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arXiv 1707.08784cond-mat.str-el
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电子自旋共振法探测长程自旋有序

Electron spin resonance for the detection of long-range spin nematic order

Shunsuke C. Furuya, Tsutomu Momoi

摘要:

在本文中,我们提出,电子自旋共振(ESR)测量使我们能够检测到的长程自旋有序。结果表明,铁四极序参量与其它参量一起使ESR谱中的顺磁共振峰的频率发生移动。铁四极序参量可从频移的角度依赖性中提取。相反,反铁四极序参量在频移中通常是不可见的。相反,长程反铁四极序在ESR谱中产生一个特征共振峰,我们称之为磁振子对共振峰。该共振对应于波矢$\bm k={\bm 0}$处的束缚磁振子对的激发。磁振子对共振频率的场依赖性反映了束缚磁振子对的凝聚,在饱和场处表现出奇异的上弯。此外,磁振子对共振峰的强度表现出特征的角度依赖性,当磁场平行于对角化弱各向异性相互作用的轴之一时,它消失。我们通过在线性味波近似下研究正方晶格上的$S=1$双线性-双二次模型,证实了自旋π相位中磁振子对共振峰的这些一般性质。此外,我们还讨论了$S=1/2$阻挫铁磁体和$S=1/2$正交二聚体自旋系统SrCu $_2$(BO $_3$)$_2$的应用,这两种材料都是自旋向列相的候选材料.我们的反铁四极有序相的理论是一致的磁振子对共振峰实验观察到的SrCu $_2$(BO $_3$)$_2$的低磁化制度的许多功能。

英文摘要:

In this paper we propose that electron spin resonance (ESR) measurements enable us to detect the long-range spin nematic order. We show that the frequency of the paramagnetic resonance peak in the ESR spectrum is shifted by the ferroquadrupolar order parameter together with other quantities. The ferroquadrupolar order parameter is extractable from the angular dependence of the frequency shift. In contrast, the antiferroquadrupolar order parameter is usually invisible in the frequency shift. Instead, the long-range antiferroquadrupolar order yields a characteristic resonance peak in the ESR spectrum, which we call a magnon-pair resonance peak. This resonance corresponds to the excitation of the bound magnon pair at the wave vector $\bm k={\bm 0}$. Reflecting the condensation of bound magnon pairs, the field dependence of the magnon-pair resonance frequency shows a singular upturn at the saturation field. Moreover, the intensity of the magnon-pair resonance peak shows a characteristic angular dependence and it vanishes when the magnetic field is parallel to one of the axes that diagonalize the weak anisotropic interactions. We confirm these general properties of the magnon-pair resonance peak in the spin nematic phase by studying an $S=1$ bilinear-biquadratic model on the square lattice in the linear flavor-wave approximation. In addition, we argue applications to the $S=1/2$ frustrated ferromagnets and also the $S=1/2$ orthogonal dimer spin system SrCu$_2$(BO$_3$)$_2$, both of which are candidate materials of spin nematics. Our theory for the antiferroquadrupolar ordered phase is consistent with many features of the magnon-pair resonance peak experimentally observed in the low-magnetization regime of SrCu$_2$(BO$_3$)$_2$.

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