We investigate the optical response of strongly disordered quantum Hall states in two-dimensional Dirac materials and find qualitatively different effects in the radiation properties of the bulk versus the edge. We show that the far-field radiation from the edge is characterized by large multipole moments (> 50) due to the efficient transfer of angular momentum from the electrons into the scattered light. The maximum multipole transition moment is a direct measure of the coherence length of the edge states. Accessing these multipole transitions would provide new tools for optical spectroscopy and control of quantum Hall edge states. On the other hand, the far-field radiation from the bulk appears as random dipole emission with spectral properties that vary with the local disorder potential. We determine the conditions under which this bulk radiation can be used to image the disorder landscape. Such optical measurements can probe sub-micron length scales over large areas and provide complementary information to scanning probe techniques. Spatially resolving this bulk radiation would serve as a novel probe of the percolation transition near half-filling.
The effective action for low-energy excitations of Laughlin's states is obtained by systematic expansion in inverse powers of the magnetic field. It is based on the W-infinity symmetry of quantum incompressible fluids and the associated higher-spin fields. Besides reproducing the Wen and Wen-Zee actions and the Hall viscosity, this approach further indicates that the low-energy excitations are extended objects with dipolar and multipolar moments.
Various nonlinear characteristics of solid states, such as the circular photogalvanic effect of time-reversal symmetric insulators, the quantized photogalvanic effect of Weyl semimetals, and the nonlinear Hall effect of time-reversal symmetric metals, have been associated with the Berry curvature dipole (BCD). Here, we explore the question of whether the Berry curvature dipole and multipoles of time-reversal symmetric insulators can be traced in the nonlinear optical responses. We performed real-time time-dependent density functional theory calculations and examined the second harmonic generat…
Graphene bilayers with layer antisymmetric strains are studied using the Dirac-Harper model for a pair of single layer Dirac Hamiltonians coupled by a one-dimensional moiré-periodic interlayer tunneling amplitude. This model hosts low energy, nearly dispersionless bands near charge neutrality that support anomalous polarizations of its charge multipole distributions. These are analyzed introducing a generalized Berry curvature that encodes the field-induced dynamics of multipole fields allowed in a chiral medium with time reversal symmetry. The formulation identifies a reciprocity relation bet…
Employing the quantum Liouville equation with phenomenological dissipation, we investigate the transport properties of massless and massive Dirac fermion systems that mimics graphene and topological insulators, respectively. The massless Dirac fermion system does not show an intrinsic Hall effect, but it shows a Hall current under the presence of circularly-polarized laser fields as a nature of a optically-driven nonequilibrium state. Based on the microscopic analysis, we find that the light-induced Hall effect mainly originates from the imbalance of photocarrier distribution in momentum space…
We propose an unconventional type of Hall effect in a topological Dirac semimetal with ferromagnetic electrodes. The topological Dirac semimetal itself has time-reversal symmetry, whereas attached ferromagnetic electrodes break it, causing the large Hall response. This induced Hall effect is a characteristic of the helical surface/edge states that arise in topological materials, such as topological Dirac semimetals or quantum spin Hall insulators. We compute the Hall conductance/resistance and the Hall angle by using a lattice model with four-terminal geometry. For topological Dirac semimetals…
In addition to the well known chiral anomaly, Dirac semimetals have been argued to exhibit mirror anomaly, close analogue to the parity anomaly of ($2+1$)-dimensional massive Dirac fermions. The observable response of such anomaly is manifested in a singular step-like anomalous Hall response across the mirror-symmetric plane in the presence of a magnetic field. Although this result seems to be valid in type-II Dirac semimetals (strictly speaking, in the linearized theory), we find that type-I Dirac semimetals do not possess such an anomaly in anomalous Hall response even at the level of the li…
We study the quantum Hall effect of Dirac fermions on the surface of a Wilson-Dirac type topological insulator thin film in the strong topological insulating phase. Although a magnetic field breaks time reversal symmetry of the bulk, the surface states can survive even in a strong field regime. We examine how the Landau levels of the surface states are affected by symmetry breaking perturbations.
We derive the effective field theory from the microscopic Hamiltonian of interacting two-dimensional (pseudo) Dirac electrons by performing a statistic gauge transformation. The quantized Hall conductance are expected to be $σ_{xy}=\frac{e^2}{h}(2k-1)$ with $k$ is arbitrary integer. There are also topological excitations which have fractional charge and obey fractional statistics.
