It has been shown that there are not only transverse but also longitudinal couplings between microwave fields and a superconducting qubit with broken inversion symmetry of the potential energy. Using multiphoton processes induced by longitudinal coupling fields and frequency matching conditions, we design a universal algorithm to produce arbitrary superpositions of two-mode photon states of microwave fields in two separated transmission line resonators, which are coupled to a superconducting qubit. Based on our algorithm, we analyze the generation of evenly-populated states and NOON states. Compared to other proposals with only single-photon process, we provide an efficient way to produce entangled microwave states when the interactions between superconducting qubits and microwave fields are in the ultrastrong regime.
Multiphoton entanglement plays a critical role in quantum information processing, and greatly improves our fundamental understanding of the quantum world. Despite tremendous efforts in either bulk media or fiber-based devices, nonlinear interactions in integrated circuits show great promise as an excellent platform for photon pair generation with its high brightness, stability and scalability \cite{Caspani2017}. Here, we demonstrate the generation of bi- and multiphoton polarization entangled qubits in a single silicon nanowire waveguide, and these qubits directly compatible with the dense wav…
Bound entangled states are the exotic objects in the entangled world. They require entanglement to create them, but once they are formed, it is not possible to locally distill any free entanglement from them. It is only until recently that a few bound entangled states were realized in the laboratory. Motivated by these experiments, we propose schemes for creating various classes of bound entangled states with photon polarization. These include Acin-Bruss-Lewenstein-Sanpara states, Dur's states, Lee-Lee-Kim bound entangled states, and an unextendible-product-basis bound entangled state.
We propose a fruitful scheme for exploring multiphoton entangled states based on linear optics and weak nonlinearities. Compared with the previous schemes the present method is more feasible because there are only small phase shifts instead of a series of related functions of photon numbers in the process of interaction with Kerr nonlinearities. In the absence of decoherence we analyze the error probabilities induced by homodyne measurement and show that the maximal error probability can be made small enough even when the number of photons is large. This implies that the present scheme is quit…
We theoretically investigate the spectral entanglement of a multiphoton source generated from the cascade emissions in the cascaded cold atomic ensembles.\ This photon source is highly directional, guaranteed under the four-wave mixing condition, and is also highly frequency-correlated due to finite driving pulse durations and superradiant decay constants.\ We utilize Schmidt decomposition to study the bipartite entanglement of the biphoton states projected from the multiphoton ones.\ This entropy of entanglement can be manipulated by controlling the driving parameters and superradiant decay r…
We study multiphoton blockade and photon-induced tunneling effects in the two-photon Jaynes-Cummings model, where a single-mode cavity field and a two-level atom are coupled via a two-photon interaction. We consider both the cavity-field-driving and atom-driving cases, and find that single-photon blockade and photon-induced tunneling effects can be observed when the cavity mode is driven, while the two-photon blockade effect appears when the atom is driven. For the atom-driving case (the two-photon transition process), we present a criterion of the correlation functions for the multiphoton blo…
When an atom is strongly coupled to a cavity, the two systems can exchange a single photon through a coherent Rabi oscillation. This process enables precise quantum-state engineering and manipulation of atoms and photons in a cavity, which play a central role in quantum information and measurement. Recently, a new regime of cavity QED has been reached experimentally where the strength of the interaction between light and artificial atoms (qubits) becomes comparable to the atomic transition frequency or the resonance frequency of the cavity mode. Here we show that this regime can strongly modif…
We present a study of manipulating the multiphoton blockade phenomenon in a single mode cavity with two ladder-type three-level atoms. Combining the cavity QED with electromagnetically induced transparency technique, we show that it is possible to actively manipulate the photon blockade when two atoms are in phase radiations. As a result, the two-photon blockade can be changed to three-photon blockade by changing the control field Rabi frequency. In the case of out-phase radiations, we show that the three-photon blockade can be improved with enhanced mean photon number. In addition, we show th…
