We present a formalism to calculate the orbital magnetization of interacting Dirac fermions under a magnetic field. In this approach, the divergence difficulty is overcome with a special limit of the derivative of the thermodynamic potential with respect to the magnetic field. The formalism satisfies the particle-hole symmetry of the Dirac fermions system. We apply the formalism to the interacting Dirac fermions in graphene. The charge and spin orderings and the exchange interactions between all the Landau levels are taken into account by the mean-field theory. The results for the orbital magnetization of interacting Dirac fermions are compared with that of non-interacting cases.
The aim of this work is to describe the spin magnetization of graphene with Rashba spinorbit coupling and Zeeman effect. It is shown that the magnetization depends critically on the spin-orbit coupling l that is controlled with an external electric field. In turn, by manipulating the density of charge carriers, it is shown that spin up and down Landau levels mix introducing jumps in the spin magnetization. Two magnetic oscillations phases are described that can be tunable through the applied external fields. The maximum and minimum of the oscillations can be alternated by taking into account h…
With a conserving formalism within the self-consistent Born approximation, we study the Hall conductivity of Dirac fermions in graphene under charged impurity scatterings. The calculated inverse Hall coefficient is compared with the experimental data. It is shown that the present calculations for the Hall coefficient and the electric conductivity are in good agreement with the experimental measurements.
We study the effects of the rippling of the graphene sheet on the quasiparticle dispersion. This is achieved using a generalization to the honeycomb lattice of the Momentum Average approximation, which is accurate for all coupling strengths and at all energies. We show that even though the position of the Dirac points may move and the Fermi speed can be renormalized significantly, quasiparticles with very long lifetimes survive near the Dirac points even for very strong couplings.
Epitaxial graphene on Ir(111) prepared in excellent structural quality is investigated by angle-resolved photoelectron spectroscopy. It clearly displays a Dirac cone with the Dirac point shifted only slightly above the Fermi level. The moire resulting from the overlaid graphene and Ir(111) surface lattices imposes a superperiodic potential giving rise to Dirac cone replicas and the opening of minigaps in the band structure.
We study the role of long-range electron-electron interactions in a system of two-dimensional anisotropic Dirac fermions, which naturally appear in uniaxially strained graphene, graphene in external potentials, some strongly anisotropic topological insulators, and engineered anisotropic graphene structures. We find that while for small interactions and anisotropy the system restores the conventional isotropic Dirac liquid behavior, strong enough anisotropy can lead to the formation of a quasi-one dimensional electronic phase with dominant charge order (anisotropic excitonic insulator).
The coupling of monochromatic light fields and solids introduces nonequilibrium Floquet states, offering opportunities to create and explore new topological phenomena. Using combined first-principles and Floquet analysis we show that one can freely engineer Floquet-Dirac fermions (FDFs) in graphene by tuning the frequency and intensity of linearly polarized light. Not only type-II FDFs are created, but they also coexist with type-I FDFs near the Fermi level. Intriguingly, novel topologically nontrivial edge states connecting type-I and type-II Floquet-Dirac points emerge in photodriven graphen…
Motivated by the results of recent photoemission and tunneling studies, we discuss potential many-body sources of a finite gap in the Dirac fermion spectrum of graphene. Specifically, we focus on the putative Peierls- and Cooper-like pairing instabilities which can be driven by sufficiently strong Coulomb and electron-phonon interactions, respectively. Our results compare favorably with the available experimental and Monte Carlo data.
Tuning interactions between Dirac states in graphene has attracted enormous interest because it can modify the electronic spectrum of the two-dimensional material, enhance electron correlations, and give rise to novel condensed-matter phases such as superconductors, Mott insulators, Wigner crystals and quantum anomalous Hall insulators. Previous works predominantly focus on the flat band dispersion of coupled Dirac states from different graphene layers. In this work, we propose a new route to realizing flat band physics in monolayer graphene under a periodic modulation from substrates. We take…
Theory of nuclear magnetic resonance (NMR) in graphene is presented. The canonical form of the electron-nucleus hyperfine interaction is strongly modified by the linear electronic dispersion. The NMR shift and spin-lattice relaxation time are calculated as function of temperature, chemical potential, and magnetic field and three distinct regimes are identified: Fermi-, Dirac-gas, and extreme quantum limit behaviors. A critical spectrometer assessment shows that NMR is within reach for fully 13C enriched graphene of reasonable size.
We study interacting Dirac quasiparticles in disordered graphene and find that an interplay between the unscreened Coulomb interactions and pseudo-relativistic quasiparticle kinematics can be best revealed in the ballistic regime, whereas in the diffusive limit the behavior is qualitatively (albeit, not quantitatively) similar to that of the ordinary 2DEG with parabolic dispersion. We calculate the quasiparticle width and density of states that can be probed by photoemission, tunneling, and magnetization measurements.
The derivation for the transport coefficients of an electron system in the presence of temperature gradient and the electric and magnetic fields are presented. The Nernst conductivity and the transverse thermoelectric power of the Dirac fermions in graphene under charged impurity scatterings and weak magnetic field are calculated on basis of the self-consistent Born approximation. The result is compared with so far the available experimental data.
It is shown that in the absence of spontaneous symmetry breaking the Dirac cones in the system of interacting electrons on honeycomb lattice are isotropic at low energies. The effect is due to the $Z_3$ subgroup of the $D_3$ symmetry group of the dispersion relation of Dirac quasiparticles. Consequences of the violations of the $Z_3$ or the sublattice symmetry are discussed.
