Coherent transfer of electron spin correlations assisted by dephasing noise
Takashi Nakajima, Matthieu R. Delbecq, Tomohiro Otsuka, Shinichi Amaha, Jun Yoneda, Akito Noiri, Kenta Takeda, Giles Allison, Arne Ludwig, Andreas D. Wieck, Xue… 展开作者
Takashi Nakajima, Matthieu R. Delbecq, Tomohiro Otsuka, Shinichi Amaha, Jun Yoneda, Akito Noiri, Kenta Takeda, Giles Allison, Arne Ludwig, Andreas D. Wieck, Xuedong Hu, Franco Nori, Seigo Tarucha
Quantum coherence of superposed states, especially of entangled states, is indispensable for many quantum technologies. However, it is vulnerable to environmental noises, posing a fundamental challenge in solid-state systems including spin qubits. Here we show a scheme of entanglement engineering where pure dephasing assists the generation of quantum entanglement at distant sites in a chain of electron spins confined in semiconductor quantum dots. One party of an entangled spin pair, prepared at a single site, is transferred to the next site and then adiabatically swapped with a third spin using a transition across a multi-level avoided crossing. This process is accelerated by the noise-induced dephasing through a variant of the quantum Zeno effect, without sacrificing the coherence of the entangled state. Our finding brings insight into the spin dynamics in open quantum systems coupled to noisy environments, opening an avenue to quantum state manipulation utilizing decoherence effects.
Environmental noise usually hinders the efficiency of charge transport through coherent quantum systems; an exception is dephasing-assisted transport (DAT). We show that linear triple quantum dots in a transport configuration and subjected to pure dephasing exhibit DAT if the coupling to the drain reservoir exceeds a threshold. DAT occurs for arbitrarily weak dephasing and the enhancement can be directly controlled by the coupling to the drain. Moreover, for specific settings, the enhanced current is accompanied by a reduction in relative shot noise. We identify the quantum Zeno effect and lon…
Motivated by recent experiments, we analyse the phonon-assisted steady-state gain of a microwave field driving a double quantum-dot in a resonator. We apply the results of our companion paper, which derives the complete set of fourth-order Lindblad dissipators using Keldysh methods, to show that resonator gain and loss are substantially affected by dephasing-assisted dissipative processes in the quantum-dot system. These additional processes, which go beyond recently proposed polaronic theories, are in good quantitative agreement with experimental observations
We analyze dephasing in single and double quantum dot systems. The decoherence is introduced by the Büttiker model with current conserving fictitious voltage leads connected to the dots. By using the non-equilibrium Green function method, we investigate the dephasing effect on the tunneling current. It is shown that a finite dephasing rate leads to observable effects. The result can be used to measure dephasing rates in quantum dots.
We show that an Aharonov-Bohm (AB) ring with asymmetric electron injection can act as a coherent detector of electron dephasing. The presence of a dephasing source in one of the two arms of a moderately-to-highly asymmetric ring changes the response of the system from total reflection to complete transmission while preserving the coherence of the electrons propagating from the ring, even for strong dephasing. We interpret this phenomenon as an implementation of an interaction-free measurement.