Multiphoton entanglement, as a quantum resource, plays an essential role in linear optical quantum information processing. Krenn et al. (Phys. Rev. Lett. 118, 080401 2017) proposed an innovative scheme that generating entanglement by path identity, in which two-photon interference (called Hong-Ou-Mandel effect) is not necessary in experiment. However, the experiments in this scheme have strict requirements in stability and scalability, which is difficult to be realized in bulk optics. To solve this problem, in this paper we first propose an on-chip scheme to generate multi-photon polarization …
Engineering multiphoton states is an outstanding challenge with applications in multiple fields, such as quan- tum metrology, quantum lithography or even biological systems. State-of-the-art methods to obtain them rely on post-selection, multi-level systems or Rydberg atomic ensembles. Recently, it was shown that a strongly driven two-level system interacting with a detuned cavity mode can be engineered to continuously emit n-photon states. In the present work, we show that spectral filtering of its emission relaxes considerably the requirements on the system parameters even to the more access…
Multiphoton path entanglement is created without applying post-selection, by manipulating the state of stimulated parametric down-conversion. A specific measurement on one of the two output spatial modes leads to the non-local bunching of the photons of the other mode, forming the desired multiphoton path entangled state. We present experimental results for the case of a heralded two-photon path entangled state and show how to extend this scheme to higher photon numbers.
Manipulating photons is an essential technique in quantum communication and computation. Combining the Raman electromagnetically induced transparency technology, we show that the photon blockade behavior can be actively controlled by using an external control field in a two atoms cavity-QED system. As a result, a versatile photon gateway can be achieved in this system, which changes the cavity photons from classical to quantum property and allows one photon, two photon and classical field leaking from the cavity. The proposal presented here has many potential applications for quantum informati…
Within the matrix product state framework, we study the non-Markovian feedback dynamics of a two-level system interacting with the electromagnetic field inside a semi-infinite waveguide where the excitation of an atom-photon bound state is possible. Taking the steady-state excitation of the emitter as a figure of merit, we compare the trapped excitation for an initially excited quantum emitter and an emitter prepared via quantized pulses containing up to four photons. In the latter case, we find that for large feedback delay times, multi-photon pulses can yield a significantly higher steady-st…
We develop a theory for the interaction of multi-level atoms with multi-mode cavities yielding cavity-enhanced multi-photon resonances. The locations of the resonances are predicted from the use of effective two- and three-level Hamiltonians. As an application we show that quantum gates can be realised when photonic qubits are encoded on the cavity modes in arrangements where ancilla atoms transit the cavity. The fidelity of operations is increased by conditional measurements on the atom and by the use of a selected, dual-rail, Hilbert space. A universal set of gates is proposed, including the…
A scheme is discussed for measuring Nth-order coherences of two orthogonally polarized light fields in a single spatial mode at very limited experimental cost. To implement the scheme, the only measurements needed are the Nth-order intensity moments after the light beam has passed through two quarter-wave plates, one half-wave plate, and a polarizing beam splitter for specific settings of the wave plates. It is shown that this method can be applied for arbitrarily large N. A set of explicit values is given for the settings of the wave plates, constituting an optimal measurement of the Nth-orde…
We present the proposition of an experiment in which the multiphoton quantum superposition consisting of N= 10^5 particles generated by a quantum-injected optical parametric amplifier (QI-OPA), seeded by a single-photon belonging to an EPR entangled pair, is made to interact with a Mirror-BEC shaped as a Bragg interference structure. The overall process will realize a Macroscopic Quantum Superposition (MQS) involving a microscopic single-photon state of polarization entangled with the coherent macroscopic transfer of momentum to the BEC structure, acting in space-like separated distant places.
