One of the promising systems to realize quantum computation is a hybrid system where a superconducting flux qubit plays a role of a quantum processor and the NV center ensemble is used as a quantum memory. We have theoretically and experimentally studied the effect of magnetic fields on this hybrid system, and found that the lifetime of the vacuum Rabi oscillation is improved by applying a few mT magnetic field to the NV center ensemble. Here, we construct a theoretical model to reproduce the vacuum Rabi oscillations with/without magnetic fields applied to the NV centers, and we determine the reason why magnetic fields can affect the coherent properties of the NV center ensemble. From our theoretical analysis, we quantitatively show that the magnetic fields actually suppress the inhomogeneous broadening from the strain in the NV centers.
Three-dimensional microwave cavities have recently been combined with superconducting qubits in the circuit quantum electrodynamics (cQED) architecture. These cavities should have less sensitivity to dielectric and conductor losses at surfaces and interfaces, which currently limit the performance of planar resonators. We expect that significantly (>10^3) higher quality factors and longer lifetimes should be achievable for 3D structures. Motivated by this principle, we have reached internal quality factors greater than 0.5x10^9 and intrinsic lifetimes of 0.01 seconds for multiple aluminum super…
We study theoretically the lifetime of magnetically trapped atoms in the close vicinity of a type-II superconducting surface, in the context of superconducting atom-chips. We account for the magnetic noise created at the cloud position by the vortices present in the superconductor and give specific results for our experiment which uses a niobium film. Our main result is that atom losses are dominated by the presence of vortices. They remain however dramatically smaller than in equivalent room-temperature atom-chip setups using normal metals.
We report the realization of a quantum circuit in which an ensemble of electronic spins is coupled to a frequency tunable superconducting resonator. The spins are Nitrogen-Vacancy centers in a diamond crystal. The achievement of strong coupling is manifested by the appearance of a vacuum Rabi splitting in the transmission spectrum of the resonator when its frequency is tuned through the NV center electron spin resonance.
Very high quality factor superconducting radio frequency cavities developed for accelerators can enable fundamental physics searches with orders of magnitude higher sensitivity, as well as offer a path to a 1000-fold increase in the achievable coherence times for cavity-stored quantum states in the 3D circuit QED architecture. Here we report the first measurements of multiple accelerator cavities of $f_0=$1.3, 2.6, 5 GHz resonant frequencies down to temperatures of about 10~mK and field levels down to a few photons, which reveal record high photon lifetimes up to 2 seconds, while also further …
Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. Ideal candidates for coherent qubit interconversion are optically active spins magnetically coupled to a superconducting resonator. We report on a cavity QED experiment with magnetically anisotropic Er3+:Y2SiO5 crystals and demonstrate strong coupling of rare-earth spins to a lumped element resonator. In addition, the electron spin resonance and relaxation dynamics of the erbium spins are detected via direct microwave absorption, without a…
We demonstrate a hybrid method based on field ionization and state-selective de-excitation capable of measuring the lifetimes of high-lying Rydberg states. For nS Rydberg states of Rb atoms with principal quantum number $60\leq n\leq88$, we measure both the individual target state lifetimes and those of the ensemble of Rydberg states populated via black-body radiation-induced transitions. We find good overall agreement with numerical calculations of the expected lifetimes in both cases. However, for the target state lifetimes, we find a local deviation towards shorter lifetimes for states arou…
The rapid development in designs and fabrication techniques of superconducting qubits has helped making coherence times of qubits longer. In the near future, however, the radiative decay of a qubit into its control line will be a fundamental limitation, imposing a trade-off between fast control and long lifetime of the qubit. In this work, we successfully break this trade-off by strongly coupling another superconducting qubit along the control line. This second qubit, which we call a Josephson quantum filter (JQF), prevents the qubit from emitting microwave photons and thus suppresses its rela…
We theoretically investigate the heating rate and spin flip lifetimes due to near field noise for atoms trapped close to layered superconducting structures. In particular, we compare the case of a gold layer deposited above a superconductor with the case of a bare superconductor. We study a niobium-based and a YBCO-based chip. For both niobium and YBCO chips at a temperature of 4.2 K, we find that the deposition of the gold layer can have a significant impact on the heating rate and spin flip lifetime, as a result of the increase of the near field noise. At a chip temperature of 77 K, this eff…
Interfacing superconducting quantum processors, working in the GHz frequency range, with optical quantum networks and atomic qubits is a challenging task for the implementation of distributed quantum information processing as well as for quantum communication. Using spin ensembles of rare earth ions provide an excellent opportunity to bridge microwave and optical domains at the quantum level. In this letter, we demonstrate magnetic coupling of Er$^{3+}$ spins doped in Y$_{2}$SiO$_{5}$ crystal to a high-Q coplanar superconducting resonator.
