A theoretical study of surface plasmon polaritons (SPPs) in ultrathin lossy metal films is presented. The dispersion relation of such films is well known and can be solved numerically to obtain a combination of long-range (LR-) and short-range (SR-) eigenmodes. In this contribution, a simple solution for the SR-SPPs is derived. An approximation for the LR- eigenmodes can be found elsewhere. To validate the approximation, a two dimensional (2D) periodic array of small holes is studied subsequently. The spectral response of the array is obtained by full-wave simulations and the results compared with those calculated analytically, showing an excellent agreement for small holes.
We present plasmonic Bragg reflectors for increasing the extraordinary optical transmission through periodic arrays of subwavelength apertures in a metal film. The increase in transmission arises by preventing loss at the edges of the array. The plasmonic Bragg reflectors have periodicity of half the usual array's periodicity. Nano-hole arrays flanked thus by reflectors exchibited double the transmission as compared to the arrays without reflectors. These structures may also be used to isolate devices in plasmonic integrated circuits.
We have observed enhanced transmission of light through a gold film due to excitation of standing surface plasmon Bloch waves in a surface Fabry-Perot resonator. Our experimental results strongly contradict the recently suggested model of light transmission via excitation of a composite diffractive evanescent wave.
The properties of thermal radiation exchange between hot and cold objects can be strongly modified if they interact in the near field where electromagnetic coupling occurs across gaps narrower than the dominant wavelength of thermal radiation. Using a rigorous fluctuational electrodynamics approach, we predict that ultra-thin films of plasmonic materials can be used to dramatically enhance near-field heat transfer. The total spectrally integrated film-to-film heat transfer is over an order of magnitude larger than between the same materials in bulk form and also exceeds the levels achievable w…
We report observation of anisotropic surface plasmon-coupled emission (SPCE) from structured PMMA films doped with Rhodamine B (RhB) and deposited on silver films. For a given structure, it is observed that relative position of incident laser spot to the structured PMMA and polarization properties of the laser beam can be used to modulate the SPCE patterns. The proposed method enables azimuthally controlling directional SPCE in a deterministic manner.
The light transmission through square and rectangular holes in a metal film has been studied. By taking account of plasma response of real metal on hole walls as well as metal surface, an analytical result for the transmission has been deduced, which agrees well with the experiments. We show that the light transmission involves both the diffraction modes and the surface plasmons. Strong coupling of diffraction modes to surface plasmon polariton results in the transmission minima, whereas the coupling to cavity surface plasmon leads to the transmission maxima. The results suggest a dual-effect …
We demonstrate an efficient double-layer light absorber by exciting plasmonic phase resonances. We show that the addition of grooves can cause mode splitting of the plasmonic waveguide cavity modes and all the new resonant modes exhibit large absorptivity greater than 90%. Some of the generated absorption peaks have wide-angle characteristics. Furthermore, we find that the proposed structure is fairly insensitive to the alignment error between different layers. The proposed plasmonic nano-structure designs may have exciting potential applications in thin film solar cells, thermal emitters, nov…
A nanodiamond (ND) hosting nitrogen-vacancy (NV) color centers is attached on the apex of an optical tip for near-field microscopy. Its fluorescence is used to launch surface plasmon-polaritons (SPPs) in a thin polycrystalline gold film. It is shown that the quantum nature of the initial source of light is preserved after conversion to SPPs. This opens the way to a deterministic quantum plasmonics, where single SPPs can be injected at well-defined positions in a plasmonic device produced by top-down approaches.
Tunable terahertz plasmons are essential for reconfigurable photonics, which have been demonstrated in graphene through gating, though with relatively weak responses. Here, we demonstrate strong terahertz plasmons in graphite thin films via infrared spectroscopy, with dramatic tunability by even a moderate temperature change or an in-situ bias voltage. Meanwhile, through magneto-plasmon studies, we reveal that massive electrons and massless Dirac holes make comparable contributions to the plasmon response. Our study not only sets up a platform for further exploration of two-component plasmas, …
Evanescent waves in a metal thin film with nonlocality are found to propagate in normal direction to film surface with quenched (to zero) energy dissipation associated with intra-band electron transitions when wave numbers satisfy a resonant condition. It is shown that resonant quenching of energy dissipation (RQED) effect occurs in metal films with thicknesses of less or larger than, but still on the order of, the nonlocality scale length. RQED ceases to exist in metal films whose thickness exceeds a cutoff length or in metal films with local dielectric permittivity. Resonant quenching of ene…
The solution of a boundary--value problem formulated for the Kretschmann configuration shows that the phase speed of a surface--plasmon--polariton (SPP) wave guided by the planar interface of a sufficiently thin metal film and a sculptured thin film (STF) depends on the vapor incidence angle used while fabricating the STF by physical vapor deposition. Furthermore, it may be possible to engineer the phase speed by periodically varying the vapor incidence angle. The phase speed of the SPP wave can be set by selecting higher mean value and/or the modulation amplitude of the vapor incidence angle.