Unwanted multiphoton emission commonly reduces the degree of entanglement of photons generated by non-classical light sources and, in turn, hampers their exploitation in quantum information science and technology. Quantum emitters have the potential to overcome this hurdle but, so far, the effect of multiphoton emission on the quality of entanglement has never been addressed in detail. Here, we tackle this challenge using photon pairs from a resonantly-driven quantum dot and comparing quantum state tomography and second-order coherence measurements as a function of the excitation power. We obs…
Photon entanglement is an essential ingredient for linear optics quantum computing schemes, quantum cryptographic protocols and fundamental tests of quantum mechanics. Here we describe a setup that allows for the generation of polarisation-entangled N-photon states on demand. The photons are obtained by mapping the entangled state of N atoms, each of them trapped inside an optical cavity, onto the free radiation field. The required initial state can be prepared by performing postselective measurements on the collective emission from the cavities through a multiport beamsplitter.
We have examined both single and entangled two-mode multiphoton coherent states and shown how the `Janus-faced' properties between two partner states are mirrored in appropriate tomograms. Entropic squeezing, quadrature squeezing and higher-order squeezing properties for a wide range of nonclassical states are estimated directly from tomograms. We have demonstrated how squeezing properties of two-mode entangled states produced at the output port of a quantum beamsplitter are sensitive to the relative phase between the reflected and transmitted fields. This feature allows for the possibility of…
The generation of quantum entangled states of many particles is a central goal of quantum information science. Characterizing such states is a complex task that demands exponentially large resources as particles are being added. Previously, we demonstrated a resource efficient source that can generate, in principal, entanglement between any number of photons. This source recursively fuse photon pairs generated by a pulsed laser into a multiphoton entangled state. In the current work, we perform quantum state tomography on the photon pair source and quantum process tomography on the fusion oper…
We show that it is possible to add or subtract many photons from a cavity field by interacting it resonantly with a two-level atom. The atom, after entangling with the field inside the cavity and exiting it, may be measured in one of the Schmidt states, producing a multiphoton process (in the sense that can add or annihilate more photons than a single transition allows), i.e., adding or subtracting several photons from the cavity field.
Encoding quantum states in complex multiphoton fields can overcome loss during signal transmission in a quantum network. Transmitting quantum information encoded in this way requires that locally stored states can be converted to propagating fields. Here we experimentally show the controlled conversion of multiphoton quantum states, like "Schrödinger cat" states, from a microwave cavity quantum memory into propagating modes. By parametric conversion using the nonlinearity of a single Josephson junction, we can release the cavity state in ~500 ns, about 3 orders of magnitude faster than its int…
We address binary and quaternary communication channels based on correlated multiphoton two-mode states of radiation in the presence of losses. The protocol are based on photon number correlations and realized upon choosing a shared set of thresholds to convert the outcome of a joint photon number measurement into a symbol from a discrete alphabet. In particular, we focus on channels build using feasible photon-number entangled states (PNES) as two-mode coherently-correlated (TMC) or twin-beam (TWB) states and compare their performances with that of channels built using feasible classically co…
We extend the analysis of photon coincidence spectroscopy beyond bichromatic excitation and two-photon coincidence detection to include multichromatic excitation and multiphoton coincidence detection. Trichromatic excitation and three-photon coincidence spectroscopy are studied in detail, and we identify an observable signature of a triple resonance in an atom-cavity system.
The multiphoton Jaynes-Cummings model is investigated and applications in quantum information science are explored. Considering the strong atom-field coupling regime and an $N$-photon interaction, a nonlinear driving field can perform an arbitrary rotation in the Fock space of the cavity mode involving the vacuum and an $M$-Fock state, with $M<N$. Besides, driving the cavity mode with a linear coherent field (superposition of many Fock states), only the cavity states within the Fock subspace {$|0\rangle,|1\rangle,..., |N-1\rangle$} can be populated, i.e., we show how to implement a Fock state …
We present a scheme, based only on linear optics and standard photon detection, that allows to generate heralded multiphoton entangled states of arbitrary photon number from spontaneous parametric downconversion (PDC) in the weak interaction regime. The scheme also works in the strong interaction regime, i.e., for the production of large photon numbers, when photon-number resolving detectors with nearly perfect quantum efficiency are used. In addition, the same setup can be used for quantum metrology as multiphoton interferometer with sensitivity at the Heisenberg limit.
