Multiphoton path entanglement is created without applying post-selection, by manipulating the state of stimulated parametric down-conversion. A specific measurement on one of the two output spatial modes leads to the non-local bunching of the photons of the other mode, forming the desired multiphoton path entangled state. We present experimental results for the case of a heralded two-photon path entangled state and show how to extend this scheme to higher photon numbers.
Loss-induced anomalous generalized bunching in multiphoton interference
Graduate School of Engineering Science, The University of Osaka（大阪大学工程科学研究科）；Center for Quantum Information and Quantum Biology, The University of Osaka（大阪大学量子信息与量子生物学中心）
In quantum mechanics, photons are bosons -- there is no restriction on the number of them that occupy the same quantum state, so many of them can bunch together, and this is well known as photon bunching effect. However, photon bunching and multiphoton interference of bunched photons have never been directly observed from a broadband thermal chaotic light source. Nevertheless, it has been known that the interference intensity of a number N of bunched photons oscillates with a wavelength of N times shorter than the wavelength of the constituent single photons, which should be observable in Four…
We describe and examine entanglement between different degrees of freedom in multiphoton states based on the permutation properties. From the state description, the entanglement comes from the permutation asymmetry. According to the different permutation properties, the multiphoton states can be divided into several parts. It will help to deal with the multiphoton interference, which can be used as the measurement of the entanglement.
Dissipative entanglement generation protocols embrace environmental interactions in order to generate long-lived entangled states. In this letter, we report on the anti-bunching dynamics for a pair of actively driven quantum emitters coupled to a shared dissipative plasmonic reservoir. We find that anti-bunching is a universal signature for entangled states generated by dissipative means and examine its use as an entanglement diagnostic. We discuss the experimental validation of plasmonically mediated entanglement generation by Hanbury Brown-Twiss interferometry with picosecond timing resoluti…
Multiphoton entanglement is an important resource for linear optics quantum computing. Here we show that a wide range of highly entangled multiphoton states, including W-states, can be prepared by interfering single photons inside a Bell multiport beam splitter and using postselection. A successful state preparation is indicated by the collection of one photon per output port. An advantage of the Bell multiport beam splitter is that it redirects the photons without changing their inner degrees of freedom. The described setup can therefore be used to generate polarisation, time-bin and frequenc…
Density matrices of pure multiphoton Fock polarization states and of arising from them reduced density matrices of mixed states are expressed in similar ways in terms of matrices of correlators defined as averaged products of equal numbers of creation and annihilation operators. Degree of entanglement of considered states is evaluated for various combinations of parameters of states and character of their reduction.
In this paper we study the evolution of the two two-level atoms interacting with a single-mode quantized radiation field, namely, two-atom multiphoton Jaynes-Cummings model when the radiation field and atoms are initially prepared in the superpostion of displaced number states and excited atomic states, respectively. For this system we investigate the atomic inversion, Wigner function, phase distribution and entanglement.
We present a scheme, based only on linear optics and standard photon detection, that allows to generate heralded multiphoton entangled states of arbitrary photon number from spontaneous parametric downconversion (PDC) in the weak interaction regime. The scheme also works in the strong interaction regime, i.e., for the production of large photon numbers, when photon-number resolving detectors with nearly perfect quantum efficiency are used. In addition, the same setup can be used for quantum metrology as multiphoton interferometer with sensitivity at the Heisenberg limit.
