Computations of the breakup of a liquid bridge are used to establish the limits of applicability of similarity solutions derived for different breakup regimes. These regimes are based on particular viscous-inertial balances, that is different limits of the Ohnesorge number $Oh$. To accurately establish the transitions between regimes, the minimum bridge radius is resolved through four orders of magnitude using a purpose-built multiscale finite element method. This allows us to construct a quantitative phase diagram for the breakup phenomenon which includes the appearance of a recently discovered low-$Oh$ viscous regime. The method used to quantify the accuracy of the similarity solutions allows us to identify a number of previously unobserved features of the breakup, most notably an oscillatory convergence towards the viscous-inertial similarity solution. Finally, we discuss how the new findings open up a number of challenges for both theoretical and experimental analysis.
The breakup dynamics of a capillary bridge on a hydrophobic stripe between two hydrophilic stripes is studied experimentally and numerically using direct numerical simulations. The capillary bridge is formed from an evaporating water droplet wetting three neighboring stripes of a chemically patterned surface. By considering the breakup process in a phase space representation, the breakup dynamics can be evaluated without the uncertainty in determining the precise breakup time. The simulations are based on the Volume-of-Fluid (VOF) method implemented in Free Surface 3D (FS3D). In order to const…
The average Rayleigh capillary breakup length of a cylindrical Newtonian viscous liquid jet moving with homogeneous velocity $\hat{U}$ (negligible external forces) must be determined by the selection of normal modes with time-independent amplitude and wavelength (invariant modes, IMs). Both positive and negative group velocity IMs exist in ample ranges of the parameter domain (Weber and Ohnesorge numbers), which explains (i) the average breakup length independence on ambient conditions (long-term resonance), and (ii) its proportionality to the inverse of the spatial growth rate of the dominant…
Despite their fundamental and applied importance, a general model to predict the natural breakup length of steady capillary jets has not been proposed yet. In this work, we derive a scaling law with two universal constants to calculate that length as a function of the liquid properties and operating conditions. These constants are determined by fitting the scaling law to a large set of experimental and numerical measurements, including previously published data. Both the experimental and numerical jet lengths conform remarkably well to the proposed scaling law. This law is explained in terms o…
It was recently demonstrated that feeding a silicon-in-silica coaxial fibre into a flame$\mathord{-}$imparting a steep silica viscosity gradient$\mathord{-}$results in the formation of silicon spheres whose size is controlled by the feed speed [Gumennik et al., Nat.Commun. 4, 2216 (2013)]. A reduced model to predict the droplet size from the feed speed was then derived by Mowlavi et al. [Phys. Rev. Fluids. 4, 064003 (2019)], but large experimental uncertainties in the parameter values and temperature profile made quantitative validation of the model impossible. Here, we validate the reduced mo…
We investigated the flow profile of a polymer solution in a thinning capillary bridge. Fluorescent tracer particles with a diameter of 3$μ$m were used to visualize the flow. The cylindrical shape of the filament introduced strong optical abberations that could be corrected for, and we were able to characterize the flow in filaments with a thickness ranging from 150 to 30 $μ$m. In the first regime when the filament was still sufficiently large, we used a PIV algorithm to deduce the flow field. At later stages when the number of particles in the observation plane decreased a PTV algorithm was us…
Step-emulsification is a microfluidic technique for droplet generation which relies on the abrupt decrease of confinement of a liquid filament surrounded by a continuous phase. A striking feature of this geometry is the transition between two distinct droplet breakup regimes, the "step-regime" and "jet-regime", at a critical capillary number. In the step-regime, small and monodisperse droplets break off from the filament directly at a topographic step, while in the jet-regime a jet protrudes into the larger channel region and large plug-like droplets are produced. We characterize the breakup b…
The effects of elasticity on filament thinning and breakup are investigated in microchannel cross flow. When a viscous solution is stretched by an external immiscible fluid, a low 100 ppm polymer concentration strongly affects the breakup process, compared to the Newtonian case. Qualitatively, polymeric filaments show much slower evolution, and their morphology features multiple connected drops. Measurements of filament thickness show two main temporal regimes: flow- and capillary-driven. At early times both polymeric and Newtonian fluids are flow-driven, and filament thinning is exponential. …