By using a self-consistent Maxwell-Bloch method, we demonstrate the simultaneously lasing and spasing behavior in a simple metal grating-film nanostructure, which can be attributed to spatial hole burning and the gain competition of different modes at the band edge and in the plasmonic band gap. We show three modes: one spaser mode in gap with quality factor as high as 248.54, one plasmon lasing mode at band edge which emit vertically from the grating surface, and the other plasmon lasing mode at band edge which is suppressed by the spaser mode. This method may find significant applications in…
The solution of a boundary-value problem formulated for a modified Kretschmann configuration shows that the phase speed of a surface-plasmon wave guided by the planar interface of a sufficiently thin metal film and a chiral sculptured thin film (STF) depends on the vapor incidence angle used while fabricating the chiral STF by physical vapor depoistion. Therefore, it may be possible to engineer the phase speed quite simply by selecting an appropriate value of the vapor deposition angle (in addition to the metal and the evaporant species).
The morphology of a columnar thin film (CTF) of silver renders it an effectively biaxially anisotropic continuum. CTFs of silver deposited on one-dimensional gratings of photoresist showed strong blazing action and asymmetrically coupled optical radiation to surface plasmon-polariton (SPP) waves propagating only along one direction supported by either the CTF/photoresist or the CTF/air interfaces. Homogenization of the CTFs using the Bruggeman formalism revealed them to display hyperbolic dispersion, and the dispersion of SPP waves was adequately described thereby.
An active control method of azo-polymer loaded surface plasmon-polaritons (SPPs) wave with tightly focused 532nm laser is proposed and demonstrated in this paper. Theoretical analysis and experimental results are consistent, which confirm the validity of this method. The optically active control method has the advantage of simple samples preparation, high spatial resolution and selectively control of the SPPs wave. This optical control of SPPs wave method has potential applications in integrated plasmonics.
When a sculptured thin film (STF), made of a metal and $\leq50$ nm thick, is used in lieu of a dense layer of metal in the Kretschmann configuration, experimental data for an STF comprising parallel tilted nanowires shows that a surface plasmon resonance (SPR) can still be excited. As the porosity of the chosen STF increases, experimental data and numerical simulations indicate the SPR dip with respect to the angle of incidence of the exciting plane wave widens and eventually disappears, leaving behind a a vestigial peak near the onset to the total-internal-reflection regime.
Low-dimensional plasmonic materials can function as high quality terahertz and infrared antennas at deep subwavelength scales. Despite these antennas' strong coupling to electromagnetic fields, there is a pressing need to further strengthen their absorption. We address this problem by fabricating thick films of aligned, uniformly sized carbon nanotubes and showing that their plasmon resonances are strong, narrow, and broadly tunable. With thicknesses ranging from 25 to 250 nm, our films exhibit peak attenuation reaching 70%, quality factors reaching 9, and electrostatically tunable peak freque…
The canonical problem of the propagation of surface-plasmon-polariton (SPP) waves localized to the planar interface of a metal and a sculptured nematic thin film (SNTF) that is periodically nonhomogeneous along the direction normal to the interface was formulated. Solution of the dispersion equation obtained thereby confirmed the possibility of exciting multiple SPP waves of the same frequency or color. However, these SPP waves differ in phase speed, field structure, and the e-folding distance along the direction of propagation.