We theoretically investigate the spectral entanglement of a multiphoton source generated from the cascade emissions in the cascaded cold atomic ensembles.\ This photon source is highly directional, guaranteed under the four-wave mixing condition, and is also highly frequency-correlated due to finite driving pulse durations and superradiant decay constants.\ We utilize Schmidt decomposition to study the bipartite entanglement of the biphoton states projected from the multiphoton ones.\ This entropy of entanglement can be manipulated by controlling the driving parameters and superradiant decay r…
Two-photon anti-bunching at a beamsplitter is only possible if the photons are entangled in a specific state, anti-symmetric in the spatial modes. Thus, observation of anti-bunching is an indication of entanglement in a degree of freedom which might not be easily accessible in an experiment. We experimentally demonstrate this concept in the case of the interference of two frequency entangled photons with continuous frequency detunings. The principle of anti-symmetrisation of the spatial part of a wavefunction and subsequent detection of hidden entanglement via anti-bunching at a beamsplitter m…
Protocols for probabilistic entanglement-assisted quantum teleportation and for entanglement swapping of material qubits are presented. They are based on a protocol for postselective Bell-state projection which is capable of projecting two material qubits onto a Bell state with the help of ancillary coherent multiphoton states and postselection by balanced homodyne photodetection. Provided this photonic postselection is successful we explore the theoretical possibilities of realizing unit fidelity quantum teleportation and entanglement swapping with $25\%$ success probability. This photon-assi…
We present an experimental demonstration of a modified version of the entanglement-assisted "Guess my Number" protocol for the reduction of communication complexity among three separated parties. The results of experimental measurements imply that the separated parties can compute a function of distributed inputs by exchanging less classical information than by using any classical strategy. And the results also demonstrate the advantages of entanglement-enhanced communication, which is very close to quantum communication. The advantages are based on the properties of Greenberger-Horne-Zeilinge…
It was shown that using multiphoton qubits, a nearly deterministic Bell-state measurement can be performed with linear optics and on-off photodetectors [Phys. Rev. Lett. 114, 113603 (2015)]. However, multiphoton qubits are generally more fragile than single-photon qubits under a lossy environment. In this paper, we propose and analyze a scheme to teleport multiphoton-qubit information using hybrid entanglement with a loss-tolerant carrier qubit. We consider three candidates for the carrier qubit: a coherent-state qubit, a single-photon polarization qubit, and a vacuum-and-single-photon qubit. …
It was suggested that two entangled fermions can behave like a single boson and that the bosonic quality is proportional to the degree of entanglement between the two particles. The relation between bosonic quality and entanglement is quite natural if one takes into account the fact that entanglement appears in bound states of interacting systems. However, entanglement can still be present in spatially separated subsystems that do not interact anymore. These systems are often a subject of studies on quantum nonlocality and foundations of quantum physics. Here, we ask whether an entangled spati…
Photon entanglement is an essential ingredient for linear optics quantum computing schemes, quantum cryptographic protocols and fundamental tests of quantum mechanics. Here we describe a setup that allows for the generation of polarisation-entangled N-photon states on demand. The photons are obtained by mapping the entangled state of N atoms, each of them trapped inside an optical cavity, onto the free radiation field. The required initial state can be prepared by performing postselective measurements on the collective emission from the cavities through a multiport beamsplitter.
We have developed a theory for accessing quantum coherences in mutually unbiased bases associated with generalized Pauli operators in multiphoton multimode linear optics networks (LONs). We show a way to construct complementary Pauli measurements in multiphoton LONs and establish a theory for evaluation of their photonic measurement statistics without dealing with the computational complexity of Boson samplings. This theory extends characterization of complementary properties in single-photon LONs to multiphoton LONs employing convex-roof extension. It allows us to detect quantum properties su…
We propose an entanglement purification scheme based on material qubits and ancillary coherent multiphoton states. We consider a typical QED scenario where material qubits implemented by two-level atoms fly sequentially through a cavity and interact resonantly with a single mode of the radiation field. We explore the theoretical possibilities of realizing a high-fidelity two-qubit quantum operation necessary for the purification protocol with the help of a postselective balanced homodyne photodetection. We demonstrate that the obtained probabilistic quantum operation can be used as a bilateral…
