We have developed a theory for accessing quantum coherences in mutually unbiased bases associated with generalized Pauli operators in multiphoton multimode linear optics networks (LONs). We show a way to construct complementary Pauli measurements in multiphoton LONs and establish a theory for evaluation of their photonic measurement statistics without dealing with the computational complexity of Boson samplings. This theory extends characterization of complementary properties in single-photon LONs to multiphoton LONs employing convex-roof extension. It allows us to detect quantum properties such as entanglement using complementary Pauli measurements, which reveals the physical significance of entanglement between modes in bipartite multiphoton LONs.
We present a review of theoretical and experimental aspects of multiphoton quantum optics. Multiphoton processes occur and are important for many aspects of matter-radiation interactions that include the efficient ionization of atoms and molecules, and, more generally, atomic transition mechanisms; system-environment couplings and dissipative quantum dynamics; laser physics, optical parametric processes, and interferometry. A single review cannot account for all aspects of such an enormously vast subject. Here we choose to concentrate our attention on parametric processes in nonlinear media, w…
Transformations achievable by linear optical components allow to generate the whole unitary group only when restricted to the one-photon subspace of a multimode Fock space. In this paper, we address the more general problem of encoding quantum information by multiphoton states, and elaborating it via ancillary extensions, linear optical passive devices and photodetection. Our scheme stems in a natural way from the mathematical structures underlying the physics of linear optical passive devices. In particular, we analyze an economical procedure for mapping a fiducial 2-photon 2-mode state into …
We have examined both single and entangled two-mode multiphoton coherent states and shown how the `Janus-faced' properties between two partner states are mirrored in appropriate tomograms. Entropic squeezing, quadrature squeezing and higher-order squeezing properties for a wide range of nonclassical states are estimated directly from tomograms. We have demonstrated how squeezing properties of two-mode entangled states produced at the output port of a quantum beamsplitter are sensitive to the relative phase between the reflected and transmitted fields. This feature allows for the possibility of…
We develop a theory for the interaction of multi-level atoms with multi-mode cavities yielding cavity-enhanced multi-photon resonances. The locations of the resonances are predicted from the use of effective two- and three-level Hamiltonians. As an application we show that quantum gates can be realised when photonic qubits are encoded on the cavity modes in arrangements where ancilla atoms transit the cavity. The fidelity of operations is increased by conditional measurements on the atom and by the use of a selected, dual-rail, Hilbert space. A universal set of gates is proposed, including the…
Determining an unknown quantum state from an ensemble of identical systems is a fundamental, yet experimentally demanding, task in quantum science. Here we study the number of measurement bases needed to fully characterize an arbitrary multi-mode state containing a definite number of photons, or an arbitrary mixture of such states. We show this task can be achieved using only linear optics and photon counting, which yield a practical though non-universal set of projective measurements. We derive the minimum number of measurement settings required and numerically show that this lower bound is s…
Recent progress on quantum state engineering has enabled the preparation of quantum photonic systems comprising multiple interacting particles. Interestingly, multiphoton quantum systems can host many complex forms of interference and scattering processes that are essential to perform operations that are intractable on classical systems. Unfortunately, the quantum coherence properties of multiphoton systems degrade upon propagation leading to undesired quantum-to-classical transitions. Furthermore, the manipulation of multiphoton quantum systems requires of nonlinear interactions at the few-ph…
Multiphoton entanglement, as a quantum resource, plays an essential role in linear optical quantum information processing. Krenn et al. (Phys. Rev. Lett. 118, 080401 2017) proposed an innovative scheme that generating entanglement by path identity, in which two-photon interference (called Hong-Ou-Mandel effect) is not necessary in experiment. However, the experiments in this scheme have strict requirements in stability and scalability, which is difficult to be realized in bulk optics. To solve this problem, in this paper we first propose an on-chip scheme to generate multi-photon polarization …
We present a scheme, based only on linear optics and standard photon detection, that allows to generate heralded multiphoton entangled states of arbitrary photon number from spontaneous parametric downconversion (PDC) in the weak interaction regime. The scheme also works in the strong interaction regime, i.e., for the production of large photon numbers, when photon-number resolving detectors with nearly perfect quantum efficiency are used. In addition, the same setup can be used for quantum metrology as multiphoton interferometer with sensitivity at the Heisenberg limit.
Strong correlation of photons, particularly in the single-photon regime, has recently been exploited for various applications in quantum information processing. Existing correlation measurements, however, do not fully characterize multi-photon correlation in a relevant context and may pose limitations in practical situations. We propose a conceptually rigorous, but easy-to-implement, criterion for detecting correlated multi-photon emission out of a quantum optical system, drawn from the context of wavefunction collapse. We illustrate the robustness of our approach against experimental limitati…
Photon entanglement is an essential ingredient for linear optics quantum computing schemes, quantum cryptographic protocols and fundamental tests of quantum mechanics. Here we describe a setup that allows for the generation of polarisation-entangled N-photon states on demand. The photons are obtained by mapping the entangled state of N atoms, each of them trapped inside an optical cavity, onto the free radiation field. The required initial state can be prepared by performing postselective measurements on the collective emission from the cavities through a multiport beamsplitter.