The experimental demonstration and characterization is made of the plasmon-mediated resonant transmission through an embedded undulated continuous thin metal film under normal incidence. 1D undulations are shown to enable a spatially resolved polarisation filtering whereas 2D undulations lead to spatially resolved, polarization independent transmission. Whereas the needed submicron microstructure lends itself in principle to CD-like low-cost mass replication by means of injection moulding and embossing, the present paper demonstrates the expected transmission effects on experimental models bas…
A set of grating couplers that convert plane waves into odd pairs of plasmons supported by extremely thin layers of doped indium tin oxide is designed. The inverse design approach is implemented to improve the efficiency of ordinary periodical couplers significantly. The optimization code based on the gradient descent method and direct Maxwell solver is designed in Matlab. Three models with different optimization levels are compared and discussed. The results of calculations are prepared for subsequent experimental verification. Considered odd plasmonic pairs represent an example of high quali…
Plasmonics enables deep-subwavelength concentration of light and has become important for fundamental studies as well as real-life applications. Two major existing platforms of plasmonics are metallic nanoparticles and metallic films. Metallic nanoparticles allow efficient coupling to far field radiation, yet their synthesis typically leads to poor material quality. Metallic films offer substantially higher quality materials, but their coupling to radiation is typically jeopardized due to the large momentum mismatch with free space. Here, we propose and theoretically investigate optically thin…
Surface plasmon polaritons (SPPs) at the interface of a columnar thin film (CTF) and metal exist over a range of propagation directions relative to the morphology of the CTF which depends on the tilt of the columns in the CTF. The phase speed of the SPP wave varies mainly as a function of the tilt of the CTF columns. Both the confinement of the SPP wave to the interface and the decay of the SPP wave along the direction of propagation depend strongly on the direction of propagation relative to the morphologically significant plane of the CTF. The greater the columnar tilt in relation to the int…
Two devices for subwave length focusing of light are explored. The first one is a thin film of a well reflecting metal which the converging beam of surface plasmons with a wave number $h>>ω_0/c$ is excited on. The waist of this beam has a cross section that is much smaller than $λ_0^2$. The second device is a linear nanoantenna with a gap in the middle. A resonance plasmon is excited in the antenna. The field in the gap concentrates on the spot that is much smaller than $λ_0^2$. In both cases the effect of field enhancement in the spot of subwave length focusing is greatly decreased because of…
The purpose of this comment is first to correct a misapprehension of the role played by composite wave diffraction on surface-wave generation at subwavelength structures and second to point out that periodic Bloch structures are unnecessary for the efficient production of the surface plasmon polariton (SPP) guided mode either as traveling or standing waves. Guided surface waves originate from simple slit or groove edges illuminated under normal incidence, and one-dimensional (1-D) surface cavities from these standing waves are easily realized.
The observation of the electrically tunable and highly confined plasmons in graphene has stimulated the exploration of interesting properties of plasmons in other two dimensional materials. Recently, hyperbolic plasmon resonance modes are observed in exfoliated WTe2 films, a type-II Weyl semimetal with layered structure, providing a platform for the assembly of plasmons with hyperbolicity and exotic topological properties. However, the plasmon modes were observed in relatively thick and small-area films, which restrict the tunability and application for plasmons. Here, large-area (~ cm) WTe2 f…
Surface-plasmon-polariton~(SPP) wave propagation guided by a metal slab in a periodically nonhomogeneous sculptured nematic thin film~(SNTF) was studied theoretically. The morphologically significant planes of the SNTF on both sides of the metal slab could either be aligned or twisted with respect to each other. The canonical boundary-value problem was formulated, solved for SPP-wave propagation, and examined to determine the effect of slab thickness on the multiplicity and the spatial profiles of SPP waves. Decrease in slab thickness was found to result in more intense coupling of two metal/S…
We examine the coupling of electromagnetic waves incident normal to a thin silver film that forms an oscillatory grating embedded between two otherwise uniform, semi-infinite half spaces. Two grating structures are considered, in one of which the mid point of the Ag film remains fixed whereas the thickness varies sinusoidally, while in the other the mid point oscillates sinusoidally whereas the film thicknesses remains fixed. On reducing the light wavelength from the long wavelength limit, we encounter signatures in the transmission, T, and reflection, R, coefficients associated with: i) the s…
We study the energy and momentum of the surface plasmon-polariton (SPP) excited in a symmetric 3-layer "insulator-metal-insulator" structure, which is known to support the symmetric (S) mode with the negative group velocity as well as the antisymmetric (AS) mode with only positive energy flow. The electric and magnetic field vectors are calculated via both the phenomenological and the microscopic approach; the latter involves the hydrodynamic model accounting for the quantum statistical effects for the electron gas in metal. Explicit representation for the energy and momentum constituents in t…
We report on fabrication of spatially-coherent columnar plasmonic nanostructure superlattice-type thin films with high porosity and strong optical anisotropy using glancing angle deposition. Subsequent and repeated depositions of silicon and gold lead to nanometer-dimension subcolumns with controlled lengths. The superlattice-type columns resemble bamboo structures where smaller column sections of gold form junctions sandwiched between larger silicon column sections ("nano-bamboo"). We perform generalized spectroscopic ellipsometry measurements and finite element method computations to elucida…
We measure the statistical distribution of the local density of optical states (LDOS) on disordered semi-continuous metal films. We show that LDOS fluctuations exhibit a maximum in a regime where fractal clusters dominate the film surface. These large fluctuations are a signature of surface-plasmon localization on the nanometer scale.
