The molecular photo cell, i.e., a single molecule donor-acceptor complex, beside being technologically important, is a paradigmatic example of a many-body system operating in strong non-equilibrium. The quantum transport and the photo-voltaic energy conversion efficiency of the photocell, attached to two external leads, are investigated within the open quantum system approach by solving the Lindblad master equation. The interplay of the vibrational degrees of freedom corresponding to the molecules (via the electron-phonon interaction) and the environment (via dephasing) shows its signature in the efficiency at maximum power. We find vibration assisted electron transport in the medium to strong electron-phonon coupling regime when the system does not suffer dephasing. Exposure to dephasing hampers such a vibration assisted electron transport in a specific range of dephasing rate.
The interplay between exctions and vibrations is considered to be a key factor in determining the exciton transfer properties in light-harvesting exciton transfer complexes. Here we study this interplay theoretically in a model for exciton transport, composed of two chromophores coupled to an exciton source and sink in the presence of vibrations. We consider two cases, that show qualitatively distinct transport features. In the first, the vibrations are global and affect the two chromophores simultaneously. In the second case, the vibrations are localized on each chromophore. For global vibrat…
Understanding the interplay between disorder, environment and interactions is key to elucidating the transport properties of open quantum systems, from excitons in photosynthetic networks to qubits in ion traps. This interplay is studied here theoretically in the context of environment-assisted quantum transport (ENAQT), a unique situation in open system where an environment-induced dephasing can, counter-intuitively, enhance transport. First, we show a surprising situation where the particle current grows with increasing disorder, even without dephasing. Then, we suggest a specific mechanism …
We perform photon-assisted-tunneling (PAT) experiments on a GaAs double quantum dot device under high microwave excitation power. Photon-assisted absorption of up to 14 photons is observed, when electron temperature (>1K) are far above the lattice temperature. Signatures of Landau-Zener-Stückelberg (LZS) interference are found even in this non-equilibrium PAT spectrum. In addition, the charge state relaxation time T_1~8ns measured in this out of thermal equilibrium double quantum dot is in agreement with other previous reports.
We focus on a recently experimentally realized scenario of normal-metal-insulator-superconductor tunnel junctions coupled to a superconducting resonator. We develop a first-principles theory to describe the effect of photon-assisted electron tunneling on the quantum state of the resonator. Our results are in very good quantitative agreement with the previous experiments on refrigeration and heating of the resonator using the photon-assisted tunneling, thus providing a stringent verification of the developed theory. Importantly, our results provide simple analytical estimates of the voltage-tun…
We demonstrate that the radiation induced "zero-resistance state" observed in a two-dimensional electron gas is a result of the non-trivial structure of the density of states of the systems and the photon assisted transport. A toy model of a structureless quantum tunneling junction where the system has oscillatory density of states catches most of the important features of the experiments. We present a generalized Kubo-Greenwood conductivity formula for the photon assisted transport in a general system, and show essentially the same nature of the transport anomaly in a uniform system.
The low temperature spin dynamics of a Fe8 Single-Molecule Magnet was studied under circularly polarized electromagnetic radiation allowing us to establish clearly photon-assisted tunneling. This effect, while linear at low power, becomes highly non-linear above a relatively low power threshold. This non-linearity is attributed to the nature of the coupling of the sample to the thermostat.These results are of great importance if such systems are to be used as quantum computers.
Transport of excitons through transfer networks is a unique example where the interplay between quantum coherence and environment-induced dephasing leads to non-trivial effects. One exciting example is the "environment-assisted quantum transport", (ENAQT), where, counter intuitively, the environment interrupts quantum transport in a way that enhances the transfer efficiency. Here we show that the interplay between dephasing and quantum coherence can lead to an additional function in exciton transport - photo-protection, that is the reduction of current upon increased excitation. We start by de…
We calculate the contribution of the photon-assisted interaction of electrons with leaky interface phonons to the dissipative dc photoconductivity of a two-dimensional electron system in a magnetic field. The calculated photoconductivity as a function of the frequency of microwave radiation and the magnetic field exhibits pronounced oscillations. The obtained oscillation structure is different from that in the case of photon-assisted interaction with impurities. We demonstrate that at a sufficiently strong microwave radiation in the certain ranges of its frequency (or in certain ranges of the …
For a single semiconductor quantum dot embedded in a microcavity, we theoretically and experimentally investigate phonon-assisted transitions between excitons and the cavity mode. Within the framework of the independent boson model we find that such transitions can be very efficient, even for relatively large exciton-cavity detunings of several millielectron volts. Furthermore, we predict a strong detuning asymmetry for the exciton lifetime that vanishes for elevated lattice temperature. Our findings are corroborated by experiment, which turns out to be in good quantitative and qualitative agr…
Via the numerical analysis on the intraband dynamics of optically excited semiconductor superlattices, we find that time-integrated squared THz emission signals can be used for probing both dynamic localization and multi-photon resonance in the coherent regime. Competition effect between dynamic localization and photon-assisted transport has also been discussed.
