Simulations of photon propagation in scintillation detectors were performed with the aim to find the optimal scintillator geometry, surface treatment, and shape of external reflector in order to achieve maximum light collection efficiency for detector configurations that avoid direct optical coupling, a situation that is commonly found in cryogenic scintillating bolometers in experimental searches for double beta decay and dark matter. To evaluate the light collection efficiency of various geometrical configurations we used the ZEMAX ray-tracing software. It was found that scintillators in the shape of a triangular prism with an external mirror shaped as truncated cone gives the highest light collection efficiency. The results of the simulations were confirmed by carrying out measurements of the light collection efficiencies of CaWO4 crystal scintillators. A comparison of simulated and measured values of light output shows good agreement
Cryogenic phonon-scintillation detectors (CPSD) for rare event search experiments require reliable, efficient and robust photon detectors that can resolve individual photons in a scintillation event.
This paper is the first report of n-type GaAs as a cryogenic scintillation radiation detector for the detection of electron recoils from interacting dark matter (DM) particles in the poorly explored MeV/c2 mass range. Seven GaAs samples from two commercial suppliers and with different silicon and boron concentrations were studied for their low temperature optical and scintillation properties. All samples are n-type even at low temperatures and exhibit emission between silicon donors and boron acceptors that peaks at 1.33 eV (930 nm). The lowest excitation band peaks at 1.44 eV (860 nm) and the…
In this work we present an elegant solution for a scintillation counter to be integrated into a cryogenic system. Its distinguishing feature is the absence of a continuous light guide coupling the scintillation and the photodetector parts, operating at cryogenic and room temperatures respectively. The prototype detector consists of a plastic scintillator with glued-in wavelength-shifting fiber located inside a cryostat, a Geiger-mode Avalanche Photodiode (G-APD) outside the cryostat, and a lens system guiding the scintillation light re-emitted by the fiber to the G-APD through optical windows …
We have studied the scintillation of pure and doped sodium iodide crystals handled in low humidity conditions under external $α$ and $γ$ excitation from room temperature down to 4K. The light yield of pure sodium iodide was seen to increase at low temperatures by a factor 30 compared to room temperature, up to a maximum of 40 photons/keV under $γ$ excitation at 60K, stabilizing to 30 photons/keV at lower temperatures. Thallium doped sodium iodide fluctuates by 20% around the room temperature value, stabilizing at 40 photons/keV at low temperature. $α/ γ$ quenching factor stabilizes at roughly …
The high scintillation luminosity of n-type GaAs at 10K is surprising because (1) with a refractive index of about 3.5, escape is inhibited by total internal reflection and (2) narrow-beam experiments at 90K report infrared absorption coefficients of several per cm. This paper presents Monte Carlo calculations showing that the high luminosity at 10K can be explained if (1) narrow-beam absorption is almost all optical scattering and (2) the absolute absorption coefficient is below 0.1 per cm. Sixteen surface reflector configurations are simulated for a range of internal scattering and absolute …
Presented here are first tests of a Gaseous Photomultiplier based on a cascade of Thick GEM structures intended for gamma-ray position reconstruction in liquid Argon. The detector has a MgF$_2$ window, transparent to VUV light, and a CsI photocathode deposited on the first THGEM. A gain of $8\cdot10^{5}$ per photoelectron and $\sim100\%$ photoelectron collection efficiency are measured at stable operation settings. The excellent position resolution capabilities of the detector (better than 100 $μ$m) at 100 kHz readout rate, is demonstrated at room temperature. Structural integrity tests of the…
High light collection efficiency is an important requirement in any application of scintillation detectors. The purpose of this study is to investigate the possibility for improving this parameter in cryogenic scintillation bolometers, which can be considered as a promising detectors in experiments investigating neutrinoless double beta decay and dark matter. Energy resolutions and relative pulse amplitudes of scintillation detectors using ZnWO4 scintillation crystals of different shapes (cylinder 20 mm in dimater by 20 mm and hexagonal prism with diagonal 20 mm and height 20 mm), reflector ma…
