Unveiling the mechanisms of the spin Hall effect in Ta
Edurne Sagasta, Yasutomo Omori, Saül Vélez, Roger Llopis, Christopher Tollan, Andrey Chuvilin, Luis E. Hueso, Martin Gradhand, YoshiChika Otani, Fèlix Casanova
备注：
9 pages and 4 figures + Supplemental Material (2 pages, 3 figures)
Spin-to-charge current interconversions are widely exploited for the generation and detection of pure spin currents and are key ingredients for future spintronic devices including spin-orbit torques and spin-orbit logic circuits. In case of the spin Hall effect, different mechanisms contribute to the phenomenon and determining the leading contribution is peremptory for achieving the largest conversion efficiencies. Here, we experimentally demonstrate the dominance of the intrinsic mechanism of the spin Hall effect in highly-resistive Ta. We obtain an intrinsic spin Hall conductivity for $β$-Ta of -820$\pm$120 ($\hbar$/e) $Ω^{-1}cm^{-1}$ from spin absorption experiments in a large set of lateral spin valve devices. The predominance of the intrinsic mechanism in Ta allows us to linearly enhance the spin Hall angle by tuning the resistivity of Ta, reaching up to -35$\pm$3%, the largest reported value for a pure metal.
The quantum localization in the quantum Hall regime is revisited using Graphene monolayers with accurate measurements of the longitudinal resistivity as a function of temperature and current. We experimentally show for the first time a cross-over from Efros-Shklovskii Variable Range Hopping (VRH) conduction regime with Coulomb interactions to a Mott VRH regime without interaction. This occurs at Hall plateau transitions for localization lengths larger than the interaction screening length set by the nearby gate. Measurements of the scaling exponents of the conductance peak widths with both tem…
Magnons enable transferring a magnetic moment or spin over macroscopic distance. In quantum Hall ferromagnet, it has been predicted in the early 90s that spin and charges are entangled, meaning that any change of the spin texture modifies the charge distribution. As a direct consequence of this entanglement, magnons carry an electric dipole moment. Here we report the first evidence of the existence of this electric dipole moment in a graphene quantum Hall ferromagnet using a Mach-Zehnder interferometer as a quantum sensor. By propagating towards the interferometer through an insulating bulk, t…
Unveiling Topological Fusion in Quantum Hall Systems from Microscopic Principles
Jagiellonian University（雅盖隆大学）；Max-Planck-Institut für Quantenoptik（马克斯·普朗克量子光学研究所）；Munich Center for Quantum Science and Technology（慕尼黑量子科学与工程中心）；Princeton University（普林斯顿大学）；Karlstads Universitet（卡尔斯特大学）；Institute for Advanced Study, Princeton（普林斯顿高等研究院）；Indiana University（印第安纳大学）
Recent discovery of spin-orbit torques (SOTs) within magnetic single-layers has attracted attention in the field of spintronics. However, it has remained elusive as to how to understand and how to tune the SOTs. Here, utilizing the single layers of chemically disordered Fe$_x$Pt$_{1-x}$, we unveil the mechanism of the "unexpected" bulk SOTs by studying their dependence on the introduction of a controlled vertical composition gradient and on temperature. We find that the bulk damping like SOT arises from an imbalanced internal spin current that is transversely polarized and independent of the m…
Collective modes of exotic quantum fluids reveal underlying physical mechanisms responsible for emergent complex quantum ground states. We observe unexpected new collective modes in the fractional quantum Hall (FQH) regime: intra-Landau-level plasmons in the second Landau level measured by resonant inelastic light scattering. The plasmons herald rotational-symmetry-breaking phases in tilted magnetic fields and reveal long-range translational invariance in these phases. The fascinating dependence of plasmon features on filling factor provide new insights on interplays between topological quantu…
The perpendicular magnetic anisotropy (PMA) at magnetic transition metal/oxide interfaces is a key element in building out-of-plane magnetized magnetic tunnel junctions for spin-transfer-torque magnetic random access memory (STT-MRAM). Size downscaling renders magnetic properties more sensitive to thermal effects. Thus, understanding the temperature dependence of the magnetic anisotropy is crucial. In this work, we theoretically address the correlation between temperature dependence of PMA and magnetization in typical Fe/MgO-based structures. In particular, the possible mechanisms behind the e…
We report an investigation of the spin- to charge-current conversion in sputter-deposited films of topological insulator $Bi_2Se_{3}$ onto single crystalline layers of YIG $(Y_{3}Fe_{5}O_{12})$ and polycrystalline films of Permalloy $(Py = Ni_{81}Fe_{19})$. Pure spin current was injected into the $Bi_{2}Se_{3}$ layer by means of the spin pumping process in which the spin precession is obtained by exciting the ferromagnetic resonance of the ferromagnetic film. The spin-current to charge-current conversion, occurring at the $Bi_{2}Se_{3}/$ferromagnet interface, was attribute to the inverse Rashb…
In order to describe correctly the interplay of extrinsic and intrinsic spin-orbit mechanisms to the spin Hall effect, it is necessary to consider different sources of spin relaxation. We take into account the spin relaxation time $τ_{DP}$ due to the Dyakonov-Perel mechanism as well as the Elliot-Yafet spin-relaxation time $τ_s$ due to the spin-orbit scattering from impurities. The total spin Hall conductivity depends crucially on the ratio $τ_s /τ_{DP}$.
