Method calculations based on the Gogny-D1M energy density functional. Physical properties such as correlation energies, negative-parity excitation energies as well as reduced transition probabilities $B(E1)$ and …
In this work we examine the possibility to describe yrast positive- and negative-parity excitations of deformed even-even nuclei through a collective rotation model in which the nuclear surface is characterized by triaxial quadrupole and octupole deformations. The nuclear moments of inertia are expressed as sums of quadrupole and octupole parts. By assuming an adiabatic separation of rotation and vibration degrees of freedom we suppose that the structure of the positive- and negative- parity bands may be determined by the triaxial-rigid-rotor motion of the nucleus. By diagonalizing the Hamilto…
An angular momentum dependence of the parity splitting in the alternating parity bands of nuclei with strong octupole correlations is considered basing on the model of the octupole motion in a one-dimensional potential well conserving axial symmetry. A sign reversal of the parity splitting at higher values of the angular momentum is interpreted as a result of the Coriolis coupling to K=1 octupole mode. New experimental data on the spectra of the alternating parity octupole bands are used.
The interplay between quadrupole and octupole degrees of freedom is discussed in a series of U, Pu, Cm and Cf isotopes both at the mean-field level and beyond. In addition to the static Hartree-Fock-Bogoliubov approach, dynamical beyond-mean-field correlations are taken into account via both parity restoration and symmetry-conserving Generator Coordinate Method calculations based on the parametrization D1M of the Gogny energy density functional. Physical properties such as correlation energies, negative-parity excitation energies as well as reduced transition probabilities $B(E1)$ and $B(E3)$ …
The cranked Skyrme III effective Hamiltonian is applied for the analysis of the rotational dependence of the quadrupole and octupole moments in Ra, Th, and U isotopes. A comparison of the intrinsic electric dipole moments calculated in the model with available experimental and theoretical values is presented. It is found that the non-axial octupole deformation $Y_{32}$ becomes favorable at high spins for the actinide nuclei.
The evolution of quadrupole and octupole collectivity and their coupling is investigated in a series of even-even isotopes of the actinide Ra, Th, U, Pu, Cm, and Cf with neutron number in the interval $130\leqslant N\leqslant 150$. The Hartree-Fock-Bogoliubov approximation, based on the parametrization D1M of the Gogny energy density functional, is employed to generate potential energy surfaces depending upon the axially-symmetric quadrupole and octupole shape degrees of freedom. The mean-field energy surface is then mapped onto the expectation value of the $sdf$ interacting-boson-model Hamilt…
Parity and time invariance violating (${\cal P},{\cal T}$-odd) nuclear forces produce ${\cal P},{\cal T}$-odd nuclear moments, for example, the nuclear Schiff moment. In turn, this moment can induce electric dipole moments (EDMs) in atoms. We estimate the contribution to the Schiff moment from the soft collective octupole vibrations existing in many heavy nuclei. Two possible mechanisms are considered, mixing of the ground state of an odd-$A$ nucleus with the octupole phonon state, and ${\cal P},{\cal T}$-odd admixture to the single-particle wave function of the valence nucleon. We found pract…
Nuclear forces violating parity and time reversal invariance P,T-odd produce P,T-odd nuclear moments, for example, the nuclear Schiff moment. In turn, this moment can induce the electric dipole moment (EDM) in the atom. The contribution to the Schiff moment from the soft collective quadrupole and octupole vibrations in spherical nuclei is calculated in the framework of the quasiparticle random phase approximation with separable quadrupole and octupole forces. The values of nuclear Schiff moments predicted for odd 217-221Ra and 217-221Ra isotopes indicate a possibility of enhancement by a facto…
$J^π$= 0$^+$ states have been investigated in the actinide nucleus ${}^{240}$Pu up to an excitation energy of 3 MeV with a high-resolution (p,t) experiment at $E_{p}$= 24 MeV. To test the recently proposed $J^π$= 0$^+_2$ double-octupole structure, the phenomenological approach of the spdf-interacting boson model has been chosen. In addition, the total 0$^+$ strength distribution and the $0^+$ strength fragmentation have been compared to the model predictions as well as to the previously studied (p,t) reactions in the actinides. The results suggest that the structure of the 0$^+_2$ states in th…
We discuss the octupole deformation properties of many even-even actinide isotopes. The analysis is carried out in the mean field framework (Hartree-Fock-Bogoliubov approximation) by using the axially symmetric octupole moment as a constraint. A one-dimensional octupole collective Hamiltonian is used to obtain properties like excitation energies or $E1$ and $E3$ transition probabilities of the negative parity band-heads associated to the lowest lying $1^{-}$ and $3^{-}$ states. The evolution of these values with neutron number is discussed and a comparison with available experimental data is m…