Caesium iodide is one of the more extensively studied scintillators. Here we present X-ray luminescence spectra, scintillation light output and decay curves as function of temperature, from room temperature down to below 10 K. Features of the observed intrinsic luminescence are explained in terms of radiative recombination of on- and off-centre STE. A model permitting interpretation of the dynamics of luminescence changes in CsI with temperature is suggested. This model includes adiabatic potential energy surfaces (APES) associated with singlet and triplet states of self-trapped excitons (STE)…
We have developed a detector, consisting of a cryogenic calorimeter with a scintillating crystal as absorber, and a second calorimeter for the detection of the scintillation light, both operated at 12 mK. Using a CaWO4 crystal with a mass of 6g as scintillating absorber, we have achieved a discrimination of nuclear recoils against electron recoils with a suppression factor of 99.7% at energies above 15 keV. This novel method will be applied for background rejection in the CRESST (Cryogenic Rare Event Search with Superconducting Thermometers) experiment looking for dark matter Weakly Interactin…
Scintillation at cryogenic temperatures can give rise to detectors with particle discrimination for rare-event searches such as dark matter detection. We present time-resolved scintillation studies of Caesium Iodide (CsI) under excitation of both alpha and gamma particles over a long acquisition window of 1 ms to fully capture the scintillation decay between room temperature and 4 K. This allows a measurement of the light yield independent of any shaping time of the pulse. We find the light yield of CsI to increase up to two orders of magnitude from that of room temperature at cryogenic temper…
Scintillation response of cryogenic CsI to few-keV and sub-keV nuclear recoils
University of Chicago（芝加哥大学）；Donostia International Physics Center (DIPC)（多诺西亚国际物理中心）；Ikerbasque, Basque Foundation for Science（伊克尔巴斯基克，巴斯克科学基金会）；Instituto de Física Corpuscular, CSIC & Universitat de València（粒子物理研究所，西班牙国家科学研究委员会与瓦伦西亚大学）
The scintillation yield for recoil Ar ions of 5 to 250 keV energy in liquid argon have been evaluated for direct dark matter searches. Lindhard theory is taken for estimating nuclear quenching. A theoretical model based on a biexcitonic diffusion-reaction mechanism is performed for electronic (scintillation) quenching. The electronic LET (linear energy transfer) is evaluated and used to obtain the initial track structure due to recoil Ar ions. The results are compared with experimental values reported for nuclear recoils from neutrons. The behavior of scintillation and ionization on the field …
The bright scintillation of pure CsI operated at liquid-nitrogen temperature makes of this material a promising dark matter and neutrino detector. We present the first measurement of its quenching factor for nuclear recoils. Our findings indicate it is indistinguishable from that for sodium-doped CsI at room temperature. Additional properties such as light yield, afterglow, scintillation decay properties for electron and nuclear recoils, and energy proportionality are studied over the \mbox{108-165 K} temperature range, confirming the vast potential of this medium for rare-event searches.
Characteristic properties of a Geiger Mode APD (G-APD) in a THGEM-based cryogenic two-phase Ar avalanche detector were studied in view of potential applications in rare-event experiments. G-APD signal amplitude and noise characteristics at cryogenic temperatures turned out to be superior to those at room temperature. The effective detection of avalanche scintillations from THGEM-multiplier holes in two-phase Ar has been demonstrated using a G-APD without wavelength shifter. At an avalanche gain of 60, the avalanche scintillation yield measured by the G-APD was as high as 0.9 photoelectrons per…
Liquid Xe TPCs are among the most popular choices for double beta decay and WIMP dark matter searches. Gaseous Xe has intrinsic advantages when compared to Liquid Xe, specifically, tracking capability and better energy resolution for double beta decay searches. The performance of gaseous Xe can be further improved by molecular additives such as trimethylamine(TMA), which are expected to (1) cool down the ionization electrons, (2) convert Xe excitation energy to TMA ionizations through Penning transfer, and (3) produce scintillation and electroluminescence light in a more easily detectable wave…
The gaseous Xenon(Xe) time projection chamber (TPC) is an attractive detector technique for neutrinoless double beta decay and WIMP dark matter searches. While it is less dense compared to Liquid Xe detectors, it has intrinsic advantages in tracking capability and better energy resolution. The performance of gaseous Xe can be further improved by molecular additives such as trimethylamine(TMA), which is expected to (1) cool down the ionization electrons, (2) convert Xe excitation energy to TMA ionizations through Penning transfer, and (3) produce scintillation and electroluminescence light in a…