A quantum mechanical approach and local response theory are applied to study plasmons propagating in nanometer-thin gold slabs sandwiched between different dielectrics. The metal slab supports two different kinds of modes, classified as long-range and short-range plasmons. Quantum spill-out is found to significantly increase the imaginary part of their mode indices, and, surprisingly, even for slabs wide enough to approach bulk the increase is 20%. This is explained in terms of enhanced plasmonic absorption, which mainly takes place at narrow peaks located near the slab surface.
A metallic film of arbitrary thickness is considered. We show that the problem of description of surface plasma oscillations (surface plasmons) with reflection boundary conditions allows analytic solution. Besides, this problem allows generalization for more general case of conducting matter (in particular, and for semiconductors).
In this paper, we utilize coupled mode theory (CMT) to model the coupling of surface plasmon polaritons (SPPs) between tri-layered corrugated thin films (CTF) structure coupler in the terahertz region. Employing the stimulated raman adiabatic passage (STIRAP) quantum control technique, we propose a novel directional coupler based on SPPs evolution in tri-layered CTF in some curved configuration. Our calculated results show that the SPPs can be completely transferred from the input to the output CTF waveguides, and even we consider SPPs propagation loss, the transfer rate is still above 70%. Th…
The solution of a boundary-value problem formulated for a modified Kretschmann configuration shows that a surface-plasmon wave can be excited at the planar interface of a sufficiently thin metal film and a nondissipative structurally chiral medium, provided the exciting plane wave is p-polarized. An estimate of the wavenumber of the surface-plasmon wave also emerges thereby.
We address the issue of the second-order coherence of single surface plasmons launched by a quantum source of light into extended gold films. The quantum source of light is made of a scanning fluorescent nanodiamond hosting five nitrogen-vacancy (NV) color centers. By using a specially designed microscopy that combines near-field optics with far-field leakage-radiation microscopy in the Fourier space and adapted spatial filtering, we find that the quantum statistics of the initial source of light is preserved after conversion to surface plasmons and propagation along the polycrystalline gold f…
Supplementing our STM and electron emission studies investigations, concluding in electron pairing in strong laser fields [1], further time-of-flight electron emission studies were carried out, changing the angle of polarization of the incident light, exciting surface plasmon oscillations. It has been found, that those parts of the electron spectrum which have been attributed to electron pairing have a significantly different angular dependence around 80 GW/cm2 where the pairing effect has been found than outside this region (e.g. 120 GW/cm2). These results have been interpreted as the appeara…
Dewetting of thin metal films is one of the most widespread method for functional plasmonic nanostructures fabrication. However, simple thermal-induced dewetting does not allow to control degree of nanostructures order without additional lithographic process steps. Here we propose a novel method for lithography-free and large-scale fabrication of plasmonic nanostructures via controllable femtosecond laser-induced dewetting. The method is based on femtosecond laser surface pattering of a thin film followed by a nanoscale hydrodynamical instability, which is found to be very controllable under s…
The influence of the film thickness and the substrate's refractive index on the surface mode at the superstrate is an important study step that may help clearing some of the misunderstandings surrounding their propagation mechanism. A single sub-wavelength slit perforating a thin metallic film is among the simplest nanostructure capable of launching Surface Plasmon Polaritons on its surrounding surface when excited by an incident field. Here, the impact of the substrate and the film thickness on surface waves is investigated. When the thickness of the film is comparable to its skin depth, SPP …
We report on the enhancement of surface plasmon resonances in a holey bidimensional grating of subwavelength size, drilled in a gold thin film coated by a graphene sheet. The enhancement originates from the coupling between charge carriers in graphene and gold surface plasmons. The main plasmon resonance peak is located around 1.5 microns. A lower constraint on the gold-induced doping concentration of graphene is specified and the interest of this architecture for molecular sensing is also highlighted.
