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arXiv 1808.01682cond-mat.supr-con
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单层(Bi,Pb)$_{2}$(Sr,La)$_{2}$ CuO $_{6+δ}$铜酸盐超导体族中自旋激发的色散、阻尼和强度

Dispersion, damping, and intensity of spin excitations in the single-layer (Bi,Pb)$_{2}$(Sr,La)$_{2}$CuO$_{6+δ}$ cuprate superconductor family

Y. Y. Peng, E. W. Huang, R. Fumagalli, M. Minola, Y. Wang, X. Sun, Y. Ding, K. Kummer, X. J. Zhou, N. B. Brookes, B. Moritz, L. Braicovich, T. P. Devereaux, G. Ghiringhelli

摘要:

本文利用$L_3$边缘共振非弹性X射线散射(RIXS)方法,测量了高$T_\mathrm{c}$超导体(Bi,Pb)$_{2}$(Sr,La)$_{2}$ CuO $_{6+δ}$(Bi 2201)中自旋激发(磁振子和顺磁振子)的色散和阻尼。选定的测量与充分的偏振分析明确地证明了这些激发的自旋翻转字符,即使在过掺杂的样品。我们发现,无阻尼频率略有增加掺杂的所有可达的动量,而阻尼增长迅速,更快地在(0,0)$\rightarrow$(0.5,0.5)的节方向比(0,0)$\rightarrow$(0.5,0)的波腹方向。我们比较实验结果的数值精确的决定性量子蒙特卡罗(DQMC)计算,提供自旋动力学结构因子$S(\textbf{Q},ω)$的三带哈伯德模型。该理论再现以及磁激发的色散和谱权重的动量和掺杂的依赖性。这些结果提供了令人信服的证据表明,顺磁,虽然越来越阻尼,坚持整个超导圆顶的铜酸盐相图,这意味着远程反铁磁相关很快被冲走,而短程磁相互作用几乎没有受到掺杂的影响。

英文摘要:

Using Cu-$L_3$ edge resonant inelastic x-ray scattering (RIXS) we measured the dispersion and damping of spin excitations (magnons and paramagnons) in the high-$T_\mathrm{c}$ superconductor (Bi,Pb)$_{2}$(Sr,La)$_{2}$CuO$_{6+δ}$ (Bi2201), for a large doping range across the phase diagram ($0.03\lesssim p\lesssim0.21$). Selected measurements with full polarization analysis unambiguously demonstrate the spin-flip character of these excitations, even in the overdoped sample. We find that the undamped frequencies increase slightly with doping for all accessible momenta, while the damping grows rapidly, faster in the (0,0)$\rightarrow$(0.5,0.5) nodal direction than in the (0,0)$\rightarrow$(0.5,0) antinodal direction. We compare the experimental results to numerically exact determinant quantum Monte Carlo (DQMC) calculations that provide the spin dynamical structure factor $S(\textbf{Q},ω)$ of the three-band Hubbard model. The theory reproduces well the momentum and doping dependence of the dispersions and spectral weights of magnetic excitations. These results provide compelling evidence that paramagnons, although increasingly damped, persist across the superconducting dome of the cuprate phase diagram; this implies that long range antiferromagnetic correlations are quickly washed away, while short range magnetic interactions are little affected by doping.

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