Electron spins in solids are promising candidates for quantum memories for superconducting qubits because they can have long coherence times, large collective couplings, and many quantum bits can be encoded into the spin-waves of a single ensemble. We demonstrate the coupling of electron spin ensembles to a superconducting transmission-line resonator at coupling strengths greatly exceeding the cavity decay rate and comparable to spin linewidth. We also use the enhanced coupling afforded by the small cross-section of the transmission line to perform broadband spectroscopy of ruby at millikelvin…
We propose an experimentally realizable hybrid quantum circuit for achieving a strong coupling between a spin ensemble and a transmission-line resonator via a superconducting flux qubit used as a data bus. The resulting coupling can be used to transfer quantum information between the spin ensemble and the resonator. In particular, in contrast to the direct coupling without a data bus, our approach requires far less spins to achieve a strong coupling between the spin ensemble and the resonator (e.g., three to four orders of magnitude less). This proposed hybrid quantum circuit could enable a lo…
Superconducting flux qubits are a promising candidate for realizing quantum information processing and quantum simulations. Such devices behave like artificial atoms, with the advantage that one can easily tune the "atoms" internal properties. Here, by harnessing this flexibility, we propose a technique to minimize the inhomogeneous broadening of a large ensemble of flux qubits by tuning only the external flux. In addition, as an example of many-body physics in such an ensemble, we show how to observe superradiance, and its quadratic scaling with ensemble size, using a tailored microwave contr…
Using a consistent quantum-mechanical treatment for the electromagnetic radiation, we theoretically investigate the magnetic spin-flip scatterings of a neutral two-level atom trapped in the vicinity of a superconducting body. We derive a simple scaling law for the corresponding spin-flip lifetime for such an atom trapped near a superconducting thick slab. For temperatures below the superconducting transition temperature T_c, the lifetime is found to be enhanced by several orders of magnitude in comparison to the case of a normal conducting slab. At zero temperature the spin-flip lifetime is gi…
Electron-spin nitrogen-vacancy color centers in diamond are a natural candidate to act as a quantum memory for superconducting qubits because of their large collective coupling and long coherence times. We report here the first demonstration of strong coupling and coherent exchange of a single quantum of energy between a flux-qubit and an ensemble of nitrogen-vacancy color centers.
In the present paper we study the spontaneous photon emission due to a magnetic spin-flip transition of a two-level atom in the vicinity of a dielectric body like a normal conducting metal or a superconductor. For temperatures below the transition temperature T_c of a superconductor, the corresponding spin-flip lifetime is boosted by several orders of magnitude as compared to the case of a normal conducting body. Numerical results of an exact formulation are also compared to a previously derived approximative analytical expression for the spin-flip lifetime and we find an excellent agreement. …
We examine the possibility of coherent, reversible information transfer between solid-state superconducting qubits and ensembles of ultra-cold atoms. Strong coupling between these systems is mediated by a microwave transmission line resonator that interacts near-resonantly with the atoms via their optically excited Rydberg states. The solid-state qubits can then be used to implement rapid quantum logic gates, while collective metastable states of the atoms can be employed for long-term storage and optical read-out of quantum information.