We study photon-assisted transport in a single-level quantum dot system under a periodically oscillating field. Photon-assisted current noises in the presence of the Coulomb interaction are calculated based on a gauge-invariant formulation of time-dependent transport. We derive the vertex corrections within the self-consistent Hartree-Fock approximation in terms the Floquet-Green's functions (Floquet-GFs), and examine the effects of the Coulomb interaction on the photon-assisted current noises. Moreover, we introduce a concept of an effective temperature to characterize nonequilibrium properti…
Photo-assisted transport through a mesoscopic conductor occurs when an oscillatory (AC) voltage is superposed to the constant (DC) bias which is imposed on this conductor. Of particular interest is the photo assisted shot noise, which has been investigated theoretically and experimentally for several types of samples. For DC biased conductors, a detection scheme for finite frequency noise using a dissipative resonant circuit, which is inductively coupled to the mesoscopic device, was developped recently. We argue that the detection of the finite frequency photo-assisted shot noise can be achie…
We report measurements of photon-assisted transport and noise in a tunnel junction in the regime of dynamical Coulomb blockade. We have measured both dc non-linear transport and low frequency noise in the presence of an ac excitation at frequencies up to 33 GHz. In both experiments we observe replicas at finite voltage of the zero bias features, a phenomenon characteristic of photon emission/absorption. However, the ac voltage necessary to explain our data is notably different for transport and noise, indicating that usual theory of photon-assisted phenomena fails to account for our observatio…
We report on electron transport through an artificial molecule formed by two tunnel coupled quantum dots, which are laterally confined in a two-dimensional electron system of an Al$_x$Ga$_{1-x}$As/GaAs heterostructure. Coherent molecular states in the coupled dots are probed by photon-assisted tunneling (PAT). Above 10 GHz, we observe clear PAT as a result of the resonance between the microwave photons and the molecular states. Below 8 GHz, a pronounced superposition of phonon- and photon-assisted tunneling is observed. Coherent superposition of molecular states persists under excitation of ac…
We report measurements of the low frequency current fluctuations of a tunnel junction placed at very low temperature biased by a time-dependent voltage $V(t)=V(1+\cos 2πνt)$. We observe that the excess noise generated by the ac excitation exhibits quantum oscillations as a function of the dc bias, with a period given by $hν/e$ with $e$ the charge of a single electron. This is a direct consequence of the quantum nature of electricity in a normal conductor.
We used a complete tight-binding band structure of graphene nanoribbon to obtain, for the first time, analytical techniques for observing photon assisted transport, and dynamic localization of electrons in the graphene nanoribbons. When the ribbons are subject to a multi-frequency dc-ac field, photon assisted replicas show up at rather strong drive force. The strong dependence of the photon peaks on ac amplitudes allow for high-harmonic dynamic oscillations at these amplitudes. We identified regions of positive differential conductivity where a nanoelectronic graphene device may be operated as…
When subjected to electromagnetic radiation, the fluctuation of the electronic current across a quantum conductor increases. This additional noise, called photon-assisted shot noise, arises from the generation and subsequent partition of electron-hole pairs in the conductor. The physics of photon-assisted shot noise has been thoroughly investigated at microwave frequencies up to 20 GHz, and its robustness suggests that it could be extended to the Terahertz (THz) range. Here, we present measurements of the quantum shot noise generated in a graphene nanoribbon subjected to a THz radiation. Our r…
The influence of strong internal forces on photon-assisted scattering and on the displacement mechanism of magnetoconductivity oscillations in a two-dimensional (2D) electron gas is theoretically studied. The theory is applied to the highly correlated system of surface electrons on liquid helium under conditions that the microwave frequency is substantially different from inter-subband resonance frequencies. A strong dependence of the amplitude of magnetoconductivity oscillations on the electron density is established. The possibility of experimental observation of such oscillations caused by …
It is argued that Trauzettel et al. [Phys. Rev. B 75, 035305 (2007)] made some mistakes in their calculations regarding the photon-assisted transport in graphene that lead to uncoupled sidebands and emergence of step-like features in dG/dV (G is differential conductance and V is the bias voltage). We discuss the relevant corrections and explain in detail how the correct results are expected to be quite different than the incorrect ones.