We report microwave-driven photon-assisted tunneling in a suspended carbon nanotube double quantum dot. From the resonant linewidth at a temperature of 13 mK, the charge dephasing time is determined to be 280 +- 30 ps. The linewidth is independent of driving frequency, but increases with increasing temperature. The moderate temperature dependence is inconsistent with expectations from electron-phonon coupling alone, but consistent with charge noise arising in the device. The extracted level of charge noise is comparable with that expected from previous measurements of a valley-spin qubit, wher…
We investigate the influence of electron-phonon interactions on the dynamical properties of a quantum-dot-cavity QED system. We show that non-Markovian effects in the phonon reservoir lead to strong changes in the dynamics, arising from photon-assisted dephasing processes, not present in Markovian treatments. A pronounced consequence is the emergence of a phonon induced spectral asymmetry when detuning the cavity from the quantum-dot resonance. The asymmetry can only be explained when considering the polaritonic quasi-particle nature of the quantum-dot-cavity system. Furthermore, a temperature…
The molecular photo cell, i.e., a single molecule donor-acceptor complex, beside being technologically important, is a paradigmatic example of a many-body system operating in strong non-equilibrium. The quantum transport and the photo-voltaic energy conversion efficiency of the photocell, attached to two external leads, are investigated within the open quantum system approach by solving the Lindblad master equation. The interplay of the vibrational degrees of freedom corresponding to the molecules (via the electron-phonon interaction) and the environment (via dephasing) shows its signature in …
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps and …
We propose a scheme to prepare arbitrary superpositions of quantum states in double quantum--dots irradiated by coherent microwave pulses. Solving the equations of motion for the dot density matrix, we find that dephasing rates for such superpositions can be quantitatively infered from additional electron current pulses that appear due to a controllable breakdown of coherent population trapping in the dots.
Resonant tunneling through identical potential barriers is a textbook problem in quantum mechanics. Its solution yields total transparency (100% tunneling) at discrete energies. This dramatic phenomenon results from coherent interference among many trajectories, and it is the basis of transport through periodic structures. Resonant tunneling of electrons is commonly seen in semiconducting 'quantum dots'. Here we demonstrate that detecting (distinguishing) electron trajectories in a quantum dot (QD) renders the QD nearly insulating. We couple trajectories in the QD to a 'detector' by employing …
The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure of dots affects the exciton dephasing rates and recombination lifetimes. We find that at low temperatures, dephasing of s-shell excitons is lifetime limited, whereas p-shell excitons exhibit significant pure dephasing due to scattering between degenerate spin states. At elevated temperatures, quadratic exciton-phonon coupling plays an important role in both…
We study quantum enhancement of transport in open systems in the presence of disorder and dephasing. Quantum coherence effects may significantly enhance transport in open systems even in the deep classical regime (where the decoherence rate is greater than the inter-site hopping amplitude), as long as the disorder is sufficiently strong. When the strengths of disorder and dephasing are fixed, there is an optimal opening strength at which the coherent transport enhancement is optimized. Analytic results are obtained in two simple paradigmatic tight-binding models of large systems: the linear ch…
The coupling between single-photon emitters and phonons opens many possibilities to store and transmit quantum properties. In this paper we apply the independent boson model to describe the coupling between an optically driven two-level system and a discrete phonon mode. Tailored optical driving allows not only to generate coherent phonon states, but also to generate coherent superpositions in the form of Schrödinger cat states in the phonon system. We analyze the influence of decay and dephasing of the two-level system on these phonon preparation protocols. We find that the decay transforms t…
The influence of electron-phonon interaction on the transmission phase shift of an electron passing through a quantum dot is investigated by using the scattering theory. The transmission phase versus the intra-dot level shows a serial of phonon-induced dips. These dips are highly sensitive to electron-phonon interaction strength $λ$, and they are much more pronounced than phonon-assisted sub-peaks appeared in the conductance. Phonon-induce dephasing is also studied, and the results show that the dephasing probability $T_d$ monotonically increases with the electron-phonon interaction strength $…
In this work we investigate the interplay between coherent and incoherent charge transport in cytosine-guanine (GC) rich DNA molecules. Our objective is to introduce physically grounded approach to dephasing in large molecules and to understand the length dependent charge transport characteristics and especially the crossover from coherent tunneling to incoherent hopping regime at different temperatures. Therefore, we apply the vibronic dephasing model and compare the results to the Büttiker probe model which is commonly used to describe decoherence effects in charge transport. Using the full …
Electronic coherence is of utmost importance for the access and control of quantum-mechanical solid-state properties. Using a purely electronic observable, the photocurrent, we measure an electronic coherence time of 22 +/- 4 fs in graphene. The photocurrent is ideally suited to measure electronic coherence as it is a direct result of quantum path interference, controlled by the delay between two ultrashort two-color laser pulses. The maximum delay for which interference between the population amplitude injected by the first pulse interferes with that generated by the second pulse determines t…
The paper discusses two-photon Rabi oscillations between the ground state of a quantum dot and the biexciton state, as well as two-photon oscillations between the two single-exciton states with different circular or linear polarizations. The effect of phonon-induced decoherence on these processes is described and optimal system properties and optical driving conditions for coherent control are identified. It is shown that proper optimalization allows one to control the biexciton system via two-photon transitions with a high fidelity.