The quantum Hall effect in graphene is regarded to be involving half-integer topological numbers associated with the massless Dirac particle, this is usually not apparent due to the doubling of the Dirac cones. Here we theoretically consider two classes of lattice models in which we manipulate the Dirac cones with either (a) two Dirac points that have mutually different energies, or (b) multiple Dirac cones having different Fermi velocities. We have shown, with an explicit calculation of the topological (Chern) number for case (a) and with an adiabatic argument for case (b) that the results ar…
We study the properties of an ultracold Fermi gas loaded in an optical square lattice and subjected to an external and classical non-Abelian gauge field. We show that this system can be exploited as an optical analogue of relativistic quantum electrodynamics, offering a remarkable route to access the exotic properties of massless Dirac fermions with cold atoms experiments. In particular we show that the underlying Minkowski space-time can also be modified, reaching anisotropic regimes where a remarkable anomalous quantum Hall effect and a squeezed Landau vacuum could be observed.
We present a theoretical analysis of two-dimensional Dirac-Rashba systems in the presence of disorder and external perturbations. We unveil a set of exact symmetry relations (Ward identities) that impose strong constraints on the spin dynamics of Dirac fermions subject to proximity-induced interactions. This allows us to demonstrate that an arbitrary dilute concentration of scalar impurities results in the total suppression of nonequilibrium spin Hall currents when only Rashba spin-orbit coupling is present. Remarkably, a finite spin Hall conductivity is restored when the minimal Dirac-Rashba …
We show that an electric field applied to a strained topological Dirac semimetal, such as Na3Bi and Cd3As2, induces a spin Hall current that is quadratic in the electric field. By regarding the strain as an effective "axial magnetic field" for the Dirac electrons, we investigate the electron and spin transport semiclassically in terms of the chiral kinetic theory. The nonlinear spin Hall effect arises as the cross effect between the regular Hall effect driven by the axial magnetic field and the anomalous Hall effect coming from the momentum-space topology. It provides an efficient way to gener…
While the quantum Hall effect in graphene has been regarded as a realization of the anomaly associated with the massless Dirac particle carrying half the usual topological integer, this is hidden due to the doubling of the Dirac cones. In order to confirm the half-integer contribution from each Dirac cone, here we theoretically consider a lattice model in which the relative energy between the two Dirac points is systematically shifted. With an explicit calculation of the topological (Chern) number, we have demonstrated that each Dirac cone does indeed contribute to the Hall conductivity as the…
We investigate the topological phase derived by time-reversal breaking fields in a nonsymmorphic symmetry-protected two-dimensional Dirac semimetal. When the nonsymmorphic symmetry is preserved even in the presence of the field, the two-dimensional electronic states change into two distinct topological phases with the insulating gap. One phase is well-known as quantum Hall states with chiral edge modes accompanying the Hall current, but the other one is an unconventional topological phase with helical edge modes in the absence of time-reversal symmetry.
We demonstrate evidences of electronic transport via topological Dirac surface states in a thin film of strained HgTe. At high perpendicular magnetic fields, we show that the electron transport reaches the quantum Hall regime with vanishing resistance. Furthermore, quantum Hall transport spectroscopy reveals energy splittings of relativistic Landau levels specific to coupled Dirac surface states. This study provides new insights in the quantum Hall effect of topological insulator (TI) slabs, in the cross-over regime between two- and three-dimensional TIs, and in the relevance of thin TI films …
We analyze the coupling of elastic lattice deformations to the magnon degrees of freedom of magnon Dirac materials. For a Honeycomb ferromagnet we find that, as it happens in the case of graphene, elastic gauge fields appear coupled to the magnon pseudospinors. For deformations that induce constant pseudomagnetic fields, the spectrum around the Dirac nodes splits into pseudoLandau levels. We show that when a Dzyaloshinskii-Moriya interaction is considered, a topological gap opens in the system and a Chern-Simons effective action for the elastic degrees of freedom is generated. Such a term enco…
Here we comprehensively investigate Landau levels, Hofstadter butterfly and transport properties of a semi-Dirac nanoribbon in a perpendicular magnetic field using a recently developed real-space implementation of the Kubo formula based on Kernel Polynomial Method. A Dirac ribbon is considered to compare and contrast our results for a semi-Dirac system. We find that the Landau levels being non-equidistant from each other for the semi-Dirac case (true for a Dirac as well), the flatness of the energy bands vanishes in the bulk and becomes dispersive for a semi-Dirac ribbon in contrast to a Dirac…
Hall effects are investigated for three-dimensional Dirac electrons as a model of bismuth alloys. It is found that there is unconventional contributions to the Hall conductivity $σ_{xy}$ generated by the interband effects of a magnetic field. This phenomena is remarkable near the band-edge. The Hall coefficient exhibits two unexpected properties; a sharp peak at around the band-edges, and a drastic sign change in the band gap region. Implications of the present results to bismuth alloys are discussed.