The hybridization of distinct quantum systems is now seen as an effective way to engineer the properties of an entire system leading to applications in quantum metamaterials, quantum simulation, and quantum metrology. One well known example is superconducting circuits coupled to ensembles of microscopic natural atoms. In such cases, the properties of the individual atom are intrinsic, and so are unchangeable. However, current technology allows us to fabricate large ensembles of macroscopic artificial atoms such as superconducting flux qubits, where we can really tailor and control the properti…
We report the experimental realization of a hybrid quantum circuit combining a superconducting qubit and an ensemble of electronic spins. The qubit, of the transmon type, is coherently coupled to the spin ensemble consisting of nitrogen-vacancy (NV) centers in a diamond crystal via a frequency-tunable superconducting resonator acting as a quantum bus. Using this circuit, we prepare arbitrary superpositions of the qubit states that we store into collective excitations of the spin ensemble and retrieve back later on into the qubit. These results constitute a first proof of concept of spin-ensemb…
Recent experiments in superconducting qubit systems have shown an unexpectedly strong dependence of the qubit relaxation rate on the readout drive power. This phenomenon limits the maximum measurement strength and thus the achievable readout speed and fidelity. We address this problem here and provide a plausible mechanism for drive-power dependence of relaxation rates. To this end we introduce a two-parameter perturbative expansion in qubit anharmonicity and the drive amplitude through a unitary transformation technique introduced in Part I. This approach naturally reveals number non-conservi…
The problem of coupling multiple spin ensembles through cavity photons is revisited by using PyBTM organic radicals and a high-$T_c$ superconducting coplanar resonator. An exceptionally strong coupling is obtained and up to three spin ensembles are simultaneously coupled. The ensembles are made physically distinguishable by chemically varying the $g$ factor and by exploiting the inhomogeneities of the applied magnetic field. The coherent mixing of the spin and field modes is demonstrated by the observed multiple anticrossing, along with the simulations performed within the input-output formali…
We demonstrate the coupling of rare-earth ions locally implanted in a substrate (Gd$^{3+}$ in Al$_{2}$O$_{3}$) to a superconducting NbN lumped-element micro-resonator. The hybrid device is fabricated by a controlled ion implantation of rare-earth ions in well-defined micron-sized areas, aligned to lithographically defined micro-resonators. The technique does not degrade the internal quality factor of the resonators which remain above $10^{5}$. Using microwave absorption spectroscopy we observe electron-spin resonances in good agreement with numerical modelling and extract corresponding couplin…
We have studied the role of thermalization in lifetime reduction of quantum memory based on multi-atomic ensembles. Herein, it is shown to be impossible to remove the thermaization-caused decoherence in such systems using the methods of dynamical decoupling. We have analyzed the existing models of the thermalization and have proposed a new understanding of the thermalization as a result of the internal processes which are not described in the unitary quantum dynamics formalism. The possible ways for reducing the negative influence of thermalization on the quantum memory lifetime are also discu…
We investigate theoretically quantum entanglement of light with the collective spin polarization of a cold atomic ensemble in cavity-assisted Raman schemes. Previous works concentrated mostly on the bad cavity limit where the signals are much longer than the cavity field lifetime. In view of atomic relaxation and other imperfections, there may arise a need to speed-up the light-atoms interface operation. By increasing the cavity field lifetime, one can achieve better light-matter coupling and entanglement. In our work, we consider the non-adiabatic effects that become important beyond the bad …
Producing nano-structures with embedded bright ensembles of lifetime-limited emitters is a challenge with potential high impact in a broad range of physical sciences. In this work, we demonstrate controlled charge transfer to and from dark states exhibiting very long lifetimes in high density ensembles of SiV centers hosted in a CVD-grown diamond nano-pyramid. Further, using a combination of resonant photoluminescence excitation and a frequency-selective persistent hole burning technique that exploits such charge state transfer, we could demonstrate close to lifetime-limited linewidths from th…
The dynamics of a weakly anharmonic superconducting qubit in a complex electromagnetic environment is generally well-described by an effective multimode Kerr Hamiltonian at sufficiently weak excitation. This Hamiltonian can be embedded in a master equation with losses determined by the details of the electromagnetic environment. Recent experiments indicate, however, that when a superconducting circuit is driven with microwave signals the observed relaxation rates appear to be substantially different from expectations based on the electromagnetic environment of the qubit alone. This issue is a …
We study spin relaxation and diffusion in an electron-spin ensemble of nitrogen impurities in diamond at low temperature (0.25-1.2 K) and polarizing magnetic field (80-300 mT). Measurements exploit mode- and temperature-dependent coupling of hyperfine-split sub-ensembles to the resonator. Temperature-independent spin linewidth and relaxation time suggest that spin diffusion limits spin relaxation. Depolarization of one sub-ensemble by resonant pumping of another indicates fast cross-relaxation compared to spin diffusion, with implications on use of sub-ensembles as independent quantum memories…
We demonstrate the use of high-Q superconducting coplanar waveguide (CPW) microresonators to perform rapid manipulations on a randomly distributed spin ensemble using very low microwave power (400 nW). This power is compatible with dilution refrigerators, making microwave manipulation of spin ensembles feasible for quantum computing applications. We also describe the use of adiabatic microwave pulses to overcome microwave magnetic field ($B_{1}$) inhomogeneities inherent to CPW resonators. This allows for uniform control over a randomly distributed spin ensemble. Sensitivity data are reported …
A quantum coherent interface between optical and microwave photons can be used as a basic building block within a future quantum information network. The interface is envisioned as an ensemble of rare-earth ions coupled to a superconducting resonator, allowing for coherent transfer between optical and microwave photons. Towards this end, we have realized a hybrid device coupling a Er$^{3+}$ doped Y$_2$SiO$_5$ crystal in a superconducting coplanar waveguide cavity. We observe a collective spin coupling of 4 MHz and a spin linewdith of down to 75 MHz.