We show that the amount of coherent quantum information that can be reliably transmitted down a dephasing channel with memory is maximized by separable input states. In particular, we model the channel as a Markov chain or a multimode environment of oscillators. While in the first model the maximization is achieved for the maximally mixed input state, in the latter it is convenient to exploit the presence of a decoherence-protected subspace generated by memory effects. We explicitly compute the quantum channel capacity for the first model while numerical simulations suggest a lower bound for t…
Using femtosecond pump-probe spectroscopy, we identify excitation induced dephasing as a major mechanism responsible for the breaking of the strong-coupling between excitons and photons in a semiconductor microcavity. The effects of dephasing are observed on the transmitted probe pulse spectrum as a density dependent broadening of the exciton-polariton resonances and the emergence of a third resonance at high excitation density. A striking asymmetry in the energy shift between the upper and the lower polaritons is also evidenced. Using the excitonic Bloch equations, we quantify the respective …
In solids and organic materials, environment-induced dephasing of particles and long-lived excitations leads to the crossover in their transport properties between quantum wave-like propagation and classical diffusive motion. In this work, we demonstrate that dynamics of single carriers in this intermediate crossover regime can exhibit distinct signatures such as the formation of vortices and viscous flow, the phenomena typically considered as manifestations of hydrodynamic transport. We explain this effect by modeling suppressed quantum interference of carriers, and we show that the resulting…
Transport of excitons through transfer networks is a unique example where the interplay between quantum coherence and environment-induced dephasing leads to non-trivial effects. One exciting example is the "environment-assisted quantum transport", (ENAQT), where, counter intuitively, the environment interrupts quantum transport in a way that enhances the transfer efficiency. Here we show that the interplay between dephasing and quantum coherence can lead to an additional function in exciton transport - photo-protection, that is the reduction of current upon increased excitation. We start by de…
We study dynamics of the measurement process in quantum dot systems, where a particular state out of coherent superposition is observed. The ballistic point-contact placed near one of the dots is taken as a noninvasive detector. We demonstrate that the measurement process is fully described by the Bloch-type equations applied to the whole system. These equations clearly reproduce the collapse of the density-matrix into the statistical mixture in the course of the measurement process. The corresponding dephasing width is uniquely defined. We show that the continuous observation of one of the st…
Carrier spins in semiconductor nanocrystals are promising candidates for quantum information processing. Using a combination of time-resolved Faraday rotation and photoluminescence spectroscopies, we demonstrate optical spin polarization and coherent spin precession in colloidal CsPbBr3 nanocrystals that persists up to room temperature. By suppressing the influence of inhomogeneous hyperfine fields with a small applied magnetic field, we demonstrate inhomogeneous hole transverse spin-dephasing times (T2*) that approach the nanocrystal photoluminescence lifetime, such that nearly all emitted ph…
We study a dephasing channel with memory, modelled by a multimode environment of oscillators. Focusing on the case of two channel uses, we show that memory effects can enhance the amount of coherent quantum information transmitted down the channel. We also show the Kraus representation for two channel uses. Finally, we propose a coding-decoding scheme that takes advantage of memory to improve the fidelity of transmission.