Dirac fermions are actively investigated, and the discovery of the quantized anomalous Hall effect of massive Dirac fermions has spurred the promise of low-energy electronics. Some materials hosting Dirac fermions are natural platforms for interlayer coherence effects such as Coulomb drag and exciton condensation. Here we determine the role played by the anomalous Hall effect in Coulomb drag in massive Dirac fermion systems. We focus on topological insulator films with out-of plane magnetizations in both the active and passive layers. The transverse response of the active layer is dominated by…
We review the recently proposed Dirac composite fermion theory of the half-filled Landau level. This paper is based on a talk given at the Nambu Symposium at University of Chicago, March 11-13, 2016.
We consider spin Hall effect in a system of massless Dirac fermions in a graphene lattice. Two types of spin-orbit interaction, pertinent to the graphene lattice, are taken into account - the intrinsic and Rashba terms. Assuming perfect crystal lattice, we calculate the topological contribution to spin Hall conductivity. When both interactions are present, their interplay is shown to lead to some peculiarities in the dependence of spin Hall conductivity on the Fermi level.
We experimentally investigate a non-linear Hall effect for three-dimensional WTe$_2$ and Cd$_3$As$_2$ single crystals, representing Weyl and Dirac semimetals, respectively. We observe finite second-harmonic Hall voltage, which depends quadratically on the longitudinal current in zero magnetic field. Despite this observation well corresponds to the theoretical predictions, only magnetic field dependence allows to distinguish the non-linear Hall effect from a thermoelectric response. We demonstrate that second-harmonic Hall voltage shows odd-type dependence on the direction of the magnetic field…
Observations of $ν=1$ Quantum Hall Effect and Inter-Band Effects of Magnetic fields on Hall Conductivity in Organic Massless Dirac Fermion System $α$-(BETS)$_2$I$_3$ under Pressure
本文在压力下的 α-(BETS)₂I₃ 有机无质量 Dirac 费米子体系中观测到 ν=1 量子 Hall 态，并通过化学势跨越 Dirac 点揭示了磁场对 Hall 电导率的带间效应。
The fractal spectrum of magnetic minibands (Hofstadter butterfly), induced by the moiré super- lattice of graphene on an hexagonal crystal substrate, is known to exhibit gapped Dirac cones. We show that the gap can be closed by slightly misaligning the substrate, producing a hierarchy of conical singularities (Dirac points) in the band structure at rational values Phi = (p/q)(h/e) of the magnetic flux per supercell. Each Dirac point signals a switch of the topological quantum number in the connected component of the quantum Hall phase diagram. Model calculations reveal the scale invariant cond…
Concept of the topological order is useful to characterize anisotropic superconductivities. The spin Hall conductance distinguishes superconductivities with the same symmetry. The Chern number for the spin Hall conductance is given by the covering degree of a closed surface around the Dirac monopole. It gives a clear illustration for the on-critical condition for the $d_{x^2-y^2}$ supreconductivitiy with non zero chemical potential. Non trivial topological orders on the triangular lattice are also presented and demonstrated by the topological objects.
Features of electronic currents in solids are truly diverse depending on circumstances, e.g. non-equilibrium transport currents leading to dissipation and persistent currents flowing in equilibrium. Differences between these currents may be clear in many cases, while there are some where they are not. Results of theoretical studies on the latter cases will be introduced briefly focusing on the inter-band effects of magnetic fields in orbital magnetisms and Hall effects of Dirac electrons.
We theoretically investigate the spin Hall conductivity (SHC) in topological Dirac semimetals (TDSMs) whose Dirac points are protected by rotational symmetry. On the basis of a general phase diagram of the system with time-reversal, inversion and four-fold rotational symmetries, we reveal that the SHC is sensitive to the phase to which the system belong. The phase and the SHC are characterized by the mirror Chern numbers and the presence or absence of gapless bulk Dirac points. It is also found that the representative TDSM Cd$_3$As$_2$ supports a large and negative SHC $σ_{xy}^z\sim -10^4 (\hb…
The unconventional (half-integer) quantum Hall effect for a single species of Dirac fermions is analyzed. We discuss possible experimental measurements of the half-integer Hall conductance $g_{xy}$ of topological insulator surface states and explain how to reconcile Laughlin's flux insertion argument with half-integer $g_{xy}$. Using a vortex state representation of Landau Level wavefunctions, we calculate current density beyond linear response, which is in particular relevant to the topological image monopole effect. As a major result, the field theory describing the localization physics of t…
An interaction-driven nonzero quantum Hall conductivity is shown to occur in time-reversal symmetric massive Dirac materials, in the absence of any external agent. The effect is produced through the dynamical breakdown of time-reversal symmetry, which is generated by quantum fluctuations, when the full dynamical electromagnetic interaction among the electrons is taken into account. The manifestation of this emergent parity anomaly should be observed in materials such as silicene, stanene, germanene and transition metal dichalcogenides, at low enough temperatures.