The thesis is divided into three parts. In the first part a new theoretical analysis of interferometric experiments by Alley-Shih, Ou-Mandel and the entanglement swapping experiment is performed. It is shown that the double- and single-photon distinguishability is not necessary for the experiments to be genuine tests against local realism. In the second part, basing on simple geometrical properties of Hilbert space, new, stronger Bell inequalities for M qubits in a maximally entangled state are derived. Application of the same method to two maximally entangled qubits yields an inequality for a…
We calculate the cavity-field distribution in the Wigner representation for the two-photon resonance of the weakly driven Jaynes-Cummings (JC) oscillator in its strong-coupling limit. Using an effective four-level system, we analytically demonstrate the presence of steady-state and transient bimodality which breaks azimuthal symmetry in phase space. The two steady-state peaks are located at opposite positions and do not correspond to the two-photon amplitude of the driven transition. The developing bimodality is portrayed in parallel with the evolution of the intensity correlation function for…
We investigate the multiphoton quantum dynamics of a leaking single-mode quantized cavity field coupled with a resonantly driven two-level system possessing permanent dipoles. The frequencies of the interacting subsystems are being considered very different, e.g., microwave ranges for the cavity and optical domains for the frequency of the two-level emitter, respectively. In this way, the emitter couples to the resonator mode via its diagonal dipole moments only. Furthermore, the generalized Rabi frequency resulting form the external coherent driving of the two-level subsystem is assumed as we…
We propose to control spin-mixing dynamics in a gas of spinor atoms, via the combination of two off-resonant Raman transition pathways, enabled by a common cavity mode and a bichromatic pump laser. The mixing rate, which is proportional to the synthesized spin-exchange interaction strength, and the effective atomic quadratic Zeeman shift (QZS), can both be tuned by changing the pump laser parameters. Quench and driving dynamics of the atomic collective spin are shown to be controllable on a faster time scale than in existing experiments based on inherent spin-exchange collision interactions. T…
We study the sensitive detection of a weak static magnetic field via Faraday rotation induced by an ensemble of spins in a bimodal degenerate microwave cavity. We determine the limit of the resolution for the sensitivity of the magnetometry achieved using either single-photon or multiphoton inputs. For the case of a microwave cavity containing an ensemble of Nitrogen-vacancy defects in diamond, we obtain a magnetometry sensitivity exceeding $0.5~\text{\nano\tesla}/\sqrt{\text{\hertz}}$, utilizing a single photon probe field, while for a multiphoton input we achieve a sensitivity about $1 \text…
Multiphoton entanglement is an important resource for linear optics quantum computing. Here we show that a wide range of highly entangled multiphoton states, including W-states, can be prepared by interfering single photons inside a Bell multiport beam splitter and using postselection. A successful state preparation is indicated by the collection of one photon per output port. An advantage of the Bell multiport beam splitter is that it redirects the photons without changing their inner degrees of freedom. The described setup can therefore be used to generate polarisation, time-bin and frequenc…
Photon coincidence spectroscopy relies on detecting multiphoton emissions from the combined atom-cavity system in atomic beam cavity quantum electrodynamics experiments. These multiphoton emissions from the cavity are nearly simultaneous approximately on the cavity lifetime scale. We determine the optimal time for the detection window of photon pairs in two-photon coincidence spectroscopy. If the window time is too short, some photon pairs will not be detected; if the window time is too long, too many nearly coincident independent single photons will be falsely interpreted as being a photon pa…
Dynamical decoupling of a quantum dot spin in a micropillar cavity for spin-multiphoton entanglement
Université Paris-Saclay（巴黎萨克雷大学）；Centre de Nanosciences et de Nanotechnologies, CNRS（国家科学研究中心纳米科学和纳米技术研究中心）；Quandela SAS（Quandela公司）；Johns Hopkins Applied Physics Laboratory（约翰斯·霍普金斯大学应用物理实验室）；University of Delaware（特拉华大学）
We propose novel types of parametric oscillators generating both three-photon and four-photon bright light which are accessible for an experiment. The devices are based on the cascaded down-conversion processes and consist of second-order media inserted in two-resonant mode cavity. Discussion of dissipation and quantum features of the system are performed by the quantum-jump simulation method and concerns to the Wigner functions. The phase-space multistabilities and critical threshold behavior of three- and four-photon subharmonics are obtained.