We study electron spin decoherence in a two-electron double quantum dot due to the hyperfine interaction, under spin-echo conditions as studied in recent experiments. We develop a semi-classical model for the interaction between the electron and nuclear spins, in which the time-dependent Overhauser fields induced by the nuclear spins are treated as classical vector variables. Comparison of the model with experimentally-obtained echo signals allows us to quantify the contributions of various processes such as coherent Larmor precession and spin diffusion to the nuclear spin evolution.
We study dephasing of electrons induced by a which path detector and thus verify Bohr's complementarity principle for fermions. We utilize a double path interferometer with two slits, with one slit being replaced by a coherent quantum dot (QD). A short one dimensional channel, in the form of a quantum point contact (QPC), in close proximity to the QD, serves as a which path detector. We find that by varying the properties of the QPC detector we affect the visibility of the interference, inducing thus dephasing. We develop a simple model to explain the dephasing due to the nearby detector and f…
The full time-dependent four-wave mixing polarization in quantum dots is microscopically calculated, taking into account acoustic phonon-assisted transitions between different exciton states of the dot. It is shown that quite different dephasing times of higher exciton states in pancake anisotropic InGaAs quantum dots are responsible for the experimentally observed [1] double-exponential decay in the photon echo signal.
Environment-assisted quantum transport (ENAQT) is the possibility of an external environment to enhance transport efficiency of quantum particles. This idea has generated much excitement over recent years, especially due to the experimentally-motivated possibility of ENAQT in photo-synthetic exciton transfer complexes. Many theoretical calculations have shown ENAQT, but the explanations for its origin differ, and a universal explanation has been elusive. Here we demonstrate a universal origin for ENAQT in quantum networks with a dephasing environment, based on a relation between exciton curren…
We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quantum aggregate. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phon…
Controlled dephasing of electrons, via 'which path' detection, involves, in general, coupling a coherent system to a current driven noise source. However, here, we present a case in which a nearly isolated electron puddle at thermal equilibrium strongly affects the coherence of a nearby electronic interferometer. Moreover, for certain average electron occupations of the puddle, the interferometer exhibits complete dephasing. This robust phenomenon stems from the Friedel Sum Rule, which relates a system's occupation with its scattering phases. The interferometer opens a peeping window into phys…
This is a review of the phase coherent transmission through interacting mesoscopic conductors. As a paradigm we study the transmission amplitude and the dephasing rate for electron transport through a quantum dot in the Coulomb blockade regime. We summarize experimental and theoretical work devoted to the phase of the transmission amplitude. It is shown that the evolution of the transmission phase may be dominated by non-universal features in the short-time dynamics of the quantum dot. The controlled dephasing in Coulomb coupled conductors is investigated. Examples comprise a single or multipl…
We report high resolution coherent population trapping on a single hole spin in a semiconductor quantum dot. The absorption dip signifying the formation of a dark state exhibits an atomic physics-like dip width of just 10 MHz. We observe fluctuations in the absolute frequency of the absorption dip, evidence of very slow spin dephasing. We identify this process as charge noise by, first, demonstrating that the hole spin g-factor in this configuration (in-plane magnetic field) is strongly dependent on the vertical electric field, and second, by characterizing the charge noise through its effects…
Understanding the interplay between disorder, environment and interactions is key to elucidating the transport properties of open quantum systems, from excitons in photosynthetic networks to qubits in ion traps. This interplay is studied here theoretically in the context of environment-assisted quantum transport (ENAQT), a unique situation in open system where an environment-induced dephasing can, counter-intuitively, enhance transport. First, we show a surprising situation where the particle current grows with increasing disorder, even without dephasing. Then, we suggest a specific mechanism …
Excitonic transport in static disordered one dimensional systems is studied in the presence of thermal fluctuations that are described by the Haken-Strobl-Reineker model. For short times, non-diffusive behavior is observed that can be characterized as the free-particle dynamics in the Anderson localized system. Over longer time scales, the environment-induced dephasing is sufficient to overcome the Anderson localization caused by the disorder and allow for transport to occur which is always seen to be diffusive. In the limiting regimes of weak and strong dephasing quantum master equations are …
