Within the universal zero-range theory, we compute the three-body recombination rate to deep molecular states for two identical bosons resonantly interacting with each other and with a third atom of another species, in the absence of weakly bound dimers. The results allow for a quantitative understanding of loss resonances at finite temperature and, combined with experimental data, can be used for testing the Efimov universality and extracting the corresponding three-body parameters in a given system. Curiously, we find that the loss rate can be dramatically enhanced by the resonant heavy-heavy interaction, even for large mass ratios where this interaction is practically irrelevant for the Efimov scaling factor. This effect is important for analysing the recent loss measurements in the Cs-Li mixture.
The mass-imbalanced three-body recombination process that forms a shallow dimer is shown to possess a rich Efimov-Stückelberg landscape, with corresponding spectra that differ fundamentally from the homonuclear case. A semi-analytical treatment of the three-body recombination predicts an unusual spectra with intertwined resonance peaks and minima, and yields in-depth insight into the behavior of the corresponding Efimov spectra. In particular, the patterns of the Efimov-Stückelberg landscape are shown to depend inherently on the degree of diabaticity of the three-body collisions, which strongl…
We present the essential experimental steps of our all-optical approach to prepare a double-degenerate Fermi-Fermi mixture of 6Li and 40K atoms, which then serves as a starting point for molecule formation. We first describe the optimized trap loading procedures, the internal-state preparation of the sample, and the combined evaporative and sympathetic cooling process. We then discuss the preparation of the sample near an interspecies Feshbach resonance, and we demonstrate the formation of heteronuclear molecules by a magnetic field ramp across the resonance.
We consider a homogeneous heteronuclear Bose mixture with contact interactions at the mean-field collapse, i.e. with interspecies attraction equal to the mean geometrical intraspecies repulsion. We show that the Lee-Huang-Yang (LHY) energy functional is accurately approximated by an expression that has the same functional form as in the homonuclear case. The approximated energy functional is characterized by two exponents, which can be treated as fitting parameters. We demonstrate that the values of these parameters which preserve the invariance under permutation of the two atomic species are …
We report on the formation of heteronuclear quantum droplets in an attractive bosonic mixture of 41K and 87Rb. We observe long-lived self-bound states, both in free space and in an optical waveguide. In the latter case, the dynamics under the effect of a species-dependent force confirms their bound nature. By tuning the interactions from the weakly to the strongly attractive regime, we study the transition from expanding to localized states, in both geometries. We compare the experimental results with beyond mean-field theory and we find a good agreement in the full range of explored interacti…
Effective scatterings and universal clusters of heteronuclear ultracold mixtures in quasi-low dimensions
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）
We study the recombination process of three atoms scattering into an atom and diatomic molecule in heteronuclear mixtures of ultracold atomic gases with large and positive interspecies scattering length at finite temperature. We calculate the temperature dependence of the three-body recombination rates by extracting universal scaling functions that parametrize the energy dependence of the scattering matrix. We compare our results to experimental data for the 40K-87Rb mixture and make a prediction for 6Li-87Rb. We find that contributions from higher partial wave channels significantly impact th…
We derive the complete mixing-demixing phase-diagram relevant to a bosonic binary mixture confined in a ring trimer and modeled within the Bose-Hubbard picture. The mixing properties of the two quantum fluids, which are shown to be strongly affected by the fragmented character of the confining potential, are evaluated by means of a specific indicator imported from Statistical Thermodynamics and are shown to depend only on two effective parameters incorporating the asymmetry between the heteronuclear species. To closely match realistic experimental conditions, our study is extended also beyond …
We propose a general scheme for inducing resonant exchange between spins or pseudo-spins of unmatched levels via periodic driving. The basic idea is illustrated for a system of two heteronuclear atoms, for which analytical results are provided for the effective spin exchange (SE) interaction strength. It is then applied to the mixture of 23Na and 87Rb atoms with a radio-frequency (rf) or microwave field near-resonant to the mismatched Zeeman level spacings. SE interaction engineered this way is applicable to ultracold quantum gas mixtures involving spinor Bose-Bose, Bose-Fermi, and Fermi-Fermi…