We propose a protocol for state transfer and entanglement generation between two distant spin qubits (sender and receiver) that have different energies. The two qubits are permanently coupled to a far off-resonant spin-chain, and the qubit of the sender is driven by an external field, which provides the energy required to bridge the energy gap between the sender and the receiver. State transfer and entanglement generation are achieved via virtual single-photon and multi-photon transitions to the eigenmodes of the channel.
We investigate both experimentally and theoretically a simple yet more robust and flexible alternative to Rabi oscillation-type biexciton preparation protocols traditionally used for semiconductor quantum dots. The quantum dot is excited by a strong laser pulse positively detuned from the two-photon resonance yielding an on demand initialization of the biexciton state by making use of the phonon-induced thermalization of the photon dressed states. It is shown that for excitation pulses in the picosecond range, a stable and high fidelity of up to $f_{XX}=0.98\pm 0.01$ is reached. Notably, the g…
We review experiments on single electron transport through single quantum dots in the presence of a microwave signal. In the case of a small dot with well-resolved discrete energy states, the applied high-frequency signal allows for inelastic tunnel events that involve the exchange of photons with the microwave field. These photon assisted tunneling (PAT) processes give rise to sideband resonances in addition to the main resonance. Photon absorption can also lead to tunneling via excited states instead of tunneling via the ground state of the quantum dot.
Schrödinger cat states are useful for many applications, ranging from quantum information processing to high-precision measurements. In this paper we propose a conceptually new method for creating such cat states, based on photon-assisted Landau-Zener-Stückelberg interferometry in a hybrid system consisting of a qubit coupled to a photon cavity. We show that by initializing the qubit in one of its basis states, performing three consecutive sweeps of the qubit energy splitting across the 1-photon resonance, and finally projecting the qubit to the same basis state, the parity of the photon field…
We report on the observation of the cyclotron-resonance-assisted photon drag effect. Resonant photocurrent is detected in InSb/InAlSb quantum wells structures subjected to a static magnetic field and excited by terahertz radiation at oblique incidence. The developed theory based on Boltzmann's kinetic equation is in a good agreement with the experimental findings. We show that the resonant photocurrent originates from the transfer of photon momentum to free electrons drastically enhanced at cyclotron resonance.
We consider the fluctuations of the electrical current (shot noise) in the presence of a voltage time-modulation. For a non-interacting metal, it is known that the derivative of the photo-assisted noise has a staircase behavior. In the presence of Coulomb interactions, we show that the photo-assisted noise presents a more complex profile, in particular for the two following systems: 1) a two-dimensional electron gas in the fractional quantum Hall regime for which we have obtained evenly spaced singularities in the noise derivative, with a spacing related to the filling factor and, 2) a carbon …
We have studied the Fano resonance in photon-assisted transport in a quantum dot and calculated both the coherent current and spectral density of shot noise. It is predicted, for the first time, that the shape of Fano profile will also appear in satellite peaks. It is found that the variations of Fano profiles with the strengths of nonresonant transmissions are not synchronous in absorption and emission sidebands. The effect of interference on photon-assisted pumped current has been also investigated. We further predict the current and spectral density of shot noise as a function of the phase,…
We report both photon- and phonon-assisted tunneling transitions in a linear array of three quantum dots, which can only be understood by considering the full three-dimensionality of the charge stability diagram. Such tunneling transitions potentially contribute to leakage of qubits defined in this system. A detailed understanding of these transitions is important as they become more abundant and complex to analyze as quantum dot arrays are scaled up.
