We address the issue of the second-order coherence of single surface plasmons launched by a quantum source of light into extended gold films. The quantum source of light is made of a scanning fluorescent nanodiamond hosting five nitrogen-vacancy (NV) color centers. By using a specially designed microscopy that combines near-field optics with far-field leakage-radiation microscopy in the Fourier space and adapted spatial filtering, we find that the quantum statistics of the initial source of light is preserved after conversion to surface plasmons and propagation along the polycrystalline gold film.
A plasmonic coupled-cavity system, which consists of a quarter-wave coupler cavity, a resonant Fabry-Perot detector nanocavity, and an off-resonant reflector cavity, is used to enhance the localization of surface plasmons in a plasmonic detector. The coupler cavity is designed based on transmission line theory and wavelength scaling rules in the optical regime, while the reflector cavity is derived from off-resonant resonator structures to attenuate transmission of plasmonic waves. We observed strong coupling of the cavities in simulation results, with an 86% improvement of surface plasmon loc…
In this work, we present a fully quantum theory of the plasmonic nanolaser, based on the maser model. Theory can be applied both to the microlasers with high Q-factor cavities and plasmonic nanolasers. We show that the latter is essentially a thresholdless device. We obtain the statistics of quanta, spectrum of the plasmonic radiation and the second-order coherence degree in the steady state. The limits of the model applicability are discussed in detail. All results are compared with the full numerical simulation.
The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with $1L-WS_2$ by transferring it onto a plasmonic nanoantenna array, a hybrid metasurface is realized impacting the polarization dependency of its SHG. Here, we investigate how plasmonic dipole resonances affect the process of SHG in plasmonic-TMD hybrid metasurfaces by nonlinear spectroscopy. We show, that the polarization dependency is affected by the lattice str…
We investigate the propagation of surface plasmons (SPPs) in a thin layer of copper surrounded by copper oxide Cu$_2$O. It is shown that particularly strong excitons in Cu$_2$O can have considerable impact on plasmon propagation, providing many opportunities for plasmon-exciton and plasmon-plasmon interactions. It is demonstrated that by the use of sufficiently thin metal layer, one can excite the so-called long range plasmons (LRSPPs) which can overcome the inherently high ohmic losses of Cu as compared to usual plasmonic metals such as silver. Analytical results are confirmed by numerical ca…
We present an optical investigation of surface plasmon polaritons propagating along nanoscale Au-wires, lithographically defined on GaAs substrates. A two-axis confocal microscope was used to perform spatially and polarization resolved measurements in order to confirm the guiding of surface plasmon polaritons over lengths ranging from $5-20 μm$ along nanowires with a lateral dimension of only $\approx 100 nm$. Finite difference time domain simulations are used to corroborate our experimental observations and highlight the potential to couple proximal quantum dot emitters to propagating plasmon…
Quantum photonics holds great promise for future technologies such as secure communication, quantum computation, quantum simulation, and quantum metrology. An outstanding challenge for quantum photonics is to develop scalable miniature circuits that integrate single-photon sources, linear optical components, and detectors on a chip. Plasmonic nanocircuits will play essential roles in such developments. Plasmonic components feature ultracompact geometries and can be controlled more flexibly and more energy-efficiently compared to conventional dielectric components due to strong field confinemen…
We demonstrate `deterministic' launching of propagative quantum surface-plasmon polaritons at freely chosen positions on gold plasmonic receptacles. This is achieved by using as plasmon launcher a near-field scanning optical source made of a diamond nanocrystal with two Nitrogen-Vacancy color-center occupancy. Our demonstration relies on leakage-radiation microscopy of a thin homogeneous gold film and on near-field optical microscopy of a nanostructured thick gold film. Our work paves the way to future fundamental studies and applications in quantum plasmonics that require an accurate position…
We study arrays of plasmonic nanoparticles combined with quantum emitters, quantum plasmonic lattices, as a platform for room temperature studies of quantum many-body physics. We outline a theory to describe surface plasmon polariton distributions when they are coupled to externally pumped molecules. The possibility of tailoring the dispersion in plasmonic lattices allows realization of a variety of distributions, including the Bose-Einstein distribution as in photon condensation. We show that the presence of losses can relax some of the standard dimensionality restrictions for condensation.