We have theoretically investigated the structure of spinning self-bound droplets made of $^{41}$K-$^{87}$Rb Bose mixture by solving the Gross-Pitaevskii equation including beyond-mean-field correction in the Lee-Huang-Yang form. The structure and energetics of vortex formation in the self-bound mixture have been elucidated, showing that the formation of linear vortices in the heavier species is energetically favoured over other configurations. A fake (partially filled) core develops as a consequence in the other species, resulting in a hole which might be imaged in experiments. The interplay b…
We report the observation of coherent heteronuclear spin dynamics driven by inter-species spin-spin interaction in an ultracold spinor mixture, which manifests as periodical and well correlated spin oscillations between two atomic species. In particular, we investigate the magnetic field dependence of the oscillations and find a resonance behavior which depends on {\em both} the linear and quadratic Zeeman effects and the spin-dependent interaction. We also demonstrate a unique knob for controlling the spin dynamics in the spinor mixture with species-dependent vector light shifts. Our finds ar…
Formation Dynamics of Quantum Droplets for Homonuclear and Heteronuclear Mixtures
Instituto de Física, Universidade Federal do Rio Grande do Sul（南里奥格兰德联邦大学物理研究所）；Departamento de Psiquiatria, Universidade Federal do Rio Grande do Sul（南里奥格兰德联邦大学精神病学系）
We study the three-body problem of two ultracold identical bosonic atoms (denoted by $B$) and one extra atom (denoted by $X$), where the scattering length $a_{BX}$ between each bosonic atom and atom $X$ is resonantly large and positive. We calculate the scattering length $a_{\rm ad}$ between one bosonic atom and the shallow dimer formed by the other bosonic atom and atom $X$, and investigate the effect induced by the interaction between the two bosonic atoms. We find that even if this interaction is weak (i.e., the corresponding scattering length $a_{BB}$ is of the same order of the van der Wa…
We study the fate of an impurity in an ultracold heteronuclear Bose mixture, focusing on the experimentally relevant case of a $^{41}$K-$^{87}$Rb mixture, with the impurity in a $^{41}$K hyperfine state. Our work provides a comprehensive description of an impurity in a BEC mixture with contact interactions across its phase diagram. We present results for the miscible and immiscible regimes, as well as for the impurity in a self-bound quantum droplet. Here, varying the interactions, we find novel, exotic states where the impurity localizes either at the center or at the surface of the droplet.
We use an effective-field-theory framework to analyze the Efimov effect in heteronuclear three-body systems consisting of two species of atoms with a large interspecies scattering length. In the leading-order description of this theory, various three-body observables in heteronuclear mixtures can be universally parameterized by one three-body parameter. We present the next-to-leading corrections, which include the effects of the finite interspecies effective range and the finite intraspecies scattering length, to various three-body observables. We show that only one additional three-body param…
Temperature-Controlled Resonance in a Heteronuclear Quantum Gas Mixture
Xi'an Jiaotong University（西安交通大学）；Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (Guangdong)（粤港澳大湾区量子科学中心（广东））；Hefei National Laboratory（合肥国家实验室）
Ultracold atomic gases have recently become a driving force in few-body physics due to the observation of the Efimov effect. While initially observed in equal mass systems, one expects even richer few-body physics in the heteronuclear case. In previous experiments with ultracold mixtures of potassium and rubidium, an unexpected non-universal behavior of Efimov resonances was observed. In contrast, we measure the scattering length dependent three-body recombination coefficient in ultracold heteronuclear mixtures of $^{39}\mathrm{K}$-\87Rb and $^{41}\mathrm{K}$-\87Rb and do not observe any signa…
We use the zero-range approximation to study a system of two identical bosons interacting resonantly with a third particle. The method is derived from effective field theory. It reduces the three-body problem to an integral equation which we then solve numerically. We also develop an alternative approach which gives analytic solutions of the integral equation in coordinate representation in the limit of vanishing total energy. The atom-dimer scattering length, the rates of atom-dimer relaxation and three-body recombination to shallow and to deep molecular states are calculated either analytica…