We introduce a scheme that combines photon-assisted tunneling by a moving optical lattice with strong Hubbard interactions, and allows for the quantum simulation of paradigmatic quantum many-body models. We show that, in a certain regime, this quantum simulator yields an effective Hubbard Hamiltonian with tunable bond-charge interactions, a model studied in the context of strongly-correlated electrons. In a different regime, we show how to exploit a correlated destruction of tunneling to explore Nagaoka ferromagnetism at finite Hubbard repulsion. By changing the photon-assisted tunneling param…
We investigate transient transport of electrons through a single-quantum-dot controlled by a plunger gate. The dot is embedded in a finite wire that is weakly coupled to leads and strongly coupled to a single cavity photon mode. A non-Markovian density-matrix formalism is employed to take into account the full electron-photon interaction in the transient regime. In the absence of a photon cavity, a resonant current peak can be found by tuning the plunger gate voltage to lift a many-body state of the system into the source-drain bias window. In the presence of an $x$-polarized photon field, add…
Quantum state transfer is crucial for quantum information processing and quantum computation. Here, we propose a hybrid optomechanical system capable of coupling a qubit, an optical mode and a mechanical oscillator. The displacement of the mechanical oscillator,due to radiation pressure, induces spatial variation in the cavity field, which in turn couples the qubit with phonon mode. This allows state transfer between the cavity mode and the qubit without an actual interaction between them. We present a scheme for the transitionless quantum state transfer based on the transitionless quantum dri…
The photo-assisted heat current through a metal/dot/metal junction and its associated Peltier coefficient are computed in the framework of the time-dependent out-of-equilibrium Keldysh formalism in the presence of a dot energy modulation. When the frequency of the modulation is much larger than the amplitude of the modulation, the heat current follows the sinusoidal time evolution of the dot energy. This is no longer the case when the modulation frequency becomes of the order or smaller than the amplitude of the modulation. To characterize this non sinusoidal behavior, we have calculated the h…
We propose a theory for photon-assisted macroscopic quantum tunneling (MQT) in a stack of capacitively-coupled intrinsic Josephson junctions in which the longitudinal Josephson plasma, i.e., longitudinal collective phase oscillation modes, is excited. The scheme of energy-level quantization in the collective oscillatory states is clarified in the $N$-junction system. When the MQT occurs from the single-plasmon states excited by microwave irradiation in the multi-photon process to the uniform voltage state, our theory predicts that the escape rate is proportional to $N^2$. This result is consis…
We investigate real-time dynamics of spin-polarized current in a quantum dot coupled to ferromagnetic leads in both parallel and antiparallel alignments. While an external bias voltage is taken constant in time, a gate terminal, capacitively coupled to the quantum dot, introduces a periodic modulation of the dot level. Using non equilibrium Green's function technique we find that spin polarized electrons can tunnel through the system via additional photon-assisted transmission channels. Owing to a Zeeman splitting of the dot level, it is possible to select a particular spin component to be pho…
We study transport through one or two ultrasmall quantum dots with discrete energy levels to which a time-dependent field is applied (e.g., microwaves). The AC field causes photon-assisted tunneling and also transitions between discrete energy levels of the dot. We treat the problem by introducing a generalization of the rotating-wave approximation to arbitrarily many levels. We calculate the dc-current through one dot and find satisfactory agreement with recent experiments by Oosterkamp et al. . In addition, we propose a novel electron pump consisting of two serially coupled single-level quan…
Graphene electrodes provide a suitable alternative to metal contacts in molecular conduction nanojunctions. Here, we propose to use graphene electrodes as a platform for effective photon assisted tunneling through molecular conduction nanojunctions. We predict dramatic increasing currents evaluated at side-band energies $\sim n\hbarω$ ($n$ is a whole number) related to the modification of graphene gapless spectrum under the action of external electromagnetic field of frequency $ω$. A side benifit of using doped graphene electrodes is the polarization control of photocurrent related to the proc…
Based on exactly mapping of a many-body electron-phonon interaction problem onto a one-body problem, we apply the well-established nonequilibrium Green function technique to solve the time-dependent phonon-assisted tunneling at low temperature through a single-molecular quantum dot connected to two leads, which is subject to a microwave irradiation field. It is found that in the presence of the electron-phonon interaction and the microwave irradiation field, the time-average transmission and the nonlinear differential conductance display additional peaks due to pure photon absorption or emissi…
We present a straightforward and computationally cheap method to obtain the phonon-assisted photocurrent in large-scale devices from first-principles transport calculations. The photocurrent is calculated using nonequilibrium Green's function with light-matter interaction from the first-order Born approximation while electron-phonon coupling (EPC) is included through special thermal displacements (STD). We apply the method to a silicon solar cell device and demonstrate the impact of including EPC in order to properly describe the current due to the indirect band-to-band transitions. The first-…
Pauli exclusion principle can lead to a supression of transport through double quantum dots, even if both quantum dots are connected by a resonant driving ac field. In this work, we study how this effect, known as spin blockade, can be removed by means of the influence of the driving field on the contacts to the leads.