Liquid xenon-based direct detection dark matter experiments have recently expanded their searches to include high-energy nuclear recoil events as motivated by effective field theory dark matter and inelastic dark matter interaction models, but few xenon recoil calibrations above 100 keV are currently available. In this work, we measured the scintillation and ionization yields of xenon recoils up to 426 keV. The experiment uses 14.1 MeV neutrons to scatter off xenon in a compact liquid xenon time projection chamber and produce quasi-monoenergetic xenon recoils between 39 keV and 426 keV. We rep…
In this paper we report on measurements of the effects of dissolved methane upon argon scintillation light. We monitor the light yield from an alpha source held 20 cm from a cryogenic photomultiplier tube (PMT) assembly as methane is injected into a high-purity liquid argon volume. We observe significant suppression of the scintillation light yield by dissolved methane at the 10 part per billion (ppb) level. By examining the late scintillation light time constant, we determine that this loss is caused by an absorption process and also see some evidence of methane-induced scintillation quenchin…
The hidden sector photon is a weakly interacting hypothetical particle with sub-eV mass that kinetically mixes with the photon. We describe a microwave frequency light shining through a wall experiment where a cryogenic resonant microwave cavity is used to try and detect photons that have passed through an impenetrable barrier, a process only possible via mixing with hidden sector photons. For a hidden sector photon mass of 53 $μ$eV we limit the hidden photon kinetic mixing parameter $χ< 1.7\times10^{-7}$, which is an order of magnitude lower than previous bounds derived from cavity experiment…
The MicroBooNE detector, to be located on axis in the Booster Neutrino Beamline (BNB) at the Fermi National Accelerator Laboratory (Fermilab), consists of two main components: a large liquid argon time projection chamber (LArTPC), and a light collection system. Thirty 8-inch diameter Hamamatsu R5912-02mod cryogenic photomultiplier tubes (PMTs) will detect the scintillation light generated in the liquid argon (LAr). This article first describes the MicroBooNE PMT performance test procedures, including how the light collection system functions in the detector, and the design of the PMT base. The…
Compelling experimental evidences of neutrino oscillations and their implication that neutrinos are massive particles have given neutrinoless double beta decay a central role in astroparticle physics. In fact, the discovery of this elusive decay would be a major breakthrough, unveiling that neutrino and antineutrino are the same particle and that the lepton number is not conserved. It would also impact our efforts to establish the absolute neutrino mass scale and, ultimately, understand elementary particle interaction unification. All current experimental programs to search for neutrinoless do…
Detection of light signals is crucial to a wide range of particle detectors. In particular, efficient detection of vacuum ultraviolet (VUV) light will provide new opportunities for some novel detectors currently being developed, but is technically challenging. In this article, we characterized the performance of Hamamatsu VUV4 silicon photomultipliers (SiPMs) for detecting VUV argon scintillation light without wavelength shifting. Using a customized cryogenic amplifier design, we operated two models of VUV4 SiPMs inside liquid argon and thoroughly examined their direct sensitivities to liquid …
Detectors for direct dark matter search using noble gases in liquid phase as detection medium need to be coupled to liquefaction, purification and recirculation systems. A dedicated cryogenic system has been assembled and operated at the INFN-Naples cryogenic laboratory with the aim to liquefy and purify the argon used as active target in liquid argon detectors to study the scintillation and ionization signals detected by large SiPMs arrays. The cryogenic system is mainly composed of a double wall cryostat hosting the detector, a purification stage to reduce the impurities below one part per b…
Detection of the vacuum ultraviolet (VUV) scintillation light produced by liquid noble elements is a central challenge in order to fully exploit the available timing, topological, and calorimetric information in detectors leveraging these media. In this paper, we characterize a novel, windowless amorphous selenium based photodetector with direct sensitivity to VUV light. We present here the manufacturing and experimental setup used to operate this detector at low transport electric fields (2.7-5.2 V/$μ$m) and across a wide range of temperatures (77K-290K). This work shows that the first proof-…