Parametrically induced strong coupling between a superconducting quantum circuit and a solid-state spin ensemble
The Grainger College of Engineering, University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校格雷格工程学院）；Materials Research Laboratory, The Grainger College of Engineering, University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校格雷格工程学院材料研究实验室）；Holonyak Micro and Nanotechnology Lab, The Grainger College of Engineering, University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校格雷格工程学院霍洛尼亚克微纳技术实验室）；National Center for Supercomputing Applications, University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校国家超级计算应用中心）
We study a hybrid quantum system consisting of spin ensembles and superconducting flux qubits, where each spin ensemble is realized using the nitrogen-vacancy centers in a diamond crystal and the nearest-neighbor spin ensembles are effectively coupled via a flux qubit.We show that the coupling strengths between flux qubits and spin ensembles can reach the strong and even ultrastrong coupling regimes by either engineering the hybrid structure in advance or tuning the excitation frequencies of spin ensembles via external magnetic fields. When extending the hybrid structure to an array with equal…
We propose an effective scheme for realizing a Jaynes-Cummings (J-C) model with the collective nitrogen-vacancy center ensembles (NVE) bosonic modes in a hybrid system. Specifically, the controllable transmon qubit can alternatively interact with one of the two NVEs, which results in the production of $N$ particle entangled states. Arbitrary $N$ particle entangled states, NOON states, N-dimensional entangled states and entangled coherent states are demonstrated. Realistic imperfections and decoherence effects are analyzed via numerical simulation. Since no cavity photons or excited levels of t…
We propose a potentially practical scheme to simulate artificial Abelian gauge field for polaritons using a hybrid quantum system consisting of nitrogen-vacancy center ensembles (NVEs) and superconducting transmission line resonators (TLR). In our case, the collective excitations of NVEs play the role of bosonic particles, and our multiport device tends to circulate polaritons in a behavior like a charged particle in an external magnetic field. We discuss the possibility of identifying signatures of the Hofstadter "butterfly" in the optical spectra of the resonators, and analyze the ground sta…
We investigate the coupling of an ensemble of phosphorus donors in an isotopically purified $^{28}$Si host lattice interacting with a superconducting coplanar waveguide resonator. The microwave transmission spectrum of the resonator shows a normal mode splitting characteristic for high cooperativity. The evaluated collective coupling strength $g_{\mathrm{eff}}$ is of the same order as the loss rate of the spin system $γ$, indicating the onset of strong coupling. We develop a statistical model to describe the influence of temperature on the coupling strength from $50\,\mathrm{mK}$ to $3.5\,\mat…
The superconducting transmon qubit is a leading platform for quantum computing and quantum science. Building large, useful quantum systems based on transmon qubits will require significant improvements in qubit relaxation and coherence times, which are orders of magnitude shorter than limits imposed by bulk properties of the constituent materials. This indicates that relaxation likely originates from uncontrolled surfaces, interfaces, and contaminants. Previous efforts to improve qubit lifetimes have focused primarily on designs that minimize contributions from surfaces. However, significant i…
This article reviews efforts to build a new type of quantum device, which combines an ensemble of electronic spins with long coherence times, and a small-scale superconducting quantum processor. The goal is to store over long times arbitrary qubit states in orthogonal collective modes of the spin-ensemble, and to retrieve them on-demand. We first present the protocol devised for such a multi-mode quantum memory. We then describe a series of experimental results using NV center spins in diamond, which demonstrate its main building blocks: the transfer of arbitrary quantum states from a qubit in…
Epitaxial NbN-junction-based self-shunted superconducting flux qubit with high anharmonicity
Tohoku University（东北大学）；RIKEN Center for Quantum Computing（理化学研究所量子计算中心）；The University of Tokyo（东京大学）；Inamori Research Institute for Science (InaRIS)（稻盛科学研究所）；National Institute of Information and Communications Technology (NICT)（信息通信研究机构）
We present a superconducting qubit design that is fabricated in a 2D geometry over a superconducting ground plane to enhance the lifetime. The qubit is coupled to a microstrip resonator for readout. The circuit is fabricated on a silicon substrate using low loss, stoichiometric titanium nitride for capacitor pads and small, shadow-evaporated aluminum/aluminum-oxide junctions. We observe qubit relaxation and coherence times ($T_1$ and $T_2$) of 11.7 $\pm$ 0.2 $μ$s and 8.7 $\pm$ 0.3 $μ$s, respectively. Calculations show that the proximity of the superconducting plane suppresses the otherwise hig…
Atom chips made of superconducting material can generate magnetic traps with significantly reduced noise. Recently, several designs for superconducting chips have been theoretically analyzed and experimentally tested, for cases with many vortices considered as an average vortex density. Here we show theoretically, for the first time, how the magnetic field of a $\it single$ vortex, pinned by a superconducting nano-disc of radius $\sim$100 nm and combined with an external bias field parallel to the disc surface, yields a closed 3D trap for cold atoms. The size of the trap, and its height above …