We discuss the possibility of realizing utlrabroadband omnidirectional absorbers and angularly selective coherent thermal emitters based on properly patterned plasmonic metastructures. Instead of relying on resonant concentration effects that inherently limit the bandwidth, we base our design on the combination of two inherently nonresonant effects: plasmonic Brewster funneling and adiabatic plasmonic focusing. With this approach, we demonstrate compact, broadband absorption and emission spanning terahertz, infrared and optical frequencies, ideal for various energy and defense applications.
Plasmonics has attracted much attention not only because it has useful properties such as strong field enhancement, but also because it reveals the quantum nature of matter. To handle quantum plasmonics effects, ab initio packages or empirical Feibelman d-parameters have been used to explore the quantum correction of plasmonic resonances. However, most of these methods are formulated within the quasi-static framework. The self-consistent hydrodynamics model offers a reliable approach to study quantum plasmonics because it can incorporate the quantum effect of the electron gas into classical el…
Graphene is a unique material to study fundamental limits of plasmonics. Apart from the ultimate single-layer thickness, its carrier concentration can be tuned by chemical doping or applying an electric field. In this manner the electrodynamic properties of graphene can be varied from highly conductive to dielectric. Graphene supports strongly confined, propagating surface plasmon-polaritons (SPPs) in a broad spectral range from terahertz to mid-infrared frequencies. It also possesses a strong magneto-optical response and thus provides complimentary architectures to conventional magneto-plasmo…
We report single plasmon generation with a self-assembled InAs/GaAs quantum dot embedded in a plasmonic microring resonator. The plasmonic cavity based on a GaAs microring is defined on an atomically-smooth silver surface. We fabricated this structure with the help of transfer printing, which enables the pick-and-place assembly of the complicated, heterogeneous three dimensional stack. We show that a high-order surface-plasmon-polariton transverse mode mediates efficient coupling between the InAs/GaAs quantum dots and the plasmonic cavity, paving the way for developing plasmonic quantum light …
We investigate an array of metal nanoparticles as a channel for nanophotonic quantum communication and the generation of quantum plasmonic interference. We consider the transfer of quantum states, including single-qubits as plasmonic wavepackets, and highlight the necessity of a quantum mechanical description by comparing the predictions of quantum theory with those of classical electromagnetic theory. The effects of loss in the metal are included, thus putting our investigation into a practical setting and enabling the quantification of the performance of realistic nanoparticle arrays as plas…
We demonstrate the generation of self-accelerating surface plasmon beams along arbitrary caustic curvatures. These plasmonic beams are excited by free-space beams through a two-dimensional binary plasmonic phase mask, which provides the missing momentum between the two beams in the direction of propagation, and sets the required phase for the plasmonic beam in the transverse direction. We examine the cases of paraxial and non-paraxial curvatures and show that this highly versatile scheme can be designed to produce arbitrary plasmonic self-accelerating beams. Several different plasmonic beams, …
A type of Tamm states inside metal-insulator-metal (MIM) waveguides is proposed. An impedance based transfer matrix method is adopted to study and optimize it. With the participation of the plasmonic Tamm states, fields could be enhanced twice: the ffirst is due to the coupling between a normal waveguide and a nanoscaled plasmonic waveguide and the second is due to the strong localization and field enhancement of Tamm states. As shown in our 2D coupling configuration, |E|^2 is enhanced up to 1050 times when 1550 nm light is coupled from an 300 nm Si slab waveguide into an 40 nm MIM waveguide.