In prospect of its application in cryogenic rare-event searches, we have investigated the low-temperature scintillation properties of CaWO4 crystals down to 3.4 K under α and γ excitation. Concerning the scintillation decay times, we observe a long component in the ms range which significantly contributes to the light yield below 40K. For the first time we have measured the temperature dependence of the α/γ- ratio of the light yield. This parameter which can be used to discriminate α and γ events in scintillating bolometers is found to be about 8-15% smaller at low temperatures compared to roo…
ProtoDUNE-DP is a 6x6x6 m3 liquid argon time-projection-chamber (LArTPC) operated at the Neutrino Platform at CERN in 2019-2020 as a prototype of the DUNE Far Detector. DUNE is a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. The light signal in these detectors is crucial to provide precise timing capabilities. In ProtoDUNE-DP, scintillation light produced by cosmic muons inthe LArTPC is collected by the photomultiplier tubes (PMTs) placed up to 7 m away from the point of interaction. The scintillation light production and…
A novel experiment for direct searches of the Dark Matter with liquid argon double-phase chamber with a mass of liquid Ar up to several hundred tons is proposed. To suppress the b-, g- and n0- backgrounds, the comparison of scintillation and ionization signals for every event is suggested. The addition in liquid Ar of photosensitive Ge(CH3)4 or C2H4 and suppression of triplet component of scintillation signals ensures the detection of scintillation signals with high efficiency and provides a complete suppression of the electron background. For the detection of photoelectrons and ionization ele…
The energy threshold of a cryogenic calorimeter can be lowered by reducing its size. This is of importance since the resulting increase in signal rate enables new approaches in rare-event searches, including the detection of MeV mass dark matter and coherent scattering of reactor or solar neutrinos. A scaling law for energy threshold vs. detector size is given. We analyze the possibility of lowering the threshold of a gram-scale cryogenic calorimeter to the few eV regime. A prototype 0.5 g Al$_2$O$_3$ device achieved an energy threshold of (${19.7\pm0.1}$) eV, the lowest value reported for a m…
We discuss recent advances in the development of cryogenic gaseous photomultipliers (GPM), for possible use in dark matter and other rare-event searches using noble-liquid targets. We present results from a 10 cm diameter GPM coupled to a dual-phase liquid xenon (LXe) TPC, demonstrating - for the first time - the feasibility of recording both primary ("S1") and secondary ("S2") scintillation signals. The detector comprised a triple Thick Gas Electron Multiplier (THGEM) structure with cesium iodide photocathode on the first element; it was shown to operate stably at 180 K with gains above 10^5,…
Molybdenum based crystals such as Li$_2$MoO$_4$ and CaMoO$_4$ are emerging as leading candidates for next generation experiments searching for neutrino-less double beta decay with cryogenic calorimeters (CUPID, AMoRE). The exquisite energy resolution and high radio-purity of these crystals come at the cost of a potentially detrimental background source: the two neutrinos double beta decay of $^{100}$Mo. Indeed, the fast half-life of this decay mode, combined with the slow response of cryogenic calorimeters, would result in pile-up events in the energy region of interest for neutrino-less doubl…
Scintillation Properties of a Stilbene Crystal for Low-Mass Dark Matter Searches
Jeju National University（济州国立大学）；Kyungpook National University（庆北国立大学）；Center for Underground Physics, Institute for Basic Science (IBS)（基础科学研究院地下物理中心）；Yemilab Operation Center, Institute for Basic Science (IBS)（基础科学研究院Yemilab运营中心）
We report on a measurement of the absorption length of scintillation light in liquid argon due to dissolved nitrogen at the part-per-million (ppm) level. We inject controlled quantities of nitrogen into a high purity volume of liquid argon and monitor the light yield from an alpha source. The source is placed at different distances from a cryogenic photomultiplier tube assembly. By comparing the light yield from each position we extract the absorption cross section of nitrogen. We find that nitrogen absorbs argon scintillation light with strength of $(1.51\pm 0.15)\times10^{-4} \;\mathrm{cm^{-…
Simulation studies have been carried out to explore the ability to discriminate between single-site and multi-site energy depositions in large scale liquid scintillation detectors. A robust approach has been found that is predicted to lead to a significant statistical separation for a large variety of event classes, providing a powerful tool to discriminate against backgrounds and break important degeneracies in signal extraction. This has particularly relevant implications for liquid scintillator searches for neutrinoless double beta decay ($0νββ$) from $^{130}$Te and $^{136}$Xe, where it is …