Dripping-onto-droplet rheometry of sodium alginate solutions
Mines Paris, PSL University（巴黎矿业学院，巴黎文理研究大学）；Universidade Estadual Paulista ‘Julio de Mesquita Filho’（圣保罗州立大学）；Universidade Federal do Rio de Janeiro（里约热内卢联邦大学）
In this paper, we experimentally explore the formation, evolution and breakup of Armstrong liquid bridge. The extremely complicated evolution stage is revealed, which involves many coupled processes including the morphology change, current variation, heat transfer, and water evaporation. By focusing on the final fate of this liquid bridge, we observe that the breakup occurs once an effective length ($\tilde{L}$) is reached. This effective length increases linearly with the applied voltage, implying a threshold electric field to sustain the liquid bridge. Moreover, by an introduced external flo…
A capillary jet falling under the effect of gravity continuously stretches while thinning downstream. We report here the effect of external periodic forcing on such a spatially varying jet in the jetting regime. Surprisingly, the optimal forcing frequency producing the most unstable jet is found to be highly dependent on the forcing amplitude. Taking benefit of the one-dimensional Eggers & Dupont (J. Fluid Mech., vol. 262, 1994, 205-221) equations, we investigate the case through nonlinear simulations and linear stability analysis. In the local framework the WKBJ formalism, established for wea…
Helped by the careful analysis of their experimental data, Worthington (1897) described roughly the mechanism underlying the formation of high-speed jets ejected after the impact of an axisymmetric solid on a liquid-air interface. In this work we combine detailed boundary-integral simulations with analytical modeling to describe the formation and break-up of such Worthington jets in two common physical systems: the impact of a circular disc on a liquid surface and the release of air bubbles from an underwater nozzle. We first show that the jet base dynamics can be predicted for both systems us…
We studied experimentally the breakup of liquid bridges made of aqueous solutions of Poly(acrylic acid) between two separating solid surfaces with freely moving contact lines. For polymer concentrations higher than a certain threshold ($\sim$ 30 ppm), the contact line on the surface with the highest receding contact angle fully retracts before the liquid bridge capillary breakup takes place at its neck. This means that all the liquid remains attached to the opposing surface when the surfaces are separated. This behavior occurs regardless of the range of liquid volume and stretching speed studi…
Breakup of water jets under gravity is a common-place phenomenon. The role of surface tension in the instability of water jets was recognized by Rayleigh and the theory propounded goes by the name of Plateau-Rayleigh theory. The necks and bulges down along the jet-length that are created by perturbation waves of wavelengths larger than a certain value keep growing with time and ultimately cause the jet to breakup into drops. The effect of perturbation waves have been investigated experimentally and found to confirm the essentials of the theory. However, there is no unanimity about the origin o…
The effect of 'bridge splitting' is considered in the case of capillary adhesion: for a fixed total volume of liquid, does having more capillary bridges increase the total adhesion force? Previous studies have shown that the capillary-induced adhesion force between two planar surfaces is only substantially enhanced by bridge splitting in specific circumstances. Here this previous result is reconsidered, and it is shown that bridge splitting may significantly increase the adhesion forces when one of the surfaces is rough. The resistance to shear is also examined, and it is shown that bridge spl…
Liquid capillary-bridge formation between solid particles has a critical influence on the rheological properties of granular materials and, in particular, on the efficiency of fluidized bed reactors. The available analytical and semi-analytical methods have inherent limitations, and often do not cover important aspects, like the presence of non-axisymmetric bridges. Here, we conduct numerical simulations of the capillary bridge formation between equally and unequally-sized solid particles using the lattice Boltzmann method, and provide an assessment of the accuracy of different families of ana…
The impact of solid and liquid objects (projectiles) onto liquids and soft solids (targets) generally results on the creation and expansion of an air cavity inside the impacted objects. The dynamics of cavity expansion and collapse depends on the projectile inertia as well as on the target properties. In this paper we study the impact of microfluidic jets generated by thermocavitation processes on a capillary bridge between two parallel planar walls. Different capillary bridge types were studied, Newtonian liquids, viscoelastic liquids and agarose gels. Thus, we compare the cavity formation an…