Strong coupling between a single quantum emitter and an electromagnetic mode is one of the key effects in quantum optics. In the cavity QED approach to plasmonics, strongly coupled systems are usually understood as single-transition emitters resonantly coupled to a single radiative plasmonic mode. However, plasmonic cavities also support non-radiative (or "dark") modes, which offer much higher coupling strengths. On the other hand, realistic quantum emitters often support multiple electronic transitions of various symmetry, which could overlap with higher order plasmonic transitions -- in the …
The possibility of using weak optical signals to perform sensing of delicate samples constitutes one of the main goals of quantum photonic sensing. Furthermore, the nanoscale confinement of electromagnetic near fields in photonic platforms through surface plasmon polaritons has motivated the development of highly sensitive quantum plasmonic sensors. Despite the enormous potential of plasmonic platforms for sensing, this class of sensors is ultimately limited by the quantum statistical fluctuations of surface plasmons. Indeed, the fluctuations of the electromagnetic field severely limit the per…
In this work, a 2D magneto-plasmonic grating structure combining materials with ferromagnetic and plasmonic properties is demonstrated. NiFe composite ferromagnetic material, as an active medium with tunable physical properties, and Au metal, as a plasmonic excitation layer, were the materials of choice. Here, we have experimentally investigated the active control of the plasmonic characteristics in Au/NiFe bilayer by the action of an external magnetic field, as well as the switching effect of the system. The active plasmonic control, can be achieved by the magnetization switching of the ferro…
We demonstrate that plasmonic helical gratings consisting of metallic nanowires imprinted with helical grooves or ridges can be used efficiently to generate plasmonic vortices with radius much smaller than the operating wavelength. In our proposed approach, these helical surface gratings are designed so that plasmon modes with different azimuthal quantum numbers (topological charge) are phase-matched, thus allowing one to generate optical plasmonic vortices with arbitrary topological charge. The general principles for designing plasmonic helical gratings that facilitate efficient generation of…
We develop a semi-analytical method for analyzing surface plasmon interferometry using near-field scanning optical sources. We compare our approach to Young double hole interferometry experiments using scanning tunneling microscope (STM) discussed in the literature and realize experiments with an aperture near-field scanning optical microscope (NSOM) source positioned near a ring like aperture slit milled in a thick gold film. In both cases the agreement between experiments and model is very good. We emphasize the role of dipole orientations and discuss the role of magnetic versus electric dip…
Plasmonic gratings of different periodicities are fabricated on top of Silicon nanocrystals embedded in Silicon Dioxide. Purcell enhancements of up to 2 were observed, which matches the value from simulations. Plasmonic enhancements are observed for the first three orders of the plasmonic modes, with the peak enhancement wavelength varying with the periodicity. Biharmonic gratings are also fabricated to extract the enhanced emission from the first order plasmonic mode, resulting in enhancements with quality factors of up to 16.
We analytically and numerically investigate magneto-plasmons in metal films surrounded by a ferromagnetic dielectric. In such waveguide using a metal film with a thickness exceeding the Skin depth, an external magnetic field in the transverse direction can induce a significant spatial asymmetry of mode distribution. Superposition of the odd and the even asymmetric modes over a distance leads to a concentration of the energy on one interface which is switched to the other interface by the magnetic field reversal. The requested magnitude of magnetization is exponentially reduced with the increas…
We report that femtosecond surface plasmon polariton pulses can propagate along a metal-dielectric waveguide and that they can be modulated on the femtosecond timescale by direct ultrafast optical excitation of the metal, thereby offering unprecedented terahertz plasmonic bandwidth - a key missing component in the development of surface plasmons as information carriers for next generation nanophotonic devices.
The concept of cross density of states characterizes the intrinsic spatial coherence of complex photonic or plasmonic systems, independently on the illumination conditions. Using this tool and the associated intrinsic coherence length, we demonstrate unambiguously the spatial squeezing of eigenmodes on disordered fractal metallic films, thus clarifying a basic issue in plasmonics.
We analyze nonlinear effects in optically driven arrays of nonlinear metallic nanoparticles. We demonstrate that such plasmonic systems are characterized by a bistable response, and they can support the propagation of dissipative switching waves (or plasmonic kinks) connecting the states with different polarization. We study numerically the properties of such plasmonic kinks which are characterized by a subwavelength extent and a tunable velocity.