Motivated by recent realizations of spin-1 NaRb mixtures in the experiments, here we investigate heteronuclear magnetism in the Mott-insulating regime. Different from the identical mixtures where the boson (fermion) statistics only admits even (odd) parity states from angular momentum composition, for heteronuclear atoms in principle all angular momentum states are allowed, which can give rise to new magnetic phases. Various magnetic phases can be developed over these degenerate spaces, however, the concrete symmetry breaking phases depend not only on the degree of degeneracy, but also the com…
We investigate the occurrence of Borromean three-body continuum s-wave resonances, in an $ααβ$ system for large negative two-body scattering lengths. The energy and width are determined by a scaling function with arguments given by energy ratios of the two-body virtual state subsystem energies with the shallowest three-body bound state. The Borromean continuum resonances emerging from Efimov states present a peculiar behavior for trapped ultracold atoms near a Feshbach resonance: two resonances with equal energies at different values of the scattering length. The corresponding three-body recom…
In this article, we revisit the heteronuclear Efimov effect in a Bose-Fermi mixture with large mass difference in the Born-Oppenheimer picture. As a specific example, we consider the combination of bosonic $^{133}\mathrm{Cs}$ and fermionic $^6\mathrm{Li}$. In a system consisting of two heavy bosons and one light fermion, the fermion-mediated potential between the two heavy bosons gives rise to an infinite series of three-body bound states. The intraspecies scattering length determines the three-body parameter and the scaling factor between consecutive Efimov states. In a second scenario, we re…
The Efimov effect in heteronuclear cold atomic systems is experimentally more easily accessible than the Efimov effect for identical atoms, because of the potentially smaller scaling factor. We focus on the case of two or three heavy identical bosons and another atom. The former case was recently observed in a mixture of 133Cs and 6Li atoms. We employ the Gaussian Expansion Method as developed by Hiyama, Kino et al.. This is a variational method that uses Gaussians that are distributed geometrically over a chosen range. Supplemental calculations are performed using the Skorniakov-Ter-Martirosi…
We investigate theoretically and experimentally the heteronuclear Efimov scenario for a three-body system that consists of two bosons and one distinguishable particle with positive intraspecies scattering lengths. The three-body parameter at the three-body scattering threshold and the scaling factor between consecutive Efimov resonances are found to be controlled by the scattering length between the two bosons, approximately independent of short-range physics. We observe two excited-state Efimov resonances in the three-body recombination spectra of an ultracold mixture of fermionic $^6 $Li and…
We discuss the stability of homonuclear and heteronuclear mixtures of 3He and 4He atoms in the metastable 2^3S_1 state (He*) and predict positions and widths of Feshbach resonances by using the Asymptotic Bound-state Model (ABM). All calculations are performed without fit parameters, using \emph{ab-initio} calculations of molecular potentials. One promising very broad Feshbach resonance (ΔB=72.9^{+18.3}_{-19.3} mT) is found that allows for tuning of the inter-isotope scattering length.
We study few-body problems in mixed dimensions with $N \ge 2$ heavy atoms trapped individually in parallel one-dimensional tubes or two-dimensional disks, and a single light atom travels freely in three dimensions. By using the Born-Oppenheimer approximation, we find three- and four-body bound states for a broad region of heavy-light atom scattering length combinations. Specifically, the existence of trimer and tetramer states persist to negative scattering lengths regime, where no two-body bound state is present. These few-body bound states are analogous to the Efimov states in three dimensio…
Hyperfine-changing collisions are of fundamental interest for the studying of ultracold heteronuclear mixtures. Here, we report the state-to-state study of the hyperfine-changing-collision dynamics in a Bose-Fermi mixture of $^6$Li and $^{41}$K atoms. The collision products are directly observed and the spin-changing dynamics is measured. Based on a two-body collision model, the experimental results are simultaneously fitted from which the spin-changing rate coefficient of $ 1.9(2)\times 10^{-12}~\rm{cm^3\cdot s^{-1}}$ is gained, being consistent with the multi-channel quantum defect theory ca…