Kondo correlation in a spin polarized quantum dot (QD) results from the dynamical formation of a spin singlet between the dot's net spin and a Kondo cloud of electrons in the leads, leading to enhanced coherent transport through the QD. We demonstrate here significant dephasing of such transport by coupling the QD and its leads to potential fluctuations in a near by 'potential detector'. The qualitative dephasing is similar to that of a QD in the Coulomb Blockade regime in spite of the fact that the mechanism of transport is quite different. A much stronger than expected suppression of coheren…
Conductance signatures that signal the presence of Majorana zero modes in a three terminal nanowire-topological superconductor hybrid system are analyzed in detail, in both the clean nanowire limit and in the presence of non-coherent dephasing interactions. In the coherent transport regime for a clean wire, we point out contributions of the local Andreev reflection and the non-local transmissions toward the total conductance lineshapes while clarifying the role of contact broadening on the Majorana conductance lineshapes at the magnetic field parity crossings. Interestingly, at larger $B$-fiel…
We calculate the dephasing rate of an electron state in a pinched quantum dot, due to Coulomb interactions between the electron in the dot and electrons in a nearby voltage biased ballistic nanostructure. The dephasing is caused by nonequilibrium time fluctuations of the electron density in the nanostructure, which create random electric fields in the dot. As a result, the electron level in the dot fluctuates in time, and the coherent part of the resonant transmission through the dot is suppressed.
A study is presented concerning the influence of flicker noise in the junction transparency on coherent transport in Andreev states. The amount of dephasing is estimated for a microwave-activated quantum interferometer. Possibilities of experimentally investigating the coupling between a superconducting quantum point contact and its electromagnetic environment are discussed.
We study phonon-assisted dephasing in optically excited semiconductor quantum dots within the frameworks of the independent Boson model and optimal control. Using a realistic description for the quantum dot states and the phonon coupling, we demonstrate that such dephasing has a drastic impact on the coherent optical response. We employ optimal control theory to search for control strategies that allow to fight decoherence, and show that appropriate tailoring of laser pulses allows a complete control of the optical excitation despite the phonon dephasing.
The dephasing time of the lowest bright exciton in CdSe/ZnS wurtzite quantum dots is measured from 5 K to 170 K and compared with density dynamics within the exciton fine structure using a sensitive three-beam four-wave-mixing technique unaffected by spectral diffusion. Pure dephasing via acoustic phonons dominates the initial dynamics, followed by an exponential zero-phonon line dephasing of 109 ps at 5 K, much faster than the ~10 ns exciton radiative lifetime. The zero-phonon line dephasing is explained by phonon-assisted spin-flip from the lowest bright state to dark exciton states. This is…
The nonlinearity exhibited by the kinetic inductance of a superconducting stripline couples stripline resonator modes together in a manner suitable for quantum non-demolition measurement of the number of photons in a given resonator mode. Quantum non-demolition measurement is accomplished by coherently driving another resonator mode, referred to as the detector mode, and measuring its response. We show that the sensitivity of such a detection scheme is directly related to the dephasing rate induced by such an intermode coupling. We show that high sensitivity is expected when the detector mode …
new defect-assisted mechanism of multiphonon intraband carrier relaxation in semiconductor quantum dots, where the carrier is found in a coherent superposition of the initial, final, and defect states, is proposed. It is shown that this mechanism is capable of explaining the observed trends in temperature dependences of the intraband relaxation rates for PbSe and CdSe colloidal nanocrystal quantum dots.
We analyze the dissipative dynamics of a two-level quantum system subject to low-frequency, e.g. 1/f noise, motivated by recent experiments with superconducting quantum circuits. We show that the effect of transverse linear coupling of the system to low-frequency noise is equivalent to that of quadratic longitudinal coupling. We further find the decay law of quantum coherent oscillations under the influence of both low- and high-frequency fluctuations, in particular, for the case of comparable rates of relaxation and pure dephasing.