Nuclei with static intrinsic octupole deformation or a soft octupole vibrational mode lead to strongly enhanced collective nuclear Schiff? moments. Interaction between electrons and these Schiff moments produce enhanced time reversal (T) and parity (P) violating electric dipole moments (EDM) in atoms and molecules. Corresponding experiments may be used to test CP-violation theories predicting T,P-violating nuclear forces and to search for axions. Nuclear octupole deformations are predicted in many short lived isotopes. This paper investigates octupole deformations in stable and very long lifet…
Nuclear fission of heavy (actinide) nuclei results predominantly in asymmetric mass-splits. Without quantum shells, which can give extra binding energy to these mass-asymmetric shapes, the nuclei would fission symmetrically. The strongest shell effects are in spherical nuclei, so naturally the spherical "doubly-magic" ${^{132}}$Sn nucleus (${Z=50}$ protons), was expected to play a major role. However, a systematic study of fission has shown that the heavy fragments are distributed around ${Z=52}$ to 56, indicating that ${^{132}}$Sn is not the only driver. Reconciling the strong spherical shell…
The quadrupole-octupole coupling and the related spectroscopic properties have been studied for the even-even light actinides $^{218-238}$Ra and $^{220-240}$Th. The Hartree-Fock-Bogoliubov approximation, based on the Gogny-D1M energy density functional, has been employed as a microscopic input, i.e., to obtain (axially symmetric) mean-field potential energy surfaces as functions of the quadrupole and octupole deformation parameters. The mean-field potential energy surfaces have been mapped onto the corresponding bosonic potential energy surfaces using the expectation value of the $sdf$ Interac…
A systematic analysis of low-lying quadrupole and octupole collective states is presented, based on the microscopic energy density functional framework. By mapping the deformation constrained self-consistent axially symmetric mean-field energy surfaces onto the equivalent Hamiltonian of the $sdf$ interacting boson model (IBM), that is, onto the energy expectation value in the boson condensate state, the Hamiltonian parameters are determined. The study is based on the global relativistic energy density functional DD-PC1. The resulting IBM Hamiltonian is used to calculate excitation spectra and …
``Beat'' patterns are shown to appear in the octupole bands of several actinides and rare earths, their appearance being independent from the formula used in order to isolate and demonstrate them. It is shown that the recent formalism, making use of discrete approximations to derivatives of the transition energies (or of the energy levels) gives results consistent with the traditional formulae. In both regions it is seen that the first vanishing of the staggering occurs at higher values of the angular momentum I in nuclei exhibiting higher staggering at low I. Since these nuclei happen to be g…
We use the Skyrme-Hartree-Fock method, allowing all symmetries to be broken, to calculate the time-reversal-violating nuclear Schiff moment (which induces atomic electric dipole moments) in the octupole-deformed nucleus 225Ra. Our calculation includes several effects neglected in earlier work, including self consistency and polarization of the core by the last nucleon. We confirm that the Schiff moment is large compared to those of reflection-symmetric nuclei, though ours is generally a few times smaller than recent estimates.
The Delta I = 1 staggering (odd--even staggering) in octupole bands of light actinides is found to exhibit a ``beat'' behaviour as a function of the angular momentum I, forcing us to revise the traditional belief that this staggering decreases gradually to zero and then remains at this zero value. Various algebraic models (spf-Interacting Boson Model, spdf-IBM, Vector Boson Model, Nuclear Vibron Model) are shown to predict in their su(3) limits constant staggering for this case, being thus unable to describe the ``beat'' behaviour. An explanation of the ``beat'' behaviour is given in terms of …
Low-energy positive and negative parity collective states in the equilibrium minimum, and the dynamics of induced fission of actinide nuclei are investigated in a unified theoretical framework based on the generator coordinate method (GCM) with the Gaussian overlap approximation (GOA). The collective potential and inertia tensor, both at zero and finite temperature, are computed using the self-consistent multidimensionally constrained relativistic mean field (MDC-RMF) model, based on the energy density functional DD-PC1. Pairing correlations are treated in the BCS approximation with a separabl…
The atomic electric dipole moment (EDM) currently searched by a number of experimental groups requires that both parity and time-reversal invariance be violated. According to current theoretical understanding, the EDM is induced by the nuclear Schiff moment. The enhancement of the Schiff moment by the combination of static quadrupole and octupole deformation was predicted earlier. Here we study a further idea of the possible enhancement in the absence of static deformation but in a nuclear system with soft collective vibrations of two types. Both analytical approximation and numerical solution…
We have developed multi-dimensional constrained covariant density functional theories (MDC-CDFT) for finite nuclei in which the shape degrees of freedom β_{λμ} with even μ, e.g., β_{20}, β_{22}, β_{30}, β_{32}, β_{40}, etc., can be described simultaneously. The functional can be one of the following four forms: the meson exchange or point-coupling nucleon interactions combined with the non-linear or density-dependent couplings. For the pp channel, either the BCS approach or the Bogoliubov transformation is implemented. The MDC-CDFTs with the BCS approach for the pairing (in the following label…