The recoil optical force that acts on emitters near a surface or waveguide relies on near-field directionality and conservation of momentum. It features desirable properties uncommon in optical forces, such as the ability to produce it via wide-area illumination of vast numbers of particles without the need for focusing, or being dynamically switchable via the polarization of light. Unfortunately, these recoil forces are usually very weak and have not been experimentally observed in small dipolar particles. Some works theoretically demonstrate orders-of-magnitude enhancement of these forces vi…
Regular arrays of metal nanoparticles on metal films have tuneable optical resonances that can be applied for surface enhanced Raman scattering or biosensing. With the aim of developing more surface selective geometries we investigate regular gold nanoparticle arrays on 25nm thick gold films, which allow to excite asymmetric surface plasmon modes featuring a much better field confinement compared to the symmetric modes used in conventional surface plasmon resonance setups. By optical extinction spectroscopy we identify the plasmonic modes sustained by our structures. Furthermore, the role of t…
The propagation of surface plasmon polariton at an interface of metallic thin film and chiral sculptured thin film theoretically has been investigated using the transfer matrix method in the Kretschman configuration. The optical absorption of structure as a function of polar incident angle for linear polarization P and S has been calculated at different structural parameters. The results show that exist multiple plasmon peaks for P-polarization, while there are the weak plasmon peaks when incident of light is S- polarized plane wave.
We introduce the concept of optical control of the fluorescence yield of CdSe quantum dots through plasmon-induced structural changes in random semicontinuous nanostructured gold films. We demonstrate that the wavelength- and polarization dependent coupling between quantum dots and the semicontinuous films, and thus the fluorescent emission spectrum, can be controlled and significantly increased through the optical extinction of a selective band of eigenmodes in the films. This optical method of effecting controlled changes in the metal nanostructure allows for versatile functionality in a sin…
A hyperbolic plasmonic surface supports highly directional propagating polaritons with extremely large density of states. Such plasmon polaritons have been realized in artificially structured metasurfaces. However, the upper bound of the achievable plasmon wave vector is limited by the structure size, which calls for a natural hyperbolic surface without any structuring. Here, we experimentally demonstrate a natural hyperbolic plasmonic surface based on thin films of WTe2 in the light wavelength range of 16 to 23 microns by far infrared absorption spectroscopy. The topological transition from t…
It is shown that a smooth metal film (or a plasma layer) can be made transparent for an electromagnetic wave when two identical subwavelength diffraction gratings are placed on both sides of the film. The electromagnetic wave transmission through the metal film is caused by excitation of evanescent surface waves (plasmons) and their transformation into propagating waves at the gratings. A model which is developed analytically shows that the problem of the wave transmission is physically equivalent to the problem of excitation of two coupled resonators of evanescent waves which are formed at th…
High-quality materials are critical for advances in plasmonics, especially as researchers now investigate quantum effects at the limit of single surface plasmons or exploit ultraviolet- or CMOS-compatible metals such as aluminum or copper. Unfortunately, due to inexperience with deposition methods, many plasmonics researchers deposit metals under the wrong conditions, severely limiting performance unnecessarily. This is then compounded as others follow their published procedures. In this perspective, we describe simple rules collected from the surface-science literature that allow high-quality…
Via exploitation of surface plasmon polaritons (SPPs), columnar thin films (CTFs) are attractive potential platforms for optical sensing as their relative permittivity dyadic and porosity can be tailored to order. Nanoscale model parameters of a CTF were determined from its measured relative permittivity dyadic, after inverting the Bruggeman homogenization formalism. These model parameters were then used to determine the relative permittivity dyadic of a fluid-infiltrated CTF. Two boundary-value problems were next solved: the first relating to SPP-wave propagation guided by the planar interfac…
