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arXiv 1608.01600cond-mat.str-el
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Hubbard模型中的输运与光学电导:高温度展开视角

Transport and Optical Conductivity in the Hubbard Model: A High-Temperature Expansion Perspective

Collège de France(法兰西学院);Centre de Physique Théorique, École Polytechnique, CNRS, Université Paris-Saclay(巴黎综合理工学院理论物理中心,法国国家科学研究中心,巴黎萨克雷大学);University of California, Santa Cruz(加州大学圣克鲁兹分校);Jožef Stefan Institute(约瑟夫·斯蒂芬研究所);San José State University(圣何塞州立大学);University of Geneva(日内瓦大学)

Edward Perepelitsky, Andrew Galatas, Jernej Mravlje, Rok Žitko, Ehsan Khatami, B Sriram Shastry, Antoine Georges

AI总结:

Hubbard模型中,通过高温度展开方法研究输运与光学电导,发现电阻率随温度线性增加,而散射时间饱和,热电功率遵循Heikes公式,洛伦兹数随温度平方倒数消失。

摘要:

我们利用高温度级数展开方法,推导出Hubbard模型动态响应函数的谱矩的解析表达式。我们考虑了通用维度d以及无限维度极限,任意电子密度n,以及有限和无限的排斥作用U。我们使用矩重建方法获得单电子能谱函数、自能和光学电导。它们在高温下都是平滑函数,并且在大U下特征无明显峰,具有特征宽度约为晶格跃迁参数t的量级。在无限维度极限下,我们将级数展开结果与精确的数值重整化群和相互作用展开量子蒙特卡洛结果进行比较。我们发现,在 surprisingly 低的温度下,结果具有很好的一致性,贯穿大部分的bad-metal区域,该区域适用于T ≳ (1-n)D,即Brinkman-Rice尺度。电阻率在高温下线性增加,没有饱和。这源于压缩性或动能的1/T行为,它们在起作用作为有效载流子数。相反,散射时间(或扩散常数)在高温下饱和。我们发现,σ(n,T) ≈ (1-n)σ(n=0,T) 对所有n来说,近似非常准确,其中σ(n=0,T) ∝ t/T 在高温下。在小n处的饱和是由于有效载流子数的密度依赖性和散射时间的密度依赖性之间的补偿。电阻率的T依赖性显示了一个膝状特征,这标志着向中间温度区域的交叉点,其中扩散常数(或散射时间)随着T的降低而增加。在高温下,热电功率遵循Heikes公式,而Wiedemann-Franz定律被违反,洛伦兹数随着1/T²消失。

英文摘要:

We derive analytical expressions for the spectral moments of the dynamical response functions of the Hubbard model using the high-temperature series expansion. We consider generic dimension $d$ as well as the infinite-$d$ limit, arbitrary electron density $n$, and both finite and infinite repulsion $U$. We use moment-reconstruction methods to obtain the one-electron spectral function, the self-energy, and the optical conductivity. They are all smooth functions at high-temperature and, at large-$U$, they are featureless with characteristic widths of order the lattice hopping parameter $t$. In the infinite-$d$ limit we compare the series expansion results with accurate numerical renormalization group and interaction expansion quantum Monte-Carlo results. We find excellent agreement down to surprisingly low temperatures, throughout most of the bad-metal regime which applies for $T \gtrsim (1-n)D$, the Brinkman-Rice scale. The resistivity increases linearly in $T$ at high-temperature without saturation. This results from the $1/T$ behaviour of the compressibility or kinetic energy, which play the role of the effective carrier number. In contrast, the scattering time (or diffusion constant) saturate at high-$T$. We find that $σ(n,T) \approx (1-n)σ(n=0,T)$ to a very good approximation for all $n$, with $σ(n=0,T)\propto t/T$ at high temperatures. The saturation at small $n$ occurs due to a compensation between the density-dependence of the effective number of carriers and that of the scattering time. The $T$-dependence of the resistivity displays a knee-like feature which signals a cross-over to the intermediate-temperature regime where the diffusion constant (or scattering time) start increasing with decreasing $T$. At high-temperatures, the thermopower obeys the Heikes formula, while the Wiedemann-Franz law is violated with the Lorenz number vanishing as $1/T^2$.

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