The interaction between coherent polaritons and incoherent excitons plays an important role in polariton physics. Using resonant pump-probe spectroscopy with selective excitation of single polariton branches, we investigate the different dephasing mechanisms responsible for generating a long-lived exciton reservoir. As expected, pumping the upper polariton results in a strong dephasing process that leads to the generation of a long lived reservoir. Unexpectedly, we observe an efficient reservoir creation while exciting only the lower polariton branch when the detuning is increased towards posi…
We study cotunneling in a double junction Coulomb blockade device under the influence of time dependent potentials. It is shown that the ac-bias leads to photon assisted cotunneling which in some cases may dominate the transport. We derive a general non-perturbative expression for the tunneling current in the presence of oscillating potentials and give a perturbative expression for the photon assisted cotunneling current.
We present time-resolved measurements of spin-flip photon-assisted tunneling and spin-flip relaxation in a doubly occupied double quantum dot. The photon-assisted excitation rate as a function of magnetic field indicates that spin-orbit coupling is the dominant mechanism behind the spin-flip under the present conditions. We are able to extract the resulting effective `spin-flip tunneling' energy, which is found to be three orders of magnitude smaller than the regular spin-conserving tunneling energy. We also measure the relaxation and dephasing times of a qubit formed out of two two-electron s…
The longstanding problem of the Hall resistivity rho(x,y) in the Hall insulator phase is addressed using four-lead Chalker-Coddington networks. Electron interaction effects are introduced via a finite dephasing length. In the quantum coherent regime, we find that rho(x,y) scales with the longitudinal resistivity rho(x,x), and they both diverge exponentially with dephasing length. In the Ohmic limit, (dephasing length shorter than Hall puddles' size), rho(x,y) remains quantized and independent of rho(x,x). This suggests a new experimental probe for dephasing processes.
The observation of coherent quantum transport phenomena in metals and semiconductors is limited by the eventual loss of phase coherence of the conducting electrons. We use the weak localization effect to measure the low-temperature dephasing time in a two-dimensional electron Fermi liquid in GaAs/AlGaAs heterostructures. We use a novel temperature calibration method based on the integer quantum Hall effect in order to directly measure the electrons' temperature. The data are in excellent agreement with recent theoretical results, including contributions from the triplet channel, for a broad te…
We investigate the degree of coherence of electronic transport through a quantum dot (QD) in the presence of an intradot electron-electron interaction. By using an open multi-terminal Aharonov-Bohm (AB) setup, we find that the intradot interaction does not induce any dephasing effect and the electron transport through the QD is fully coherent. We also observe that the asymmetric amplitude of the AB oscillation in the conductance through the two-terminal AB setup originates from the interplay between the confined structure and the electron-electron interaction. Thus, one can not associate a dep…
By examining the full counting statistics of a non adiabatic pure spin pump with particular emphasis on the second and third moments, it is shown that incoherent or sequential transport, in contrast to coherent transport, can change non-local spin shot noise cross-correlations from being anti-correlated to being completely correlated, a truly counterintuitive result. The third moment on the other hand is shown to be much more resilient and its nature remains unaltered in incoherent transport regime. However, phenomenologically including dephasing modifies this picture as both Shot noise and mo…
Coherent Rashba spin precession along interacting multi-mode quantum channels is investigated, revisiting the theory of coupled Tomonaga-Luttinger liquids. We identify susceptibilities as the key-parameters to govern exponents and Rashba precession lengths. In semiconducting quantum wires spins of different transport channels are found to {\em dephase} in their respective precession angles with respect to one another, as a result of the interaction. This could explain the experimental difficulty to realize the Datta Das transistor. In single walled carbon nanotubes, on the other hand, interact…