We have analyzed analytically the Faraday rotation of an electromagnetic wave for magnetoactive thin metallic film with a nanostructured surface profile. Periodical as well as random surface profiles were considered. The plasmon contribution to the Faraday angle was studied. For periodical grating case, we have shown that the maximum of rotation angle is achieved when surface plasmon wave number coincides with one of the wave numbers of the inverse lattice. Enhancement of the Faraday angle at plasmonic band edges is predicted. In the case of random surface profile, it is shown that the diffusi…
Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain mea…
We propose and analyze surface-plasmon-driven electron spin currents in a thin metallic film. The electron gas in the metal follows the transversally rotating electric fields of the surface plasmons (SPs), which leads to a static magnetization gradient. We consider herein SPs in a thin-film insulator-metal-insulator structure and solve the spin diffusion equation in the presence of a magnetization gradient. The results reveal that the SPs at the metal interfaces generate spin currents in the metallic film. For thinner film, the SPs become strongly hybridized, which increases the magnetization …
We have observed laser-like emission of surface plasmon polaritons (SPPs) decoupled to the glass prism in an attenuated total reflection setup. SPPs were excited by optically pumped molecules in a polymeric film deposited on the top of the silver film. Stimulated emission was characterized by a distinct threshold in the input-output dependence and narrowing of the emission spectrum. The observed stimulated emission and corresponding to it compensation of the metallic absorption loss by gain enables many applications of metamaterials and nanoplasmonic devices.
We report the excitation of a surface plasmon resonance (SPR) close to the orthogonal axis of a gold (Au) film on borosilicate glass. Direct spectroscopic measurement of SPR shifts using different liquids are made at ~5° incidence within a reflection spectrophotometer. Scattering of light that is able to penetrate across the film at the interfaces is the proposed mechanism by which coupling, and plasmon localization, is established.
We explored the effects of relative motion on the excitation of surface-plasmon-polariton (SPP) waves guided by the planar interface of a metal film and a dielectric slab, both materials being isotropic and homogeneous. Electromagnetic phasors in moving and non-moving reference frames were related directly using the corresponding Lorentz transformations. Our numerical studies revealed that, in the case of a uniformly moving dielectric slab, the angle of incidence for SPP-wave excitation is highly sensitive to (i) the ratio $β$ of the speed of motion to speed of light in free space and (ii) the…
The surface states of the 3D topological insulator (TI), Bi$_2$Se$_3$, are known to host two-dimensional Dirac plasmon polaritons (DPPs) in the terahertz spectral range. In TI thin films, the DPPs excited on the top and bottom surfaces couple, leading to an acoustic and an optical plasmon mode. Vertical coupling in these materials is therefore reasonable well-understood, but in-plane coupling among localized TI DPPs has yet to be investigated. In this paper, we demonstrate in-plane DPP coupling in TI stripe arrays and show that they exhibit dipole-dipole type coupling. The coupling becomes neg…
We theoretically investigated the magnetically-tunable cutoff of long-range surface plasmon polariton along thin metal film surrounded by a magneto-optic material on one side and by a nonmagnetic dielectric on the other side. The analytically derived cutoff condition predicts that a magnetic field bias can induce a novel degenerate cutoff-state near which the beyond-cutoff radiation in one side can be switched to that in the other side by a minor variation of the magnetic field from the bias. The magnetization bias needed for the degeneracy is in proportion to the metal film thickness and in i…
We numerically study the effect of the quantum spill-out (QSO) on the plasmon mode indices of an ultra-thin metallic slab, using the Fourier modal method (FMM). To improve the convergence of the FMM results, a novel nonlinear coordinate transformation is suggested and employed. Furthermore, we present a perturbative approach for incorporating the effects of QSO on the plasmon mode indices, which agrees very well with the full numerical results. The perturbative approach also provides additional physical insight, and is used to derive analytical expressions for the mode indices using a simple m…
Extending plasmonics into the ultraviolet range imposes the use of aluminum to achieve the best optical performance. However, water corrosion is a major limiting issue for UV aluminum plasmonics, as this phenomenon occurs significantly faster in presence of UV light, even at low laser powers of a few microwatts. Here we assess the performance of nanometer-thick layers of various metal oxides deposited by atomic layer deposition (ALD) and plasma-enhanced chemical vapor deposition (PECVD) on top of aluminum nanoapertures to protect the metal against UV photocorrosion. The combination of a 5 nm A…
