Reorientation of the bicollinear antiferromagnetic structure at the surface of Fe$_{1+y}$Te bulk and thin films
Torben Hänke, Udai Raj Singh, Lasse Cornils, Sujit Manna, Anand Kamlapure, Martin Bremholm, Ellen Marie Jensen Hedegaard, Bo Brummerstedt Iversen, Philip Hofman… 展开作者
Torben Hänke, Udai Raj Singh, Lasse Cornils, Sujit Manna, Anand Kamlapure, Martin Bremholm, Ellen Marie Jensen Hedegaard, Bo Brummerstedt Iversen, Philip Hofmann, Jin Hu, Jens Wiebe, Zhiqiang Mao, Roland Wiesendanger
建立非常规超导体的非超导母体化合物中普遍存在的反铁磁性与其超导相之间的关系,被认为是理解这些材料中复杂物理的重要因素。从块体系统到薄膜的发展强烈地影响了非常规超导体的相图。对于Fe $_{1+y}$ Se $_{1-x}$ Te $_x$超导体的母体化合物Fe $_{1+y}$ Te,体敏中子衍射揭示了面内取向的双共线反铁磁结构。在这里,我们表明,通过自旋分辨扫描隧道显微镜,在体Fe $_{1+y}$ Te的表面上,以及在拓扑绝缘体Bi $_2$ Te $_3$上生长的薄膜上,自旋方向倾斜远离表面平面和表面单元格的高对称性方向,同时保持双共线磁性结构。我们的研究结果表明,在Fe-硫属化物表面的磁性显着偏离一个简单的面内取向的双共线反铁磁结构,这意味着在相关的超导化合物的表面的配对可能是不同的,在体。
英文摘要:
Establishing the relation between the ubiquitous antiferromagnetism in the non-superconducting parent compounds of unconventional superconductors and their superconducting phase is believed to be important for the understanding of the complex physics in these materials. Going from the bulk systems to thin films strongly affects the phase diagram of unconventional superconductors. For Fe$_{1+y}$Te, the parent compound of the Fe$_{1+y}$Se$_{1-x}$Te$_x$ superconductors, bulk sensitive neutron diffraction has revealed an in-plane oriented bicollinear antiferromagnetic structure. Here, we show by spin-resolved scanning tunneling microscopy that on the surfaces of bulk Fe$_{1+y}$Te, as well as on thin films grown on the topological insulator Bi$_2$Te$_3$, the spin direction is canted both away from the surface plane and from the high-symmetry directions of the surface unit cell, while keeping the bicollinear magnetic structure. Our results demonstrate that the magnetism at the Fe-chalcogenide surface markedly deviates from a simple in-plane oriented bicollinear antiferromagnetic structure, which implies that the pairing at the surface of the related superconducting compounds might be different from that in the bulk.
Selective stabilization of antiferromagnetic orders in FeTe films via local strain engineering
Beijing Academy of Quantum Information Sciences(北京量子信息科学研究院);School of Physics, Renmin University of China(中国人民大学物理学院);Key Laboratory of Quantum State Construction and Manipulation (Ministry of Education), Renmin University of China(中国人民大学量子态构建与操控教育部重点实验室);Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);University of Chinese Academy of Sciences(中国科学院大学)
Magnetotransport evidence of irreversible spin reorientation in the collinear antiferromagnetic state of underdoped $\mathrm{Nd}_{2-x}\mathrm{Ce}_x\mathrm{CuO}_4$