We calculate the universal spectrum of trimer and tetramer states in heteronuclear mixtures of ultracold atoms with different masses in the vicinity of the heavy-light dimer threshold. To extract the energies, we solve the three- and four-body problem for simple two- and three-body potentials tuned to the universal region using the Gaussian expansion method. We focus on the case of one light particle of mass $m$ and two or three heavy bosons of mass $M$ with resonant heavy-light interactions. We find that trimer and tetramer cross into the heavy-light dimer threshold at almost the same point a…
We investigate a mixture of ultracold fermionic $^{40}$K atoms and weakly bound $^{6}$Li$^{40}$K dimers on the repulsive side of a heteronuclear atomic Feshbach resonance. By radio-frequency spectroscopy we demonstrate that the normally repulsive atom-dimer interaction is turned into a strong attraction. The phenomenon can be understood as a three-body effect in which two heavy $^{40}$K fermions exchange the light $^{6}$Li atom, leading to attraction in odd partial-wave channels (mainly p-wave). Our observations show that mass imbalance in a fermionic system can profoundly change the character…
The multichannel Efimov physics is investigated in ultracold heteronuclear admixtures of K and Rb atoms. We observe a shift in the scattering length where the first atom-dimer resonance appears in the $^{41}$K-$^{87}$Rb system relative to the position of the previously observed atom-dimer resonance in the $^{40}$K-$^{87}$Rb system. This shift is well explained by our calculations with a three-body model including the van der Waals interactions, and, more importantly, the multichannel spinor physics. With only minor difference in the atomic masses of the admixtures, the shift in the atom-dimer …
Recent measurements of Efimov resonances in a number of ultracold atom species have revealed an unexpected universality, in which three-body scattering properties are determined by the van der Waals length of the two-body interaction potential. To investigate whether this universality extends to heteronuclear mixtures, we measure loss rate coefficients in an ultracold trapped gas of $^{40}$K and $^{87}$Rb atoms. We find an Efimov-like resonance in the rate of inelastic collisions between $^{40}$K$^{87}$Rb Feshbach molecules and $^{87}$Rb atoms. However, we do not observe any Efimov-related res…
We report on the first realization of heteronuclear dipolar quantum mixtures of highly magnetic erbium and dysprosium atoms. With a versatile experimental setup, we demonstrate binary Bose-Einstein condensation in five different Er-Dy isotope combinations, as well as one Er-Dy Bose-Fermi mixture. Finally, we present first studies of the interspecies interaction between the two species for one mixture.
We have investigated self-bound binary ultra dilute bosonic mixtures at zero temperature within Density Functional Theory using a Local Density Approximation. We provide the explicit expression of the Lee-Huang-Yang correction in the general case of heteronuclear mixtures, and investigate the general thermodynamic conditions which lead to the formation of self-bound systems. We have determined the conditions for stability against the evaporation of one component, as well as the mechanical and diffusive spinodal lines. We have also calculated the surface tension of the self-bound state as a fun…
We report on the observation of heteronuclear magnetic Feshbach resonances in several isotope mixtures of the highly magnetic elements erbium and dysprosium. Among many narrow features, we identify two resonances with a width greater than one Gauss. We characterize one of these resonances, in a mixture of $^{168}$Er and $^{164}$Dy, in terms of loss rates and elastic cross section, and observe a temperature dependence of the on-resonance loss rate suggestive of a universal scaling associated with broad resonances. Our observations hold promise for the use of such a resonance for tuning the inte…
First-order phase transition in atom-molecule quantum degenerate mixtures with coherent three-body recombination
Missouri University of Science and Technology（密苏里科技大学）；Ben-Gurion University of the Negev（内盖夫本古里安大学）；Harvard & Smithsonian（哈佛大学与史密森尼学会）；University of Chicago（芝加哥大学）
We have studied the three-body recombination rates on both sides of the interspecies d-wave Feshbach resonance in the $^{85}$Rb\,-$^{87}$Rb-$^{87}$Rb system using the $R$-matrix propagation method in the hyperspherical coordinate frame. Two different mechanisms of recombination rate enhancement for positive and negative $^{85}$Rb\,-$^{87}$Rb d-wave scattering lengths are analyzed. On the positive scattering length side, the recombination rate enhancement occurs due to the existence of three-body shape resonance, while on the negative scattering length side, the coupling between the lowest entr…