The new process of quantum-injection into an optical parametric amplifier operating in entangled configuration is adopted to amplify into a large dimensionality spin 1/2 Hilbert space the quantum entanglement and superposition properties of the photon-couples generated by parametric down-conversion. The structure of the Wigner function and of the field's correlation functions shows a decoherence-free, multiphoton Schroedinger-cat behaviour of the emitted field which is largely detectable against the squeezed-vacuum noise. Furthermore, owing to its entanglement character, the system is found to…
Multiphoton entanglement is an important resource for linear optics quantum computing. Here we show that a wide range of highly entangled multiphoton states, including W-states, can be prepared by interfering single photons inside a Bell multiport beam splitter and using postselection. A successful state preparation is indicated by the collection of one photon per output port. An advantage of the Bell multiport beam splitter is that it redirects the photons without changing their inner degrees of freedom. The described setup can therefore be used to generate polarisation, time-bin and frequenc…
In this contribution, we show that the use of conditional measurements in the resonant interaction of two quantized electromagnetic fields gives rise to nonclassical multiphoton processes. Furthermore, we demonstrate that this phenomenon may enable a robust integrated-optics protocol to engineer quantum states containing a high number of photons, thus making it a potentially appealing platform for exploring mesoscopic quantum phenomena.
Many recent experiments employ several parametric down conversion (PDC) sources to get multiphoton interference. Such interference has applications in quantum information. We study here how effects due to photon statistics, misalignment, and partial distinguishability of the PDC pairs originating from different sources may lower the interference contrast in the multiphoton experiments.
We propose and theoretically investigate an unambiguous Bell measurement of atomic qubits assisted by multiphoton states. The atoms interact resonantly with the electromagnetic field inside two spatially separated optical cavities in a Ramsey-type interaction sequence. The qubit states are postselected by measuring the photonic states inside the resonators. We show that if one is able to project the photonic field onto two coherent states on opposite sites of phase space, an unambiguous Bell measurement can be implemented. Thus our proposal may provide a core element for future components of q…
We consider a multiphoton Bell-type inequality to study nonlocality in four-mode continuous variable systems, which goes beyond two-photon states and can be applied to mixed as well as states with fluctuating photon number. We apply the inequality to a wide variety of states such as pure and mixed Gaussian states (including squeezed thermal states) and non-Gaussian states. We consider beam splitters as a model for leakage and show that the inequality is able to detect nonclassicality of noisy Gaussian states as well. Finally, we investigate nonlocality in pair-coherent states and entangled coh…
We present the proposition of an experiment in which the multiphoton quantum superposition consisting of N= 10^5 particles generated by a quantum-injected optical parametric amplifier (QI-OPA), seeded by a single-photon belonging to an EPR entangled pair, is made to interact with a Mirror-BEC shaped as a Bragg interference structure. The overall process will realize a Macroscopic Quantum Superposition (MQS) involving a microscopic single-photon state of polarization entangled with the coherent macroscopic transfer of momentum to the BEC structure, acting in space-like separated distant places.