We describe the emission, detection and structure of multiphoton states of light. We include the effect of frequency filtering, which describes, at a fundamental level, physical detection of a quantum emitter. The case of the spontaneous emission of Fock states is treated fully and analytically. We stress this picture by contrasting it to the numerical simulation of two-photon bundles emitted from a two-level system in a cavity. We show that dynamical factors exist that allow for a more robust multiphoton emission than spontaneous emission. We also describe how this relates to thermal light.
We present a scheme to generate maximally entangled states of two three-level atoms with a nonresonant cavity by cavity-assisted collisions. Since the cavity field is only virtually excited no quantum information will be transferred from the atoms to the cavity.
Based on a multimode multilevel Jaynes-Cummings model and multiphoton resonance theory, a set of universal two- and three-qubit gates, namely the iSWAP and the Fredkin gates, has been realized where dual-rail qubits are encoded in cavities. In this way the information has been stored in cavities and the off-resonant atomic levels have been eliminated by the semi-classical theory of an effective two-level Hamiltonian. A further semi-classical model, namely the spin-$J$ model, has been introduced so that a complete population inversion for levels of interest has been achieved and periodic multil…
In this paper, we present a scheme to generate an entangled coherent state by considering a three-level Λ- type atom interacting with a two-mode cavity driven by classical fields. The two-mode entangled coherent state can be obtained under large detuning conditions. Considering the cavity decay, an analytical solution is deduced.
WaveguideQEDoffers the possibility of generating strong coherent atomic interactions either through appropriate atomic configurations in the dissipative regime or in the bandgap regime. In this work, we show how to harness these interactions in order to herald the generation of highly entangled atomic states, which afterwards can be mapped to generate single mode multi-photonic states with high fidelities.Weintroduce two protocols for the preparation of the atomic states, we discuss their performance and compare them to previous proposals. In particular, we show that one of them reaches high p…
We propose a scheme for implementing a multipartite quantum filter that uses entangled photons as a resource. It is shown that the success probability for the 2-photon parity filter can be as high as 1/2, which is the highest that has so far been predicted without the help of universal two-qubit quantum gates. Furthermore, the required number of ancilla photons is the least of all current parity filter proposals. Remarkably, the quantum filter operates with probability 1/2 even in the N-photon case, irregardless of the number of photons in the input state.
The dynamics of an entangled atomic system in a partial interaction with entangled cavity fields, characterizing an entanglement swapping, have been studied through the use of Von Neuman entropy. We consider the interaction via two-photon process given by a full microscopical Hamiltonian approach. The explicit expression of the entropy is obtained, wherewith we estimated the largest period. The numerical simulation of the entropy of the entangled atomic and cavity systems shows that its time evolution presents multi-periodicity. The effects of detuning parameter on the period and the amplitude…
A protocol is proposed to generate atomic entangled states in a cavity QED system. It utilizes Raman transitions or stimulated Raman adiabatic passages between two systems to entangle the ground states of two three-state $Λ$-type atoms trapped in a single mode cavity. It does not need the measurements on cavity field nor atomic detection and can be implemented in a deterministic fashion. Since the present protocol is insensitive to both cavity decay and atomic spontaneous emission, the produced entangled states may have some interesting applications in quantum information processing.
We present a scheme to generate a maximally entangled state of two three-level atoms in a cavity. The success or failure of the generation of the desired entangled state can be determined by detecting the polarization of the photon leaking out of the cavity. With the use of an automatic feedback, the success probability of the scheme can be made to approach unity.