We consider a heteronuclear fermionic mixture on the molecular side of an interspecies Feshbach resonance and discuss atom-dimer scattering properties in uniform space and in the presence of an external confining potential, restricting the system to a quasi-2D geometry. We find that there is a peculiar atom-dimer p-wave resonance which can be tuned by changing the frequency of the confinement. Our results have implications for the ongoing experiments on Lithium-Potassium mixtures, where this mechanism allows for switching the p-wave interaction between a K atom and Li-K dimer from attractive t…
Magnetic Feshbach resonances have allowed great success in the production of ultracold diatomic molecules from bi-alkali mixtures, but have so far eluded observation in mixtures of alkali and alkaline-earth-like atoms. Inelastic collisional properties of ultracold atomic systems exhibit resonant behavior in the vicinity of such resonances, providing a detection signature. We study magnetic field dependent inelastic effects via atom loss spectroscopy in an ultracold heteronuclear mixture of alkali $^6$Li in the ground state and alkaline-earth-like $^{174}$Yb in an excited electronic metastable …
We study Efimov resonances via three-body loss in an ultracold two-component gas of fermionic $^6$Li and bosonic $^{133}$Cs atoms close to a Feshbach resonance at 843~G, extending results reported previously [Pires \textit{et al.}, Phys. Rev. Lett. 112, 250404 (2014)] to temperatures around 120~nK. The experimental scheme for reaching lower temperatures is based upon compensating the gravity-induced spatial separation of the mass-imbalanced gases with bichromatic optical dipole traps. We observe the first and second excited Li-Cs-Cs Efimov resonance in the magnetic field dependence of the thre…
In few-body physics, Efimov states are an infinite series of three-body bound states that obey universal discrete scaling symmetry when pairwise interactions are resonantly enhanced. Despite abundant reports of Efimov states in recent cold atom experiments, direct observation of the discrete scaling symmetry remains an elusive goal. Here we report the observation of three consecutive Efimov resonances in a heteronuclear Li-Cs mixture near a broad interspecies Feshbach resonance. The positions of the resonances closely follow a geometric series $1$, $λ$, $λ^2$. The observed scaling constant $λ_…
We study three-body recombination in an ultracold Bose-Fermi mixture. We first show theoretically that, for weak inter-species coupling, the loss rate is proportional to Tan's contact. Second, using a 7 Li/ 6 Li mixture we probe the recombination rate in both the thermal and dual superfluid regimes. We find excellent agreement with our model in the BEC-BCS crossover. At unitarity where the fermion-fermion scattering length diverges, we show that the loss rate is proportional the 4/3 power of the fermionic density. Our results demonstrate that impurity-induced losses can be used as a quantitati…
The preparation of a quantum degenerate gas of heteronuclear molecules has been an outstanding challenge. We use path integral Quantum Monte Carlo simulations to understand the role of interactions and finite temperature effects in the protocol currently employed to adiabatically prepare a low-entropy gas of polar molecules in a lattice starting from an ultracold Bose-Fermi mixture. We find that interspecies interactions affect the final temperature of the mixture after the adiabatic loading procedure and detrimentally limit the molecular peak filling. Our conclusions are in agreement with rec…
We observe two consecutive heteronuclear Efimov resonances in an ultracold Li-Cs mixture by measuring three-body loss coefficients as a function of magnetic field near a Feshbach resonance. The first resonance is detected at a scattering length of $a_-^{(1)}=-320(10)~a_0$ corresponding to $\sim 7 $ ($\sim 3$) times the Li-Cs (Cs-Cs) van der Waals range. The second resonance appears at $5.8(1.0) a_-^{(1)}$ close to the unitarity-limited regime at the sample temperature of 450 nK. Indication of a third resonance is found in the atom loss spectra. The scaling of the resonance positions is close t…
We experimentally and theoretically study the effect of the intraspecies scattering length onto the heteronuclear Efimov scenario, following up on our earlier observation of Efimov resonances in an ultracold Cs-Li mixture for negative [Pires et al., Phys. Rev. Lett. 112, 250404 (2014)] and positive Cs-Cs scattering length [Ulmanis et al., Phys. Rev. Lett. 117, 153201 (2016)]. Three theoretical models of increasing complexity are employed to quantify its influence on the scaling factor and the three-body parameter: a simple Born-Oppenheimer picture, a zero-range theory, and a spinless van der W…