Magnetically induced electric polarization reversal in multiferroic TbMn$_2$O$_5$: Terbium spin reorientation studied by resonant x-ray diffraction
在多铁性TbMn $_2$ O $_5$中,铽离子的行为形成磁电耦合的关键部分。结果是在2 T下磁感应电极化的强度反转。在这篇文章中,我们提出了在外加磁场下的铽磁性结构的第一个直接测量。与目前对\tmo磁性的解释相反,我们表明,在电极化的强度反转时,铽子晶格采用倾斜的反铁磁结构,具有平行于\textit{a}轴的磁矩的大分量。此外,我们提供的证据之间的耦合锰的3D磁性结构和铽$4f$磁性,这是在难以捉摸的磁电机制发挥重要的意义。
Thermal evolution of antiferromagnetic correlations and tetrahedral bond angles in superconducting FeTe$_{1-x}$Se$_x$
最近已经证明,在铁硫属化物中通过中子散射测量的动态磁关联可以用短程关联的模型来描述,该短程关联的特征在于特定的{选择四自旋斑,其中适当的选择随着}母体材料被掺杂朝向超导性而改变。在这里,我们应用这样的模型来描述测量地图的磁散射作为二维波矢量的函数获得的最佳超导晶体FeTe $_{1-x}$ Se $_x$。我们发现,特征反铁磁波矢量的演变,发现在欠掺杂的硫族化物(在高温下)的双共线结构与条纹结构的反铁磁铁砷化物(在低温下); {这些都可以描述相同的本地元格,但不同的元格间的相关性}。虽然低能磁谱权重的大小在所有温度下都很大,但它实际上在低温下有所减弱,其中载流子变得更加巡回。所观察到的自旋相关性的变化与电子散射率的急剧下降和冷却时的体散射响应的增长相关。最后,我们还提出了粉末中子衍射结果的晶格参数在FeTe $_{1-x}$ Se $_x$表明四面体键角趋于增加对冷却的理想值,在协议的增加屏蔽的晶体场更多的巡回电子和相应较小的分裂的Fe $3d$轨道。
Angle dependent field-driven reorientation transitions in uniaxial antiferromagnet MnBi$_2$Te$_4$ single crystal
Center for Quantum Materials & Devices and College of Physics, Chongqing University(重庆大学量子材料与器件中心及物理学院);Low Temperature Physics Laboratory, College of Physics, Chongqing University(重庆大学物理学院低温物理实验室)
Topological Electronic Structure Evolution with Symmetry Breaking Spin Reorientation in (Fe$_{1-x}$Co$_{x}$)Sn
由于拓扑结构、磁性和电子关联之间的相互作用,具有可果美晶格的拓扑材料引起了人们的广泛关注。(Fe $_{1-x}$ Co $_x$)Sn系统不仅具有可果美晶格,而且具有随温度和掺杂可调的对称破缺磁矩。在这项研究中,角分辨光电子能谱和第一性原理计算被用来研究拓扑电子结构和不同的磁矩从平面到轴向反铁磁相之间的相互作用。在狄拉克点的理论预测的间隙揭示在低温轴向阶段,但没有观察到跨温度依赖的磁相变的间隙开放。然而,拓扑表面带被观察到转移的能量作为表面磁矩减少或变得无序随着时间的推移在实验测量。移动的表面带可能会排除温度相关的散装间隙的确定,但突出了磁性和拓扑结构之间的复杂连接与表面/散装二分法,可以影响材料的性能和它们的询问。
Reversible tuning of magnetic order and intrinsic superconductivity in strained FeTe films via stoichiometry control
Beijing Academy of Quantum Information Sciences(北京量子信息科学研究院);Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);University of Chinese Academy of Sciences(中国科学院大学);Renmin University of China(中国人民大学);Shanxi Normal University(山西师范大学);Tsinghua University(清华大学)
Spin reorientation of the Fe moments in Eu$_{0.5}$Ca$_{0.5}$Fe$_{2}$As$_{2}$: Evidence for a strong interplay of Eu and Fe magnetism
用互补极化和非极化单晶中子衍射方法研究了Eu $_{0.5}$ Ca $_{0.5}$ Fe $_{2}$ As $_{2}$的温度相关磁性结构。在A型反铁磁(AFM)结构中,当Eu位被等价的Ca $^{2+}$稀释50%时,在低于$\mathit{T_{Eu}}$ = 10 K的温度下,Eu亚晶格仍然是长程有序的.在2.5 K时,Eu $^{2+}$自旋的磁矩大小为6.74(4)$μ_{B}$. Fe亚晶格在$\mathit{T_{SDW}}$ = 192(2)K时经历自旋密度波转变,并在$\mathit{T_{Eu}}$上方显示面内AFM结构。而在2.5 K时,Fe的$^{2+}$矩在与$\mathit{ab}$平面成14(4)°的倾斜AFM结构中是有序的.低于Eu的AFM有序温度的Fe的自旋重取向提供了Eu $_{0.5}$ Ca $_{0.5}$ Fe $_{2}$ As $_{2}$中两个磁性亚晶格之间强相互作用的直接证据。