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arXiv 1801.02018cond-mat.mtrl-sci
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准一维Ta2NiSe7中电荷密度波的带相关性

Band dependence of charge density wave in quasi-one-dimensional Ta2NiSe7 probed by orbital magnetoresistance

Jiaming He, Yiran Zhang, Libin Wen, Yusen Yang, Jinyu Liu, Yueshen Wu, Hailong Lian, Hui Xing, Shun Wang, Zhiqiang Mao, Ying Liu

摘要:

Ta2NiSe7是一种准一维(准一维)过渡金属硫属化合物,具有Ta和Ni链状结构。一个无公度的电荷密度波(CDW)在这个准一维结构的研究,以前使用隧道谱,X射线和电子衍射,而其输运性质和潜在的电子状态的关系仍有待探讨。在这里,我们报告我们的磁电阻(MR)的Ta2NiSe7的结果。当进入CDW状态时,发现科勒规则的崩溃。同时,观察到MR的场依赖性中的曲率的明显变化。我们发现,曲率的变化是很好地描述了两个频带的轨道MR,与空穴密度被强烈抑制在CDW状态,表明$p$轨道从硒原子占主导地位的变化,通过CDW过渡的运输。

英文摘要:

Ta2NiSe7 is a quasi-one-dimensional (quasi-1D) transition-metal chalcogenide with Ta and Ni chain structure. An incommensurate charge-density wave (CDW) in this quasi-1D structure was well studied previously using tunnelling spectrum, X-ray and electron diffraction, whereas its transport property and the relation to the underlying electronic states remain to be explored. Here we report our results of magnetoresistance (MR) on Ta2NiSe7. A breakdown of the Kohler's rule is found upon entering the CDW state. Concomitantly, a clear change of curvature in the field dependence of MR is observed. We show that the curvature change is well described by two-band orbital MR, with the hole density being strongly suppressed in the CDW state, indicating that the $p$ orbitals from Se atoms dominate the change in transport through the CDW transition.

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