We propose a Bell measurement scheme by employing a logical qubit in Greenberger-Horne-Zeilinger (GHZ) entanglement with an arbitrary number of photons. Remarkably, the success probability of the Bell measurement as well as teleportation of the GHZ entanglement can be made arbitrarily high using only linear optics elements and photon on-off measurements as the number of photons increases. Our scheme outperforms previous proposals using single photon qubits when comparing the success probabilities in terms of the average photon usages. It has another important advantage for experimental feasibi…
Multiphoton quantum interference underpins fundamental tests of quantum mechanics and quantum technologies. Consequently, the detrimental effect of photon distinguishability in multiphoton interference experiments can be catastrophic. Here, we employ correlation measurements in the photonic inner modes, time or frequency, to restore quantum interference between photons differing in their colors or injection times in arbitrary linear optical networks, without the need for additional filtering or post selection. Interestingly, we demonstrate how harnessing the multiphoton inner-mode quantum info…
The estimation of high order correlation function values is an important problem in the field of quantum computation. We show that the problem can be reduced to preparation and measurement of optical quantum states resulting after annihilation of a set number of quanta from the original beam. We apply this approach to explore various photon bunching regimes in optical states with gamma-compounded Poisson photon number statistics. We prepare and perform measurement of the thermal quantum state as well as states produced by subtracting one to ten photons from it. Maximum likelihood estimation is…
In spite of decades of effort, it has not yet been possible to create single-mode multiphoton states of light with high success probability and near unity fidelity. Complex quantum states of propagating optical photons would be an enabling resource for diverse protocols in quantum information science, including for interconnecting quantum nodes in quantum networks. Here, we propose several methods to generate heralded mutipartite entangled atomic and photonic states by using the strong and long-range dissipative couplings between atoms emerging in waveguide QED setups. Our theoretical analysis…
The multiphoton Jaynes-Cummings model is investigated and applications in quantum information science are explored. Considering the strong atom-field coupling regime and an $N$-photon interaction, a nonlinear driving field can perform an arbitrary rotation in the Fock space of the cavity mode involving the vacuum and an $M$-Fock state, with $M<N$. Besides, driving the cavity mode with a linear coherent field (superposition of many Fock states), only the cavity states within the Fock subspace {$|0\rangle,|1\rangle,..., |N-1\rangle$} can be populated, i.e., we show how to implement a Fock state …
Triggered single-photon sources produce the vacuum state with non-negligible probability, but produce a much smaller multiphoton component. It is therefore reasonable to approximate the output of these photon sources as a mixture of the vacuum and single-photon states. We show that it is impossible to increase the probability for a single photon using linear optics and photodetection on fewer than four modes. This impossibility is due to the incoherence of the inputs; if the inputs were pure-state superpositions, it would be possible to obtain a perfect single-photon output. In the more genera…
We introduce a formalism of nonlinear canonical transformations for general systems of multiphoton quantum optics. For single-mode systems the transformations depend on a tunable free parameter, the homodyne local oscillator angle; for n-mode systems they depend on n heterodyne mixing angles. The canonical formalism realizes nontrivial mixings of pairs of conjugate quadratures of the electromagnetic field in terms of homodyne variables for single-mode systems; and in terms of heterodyne variables for multimode systems. In the first instance the transformations yield nonquadratic model Hamilton…
It was shown that using multiphoton qubits, a nearly deterministic Bell-state measurement can be performed with linear optics and on-off photodetectors [Phys. Rev. Lett. 114, 113603 (2015)]. However, multiphoton qubits are generally more fragile than single-photon qubits under a lossy environment. In this paper, we propose and analyze a scheme to teleport multiphoton-qubit information using hybrid entanglement with a loss-tolerant carrier qubit. We consider three candidates for the carrier qubit: a coherent-state qubit, a single-photon polarization qubit, and a vacuum-and-single-photon qubit. …
We investigate the multiphoton quantum dynamics of a leaking single-mode quantized cavity field coupled with a resonantly driven two-level system possessing permanent dipoles. The frequencies of the interacting subsystems are being considered very different, e.g., microwave ranges for the cavity and optical domains for the frequency of the two-level emitter, respectively. In this way, the emitter couples to the resonator mode via its diagonal dipole moments only. Furthermore, the generalized Rabi frequency resulting form the external coherent driving of the two-level subsystem is assumed as we…
The quantum statistical fluctuations of the electromagnetic field establish a limit, known as the shot-noise limit, on the sensitivity of optical measurements performed with classical technologies. However, quantum technologies are not constrained by this shot-noise limit. In this regard, the possibility of using every photon produced by quantum sources of light to estimate small physical parameters, beyond the shot-noise limit, constitutes one of the main goals of quantum optics. Here we experimentally demonstrate a scalable protocol for quantum-enhanced optical phase estimation across a broa…
Extending the scheme developed for a single mode of the electromagnetic field in the preceding paper ``Structure of multiphoton quantum optics. I. Canonical formalism and homodyne squeezed states'', we introduce two-mode nonlinear canonical transformations depending on two heterodyne mixing angles. They are defined in terms of hermitian nonlinear functions that realize heterodyne superpositions of conjugate quadratures of bipartite systems. The canonical transformations diagonalize a class of Hamiltonians describing non degenerate and degenerate multiphoton processes. We determine the coherent…
Protocols for probabilistic entanglement-assisted quantum teleportation and for entanglement swapping of material qubits are presented. They are based on a protocol for postselective Bell-state projection which is capable of projecting two material qubits onto a Bell state with the help of ancillary coherent multiphoton states and postselection by balanced homodyne photodetection. Provided this photonic postselection is successful we explore the theoretical possibilities of realizing unit fidelity quantum teleportation and entanglement swapping with $25\%$ success probability. This photon-assi…
We investigate how multiphoton quantum states obtained through optical parametric amplification can be manipulated by performing a measurement on a small portion of the output light field. We study in detail how the macroqubit features are modified by varying the amount of extracted information and the strategy adopted at the final measurement stage. At last the obtained results are employed to investigate the possibility of performing a microscopic-macroscopic non-locality test free from auxiliary assumptions.