We demonstrate controlled entanglement routing between bunching and antibunching path-entangled two-photon states in an unbalanced Mach-Zehnder interferometer (UMZI), in which the routing process is controlled by the relative phase difference in the UMZI. Regarding bunching and antibunching path-entangled two-photon states as two virtual ports, we can consider the UMZI as a controlled entanglement router, which bases on the coherent manipulation of entanglement. Half of the entanglement within the input two-photon state is coherently routed between the two virtual ports, while the other is los…
The estimation of high order correlation function values is an important problem in the field of quantum computation. We show that the problem can be reduced to preparation and measurement of optical quantum states resulting after annihilation of a set number of quanta from the original beam. We apply this approach to explore various photon bunching regimes in optical states with gamma-compounded Poisson photon number statistics. We prepare and perform measurement of the thermal quantum state as well as states produced by subtracting one to ten photons from it. Maximum likelihood estimation is…
Multiphoton quantum interference underpins fundamental tests of quantum mechanics and quantum technologies. Consequently, the detrimental effect of photon distinguishability in multiphoton interference experiments can be catastrophic. Here, we employ correlation measurements in the photonic inner modes, time or frequency, to restore quantum interference between photons differing in their colors or injection times in arbitrary linear optical networks, without the need for additional filtering or post selection. Interestingly, we demonstrate how harnessing the multiphoton inner-mode quantum info…
Multiphoton entanglement plays a critical role in quantum information processing, and greatly improves our fundamental understanding of the quantum world. Despite tremendous efforts in either bulk media or fiber-based devices, nonlinear interactions in integrated circuits show great promise as an excellent platform for photon pair generation with its high brightness, stability and scalability \cite{Caspani2017}. Here, we demonstrate the generation of bi- and multiphoton polarization entangled qubits in a single silicon nanowire waveguide, and these qubits directly compatible with the dense wav…
Multiphoton entanglement, as a quantum resource, plays an essential role in linear optical quantum information processing. Krenn et al. (Phys. Rev. Lett. 118, 080401 2017) proposed an innovative scheme that generating entanglement by path identity, in which two-photon interference (called Hong-Ou-Mandel effect) is not necessary in experiment. However, the experiments in this scheme have strict requirements in stability and scalability, which is difficult to be realized in bulk optics. To solve this problem, in this paper we first propose an on-chip scheme to generate multi-photon polarization …
The negativity of the Wigner function is discussed as a measure of the non classicality and the quantum interference pattern obtained therein as a possible measure of the entanglement between the two modes of the vortex states. This measure of entanglement is compared with the results obtained from concurrence.
Experimental observation of counter-intuitive features of photonic bunching
Sapienza Università di Roma（罗马大学）；International Iberian Nanotechnology Laboratory (INL)（国际伊比利亚纳米技术实验室）；Consiglio Nazionale delle Ricerche（意大利国家研究委员会）；Politecnico di Milano（米兰理工大学）
The local multiphoton absorption rate for an arbitrary quantum state of monochromatic light, taking into account the photon number, momentum, and polarization degrees of freedom, is shown to have an upper bound that can be reached by coherent fields. This surprising result rules out any quantum enhancement of the multiphoton absorption rate by momentum entanglement.
We describe a protocol to entangle two qubits at a distance by using resonance fluorescence. The scheme makes use of the postselection of large and distinguishable fluorescence signals corresponding to entangled and unentangled qubit states and has the merits of both high success probability and high entanglement fidelity owing to the multiphoton nature. Our result shows that the entanglement generation is robust against photon fluctuations in the fluorescence signals for a wide range of driving fields. We also demonstrate that this new protocol has an average entanglement duration within the …
Bound entangled states are the exotic objects in the entangled world. They require entanglement to create them, but once they are formed, it is not possible to locally distill any free entanglement from them. It is only until recently that a few bound entangled states were realized in the laboratory. Motivated by these experiments, we propose schemes for creating various classes of bound entangled states with photon polarization. These include Acin-Bruss-Lewenstein-Sanpara states, Dur's states, Lee-Lee-Kim bound entangled states, and an unextendible-product-basis bound entangled state.