We present plasmonic Bragg reflectors for increasing the extraordinary optical transmission through periodic arrays of subwavelength apertures in a metal film. The increase in transmission arises by preventing loss at the edges of the array. The plasmonic Bragg reflectors have periodicity of half the usual array's periodicity. Nano-hole arrays flanked thus by reflectors exchibited double the transmission as compared to the arrays without reflectors. These structures may also be used to isolate devices in plasmonic integrated circuits.
Plasmonics can be used to improve absorption in optoelectronic devices and has been intensively studied for solar cells and photodetectors. Graphene has recently emerged as a powerful plasmonic material. It shows significantly less losses compared to traditional plasmonic materials such as gold and silver and its plasmons can be tuned by changing the Fermi energy with chemical or electrical doping. Here we propose the usage of graphene plasmonics for light trapping in optoelectronic devices and show that the excitation of localized plasmons in doped, nanostructured graphene can enhance optical…
We theoretically investigated the transmission properties of a single plasmon interacting with two-level quantum dots (QDs) and a V-type three-level QD, coupled to plasmonic waveguide, respectively. We investigated the transmission of a single plasmon by a system including a V-type three-level QD and compared it with that by a system including only two-level QDs.
Absorbing and emitting optical properties of a spherical plasmonic nanoantenna are described in terms of the size dependent resonance frequencies and damping rates of the multipolar surface plasmons (SP). We provide the plasmon size characteristics for gold and silver spherical particles up to the large size retardation regime where the plasmon radiative damping is significant. We underline the role of the radiation damping in comparison with the energy dissipation damping in formation of receiving and transmitting properties of a plasmonic particle. The size dependence of both: the multipolar…
Localized surface plasmon polaritons in conducting structures give rise to enhancements of electromagnetic local fields and extinction efficiencies. Resonant conducting structures are conventionally fabricated with a fixed geometry that determines their plasmonic response. Here, we challenge this conventional approach by demonstrating the photo-generation of plasmonic materials (THz plasmonic antennas) on a flat semiconductor layer by the structured optical illumination through a spatial light modulator. Free charge carriers are photo-excited only on selected areas, which enables the definitio…
Plasmonic fields are usually considered non-chiral because of the transverse magnetic polarization of surface plasmon modes. We however show here that an optical lattice created from the intersection of two coherent surface plasmons propagating on a smooth metal film can generate optical chirality in the interfering near field. We reveal in particular the emergence of plasmonic potentials relevant to the generation of near-field chiral forces. This draws promising perspectives for performing enantiomeric separation schemes within the near field.
The development of metamaterials, data processing circuits and sensors for the visible and UV parts of the spectrum is hampered by the lack of low-loss media supporting plasmonic excitations and drives the intense search for plasmonic materials beyond noble metals. By studying plasmonic nanostructures fabricated on the surface of topological insulator $\mbox{Bi}_{1.5}\mbox{Sb}_{0.5}\mbox{Te}_{1.8}\mbox{Se}_{1.2}$ we found that it is orders of magnitude better plasmonic material than gold and silver in the blue-UV range. Metamaterial fabricated from $\mbox{Bi}_{1.5}\mbox{Sb}_{0.5}\mbox{Te}_{1.8…
The field of plasmonics offers a route to control light fields with metallic nanostructures through the excitation of Surface Plasmon Polaritons (SPPs). These surface waves, bound to a metal dielectric interface, tightly confine electromagnetic energy. Active control over SPPs has potential for applications in sensing, photovoltaics, quantum communication, nano circuitry, metamaterials and super-resolution microscopy. We achieve here a new level of control of plasmonic fields using a digital spatial light modulator. Optimizing the plasmonic phases via feedback we focus SPPs at a freely pre-cho…
Plasmonic nanolithography is a nanofabrication technique which exploits surface plasmons to generate subdiffraction patterns. In this review, we highlight the key concepts in plasmonic nanolithography, review the pioneering papers and provide a classification that can be useful in determining the proper method and tool for subdiffraction patterning. Considering the ongoing developments in the field of plasmonics, lithography using surface plasmons is an extremely promising approach for development of high-throughput nanofabrication techniques.
