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arXiv 1502.04688cond-mat.supr-con
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(Li0)OHFe0.98 Se超导体:离子交换合成大单晶和高二维电子性质

(Li0.84Fe0.16)OHFe0.98Se superconductor: Ion-exchange synthesis of large single crystal and highly two-dimensional electron properties

Xiaoli Dong, Kui Jin, Dongna Yuan, Huaxue Zhou, Jie Yuan, Yulong Huang, Wei Hua, Junliang Sun, Ping Zheng, Wei Hu, Yiyuan Mao, Mingwei Ma, Guangming Zhang, Fang… 展开作者

Xiaoli Dong, Kui Jin, Dongna Yuan, Huaxue Zhou, Jie Yuan, Yulong Huang, Wei Hua, Junliang Sun, Ping Zheng, Wei Hu, Yiyuan Mao, Mingwei Ma, Guangming Zhang, Fang Zhou, Zhongxian Zhao

摘要:

采用水热离子交换法成功地合成了(Li_(1-x)Fe_(1-y)Se_x)OHFe_(1-x)Se_x超导体的优质单晶(Li_(0.84)Fe_(0.16)OHFe_(0.98)Se)。通过磁化率和电阻率测量确定了超导转变温度(Tc)为42 K,沿c轴和ab平面的零温上临界磁场分别为79和313特斯拉。面外电阻率与面内电阻率之比\r{ho} c/ \r{ho} ab随温度的降低而增大,在50 K时达到2500,在特征温度T*=120 K时出现明显的扭折。负的面内霍尔系数表明电子载流子在电荷传输中占主导地位,并且随着温度降低至接近T*,空穴贡献显著降低。从T* 下降到Tc,我们观察到FeSe层的面内电阻率和磁化率的线性温度依赖性。因此,我们的研究结果表明,正常状态的(Li0.84Fe0.16)OHFe0.98Se变得高度二维和异常之前的超导转变,提供了一个新的见解高Tc超导机制。

英文摘要:

A large and high-quality single crystal (Li0.84Fe0.16)OHFe0.98Se, the optimal superconductor of newly reported (Li1-xFex)OHFe1-ySe system, has been successfully synthesized via a hydrothermal ion-exchange technique. The superconducting transition temperature (Tc) of 42 K is determined by magnetic susceptibility and electric resistivity measurements, and the zero-temperature upper critical magnetic fields are evaluated as 79 and 313 Tesla for the field along the c-axis and the ab-plane, respectively. The ratio of out-of-plane to in-plane electric resistivity,\r{ho}c/\r{ho}ab, is found to increases with decreasing temperature and to reach a high value of 2500 at 50 K, with an evident kink occurring at a characteristic temperature T*=120 K. The negative in-plane Hall coefficient indicates that electron carriers dominate in the charge transport, and the hole contribution is significantly reduced as the temperature is lowered to approach T*. From T* down to Tc, we observe the linear temperature dependences of the in-plane electric resistivity and the magnetic susceptibility for the FeSe layers. Our findings thus reveal that the normal state of (Li0.84Fe0.16)OHFe0.98Se becomes highly two-dimensional and anomalous prior to the superconducting transition, providing a new insight into the mechanism of high-Tc superconductivity.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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