Symplectic connection third-order Hall effect in a room-temperature ferromagnet
Tsung-Dao Lee Institute, Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), School of Physics and Astronomy, Shanghai Jiao Tong University（上海交大李政道研究所，教育部人工结构与量子控制重点实验室，物理与天文学院，上海交通大学）；Interdisciplinary Center for Theoretical Physics and Information Sciences (ICTPIS), Fudan University（复旦大学理论物理与信息科学交叉中心）；School of Physics, Beihang University（北京航空航天大学物理学院）；Shanghai Engineering Research Center of Energy Efficient and Custom AI IC, School of Information Science and Technology, ShanghaiTech University（上海科技大学信息科学与技术学院，能效与定制AI集成电路上海市工程研究中心）；Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology and School of Physics Science and Engineering, Tongji University（同济大学物理科学与工程学院，特种人工微结构材料与技术上海市重点实验室）；Research Laboratory for Quantum Materials, Department of Applied Physics, The Hong Kong Polytechnic University（香港理工大学应用物理系，量子材料研究实验室）
We theoretically study the interplay between bulk Weyl electrons and magnetic topological defects, including magnetic domains, domain walls, and $\mathbb{Z}_6$ vortex lines, in the antiferromagnetic Weyl semimetals \mnsn\ and Mn$_3$Ge with negative vector chirality. We argue that these materials possess a hierarchy of energies scales which allows a description of the spin structure and spin dynamics using a XY model with $\mathbb{Z}_6$ anisotropy. We propose a dynamical equation of motion for the XY order parameter, which implies the presence of $\mathbb{Z}_6$ vortex lines, the double-domain p…
Unveiling the impact of anti-site defects in magnetic transitions of few-layer MnBi2Te4 by operando heating
State Key Laboratory of Surface Physics and Department of Physics, Fudan University（复旦大学表面物理国家重点实验室和物理系）；Institute for Nanoelectronic Devices and Quantum Computing, Fudan University（复旦大学纳米电子器件与量子计算研究所）；Key Laboratory of Micro and Nano Photonic Structures (MOE), Fudan University（复旦大学微纳光子结构教育部重点实验室）；Shanghai Branch, Hefei National Laboratory（合肥国家实验室上海分部）；Shanghai Research Center for Quantum Sciences（上海量子科学研究中心）；New Cornerstone Science Laboratory（新基石科学实验室）
Magnetic skyrmions are topologically wound nanoscale textures of spins whose ambient stability and electrical manipulation in multilayer films have led to an explosion of research activities. While past efforts focused predominantly on isolated skyrmions, recently ensembles of chiral spin textures, consisting of skyrmions and magnetic stripes, were shown to possess rich interactions with potential for device applications. However, several fundamental aspects of chiral spin texture phenomenology remain to be elucidated, including their domain wall structure, thermodynamic stability, and morphol…
Recently, it has been known that the hidden Rashba (R-2) effect in two-dimensional materials gives rise to a novel physical phenomenon called spin-layer locking (SLL). However, not only has its underlying fundamental mechanism been unclear, but also there are only a few materials exhibiting weak SLL. Here, through the first-principles density functional theory and model Hamiltonian calculation, we reveal that the R-2 SLL can be determined by the competition between the sublayer-sublayer interaction and the spin-orbit coupling (SOC), which is related to the Rashba strength. In addition, the orb…
We propose a mechanism of intrinsic spin Hall effect (SHE). In this mechanism, local orbital angular momentum (OAM) induces electron position shift and couples with the bias electric field to generate orbital Hall effect (OHE). SHE then emerges as a concomitant effect of OHE through the atomic spin-orbit coupling. Spin Hall conductivity due to this mechanism is estimated to be comparable to experimental values for heavy metals. This mechanism predicts the sign change of the spin Hall conductivity as the spin-orbit polarization changes its sign, and also correlation between the spin Hall conduc…
