Spatial phase separation into mesoscopic domains of non-magnetic [superconducting (SC) below Tc = 25.5 K] and two kinds of magnetic phases, one showing disordered spin density wave (d-SDW) order and another associated with glassy weak magnetism (WM), are observed below ~100 K by muon spin rotation (muSR) in LaFeAsO1-xFx for x = 0.057(3) which is near the boundary of these phases on the doping phase diagram. In contrast to the competing order observed in the regular SDW phase of Ba(Fe1-xCox)2As2, the WM domain exhibits cooperative coupling of superconducting and magnetic order parameters as inferred from strong diamagnetism and associated negative shift of muSR frequency just below Tc.
Origin of doping-induced suppression and reemergence of magnetism in LaFeAsO$_{1-x}$H$_x$
利用动力学平均场理论结合密度泛函理论研究了铁基超导体LaFeAsO $_{1-x}$ H $_x$中氢掺杂对磁性的影响.我们发现,两个独立的结果的掺杂,电子占据和结构修改的增加,有相反的影响的电子相关性和磁性的强度,导致在中间掺杂水平附近的计算磁矩的最小值作为$x$的函数。我们的结果提供了一个自然的解释,令人费解的最近实验发现的两个分离的反铁磁相在低和高掺杂限制。此外,随着掺杂量的增加,轨道占有率和关联强度的增加,导致$d_{xz/yz}$轨道极化率的降低和$d_{xy}$轨道在磁性中的作用的增强,并结合磁性的本质作用讨论了它们对超导性的可能影响.
A unified phase diagram of F-doped LaFeAsO by means of NMR and NQR parameters
我们目前$^{75}$作为核磁共振和四极共振结果(NMR,NQR)的一组新的LaFeAsO $_{1-x}$ F $_x$多晶样品。改进的合成条件导致更均匀的样品,更好地控制氟含量。结构$\equiv$的磁,超导转变温度已被确定的NMR自旋晶格弛豫率和交流磁化率测量。如此确定的相图偏离公布的一个,特别是低F掺杂浓度。然而,如果从NQR谱确定掺杂水平,则两个相图可以被调和。磁性和超导性的本体共存和纳米级分离成低掺杂样和高掺杂样区域的情况下,已被证实。在磁性和超导性的边界处对欠掺杂样品的附加频率依赖的强度、自旋-自旋和自旋-晶格弛豫率测量表明,正交性和磁性起源于低掺杂区,超导性首先在高掺杂区发展。
Doping dependence of Normal-state Property in the Iron-based Oxypnictide Superconductors LaFeAsO1-y probed by 57Fe-NMR and 75As-NMR/NQR
本文报道了贫氧铁基氧氮族化合物超导体LaFeAsO_{1-y} $. A microscopic phase separation between superconducting domains and magnetic domains is shown to take place in the underdoped sample, indicating a local inhomogeneity in association with the density distribution of oxygen deficiencies. As a result, 1/T_1T in the normal state of the superconducting domain decreases significantly upon cooling at both the Fe and As sites regardless of the electron-doping level in LaFeAsO_{1-y}. On the basis of this result, we claim that $ 1/T_1 T $ is not always enhanced by antiferromagnetic fluctuations close to an antiferromagn…
通过X射线衍射、电阻率、磁化率和热容的测量,研究了LaFe $_{1-x}$ Ni $_{x}$ AsO($0\leq x \leq0.1$)中Ni的替代效应。镍掺杂大大抑制了与自旋密度波有序在母体化合物的电阻率异常。超导电性出现在$0.03\leq x \leq0.06$的一个狭窄区域,在$x$ =0.04时,最大$T_c$为6.5 K,在此区域,磁化率增强。在零温度下的上临界场估计超过泡利顺磁极限。与LaFeAsO $_{1-x}$ F $_{x}$系统相比,$T_c$大大降低。
The intrinsic electronic phase diagram of iron-oxypnictide superconductors
我们提出了第一个全面的推导的铁氧铌酸盐超导体在正常状态下的电阻率$ρ$的LaFeAsO $_{1-x}$ F $_x$和SmFeAsO $_{1-x}$ F $_x$的掺杂范围宽的基础上的分析。我们的数据为这些新材料中不寻常的正常状态属性提供了明确的证据。特别地,在低掺杂水平下超导性的出现伴随着正常状态的$ρ$中的明显异常输运行为,这让人想起母体材料中的自旋密度波(SDW)特征。在较高的掺杂水平下,LaFeAsO $_{1-x}$ F $_x$的$ρ$显示出从这种赝隙状行为到费米液体状行为的明显转变,模仿了铜酸盐的相图。此外,我们的数据揭示了异常特征的强度和超导相的稳定性之间的相关性。在SmFeAsO $_{1-x}$ F $_x$中,超导电性增强,类赝隙特征增强,而在具有类费米液体行为的掺杂区,超导电性降低,类赝隙特征消失.
Cooperative effect of doping and temperature on the polaronic band structure in strongly correlated electron systems with strong electron-phonon interaction
Reentrant metallic transition at a temperature above Tc at the breakdown of cooperative Jahn-Teller orbital order in perovskite manganites
我们报告了一个有趣的重入金属电阻率图案超过一个特征温度T*,这是高于其他这样的特征转变温度,如T(c)(居里点),T(N)(Neel点),T(CO)(充电顺序开始点)或T(OO)(轨道序起始点)在稀土钙钛矿锰氧化物(RE(1-x)A(x)MnO(3); RE = La,Nd,Y; A = Sr,Ca; x = 0.0-0.5)范围内。这种行为通常在掺杂水平(x)高于出现金属基态所需的临界掺杂水平x(c)(= 0.17-0.22)的掺杂锰氧化物中观察到,因此在合作的Jahn-Teller轨道序已经发生击穿的系统中观察到。然而,在La(1-x)Ca(x)MnO(3)(x = 0.0-0.5)系列中所做的观察结果证明是这种总趋势的例外。
Reconfigurable flat bands from cooperative moiré and charge order
University of St Andrews(圣安德鲁斯大学);Diamond Light Source(钻石光源);Max Planck Institute for Chemical Physics of Solids(马克斯·普朗克固体化学物理研究所);Lund University(隆德大学)