Three symmetries prevent a twisted bilayer of graphene from developing an in-plane spontaneous magnetization in the absence of a magnetic field - time reversal symmetry, $C_2$ symmetry to $π$ rotation and $C_3$ symmetry to $2π/3$ rotation. In contrast, there are experimental and theoretical indications that, at certain electron densities, time reversal and $C_2$ symmetries are broken spontaneously, while the $C_3$ symmetry is often broken due to strain. We show that in-plane orbital magnetization is a very sensitive probe to the simultaneous breaking of these three symmetries, exhibiting surpr…
The quasi-2D electrons in graphene behave as massless fermions obeying a Dirac-Weyl equation in the low-energy regime near the two Fermi points. The stability of spin-polarized phases (SPP) in graphene is considered. The exchange energy is evaluated from the analytic pair-distribution functions, and the correlation energies are estimated via a closely similar four-component 2D electron fluid which has been investigated previously. SPPs appear for sufficiently high doping, when the exchange energy alone is considered. However, the inclusion of correlations is found to {\it suppress} the spin-ph…
Spectral analysis of Shubnikov de Haas (SdH) oscillations of magnetoresistance and of Quantum Hall Effect (QHE) measured in quasi-2D highly oriented pyrolytic graphite (HOPG) [Phys. Rev. Lett. 90, 156402 (2003)] reveals two types of carriers: normal (massive) electrons with Berry phase 0 and Dirac-like (massless) holes with Berry phase pi. We demonstrate that recently reported integer- and semi-integer QHE for bi-layer and single-layer graphenes take place simultaneously in HOPG samples.
Electrons in quantum materials exhibiting coexistence of dispersionless (flat) bands piercing dispersive (steep) bands can give rise to strongly correlated phenomena, and are associated with unconventional superconductivity. It is known that in twisted trilayer graphene steep Dirac cones can coexist with band flattening, but the phenomenon is not stable under layer misalignments. Here we show that such a twisted sandwiched graphene (TSWG) -- a three-layer van der Waals heterostructure with a twisted middle layer -- can have very stable flat bands coexisting with Dirac cones near the Fermi ener…
Using density-functional theory, we calculate the electronic bandstructure of single-layer graphene on top of hexagonal In_2Te_2 monolayers. The geometric configuration with In and Te atoms at centers of carbon hexagons leads to a Kekule' texture with an ensuing bandgap of 20 meV. The alternative structure, nearly degenerate in energy, with the In and Te atoms on top of carbon sites is characterized instead by gapless spectrum with the original Dirac cones of graphene reshaped, depending on the graphene-indium chalcogenide distance, either in the form of an undoubled pseudo-spin one Dirac cone…
Graphene, the atomic-thin layer of carbon atoms, was first isolated on an insulating substrate in 2004 by two groups in Manchester University [1, 2] and Columbia [3]. Those milestone experiments established the Dirac nature of the charge carriers in graphene. The same year, C.L. Kane and E.G. Mele predicted that intrinsic spin-orbit coupling in graphene, if strong enough, would lead to a novel state of electronic matter called the Quantum Spin Hall (QSH) state [4, 5]. The QSH state is characterized by conducting gapless edge states circulating around an insulating bulk. Those edge states are p…
Recent studies show that periodic potentials can generate superlattice Dirac points at energies in graphene (is the Fermi velocity of graphene and G is the reciprocal superlattice vector). Here, we perform scanning tunneling microscopy and spectroscopy studies of a corrugated graphene monolayer on Rh foil. We show that the quasi-periodic ripples of nanometer wavelength in the corrugated graphene give rise to weak one-dimensional (1D) electronic potentials and thereby lead to the emergence of the superlattice Dirac points. The position of the superlattice Dirac point is space-dependent and show…
The analytical expressions for both diagonal and off-diagonal ac and dc conductivities of graphene placed in an external magnetic field are derived. These conductivities exhibit rather unusual behavior as functions of frequency, chemical potential and applied field which is caused by the fact that the quasiparticle excitations in graphene are Dirac-like. One of the most striking effects observed in graphene is the odd integer quantum Hall effect. We argue that it is caused by the anomalous properties of the Dirac quasiparticles from the lowest Landau level. Other quantities such as Hall angle …
We compute the magnetization of graphene in a magnetic field, taking into account for generality the possibility of a mass gap. We concentrate on the physical regime where quantum oscillations are not observed due to the effect of the temperature or disorder and show that the magnetization exhibits non-linear behaviour as a function of the applied field, reflecting the strong non-analyticity of the two-dimensional effective action of Dirac electrons. The necessary values of the magnetic field to observe this non-linearity vary from a few Teslas for very clean suspended samples to 20 - 30 Tesla…
We report measurements of the cyclotron mass in graphene for carrier concentrations n varying over three orders of magnitude. In contrast to the single-particle picture, the real spectrum of graphene is profoundly nonlinear so that the Fermi velocity describing the spectral slope reaches ~3x10^6 m/s at n <10^10 cm^-2, three times the value commonly used for graphene. The observed changes are attributed to electron-electron interaction that renormalizes the Dirac spectrum because of weak screening. Our experiments also put an upper limit of ~0.1 meV on the possible gap in graphene.
A recently constructed model for low lying excitations in bilayer graphene exhibits mid-gap, zero energy modes in its Dirac-like spectrum, when a scalar order parameter takes a vortex profile. We show that these modes persist when the dynamics is extended by a gauge field interaction, which also renders finite the vortex energy. The effect of the gauge field on the zero energy wave function is to shift the phase of the (damped) oscillatory component of the wave function in the absence of the gauge field.
