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arXiv 1702.02782cond-mat.supr-concond-mat.str-el
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轨道杂化掺杂铜氧化物超导体中的阻尼自旋激发

Damped spin excitations in a doped cuprate superconductor with orbital hybridization

O. Ivashko, N. E. Shaik, X. Lu, C. G. Fatuzzo, M. Dantz, P. G. Freeman, D. E. McNally, D. Destraz, N. B. Christensen, T. Kurosawa, N. Momono, M. Oda, C. Monney,… 展开作者

O. Ivashko, N. E. Shaik, X. Lu, C. G. Fatuzzo, M. Dantz, P. G. Freeman, D. E. McNally, D. Destraz, N. B. Christensen, T. Kurosawa, N. Momono, M. Oda, C. Monney, H. M. Rønnow, T. Schmitt, J. Chang

摘要:

用共振非弹性X射线散射(RIXS)方法研究了轻微欠掺杂La $_{2-x}$ Sr $_{x}$ CuO $_4$(LSCO)与$x=0.12$和$0.145$的过阻尼自旋激发.研究了三个高对称方向:(1)波腹$(0,0)\rightarrow (1/2,0)$,(2)波节$(0,0)\rightarrow (1/4,1/4)$和(3)连接这两个方向的区域边界方向$(1/2,0)\rightarrow (1/4,1/4)$。过阻尼激励沿(1)和(3)表现出很强的色散,而沿(2)则表现出较弱的色散。这与未掺杂的化合物La $_{2}$ CuO $_4$(LCO)形成强烈对比,其中沿着(1)和(2)发现最强的色散。用于解释LCO的激发光谱的$t-t^{\prime}-t^{\prime\prime}-U$ Hubbard模型预测$-$为常数$U/t$ $-$,沿着(3)的分散与$(t^{\prime}/t)^2$成比例。然而,使用单带模型在LSCO上提取的对角跳跃$t^{\prime}$是低的($t^{\prime}/t\sim-0.16$)并且随着掺杂而降低。因此,我们调用了一个双轨道($d_{x^2-y^2}$和$d_{z^2}$)模型,这意味着$t^{\prime}$增强。这种效应的作用,以提高区域边界内的扩散哈伯德模型。因此,我们得出结论,$d_{x^2-y^2}$和$d_{z^2}$状态的杂化对LSCO中的区边界色散具有显著影响。

英文摘要:

A resonant inelastic x-ray scattering (RIXS) study of overdamped spin-excitations in slightly underdoped La$_{2-x}$Sr$_{x}$CuO$_4$ (LSCO) with $x=0.12$ and $0.145$ is presented. Three high-symmetry directions have been investigated: (1) the antinodal $(0,0)\rightarrow (1/2,0)$, (2) the nodal $(0,0)\rightarrow (1/4,1/4)$ and (3) the zone boundary direction $(1/2,0)\rightarrow (1/4,1/4)$ connecting these two. The overdamped excitations exhibit strong dispersions along (1) and (3), whereas a much more modest dispersion is found along (2). This is in strong contrast to the undoped compound La$_{2}$CuO$_4$ (LCO) for which the strongest dispersions are found along (1) and (2). The $t-t^{\prime}-t^{\prime\prime}-U$ Hubbard model used to explain the excitation spectrum of LCO predicts $-$ for constant $U/t$ $-$ that the dispersion along (3) scales with $(t^{\prime}/t)^2$. However, the diagonal hopping $t^{\prime}$ extracted on LSCO using single-band models is low ($t^{\prime}/t\sim-0.16$) and decreasing with doping. We therefore invoked a two-orbital ($d_{x^2-y^2}$ and $d_{z^2}$) model which implies that $t^{\prime}$ is enhanced. This effect acts to enhance the zone-boundary dispersion within the Hubbard model. We thus conclude that hybridization of $d_{x^2-y^2}$ and $d_{z^2}$ states has a significant impact on the zone-boundary dispersion in LSCO.

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