The complex behavior of drop deposition on a hydrophobic surface is considered by looking at a model problem in which the evolution of a constant-volume liquid bridge is studied as the bridge is stretched. The bridge is pinned with a fixed diameter at the upper contact point, but the contact line at the lower attachment point is free to move on a smooth substrate. Experiments indicate that initially, as the bridge is stretched, the lower contact line slowly retreats inwards. However at a critical radius, the bridge becomes unstable, and the contact line accelerates dramatically, moving inwards…
We study both numerically and experimentally the breakup of a viscoelastic liquid bridge between two parallel electrodes. We solve the leaky-dielectric FENE-P model to describe the dynamical response of the liquid bridge under isothermal conditions. The results show that the surface charge screens the inner electric field perpendicular to the free surface over the entire dynamical process. The liquid bridge deformation produces a normal electric field on the outer side of the free surface that is commensurate with the axial one. The surface conduction does not significantly affect the current …
We propose an extension of the Maffettone-Minale (MM) model to predict the dynamics of an ellipsoidal droplet in a shear flow. The parameters of the MM model are traditionally retrieved in the framework of the perturbation theory for small deformations, i.e., small capillary numbers ($\mbox{Ca} \ll 1$) applied to Stokes equations. In this work, we take a novel route, in that we determine the model parameters at finite capillary numbers ($\mbox{Ca}\sim {\cal O}(1)$) without relying on perturbation theory results, while retaining a realistic representation in creeping time and steady deformation…
We study a liquid jet that breaks up into drops in an external co-flowing liquid inside a confining microfluidic geometry. The jet breakup can occur right after the nozzle in a phenomenon named dripping or through the generation of a liquid jet that breaks up a long distance from the nozzle, which is called jetting. Traditionally, these two regimes have been considered to reflect the existence of two kinds of spatiotemporal instabilities of a fluid jet, the dripping regime corresponding to an absolutely unstable jet and the jetting regime to a convectively unstable jet. Here, we present quanti…
We propose a combined computational approach based on the multi-phase-field and the lattice Boltzmann method for the motion of solid particles under the action of capillary forces. The accuracy of the method is analyzed by comparison with the analytic solutions for the motion of two parallel plates of finite extension connected by a capillary bridge. The method is then used to investigate the dynamics of multiple spherical solid bodies connected via capillary bridges. The amount of liquid connecting the spheres is varied, and the influence of the resulting liquid-morphology on their dynamics i…
The migration of liquids in porous media, such as sand, has been commonly considered at high saturation levels with liquid pathways at pore dimensions. In this letter we reveal a low saturation regime observed in our experiments with droplets of extremely low volatility liquids deposited on sand. In this regime the liquid is mostly found within the grain surface roughness and in the capillary bridges formed at the contacts between the grains. The bridges act as variable-volume reservoirs and the flow is driven by the capillary pressure arising at the wetting front according to the roughness le…
Liquid bridges are commonly encountered in nature and the liquid transfer induced by their rupture are widely used in various industrial applications. In this work, with the focus on the porous tip, we studied the impacts of capillary effects on the liquid transfer induced by the rupture through numerical simulations. To depict the capillary effects of a porous tip, a time scale ratio, R_T, is proposed to compare the competing mechanisms of spontaneous imbibitiona and external drag. In terms of R_T, we then develop a theoretical model for estimating the liquid retention ratio considering the g…
Deformation and breakup of a ferrofluid compound droplet migrating in a microchannel under a magnetic field: A phase-field-based multiple-relaxation time lattice Boltzmann study
We used volume-of-fluid (VOF) method to perform three-dimensional numerical simulations of droplet formation of Newtonian fluids in microfluidic T-junction devices. To evaluate the performance of the VOF method we examined the regimes of drop formation and determined droplet size as a function of system parameters. Comparison of the simulation results with four sets of experimental data from the literature showed good agreement, validating the VOF method. Motivated by the lack of adequate studies investigating the influence of viscosity ratio (λ) on the generated droplet size, we mapped the de…