We consider the photon-assisted tunneling (PAT) and the Landau-Zener-Stueckelberg (LZS) interference for double quantum dots induced electrostatically along a semiconducting carbon nanotube. An atomistic tight-binding approach and the time-dependent configuration interaction method are employed for description of the systems of a few confined electrons and holes. We reproduce the patterns of the LZS interference recently observed for the quantum double dots describing transport across hole-localized states. Moreover, we indicate that for charge configurations for which the ground-state is Paul…
The effect of an ac perturbation on the shot noise of a fractional quantum Hall fluid is studied at finite temperature. For a normal metal, it is known that the zero-frequency noise derivative exhibits steps as a function of bias voltage. In contrast, at Laughlin fractions, the backscattering noise exhibits evenly spaced singularities, which are reminiscent of tunneling density-of-states singularities for quasiparticles. The spacing is determined by the quasiparticle charge $νe$ and the ratio of the dc bias with respect to the drive frequency. Photo-assisted transport can thus be considered as…
We consider a hybrid single-electron transistor (SET) constituted by a gate-controlled normal-metal island (N) connected to two voltage-biased superconducting leads (S) by means of two tunnel junctions (S-I-N-I-S), operated as a turnstile. We show that the exchange of photons between this system and the high-temperature electromagnetic environment where it is embedded enhances Andreev reflection, thereby limiting the single-electron tunneling accuracy.
Resonant tunneling through a quantum dot coupled to superconducting reservoirs in the presence of time-dependent external voltage has been studied. A general formula of the current is derived based on the nonequilibrium Green's function technique. Using this formula photon-assisted quasiparticle transport has been investigated for the quantum dot connected to superconductors. In addition, resonant Andreev transport through a strongly correlated quantum dot connected to a normal metallic lead and a superconducting lead is studied.
Recent double-slit interference experiments have demonstrated the possibility of probing the phase of the complex transmission coefficient of a quantum dot via the Aharonov-Bohm effect. We propose an extension of these experiments: an ac voltage imposed on the side gate with the concomitant photonic sidebands leads to additional structure both in the amplitude and in the phase of the Aharonov-Bohm signal. Observation of these effects would be a definitive proof of coherent absorption and reemission of photons from the ac source.
We show that the comment by A.F. Volkov ignores a delicate issue in the conductance measurement for a hall bar system. In such system, $ρ_{xx}\approx ρ_{xy}^{2}σ_{xx}$ while $σ_{xy}\gg σ_{xx}$, as correctly pointed out in Ref.3. We clarify that the so called "zero resistance state" is actually a "zero conductance state". A discussion concerning the phase transition induced by the negative conductance is presented.
Recently, the terahertz (THz) photon-assisted tunneling (PAT) through a two-level InAs quantum dot (QD) has been successfully realized in experiment [Phys. Rev. Lett. {\bf 109}, 077401 (2012)]. The Coulomb interaction in this device is comparable with the energy difference between the two energy levels. We theoretically explore the effects of Coulomb interaction on the PAT processes and show that the main peaks of the experiment can be well derived by our model analysis. Furthermore, we find additional peaks, which were not addressed in the InAs QD experiment and may be further identified in e…
The effect of an AC perturbation on the shot noise of a fractional quantum Hall fluid is studied both in the weak and the strong backscattering regimes. It is known that the zero-frequency current is linear in the bias voltage, while the noise derivative exhibits steps as a function of bias. In contrast, at Laughlin fractions, the backscattering current and the backscattering noise both exhibit evenly spaced singularities, which are reminiscent of the tunneling density of states singularities for quasiparticles. The spacing is determined by the quasiparticle charge $νe$ and the ratio of the DC…
We theoretically investigate the production of polarization-entangled photons through the biexciton cascade decay in a single semiconductor quantum dot. In the intermediate state the entanglement is encoded in the polarizations of the first emitted photon and the exciton, where the exciton state can be effectively ``measured'' by the solid state environment through the formation of a lattice distortion. We show that the resulting loss of entanglement becomes drastically enhanced if the phonons contributing to the lattice distortion are subject to elastic scatterings at the device boundaries, w…
We analyze dephasing in single and double quantum dot systems. The decoherence is introduced by the Büttiker model with current conserving fictitious voltage leads connected to the dots. By using the non-equilibrium Green function method, we investigate the dephasing effect on the tunneling current. It is shown that a finite dephasing rate leads to observable effects. The result can be used to measure dephasing rates in quantum dots.