For the first time the potential energy surfaces of actinide nuclei in the $(β_{20}, β_{22}, β_{30})$ deformation space are obtained from a multi-dimensional constrained covariant density functional theory. With this newly developed theory we are able to explore the importance of the triaxial and octupole shapes simultaneously along the whole fission path. It is found that besides the octupole deformation, the triaxiality also plays an important role upon the second fission barriers. The outer barrier as well as the inner barrier are lowered by the triaxial deformation compared with axially sy…
Deformed nuclei possess enhanced moments violating time reversal invariance ($T$) and parity ($P$). Collective magnetic quadrupole moments (MQM) appear in nuclei with a quadrupole deformation (which have ordinary $T$,$P$-conserving collective electric quadrupole moments). Nuclei with an octupole deformation have a collective electric octupole moment, electric dipole moment (EDM), Schiff moment and MQM in the intrinsic frame which rotates with the nucleus. In a state with definite angular momentum in the laboratory frame, these moments are forbidden by $T$ and $P$ conservation, meaning their ex…
Octupole deformation results in a strongly enhanced collective Schiff moment in 229Th nucleus. An additional enhancement of time reversal (T) and parity (P) violating effects (such as T,P-violating electric dipole moments) appears in the ground 1Sigma state and in the metastable 3Delta_1 state of diatomic molecule 229ThO. Similar enhancements exist in molecular ions 229ThOH+, 229ThF+ and 225,223RaOH+. Corresponding experiments may be used to test CP-violation theories predicting T,P-violating nuclear forces and to search for axions.
We perform calculations of the CP-violating atomic and molecular electric dipole moments (EDM) induced by the interaction of the nuclear Schiff moments with electrons. EDM of atoms Eu, Dy, Gd, Ac, Th, Pa, U, Np and Pu are of special interest since they have isotopes with strongly enhanced nuclear Schiff moments caused by the octupole nuclear deformation or soft octupole vibration mode. These atoms have open 4f or 5f shells making the calculations complicated. We use our special version of the configuration interaction method combined with the many-body perturbation theory method adopted for op…
We have calculated the atomic electric dipole moments (EDMs) induced in 229Pa and 225Ac by their respective nuclear Schiff moments S. The results are d(229Pa)= - 9.5 10^{-17} [S/(e fm)] e cm= - 1.1 10^{-20} ηe cm; d(225Ac})=- 8.6 10^{-17} [S/(e fm)] e cm=- 0.8 10^{-21} ηe cm. EDM of 229 Pa is 3 10^4 times larger than 199Hg EDM and 40 times larger than 225Ra EDM. Possible use of actinides in solid state experiments is also discussed. The T,P-odd spin-axis interaction in RaO molecule is 500 times larger than in TlF.
The discovery of the atomic electric dipole moment (EDM) would reveal the simultaneous violation of parity (P) and time-reversal (T) invariance. The EDM can be induced by T-odd forces between the nucleus and atomic electrons. As the nuclear dipole moment is screened according to the Schiff theorem, the appropriate nuclear operator is the Schiff moment that may exist in nuclei under PT-violation. We briefly review the current experimental situation and discuss more in detail the ideas concerning possible collective mechanisms for the enhancement of the nuclear Schiff moment. The most promising …
Parity and time invariance violating forces produce collective P- and T- odd moments in nuclei with static octupole deformation. Collective Schiff moment, electric octupole and dipole and also magnetic quadrupole appear due to the mixing of rotational levels of opposite parity and can exceed single-particle moments by more than a factor of 100. This enhancement is due to two factors, the collective nature of the intrinsic moments and the small energy separation between members of parity doublets. The above moments induce T- and P- odd effects in atoms and molecules. Experiments with such syste…
Nuclei with an octupole deformation have a non-zero electric octupole moment, electric dipole moment (EDM), Schiff moment and magnetic quadrupole moment (MQM) in the intrinsic frame which rotates with the nucleus. In a state with definite angular momentum in the laboratory frame, these moments are forbidden by parity (P) and time reversal invariance (T) conservation, meaning their expectation values vanish due to nuclear rotation. However, nuclei with an octupole deformation have doublets of close opposite parity rotational states with the same spin, which are mixed by T,P-odd nuclear forces. …
The cranked relativistic Hartree-Bogoliubov (CRHB) theory has been applied for a systematic study of pairing and rotational properties of actinides and light superheavy nuclei. Pairing correlations are taken into account by the Brink-Booker part of finite range Gogny D1S force. For the first time in the covariant density functional theory (CDFT) framework the pairing properties are studied via the quantities (such as three-point $Δ^{(3)}$ indicators) related to odd-even mass staggerings. The investigation of the moments of inertia at low spin and the $Δ^{(3)}$ indicators shows the need for an …