Nanostructured metal surfaces comprised of periodically arranged spherical voids are grown by electrochemical deposition through a self-assembled template. Detailed measurements of the angle- and orientation-dependent reflectivity reveal the spectral dispersion, from which we identify the presence of both delocalized Bragg- and localized Mie-plasmons. These couple strongly producing bonding and anti-bonding mixed plasmons with anomalous dispersion properties. Appropriate plasmon engineering of the void morphology selects the plasmon spatial and spectral positions, allowing these plasmonic crys…
By viewing plasmon waves in metallic waveguides as propagating electric and magnetic dipoles we show that according to laws of quantum mechanics they will acquire additional phase when propagating through space with static magnetic field. The new effect is physically different from conventional magneto-plasmonic phenomena and is sufficiently strong to observe it under routinely accessible experimental conditions.
Low-profile patterned plasmonic surfaces are synergized with a broad class of silicon microstructures to greatly enhance near-field nanoscale imaging, sensing, and energy harvesting coupled with far-field free-space detection. This concept has a clear impact on several key areas of interest for the MEMS community, including but not limited to ultra-compact microsystems for sensitive detection of small number of target molecules, and surface devices for optical data storage, micro-imaging and displaying. In this paper, we review the current state-of-the-art in plasmonic theory as well as derive…
The use of nanoplasmonics to control light and heat close to the thermodynamic limit enables exciting opportunities in the field of plasmonic catalysis. The decay of plasmonic excitations creates highly nonequilibrium distributions of hot carriers that can initiate or catalyze reactions through both thermal and nonthermal pathways. In this Perspective, we present the current understanding in the field of plasmonic catalysis, capturing vibrant debates in the literature, and discuss future avenues of exploration to overcome critical bottlenecks. Our Perspective spans first-principles theory and …
Surface plasmon polaritons enable light concentration within subwavelength regions, opening thereby new avenues for miniaturizing the device and strengthening light-matter interactions. Here we realize effective electro-optic modulation in low-loss plasmonic waveguides with the aid of graphene, and the devices are fully integrated in the silicon-on-insulator platform. By advantageously exploiting low-loss plasmonic slot-waveguide modes, which weakly leak into a substrate while feature strong fields within the two-layer-graphene covered slots in metal, we successfully achieve a tunability of 0.…
An emitter in the vicinity of a metal nanostructure is quenched by its decay through non-radiative channels, leading to the belief in a zone of inactivity for emitters placed within $<$10nm of a plasmonic nanostructure. Here we demonstrate that in tightly-coupled plasmonic resonators forming nanocavities "quenching is quenched" due to plasmon mixing. Unlike isolated nanoparticles, plasmonic nanocavities show mode hybridization which massively enhances emitter excitation and decay via radiative channels. This creates ideal conditions for realizing single-molecule strong-coupling with plasmons, …
We demonstrate a plasmonic route to control the collective spontaneous emission of two-level quantum emitters. Superradiance and subradiance effects are observed over distances comparable to the operating wavelength inside plasmonic nanochannels. These plasmonic waveguides can provide an effective epsilon-near-zero operation in their cut-off frequency and Fabry-Perot resonances at higher frequencies. The related plasmonic resonant modes are found to efficiently enhance the constructive (superradiance) or destructive (subradiance) interference between different quantum emitters located inside t…
A plasmonic nanoantenna probed by a plane-polarized optical field in a medium with no gain materials can show zero absorption or even amplification, while exhibiting maximal polarizability. This occurs through coupling to an adjacent nanoantenna in a specially designed metamolecule, which is pumped by an orthogonal optical field with phase shift. The introduced scheme is a classical counterpart of an effect known in quantum optics as enhancement of the index of refraction (EIR). In contrary to electromagnetically induced transparency (EIT), where the medium is rendered highly dispersive at the…
We demonstrate that ultrafast carrier excitation can drastically affect electronic structures and induce brief surface plasmonic response in non-plasmonic metals, potentially creating a plasmonic switch. Using first-principles molecular dynamics and Kubo-Greenwood formalism for laser-excited tungsten we show that carrier heating mobilizes d electrons into collective inter and intraband transitions leading to a sign flip in the imaginary optical conductivity, activating plasmonic properties for the initial non-plasmonic phase. The drive for the optical evolution can be visualized as an increasi…
We evaluate optical forces and torques induced by a surface plasmon to a sphere of arbitrary size, i.e. beyond the point-like dipolar limit. Through a multipolar decomposition of the plasmonic field, we demonstrate that the induced torque is purely transverse to the plasmon propagation direction. Our approach removes the inherent ambiguities of the dipolar regime with respect to rotations and emphasizes the crucial role played by dissipation in the onset of the plasmonic torque. We also give realistic estimates of such plasmon-induced spinning of gold spheres immersed in water or air.