In the systems of spin $\frac12$ fermions with resonant $S$-wave interactions supporting only weakly bound dimers the antisymmetry forbids recombination of three (or more) fermions at zero energy. However, the fermion-fermion-dimer recombination is only partially suppressed. It is studied in the framework of momentum-space integral equations for the four-particle transition operators. In the vicinity of the unitary limit the fermion-fermion-dimer recombination rate, rescaled to build dimensionless quantity, is found to be linear in the effective range parameter, enabling a simple and accurate …
We report on the dynamical formation of self-bound quantum droplets in attractive mixtures of $^{39}$K atoms. Considering the experimental observations of Semeghini et al., Phys. Rev. Lett. 120, 235301 (2018), we perform numerical simulations to understand the relevant processes involved in the formation of a metastable droplet from an out-of-equilibrium mixture. We first analyze the so-called self-evaporation mechanism, where the droplet dissipates energy by releasing atoms, and then we consider the effects of losses due to three-body recombinations and to the balancing of populations in the …
We report on the observation of unusually strong interactions in a thermal mixture of ultracold atoms which cause a significant modification of the spatial distribution. A mixture of $^{87}$Rb and $^{174}$Yb with a temperature of a few $μ$K is prepared in a hybrid trap consisting of a bichromatic optical potential superimposed on a magnetic trap. For suitable trap parameters and temperatures, a spatial separation of the two species is observed. We infer that the separation is driven by a large interaction strength between $^{174}$Yb and $^{87}$Rb accompanied by a large three-body recombination…
We derive exact general relations between various observables for N bosons with zero-range interactions, in two or three dimensions, in an arbitrary external potential. Some of our results are analogous to relations derived previously for two-component fermions, and involve derivatives of the energy with respect to the two-body s-wave scattering length a. Moreover, in the three-dimensional case, where the Efimov effect takes place, the interactions are characterized not only by a, but also by a three-body parameter R\_t. We then find additional relations which involve the derivative of the ene…
We report the production of quantum degenerate Bose-Bose mixtures of Cs and Yb with both attractive (Cs + $^{174}$Yb) and repulsive (Cs + $^{170}$Yb) interspecies interactions. Dual-species evaporation is performed in a bichromatic optical dipole trap that combines light at 1070 nm and 532 nm to enable control of the relative trap depths for Cs and Yb. Maintaining a trap which is shallower for Yb throughout the evaporation leads to highly efficient sympathetic cooling of Cs for both isotopic combinations at magnetic fields close to the Efimov minimum in the Cs three-body recombination rate at …
A new narrow 3-atom loss resonance associated with an Efimov trimer crossing the 3-atom threshold has recently been discovered in a many-body system of ultracold 6Li atoms in the three lowest hyperfine spin states at a magnetic field near 895 G. O'Hara and coworkers have used measurements of the 3-body recombination rate in this region to determine the complex 3-body parameter associated with Efimov physics. Using this parameter as the input, we calculate the universal predictions for the spectrum of Efimov states and for the 3-body recombination rate in the universal region above 600 G where …
We present an exploratory study that suggests that Efimov physics, a leading research theme in few-body quantum physics, can also induce stable many-body ground states whose building blocks are universal clusters. We identify a range of parameters in a mass-and-density imbalanced two-species fermionic mixture for which the ground state is a gas of Efimov-related universal trimers. An explicit calculation of the trimer-trimer interaction reveals that the trimer phase is an SU$(3)$ Fermi liquid stable against recombination losses. We propose to experimentally observe this phase in a fermionic $^…
Tunable state-dependent interactions in collisionally stable mixtures of polar molecules
Institute for Molecules and Materials, Radboud University（分子与材料研究所，拉德堡德大学）；Institut für Theoretische Physik, Universität Heidelberg（理论物理研究所，海德堡大学）；Institute for Quantum Electronics, ETH Zürich（量子电子学研究所，苏黎世联邦理工学院）
We analyze the collision of three particles with arbitrary mass ratio at zero collision energy, assuming arbitrary short-range potentials, and generalize the three-body scattering hypervolume $D$ first defined for identical bosons in 2008. We solve the three-body Schrödinger equation asymptotically when the three particles are far apart or one pair and a third particle are far apart, deriving two asymptotic expansions of the wave function, and the parameter $D$ appears at the order $1/B^4$, where $B$ is the overall size of the triangle formed by the particles. We then analyze the ground state …
