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arXiv 2012.15628cond-mat.mes-hallcond-mat.mtrl-sci
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由贝里曲率多极矩诱导的高阶非线性反常霍尔效应

Higher-Order Nonlinear Anomalous Hall Effects Induced by Berry Curvature Multipoles

Cheng-Ping Zhang, Xue-Jian Gao, Ying-Ming Xie, Hoi Chun Po, K. T. Law

AI总结:

本研究揭示贝里曲率多极矩可诱导高阶非线性反常霍尔效应,通过对称性分析与计算验证了其在反铁磁体、拓扑绝缘体等材料中的主导阶响应,并提出了多种候选材料体系。

摘要:

近年来,研究表明贝里曲率单极子和偶极子分别在反常霍尔效应和非线性霍尔效应中发挥关键作用。本研究证明,贝里曲率多极矩(费米能级处贝里曲率的高阶矩)可诱导高阶非线性反常霍尔(NLAH)效应。具体而言,会产生垂直于电流方向的交流霍尔电压,其频率为外加电流频率的整数倍。重要的是,通过分析所有三维和二维磁性点群的对称性质,我们发现四极矩、六极矩乃至更高阶的贝里曲率矩可在特定材料中引发主导阶的倍频效应。为提供具体实例,我们指出:由于贝里曲率四极矩的存在,三阶NLAH电压可成为某些反铁磁体中的主导阶霍尔响应;而由贝里曲率六极矩诱导的四阶NLAH电压可成为拓扑绝缘体表面态中的主导响应。我们的结果通过对称性分析、有效哈密顿量及第一性原理计算得到验证。此外,我们还提出了其他支持高阶NLAH效应的材料,包括二维反铁磁体与铁磁体、外尔半金属,以及接近量子反常霍尔相的转角双层石墨烯。

英文摘要:

In recent years, it has been shown that Berry curvature monopoles and dipoles play essential roles in the anomalous Hall effect and the nonlinear Hall effect respectively. In this work, we demonstrate that Berry curvature multipoles (the higher moments of Berry curvatures at the Fermi energy) can induce higher-order nonlinear anomalous Hall (NLAH) effect. Specifically, an AC Hall voltage perpendicular to the current direction emerges, where the frequency is an integer multiple of the frequency of the applied current. Importantly, by analyzing the symmetry properties of all the 3D and 2D magnetic point groups, we note that the quadrupole, hexapole and even higher Berry curvature moments can cause the leading-order frequency multiplication in certain materials. To provide concrete examples, we point out that the third-order NLAH voltage can be the leading-order Hall response in certain antiferromagnets due to Berry curvature quadrupoles, and the fourth-order NLAH voltage can be the leading response in the surface states of topological insulators induced by Berry curvature hexapoles. Our results are established by symmetry analysis, effective Hamiltonian and first-principles calculations. Other materials which support the higher-order NLAH effect are further proposed, including 2D antiferromagnets and ferromagnets, Weyl semimetals and twisted bilayer graphene near the quantum anomalous Hall phase.

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