New Cryogenic Avalanche Detector (CRAD) with ultimate sensitivity, that will be able to detect one primary electron released in the cryogenic liquid, is under development in the Laboratory of Cosmology and Particle Physics of the Novosibirsk State University jointly with the Budker Institute of Nuclear Physics. The CRAD will use two sets of cryogenic PMTs in order to get trigger signal either from primary scintillations in liquid Ar or from secondary scintillations in high field gap above the liquid. Two types of cryogenic PMTs produced by Hamamatsu Photonics were tested and the results are pr…
We present here a comprehensive study of the light yield of primary and secondary scintillations produced in gaseous and liquid Ar in the near infrared (NIR) and visible region, at cryogenic temperatures. The measurements were performed using Geiger-mode avalanche photodiodes (GAPDs) and pulsed X-ray irradiation. The primary scintillation yield of the fast emission component in gaseous Ar was found to be independent of temperature in the range of 87-160 K; it amounted to 17000+/-3000 photon/MeV in the NIR in the range of 690-1000 nm. In liquid Ar at 87 K, the primary scintillation yield of the…
In this work we report the realization of the first low-threshold cryogenic detector that uses diamond as absorber for astroparticle physics applications. We tested two 0.175$\,$g CVD diamond samples, each instrumented with a W-TES. The sensors showed transitions at about 25 mK. We present the performance of the diamond detectors and we highlight the best performing one, where we obtained an energy threshold as low as 16.8 eV. This promising result lays the foundation for the use of diamond for different fields of applications where low threshold and excellent energy resolution are required, a…
A new type of the Multi-Pixel Photon Counter (MPPC), sensitive to Vacuum Ultra-Violet (VUV) light (wavelength λ < 150 nm), is recently developed and produced by Hamamatsu Photonics K.K. The basic properties of the new MPPC are measured at cryogenic facility of Waseda university using liquid nitrogen. Temperature dependence of breakdown voltage, capacitance, and dark count rate of the MPPC are also evaluated. In addition, the absolute photon detection efficiency (PDE) for liquid argon (LAr) scintillation light (λ = 128 nm) is estimated to be about 7% with uncertainty of 2% by using 241 Am α-ray…
Recently there is a flourishing and notable interest in the crystalline scintillator material sodium iodide (NaI) as target for direct dark matter searches. This is mainly driven by the long-reigning contradicting situation in the dark matter sector: the positive evidence for the detection of a dark matter modulation signal claimed by the DAMA/LIBRA collaboration is (under so-called standard assumptions) inconsistent with the null-results reported by most of the other direct dark matter experiments. We present the results of a first prototype detector using a new experimental approach in compa…
The use of xenon-doped liquid argon is a promising alternative for large pure liquid-argon TPCs. Not only xenon-doped liquid argon enhances the light production, mitigating the possible suppression due to impurities, but also it increases the wavelength of the scintillation light, enlarging the effective Rayleigh scattering length and improving the detection uniformity. ProtoDUNE Dual-Phase is a 300-ton active volume LAr TPC, a prototype for the Deep Underground Neutrino Experiment (DUNE), a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon …
We report a demonstration of the scalability of optically transparent xenon in the solid phase for use as a particle detector above a kilogram scale. We employ a liquid nitrogen cooled cryostat combined with a xenon purification and chiller system to measure the scintillation light output and electron drift speed from both the solid and liquid phases of xenon. Scintillation light output from sealed radioactive sources is measured by a set of high quantum efficiency photomultiplier tubes suitable for cryogenic applications. We observed a reduced amount of photons in solid phase compared to that…
The Deep Underground Neutrino Experiment (DUNE) is a leading-edge experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. ProtoDUNE-Dual Phase (DP) is a 6x6x6 m$^3$ liquid argon time-projection-chamber (LArTPC) operated at the CERN Neutrino Platform in 2019-2020 as a prototype of the DUNE Far Detector. In ProtoDUNE-DP, the scintillation and electroluminescence light produced by cosmic muons in the LArTPC is collected by photomultiplier tubes placed up to 7 m away from the ionizing track. In this paper, we present the performance of the Proto…