We analyze quantum charge pumping in an open ring with a dot embedded in one of its arms. We show that cyclic driving of the dot levels by a \textit{single} parameter leads to a pumped current when a static magnetic flux is simultaneously applied to the ring. Based on the computation of the Floquet-Green's functions, we show that for low driving frequencies $ω_0$, the interplay between the spatial interference through the ring plus photon-assisted tunneling gives an average direct current (dc) which is proportional to $ω_0^{2}$. The direction of the pumped current can be reversed by changing t…
It is shown that, although the major feature of the microwave-induced magnetoresistance oscillations in two-dimensional (2D) electron systems is insensitive to the behavior of the elastic scattering in the photon-assisted impurity scattering model [X.L. Lei and S.Y. Liu, Phys. Rev. Lett. 91, 226805 (2003)], the required microwave intensity to induce an effective oscillation depends strongly on the form of the impurity potential. A microwave electric field of a few Volts per cm in amplitude is sufficient to induce remarkable oscillations if the elastic scatterings are due to background charged …
In this review we focus on electronic transport through semiconductor nanostructures which are driven by ac fields. Along the review we describe the available experimental information on different nanostructures, like resonant tunneling diodes, superlattices or quantum dots, together with the theoretical tools needed to describe the observed features. These theoretical tools such as, for instance, the Floquet formalism, the non-equilibrium Green's function technique or the density matrix technique, are suitable for tackling with photon-assisted transport problems where the interplay of differe…
We analyze long-range transport through an ac driven triple quantum dot with one single electron. An effective model is proposed for the analysis of photoassisted cotunnel in order to account for the virtual processes which dominate the long-range transport, which takes place at n-photon resonances between the edge quantum dots. The AC field renormalizes the inter dot hopping, modifying the levels hybridization. It results in a non trivial behavior of the current with the frequency and intensity of the external ac field.
We report microwave-driven photon-assisted tunneling in a suspended carbon nanotube double quantum dot. From the resonant linewidth at a temperature of 13 mK, the charge dephasing time is determined to be 280 +- 30 ps. The linewidth is independent of driving frequency, but increases with increasing temperature. The moderate temperature dependence is inconsistent with expectations from electron-phonon coupling alone, but consistent with charge noise arising in the device. The extracted level of charge noise is comparable with that expected from previous measurements of a valley-spin qubit, wher…
Motivated by a recent experiment by L.-H. Reydellet et al., Phys. Rev. Lett. 90, 176803 (2003), we discuss an interpretation of photon-assisted shot noise in mesoscopic multiprobe conductors in terms of electron-hole pair excitations. AC-voltages are applied to the contacts of the sample. Of interest are correlations resulting from the fact that electrons and holes are generated in pairs. We show that with two out-of-phase ac-potentials of equal magnitude and frequency, applied to different contacts, it is possible to trace out the Hanbury Brown Twiss exchange interference correlations in a fo…
Photon-assisted electron transport in ballistic graphene is analyzed using scattering theory. We show that the presence of an ac signal (applied to a gate electrode in a region of the system) has interesting consequences on electron transport in graphene, where the low energy dynamics is described by the Dirac equation. In particular, such a setup describes a feasible way to probe energy dependent transmission in graphene. This is of substantial interest because the energy dependence of transmission in mesoscopic graphene is the basis of many peculiar transport phenomena proposed in the recent…
The way molecules absorb, transfer, and emit light can be modified by coupling them to optical cavities. The extent of the modification is often defined by the cavity-molecule coupling strength, which depends on the number of coupled molecules. We experimentally and numerically study the evolution of photoemission from a thin layered J-aggregated molecular material strongly coupled to a Fabry-Perot microcavity as a function of the number of coupled layers. We unveil an important difference between the strong coupling signatures obtained from reflection spectroscopy and from polariton assisted …