Hotspots of surface-enhanced resonance Raman scattering (SERRS) are localized within 1 nm at gaps or crevices of plasmonic nanoparticle (NP) dimers. We demonstrate SERRS hotspots with volumes that are extended in one dimension tens of thousand times compared to standard zero-dimensional hotspots using gaps or crevices of plasmonic nanowire (NW) dimers.
A composite plasmonic slab based on double-layer metallic gratings and a dielectric film is experimentally and numerically demonstrated in terahertz (THz) regions, which can support two resonance modes and then form a broad bandgap (40%). As compared to the double-layer metal grating, the dielectric film in composite THz slabs significantly enhances the transmission of the transverse magnetic (TM) mode. Electric field vector proved that the low-frequency resonance mode originates from the symmetric plasmonic mode and the high-frequency resonance mode is induced by the hybrid mode of plasmonic …
Plasmonic nanoparticles (NPs) hold tremendous promise for catalyzing light-driven chemical reactions. The conventionally assumed detrimental absorption loss from plasmon damping can now be harvested to drive chemical transformations of the NP adsorbent, through the excitation and transfer of energetic "hot" carriers. The rate and selectivity of plasmonic photocatalysis are dependent on the characteristics of the incident light. By engineering the strength and wavelength of the light harvesting of a NP, it is possible to achieve more efficient and predictive photocatalysts. We report a plasmoni…
We introduce the concept of polychromatic plasmonics and suggest an broadband plasmonic lens for nanofocusing of surface plasmon polaritons. The lens employs a parabolically modulated metal-dielectric-metal structure. This plasmonic lens has a bandwidth of more than an optical octave thus opening new opportunities for broadband plasmonic applications.
We demonstrate an efficient double-layer light absorber by exciting plasmonic phase resonances. We show that the addition of grooves can cause mode splitting of the plasmonic waveguide cavity modes and all the new resonant modes exhibit large absorptivity greater than 90%. Some of the generated absorption peaks have wide-angle characteristics. Furthermore, we find that the proposed structure is fairly insensitive to the alignment error between different layers. The proposed plasmonic nano-structure designs may have exciting potential applications in thin film solar cells, thermal emitters, nov…
We demonstrate thermally tunable superconductor hole array with active control over their resonant transmission induced by surface plasmon polaritons . The array was lithographically fabricated on high temperature YBCO superconductor and characterized by terahertz-time domain spectroscopy. We observe a clear transition from the virtual excitation of the surface plasmon mode to the real surface plasmon mode. The highly tunable superconducting plasmonic hole arrays may have promising applications in the design of low-loss, large dynamic range amplitude modulation, and surface plasmon based terah…
A novel plasmonic THz fiber featuring two metallic wires in a porous dielectric cladding is studied for resonant sensing applications. In our design, introduction of even lossless analytes into the fiber core leads to significant changes in the modal losses, which is used as a transduction mechanism.