We present preliminary results of measurements of the quenching factor for Na recoils in NaI(Tl) at room temperature, made at a dedicated neutron facility at the University of Sheffield. Measurements have been performed with a 2.45 MeV mono-energetic neutron generator in the energy range from 10 keV to 100 keV nuclear recoil energy. A BC501A liquid scintillator detector was used to tag neutrons. Cuts on pulse-shape discrimination from the BC501A liquid scintillator detector and neutron time-of-flight were performed on pulses recorded by a digitizer with a 2 ns sampling time. Measured quenching…
Application of CaMoO4 as a scintillation target in cryogenic rare event searches relies on the understanding of scintillation properties of the material at the temperatures at which these detectors operate. We devised and implemented a detection module with a low-temperature photomultiplier from Hamamatsu (model R8520-06) powered by a Cockcroft-Walton generator. The detector module containing the CaMoO4 crystal was placed in a 3He/4He dilution refrigerator and used to measure scintillation characteristics of CaMoO4 in the millikelvin temperature range. At the lowest temperature achieved, the e…
A novel concept of optical signal recording in two-phase avalanche detectors, with Geiger-mode Avalanche Photodiodes (G-APD) is described. Avalanche-scintillation photons were measured in a thick Gas Electron Multiplier (THGEM) in view of potential applications in rare-event experiments. The effective detection of avalanche scintillations in THGEM holes has been demonstrated in two-phase Ar with a bare G-APD without wavelength shifter, i.e. insensitive to VUV emission of Ar. At gas-avalanche gain of 400 and under \pm 70^\circ viewing-angle, the G-APD yielded 640 photoelectrons (pe) per 60 keV …
Measuring the scintillation light in noble gases is an important detection technique in particle physics. Numerous rare event searches like neutrino beam experiments, neutrino-less double beta-decay, and dark matter searches use argon-based detectors. In liquid argon, the light yield can be enhanced by the addition of a small quantity of xenon, where $\sim 10 - 1000$ ppm are added. The general enhancement mechanism and its pathway via an energy transfer between argon and xenon excimers is well known, however the importance of absorption of argon excimer emission by atomic xenon has not been fu…
Liquid argon is being employed as a detector medium in neutrino physics and Dark Matter searches. A recent push to expand the applications of scintillation light in Liquid Argon Time Projection Chamber neutrino detectors has necessitated the development of advanced methods of simulating this light. The presently available methods tend to be prohibitively slow or imprecise due to the combination of detector size and the amount of energy deposited by neutrino beam interactions. In this work we present a semi-analytical model to predict the quantity of argon scintillation light observed by a ligh…
Applications that utilize scintillation detectors at low temperatures are growing in number. Many of these require materials with high light yield and a fast response. Here we report on the low-temperature characterisation of ZnSe doped with Al or Te, respectively. The X-ray luminescence and decay curves were measured over the 77- 295 K temperature range, and alpha particle excitation was used to examine scintillation light output and decay kinetics over the range 9-295 K. A significant improvement of the scintillation characteristics was observed at cooling below 100 K. The scintillation ligh…
Liquid noble based particle detectors often use the organic wavelength shifter 1,1,4,4- tetraphenyl-1,3-butadiene (TPB) which shifts UV scintillation light to the visible regime, facilitating its detection, but which also can scintillate on its own. Dark matter searches based on this type of detector commonly rely on pulse-shape discrimination (PSD) for background mitigation. Alpha-induced scintillation therefore represents a possible background source in dark matter searches. The timing characteristics of this scintillation determine whether this background can be mitigated through PSD. We ha…
Large liquid-scintillator-based detectors have proven to be exceptionally effective for low energy neutrino measurements due to their good energy resolution and scalability to large volumes. The addition of directional information using Cherenkov light and fast timing would enhance the scientific reach of these detectors, especially for searches for neutrino-less double-beta decay. In this paper, we develop a technique for extracting particle direction using the difference in arrival times for Cherenkov and scintillation light, and evaluate several detector advances in timing, photodetector sp…