The experiments of multi-photon entanglements have been made by some groups, including Pan's group (Ref.[2],[3],[5]). Obviously, the increase number of the photon would cause a dramatically increase in the dimension of the measurement matrix, which result in a great consumption of time in the measurements. From a practical view, we wish to gain the most information through as little measurements as possible for the multi-photon entanglements. The low rank matrix recovery (LRMR) provides such a possibility to resolve all the issues of the measurement matrix based on less data. In this paper, we…
The new process of quantum-injection into an optical parametric amplifier operating in entangled configuration is adopted to amplify into a large dimensionality spin 1/2 Hilbert space the quantum entanglement and superposition properties of the photon-couples generated by parametric down-conversion. The structure of the Wigner function and of the field's correlation functions shows a decoherence-free, multiphoton Schroedinger-cat behaviour of the emitted field which is largely detectable against the squeezed-vacuum noise. Furthermore, owing to its entanglement character, the system is found to…
The generation of quantum entangled states of many particles is a central goal of quantum information science. Characterizing such states is a complex task that demands exponentially large resources as particles are being added. Previously, we demonstrated a resource efficient source that can generate, in principal, entanglement between any number of photons. This source recursively fuse photon pairs generated by a pulsed laser into a multiphoton entangled state. In the current work, we perform quantum state tomography on the photon pair source and quantum process tomography on the fusion oper…
In this theoretical study we demonstrate that entangled states are able to significantly extend the functionality of Hong-Ou-Mandel (HOM) interferometers. By generating a coherent superposition of parametric-down-conversion photons and spatial entanglement in the input channel, the coincidence probability measured at the output changes from a typical HOM-type dip (photon bunching) into much richer patterns including an anti-bunching peak and rapid oscillation fringes with twice the optical frequency. The considered system should be realizable on a single chip using current waveguide technology…
We present a detailed analysis of the Bell measurement scheme proposed in [Phys. Rev. Lett. 114, 113603 (2015)] based on a logical qubit using Greenberger-Horne-Zeilinger (GHZ) entanglement of photons. The success probability of the proposed Bell measurement can be made arbitrarily high using only linear optics as the number of photons in a logical qubit increases. We compare our scheme with all the other proposals, using single-photon qubits, coherent-state qubits or hybrid qubits, suggested to enhance the efficiency of the Bell measurement. As a remarkable advantage, our scheme requires only…
The effects of photon bunching and antibunching correspond to the classical and quantum features of the electromagnetic field, respectively. No direct evidence suggests whether these effects can be potentially related to quantum entanglement. Here we design a cavity quantum electrodynamics model with two atoms trapped in to demonstrate the connections between the steady-state photon statistics and the two-atom entanglement . It is found that within the weak dissipations and to some good approximation, the local maximal two-atom entanglements perfectly correspond to not only the quantum feature…
The first direct measurement of photon bunching (g2 correlation function) in one output arm of a spontaneous-parametric-down-conversion source operated with a continuous pump laser in the single-photon regime is demonstrated. The result is in agreement with the statistics of a thermal field of the same coherence length, and shows the feasibility of investigating photon statistics with compact cw-pumped sources. Implications for entanglement-based quantum cryptography are discussed.
"Schrodinger's cat" is a gedankenexperiment intended to highlight conceptual difficulties in the interpretation of quantum mechanics. The generation of 'cat-like' states is central to numerous quantum information protocols. In particular, much attention has been drawn by states containing N photons in a superposition of all being in one of two designated modes. These maximally path entangled states, known as 'NOON' states, exhibit enhanced phase sensitivity and allow reaching the fundamental quantum limit of precision measurement. Such states could also be used for obtaining 'super-resolution'…
Unwanted multiphoton emission commonly reduces the degree of entanglement of photons generated by non-classical light sources and, in turn, hampers their exploitation in quantum information science and technology. Quantum emitters have the potential to overcome this hurdle but, so far, the effect of multiphoton emission on the quality of entanglement has never been addressed in detail. Here, we tackle this challenge using photon pairs from a resonantly-driven quantum dot and comparing quantum state tomography and second-order coherence measurements as a function of the excitation power. We obs…
Progress in the reliable preparation, coherent propagation and efficient detection of many-body states has recently brought collective quantum phenomena of many identical particles into the spotlight. This tutorial introduces the physics of many-boson and many-fermion interference required for the description of current experiments and for the understanding of novel approaches to quantum computing. The field is motivated via the two-particle case, for which the uncorrelated, classical dynamics of distinguishable particles is compared to the quantum behaviour of identical bosons and fermions. B…
It is shown that coherent superpositions of two oppositely polarized n-photon states can be created by post-selecting the transmission of n independently generated photons into a single mode transmission line. It is thus possible to generate highly non-classical n-photon polarization states using only the bunching effects associated with the bosonic nature of photons. The effects of mode-matching errors are discussed and the possibility of creating n-photon entanglement by redistributing the photons into n separate modes is considered.