Multiphoton heralding generates large-amplitude squeezed Schrödinger cat states and parity-selective Fock superpositions from squeezed vacuum via an OPA
Single photons are a vital resource for optical quantum information processing. Efficient and deterministic single photon sources do not yet exist, however. To date, experimental demonstrations of quantum processing primitives have been implemented using non-deterministic sources combined with heralding and/or postselection. Unfortunately, even for eight photons, the data rates are already so low as to make most experiments impracticable. It is well known that quantum memories, capable of storing photons until they are needed, are a potential solution to this `scaling catastrophe'. Here, we an…
Thermal states of light are widely used in quantum optics for various quantum phenomena testing. Particularly, they can be utilized for characterization of photon creation and photon annihilation operations. During the last decade the problem of photon subtraction from multimode quantum states become of much significance. Therefore, in this work we present a technique for statistical parameter estimation of multimode multiphoton subtracted thermal states of light, which can be used for multimode photon annihilation test.
The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. For addressing systems with underlying bosonic structure, it is advantageous to utilize a naturally bosonic platform. Optical photons passing through linear networks may be configured to perform quantum simulation tasks, but the efficient preparation and detection of multiphoton quantum states of light in linear optical systems are challenging. Here, we experimentally implement a boson sampling protocol for simulating molecular vibronic spectra [Nature Photonics $\textbf{9}$…
We propose a model for computing of a certain set of analytical functions based on estimating the output distribution of multiphoton outcomes in an optical scheme with an initial single-mode squeezed vacuum (SMSV) state and photonic states measuring the number of photons in one of the output modes of the beam splitter (BS) by photon number resolving (PNR) detector. The set of considered analytical functions is polynomial expressions including arbitrary derivatives of certain functions which can take on very large values even on small interval in their argument and small values of the parameter…
We investigate which pure states of $n$ photons in $d$ modes can be transformed into each other via linear optics, without post-selection. In other words, we study the local unitary (LU) equivalence classes of symmetric many-qudit states. Writing our state as $f^\dagger|Ω\rangle$, with $f^\dagger$ a homogeneous polynomial in the mode creation operators, we propose two sets of LU-invariants: (a) spectral invariants, which are the eigenvalues of the operator $ff^\dagger$, and (b) moments, each given by the norm of the symmetric component of a tensor power of the initial state, which can be compu…
Two-color multiphoton emission from polycrystalline tungsten nanotips has been demonstrated using two-color laser fields. The two-color photoemission is assisted by a three-photon multicolor quantum channel, which leads to a twofold increase in quantum efficiency. Weak-field control of two-color multiphoton emission was achieved by changing the efficiency of the quantum channel with pulse delay. The result of this study complements two-color tunneling photoemission in strong fields, and has potential applications for nanowire-based photonic devices. Moreover, the demonstrated two-color multiph…
A scheme for the enhanced generation of higher photon-number states is realized, using an optical time-multiplexing setting that exploits a parametric down-conversion source for an iterative state generation. We use a quantum feedback mechanism for already generated photons to induce self-seeding of the consecutive nonlinear process, enabling us to coherently add photons to the light that propagates in the feedback loop. The addition can be carried out for any chosen number of round trips, resulting in a successive buildup of multiphoton states. Our system is only limited by loop losses. The l…
Thermal states of light are widely used in quantum optics due to their correlation properties. As is well known, their correlation properties and the photon number distribution as a whole are strongly dependent on the mode number selected by the detection scheme. The same changes can be caused by photon subtraction. Therefore, we describe the general case of the multimode thermal state after a multiphoton subtraction, when the photon number statistics is registered by the detector selecting a part of the initial modes. We present an analytical form of the obtained photon number distribution an…
Spatial quantum enhancement effects are studied under a unified framework. It is shown that the multiphoton absorption rate of photons with a quantum-enhanced lithographic resolution is reduced, not enhanced, contrary to popular belief. The use of adiabatic soliton expansion is proposed to beat the standard quantum limit on the optical beam displacement accuracy, as well as to engineer an arbitrary multiphoton interference pattern for quantum lithography. The proposed scheme provides a conceptually simple method that works for an arbitrary number of photons.
We present a detailed analysis of the Bell measurement scheme proposed in [Phys. Rev. Lett. 114, 113603 (2015)] based on a logical qubit using Greenberger-Horne-Zeilinger (GHZ) entanglement of photons. The success probability of the proposed Bell measurement can be made arbitrarily high using only linear optics as the number of photons in a logical qubit increases. We compare our scheme with all the other proposals, using single-photon qubits, coherent-state qubits or hybrid qubits, suggested to enhance the efficiency of the Bell measurement. As a remarkable advantage, our scheme requires only…