The effect of strong long-range disorder on the quantization of the Hall conductivity $σ_{xy}$ in graphene is studied numerically. It is shown that increasing Landau-level mixing progressively destroys all plateaus in $σ_{xy}$ except the plateaus at $σ_{xy}=\mp e^2/2h$ (per valley and per spin). The critical state at the charge-neutral Dirac point is robust to strong disorder and belongs to the universality class of the conventional plateau transitions in the integer quantum Hall effect. We propose that the breaking of time-reversal symmetry by ripples in graphene can realize this quantum crit…
We report the synthesis and magneto-transport measurements on the single crystal of Dirac semimetal PdTe$_2$. The de Haas-van Alphen oscillations with multiple frequencies have been clearly observed, from which the small effective masses and nontrivial Berry phase are extracted, implying the possible existence of the Dirac fermions in PdTe$_2$. The planar Hall effect and anisotropic longitudinal resistivity originating from the chiral anomaly and nontrivial Berry phase are observed, providing strong evidence for the nontrivial properties in PdTe$_2$. With the increase of temperature up to 150 …
Spectral analysis of Shubnikov de Haas (SdH) oscillations of magnetoresistance and of Quantum Hall Effect (QHE) measured in quasi-2D highly oriented pyrolytic graphite (HOPG) [Phys. Rev. Lett. 90, 156402 (2003)] reveals two types of carriers: normal (massive) electrons with Berry phase 0 and Dirac-like (massless) holes with Berry phase pi. We demonstrate that recently reported integer- and semi-integer QHE for bi-layer and single-layer graphenes take place simultaneously in HOPG samples.
We propose two novel two-dimensional topological Dirac materials, planar PtN4C2 and Pt2N8C6, which exhibit graphene-like electronic structures with linearly dispersive Dirac-cone states exactly at the Fermi level. Moreover, the Dirac cone is anisotropic, resulting in anisotropic Fermi velocities and making it possible to realize orientation-dependent quantum devices. Using the first-principles electronic structure calculations, we have systemically studied the structural, electronic, and topological properties. We find that spin-orbit coupling opens a sizable topological band gap so that the m…
Carrier dynamics acquire a new character in the presence of Bloch-band Berry curvature, which naturally arises in gapped Dirac materials (GDMs). Here we argue that photoresponse in GDMs with small band gaps is dramatically enhanced by Berry curvature. This manifests in a giant and saturable Hall photoconductivity when illuminated by circularly polarized light. Unlike Hall motion arising from a Lorentz force in a magnetic field, which impedes longitudinal carrier motion, Hall photoconductivity arising from Berry curvature can boost longitudinal carrier transport. In GDMs, this results in a heli…
Anisotropic magnetoresistance is the change tendency of resistance of a material on the mutual orientation of the electric current and the external magnetic field. Here, we report experimental observations in the Dirac semimetal Cd3As2 of giant anisotropic magnetoresistance and its transverse version, called the planar Hall effect. The relative anisotropic magnetoresistance is negative and up to -68% at 2 K and 10 T. The high anisotropy and the minus sign in this isotropic and nonmagnetic material are attributed to a field-dependent current along the magnetic field, which may be induced by the…
Recently, giant planar Hall effect originating from chiral anomaly has been predicted in nonmagnetic Dirac/Weyl semimetals. ZrTe5 is considered to be an intriguing Dirac semimetal at the boundary of weak topological insulators and strong topological insulators, though this claim still remains controversial. Here, we report the observation in ZrTe5 of the giant planar Hall resistivity that shows two different magnetic-field dependences as predicted by theory and a maximum at the Lifshitz transition temperature. We found that the giant planar Hall resistivity fades out with decreasing the thickn…
We investigate effects of the filled Dirac sea on the $SU(4)$ symmetry breaking in the integer quantum Hall states of graphene with long-ranged Coulomb interactions. Our model also includes Hubbard and nearest neighbour repulsive interactions with strengths $U$ and $V$ respectively. We find that the symmetry breaking of the $n=0$ Landau levels induces an $SU(4)$ polarization of the Dirac sea. This results in several phases which are absent when the effects of the Dirac sea are neglected. We compute the phase diagram in the $U$-$V$ space. We also calculate the excitation gaps in tilted magnetic…