A bipartite multiphoton entangled state is created through stimulated parametric down-conversion of strong laser pulses in a nonlinear crystal. It is shown how detectors that do not resolve photon number can be used to analyze such multiphoton states. Entanglement of up to 12 photons is detected using both the positivity of the partially transposed density matrix and a newly derived criteria. Furthermore, evidence is provided for entanglement of up to 100 photons. The multi-particle quantum state is such that even in the case of an overall photon collection and detection efficiency as low as a…
We propose a Bell measurement scheme by employing a logical qubit in Greenberger-Horne-Zeilinger (GHZ) entanglement with an arbitrary number of photons. Remarkably, the success probability of the Bell measurement as well as teleportation of the GHZ entanglement can be made arbitrarily high using only linear optics elements and photon on-off measurements as the number of photons increases. Our scheme outperforms previous proposals using single photon qubits when comparing the success probabilities in terms of the average photon usages. It has another important advantage for experimental feasibi…
With the Jaynes-Cummings model, we have studied the atom and light field quantum entanglement of multiphoton transition, and researched the effect of initial state superposition coefficient $C_{1}$, the transition photon number $N$, the quantum discord $δ$ and the nonlinear coefficient $χ$ on the quantum entanglement degrees. We have given the quantum entanglement degrees curves with time evolution, and obtained some results, which should have been used in quantum computing and quantum information.
We study a simple, effective and robust method for entangling two separate stationary quantum dot spin qubits with high fidelity using multiphoton Gaussian state. The fluorescence signals from the two dots interfere at a beam splitter. The bosonic nature of photons leads, in analogy with the Hong-Ou-Mandel effect, to selective pairing of photon holes (photon absences in the fluorescent signals). As a result, two odd photon number detections at the outgoing beams herald trion entanglement creation, and subsequent reduction of the trions to the spin ground states leads to spin-spin entanglement.…
Dynamical decoupling of a quantum dot spin in a micropillar cavity for spin-multiphoton entanglement
Université Paris-Saclay（巴黎萨克雷大学）；Centre de Nanosciences et de Nanotechnologies, CNRS（国家科学研究中心纳米科学和纳米技术研究中心）；Quandela SAS（Quandela公司）；Johns Hopkins Applied Physics Laboratory（约翰斯·霍普金斯大学应用物理实验室）；University of Delaware（特拉华大学）
Silicon single-photon detectors (SPDs) are the key devices for detecting single photons in the visible wavelength range. Here we present high detection efficiency silicon SPDs dedicated to the generation of multiphoton entanglement based on the technique of high-frequency sine wave gating. The silicon single-photon avalanche diodes (SPADs) components are acquired by disassembling 6 commercial single-photon counting modules (SPCMs). Using the new quenching electronics, the average detection efficiency of SPDs is increased from 68.6% to 73.1% at a wavelength of 785 nm. These sine wave gating SPD…
Bright, entangled multiphoton sources based on atom photon interactions are an essential requirement in the realization of several quantum information and quantum computation schemes based on photonic quantum systems. Here, we experimentally demonstrate a four photon polarization entangled GHZ state obtained from Doppler broadened atomic ensembles of 87Rb atoms. Owing to collective two photon coherence in the Doppler broadened cascade-type atomic system, our setup enables the generation of robust four photon GHZ states with a fidelity of 0.82 and a measured four photon average coincidence rate…