Droplet breakup is a well studied phenomena in Newtonian fluids. One property of this behavior is that, independent of initial conditions, the minimum radius exhibits power law scaling with the time left to breakup tau. Because they have additional structure and shear dependent viscosity, liquid crystals pose an interesting complication to such studies. Here, we investigate the breakup of a synthetic nematic liquid crystal known as MBBA. We determine the phase of the solution by using a cross polarizer setup in situ with the liquid bridge breakup apparatus. Consistent with previous studies of …
In this fluid dynamics video, we report on experiments of large aspect ratio capillary surfaces supported by a helical wire. These open channels are potentially useful for fluid management at low Bond numbers. The experiments were performed in a Plateau tank, injecting 2-fluorotoluene into distilled water, density matched at 26.5 $^{o}$C. Extension springs with a nominal diameter of 0.24 inches and with a wire diameter of 0.018 inches were used. At small extensions, liquid can be injected into the spring from one side. The injected free-ended liquid columns are stable. Volume-constrained stabi…
We analyze both theoretically and experimentally the breakup of a pendant water droplet loaded with Sodium Dodecyl Sulfate (SDS). The free surface minimum radius measured in the experiments is compared with that obtained from a numerical solution of the full Navier-Stokes equations for different values of the shear and dilatational surface viscosities. This comparison shows the small but measurable effect of the surface viscous stresses on the system dynamics for sufficiently small spatiotemporal distances from the breakup point, and allows to establish upper bounds for the values of the shear…
The breakup of an interface into a cascade of droplets and their subsequent coalescence is a generic problem of central importance to a large number of industrial settings such as mixing, separations, and combustion. We study the breakup of a liquid jet introduced through a cylindrical nozzle into a stagnant viscous phase via a hybrid interface-tracking/level-set method to account for the surface tension forces in a three-dimensional Cartesian domain. Numerical solutions are obtained for a range of Reynolds (Re) and Weber (We) numbers. We find that the interplay between the azimuthal and strea…
We report an experimental and theoretical study of the global stability and nonlinear dynamics of vertical jets of viscous liquid confined in the axial direction due to their impact on a bath of the same liquid. Previous works demonstrated that in the absence of axial confinement the steady liquid thread becomes unstable due to an axisymmetric global mode for values of the flow rate, $Q$, below a certain critical value, $Q_c$, giving rise to oscillations of increasing amplitude that finally lead to a dripping regime (Sauter & Buggisch, J. Fluid Mech., 2005; Rubio-Rubio et al., J. Fluid Mech., …
When a liquid viscous bridge between two parallel substrates is stretched by accelerating one substrate, its interface recedes in the radial direction. In some cases the interface becomes unstable. Such instability leads to the emergence of a network of fingers. In this study the mechanisms of the fingering are studied experimentally and analysed theoretically. The experimental setup allows a constant acceleration of the movable substrate with up to 180 m/s$^2$. The phenomena are observed using two high-speed video systems. The number of fingers is measured for different liquid viscosities and…
The secondary atomization of liquid droplets is a common physical phenomenon in many industrial and engineering applications. Atomization in high speed compressible flows is less well understood than its more frequently studied low Mach number counterpart. The key to understanding the mechanisms of secondary atomization is examination of the breakup characteristics and droplet trajectories across a range of physical conditions. In this study, a planar shock wave impacting a cylindrical water column ($ρ_l=1000 \rm~kg/m^3$) is simulated for a range of Weber numbers ranging three orders of magnit…
Analyzing a capillary minimizing problem for a higher-dimensional extended fluid, we find that there exist startling similarities between the black hole-black string system (the Gregory-Laflamme instability) and the liquid drop-liquid bridge system (the Rayleigh-Plateau instability), which were first suggested by a perturbative approach. In the extended fluid system, we confirm the existence of the critical dimension above which the non-uniform bridge (NUB, i.e., {\it Delaunay unduloid}) serves as the global minimizer of surface area. We also find a variety of phase structures (one or two cusp…