A cold atomic ensemble suits well for optical quantum memories, and its entanglement with a single photon forms the building block for quantum networks that give promise for many revolutionary applications. Efficiency and lifetime are among the most important figures of merit for a memory. In this paper, we report the realization of entanglement between an atomic ensemble and a single-photon with subsecond lifetime and high efficiency. We engineer dual control modes in a ring cavity to create entanglement and make use of 3-dimensional optical lattice to prolong memory lifetime. The memory effi…
The quantized lateral motional states and the spin states of electrons trapped on the surface of superfluid helium have been proposed as basic building blocks of a scalable quantum computer. Circuit quantum electrodynamics (cQED) allows strong dipole coupling between electrons and a high-Q superconducting microwave resonator, enabling such sensitive detection and manipulation of electron degrees of freedom. Here we present the first realization of a hybrid circuit in which a large number of electrons are trapped on the surface of superfluid helium inside a coplanar waveguide resonator. The hig…
We have built a hybrid system composed of a superconducting flux qubit (the processor) and an ensemble of nitrogen-vacancy centers in diamond (the memory) that can be directly coupled to one another and demonstrated how information can be transferred from the flux qubit to the memory, stored and subsequently retrieved. We have established the coherence properties of the memory, and succeeded in creating an entangled state between the processor and memory, demonstrating how the entangled state's coherence is preserved. Our results are a significant step towards using an electron spin ensemble a…
We propose to create and stabilize long-lived macroscopic quantum superposition states in atomic ensembles. We show that using a fully quantum parametric amplifier can cause the simultaneous decay of two atoms and, in turn, create stabilized atomic Schrödinger cat states. Remarkably, even with modest parameters these intracavity atomic cat states can have an extremely long lifetime, up to \emph{4 orders of magnitude} longer than that of intracavity photonic cat states under the same parameter conditions, reaching \emph{tens of milliseconds}. This lifetime of atomic cat states is ultimately lim…
A protocol is discussed which allows one to realize a transducer for single photons between the optical and the microwave frequency range. The transducer is a spin ensemble, where the individual emitters possess both an optical and a magnetic-dipole transition. Reversible frequency conversion is realized by combining optical photon storage, by means of EIT, with the controlled switching of the coupling between the magnetic-dipole transition and a superconducting qubit, which is realized by means of a microwave cavity. The efficiency is quantified by the global fidelity for transferring coheren…
Spin echo is a powerful technique to extend atomic or nuclear coherence time by overcoming the dephasing due to inhomogeneous broadening. However, applying this technique to an ensemble-based quantum memory at single-quanta level remains challenging. In our experimental study we find that noise due to imperfection of the rephasing pulses is highly directional. By properly arranging the beam directions and optimizing the pulse fidelities, we have successfully managed to operate the spin echo technique in the quantum regime and observed nonclassical photon-photon correlations. In comparison to t…
Microscopic two-level system (TLS) defects at dielectric surfaces and interfaces are among the dominant sources of loss in superconducting quantum circuits, and their properties have been extensively probed using superconducting resonators and qubits. We report on spectroscopy of TLSs coupling to the strain field in a surface acoustic wave (SAW) resonator. The narrow free spectral range of the resonator allows for two-tone spectroscopy where a strong pump is applied at one resonance while a weak signal is used to probe a different mode. We map the spectral hole burnt by the pump tone as a func…
We investigate the electron spin resonance of an ensemble of Nitrogen-Vacancy (NV) color centers in a bulk diamond crystal. The four possible orientations of the NV-center in the lattice lead to different dependences on the magnitude and the orientation of an external static magnetic field. Experimental results obtained with a continuous microwave excitation are in good agreement with simulations. In addition, we observe that the average radiative lifetime of the NV color center is also modified when the external magnetic field is applied. This variation is explained by the mixing between mS =…
Dielectric loss is one of the major decoherence sources of superconducting qubits. Contemporary high-coherence superconducting qubits are formed by material systems mostly consisting of superconducting films on substrate with low dielectric loss, where the loss mainly originates from the surfaces and interfaces. Among the multiple candidates for material systems, a combination of titanium nitride (TiN) film and sapphire substrate has good potential because of its chemical stability against oxidization, and high quality at interfaces. In this work, we report a TiN film deposited onto sapphire s…