The co-presence of multiple Dirac bands in few-layer graphene leads to a rich phase diagram in the quantum Hall regime. Using transport measurements, we map the phase diagram of BN-encapsulated ABA-stacked trilayer graphene as a function charge density n, magnetic field B and interlayer displacement field D, and observe transitions among states with different spin, valley, orbital and parity polarizations. Such rich pattern arises from crossings between Landau levels from different subbands, which reflect the evolving symmetries that are tunable in situ. At D=0, we observe fractional quantum H…
We present complete analytical and numerical results that demonstrate the anomalous universal fluctuations of the spin-Hall conductance in chiral materials such as graphene and topological insulators. We investigated both the corresponding fluctuations, the Universal Fractionated and the Universal Quantized, and also the open channels orbital number crossover between the two regimes. In particular, we show that the Wigner-Dyson symmetries does not properly describe such conductances and the preponderant role of the chiral classes on the Dirac quantum dots. The results are analytical and solve …
A honeycomb lattice system has four types of Dirac electrons corresponding to the spin and valley degrees of freedom. We consider a state that contains only one type of massless electrons and three types of massive ones, which we call the single Dirac-cone state. We analyze quantum Hall (QH) effects in this state. We make a detailed investigation of the Chern and spin-Chern numbers. We make clear the origin of unconventional QH effects discovered in graphene. We also show that the single Dirac-cone state may have arbitrary large spin-Chern numbers in magnetic field. Such a state will be genera…
The analytical expressions for both diagonal and off-diagonal ac and dc conductivities of graphene placed in an external magnetic field are derived. These conductivities exhibit rather unusual behavior as functions of frequency, chemical potential and applied field which is caused by the fact that the quasiparticle excitations in graphene are Dirac-like. One of the most striking effects observed in graphene is the odd integer quantum Hall effect. We argue that it is caused by the anomalous properties of the Dirac quasiparticles from the lowest Landau level. Other quantities such as Hall angle …
We have experimentally confirmed the quantum Hall ferromagnetic state with Chern number ν=0, characterized by the helical edge state, in a layered organic Dirac fermion system α-(BEDT-TTF)_2I_3. The interlayer resistance saturates at low temperatures and high magnetic fields. It does not scale with the sample cross-sectional area in the saturating region, and resonantly depends on the magnetic field direction. These results strongly suggest that the helical edge state dominates transport. This is the first observation of the topological phase in organic molecular crystals.
A semiclassical formulation of the spin Hall effect for physical systems satisfying Dirac-like equation is introduced. We demonstrated that the main contribution to the spin Hall conductivity is given by the spin Chern number whether the spin is conserved or not at the quantum level. We illustrated the formulation within the Kane-Mele model of graphene in the absence and in the presence of the Rashba spin-orbit coupling term.
We present a perturbative method for calculating the optical Hall conductivity in a tight-binding framework based on the Kubo formalism. The method involves diagonalization only of the Hamiltonian in absence of the magnetic field, and thus avoids the computational problems usually arising due to the huge magnetic unit cells required to maintain translational invariance in presence of a Peierls phase. A recipe for applying the method to numerical calculations of the magneto-optical response is presented. We apply the formalism to the case of ordinary and gapped graphene in a next-nearest neighb…
We report on the unusual nature of nu=0 state in the integer quantum Hall effect (QHE) in graphene and show that electron transport in this regime is dominated by counter-propagating edge states. Such states, intrinsic to massless Dirac quasiparticles, manifest themselves in a large longitudinal resistivity rho_xx > h/e^2, in striking contrast to rho_xx behavior in the standard QHE. The nu=0 state in graphene is also predicted to exhibit pronounced fluctuations in rho_xy and rho_xx and a smeared zero Hall plateau in sigma_xy, in agreement with experiment. The existence of gapless edge states p…
The Landau bands of mirror symmetric 2D Dirac semi-metals (for example odd-layers of ABA-graphene) can be identified by their parity with respect to mirror symmetry. This symmetry facilitates a new class of counter-propagating Hall states at opposite but equal electron and hole filling factors $|ν_{\pm}|=1/m$ ({\it m} odd). Here, we propose a Laughlin-like correlated liquid wavefunction, at the charge neutrality point, that exhibits fractionally charged quasi-particle/hole pair excitation of opposite parity. Using a bosonized one-dimensional edge state theory, we show that the longitudinal con…
