We demonstrate that the spin decoherence of nitrogen vacancy (NV) centers in diamond can be suppressed by a transverse magnetic field if the electron spin bath is the primary decoherence source. The NV spin coherence, created in "a decoherence-free subspace" is protected by the transverse component of the zero-field splitting, increasing the spin-coherence time about twofold. The decoherence due to the electron spin bath is also suppressed at magnetic fields stronger than ~25 gauss when applied parallel to the NV symmetry axis. Our method can be used to extend the spin-coherence time of similar spin systems for applications in quantum computing, field sensing, and other metrologies.
Nitrogen-vacancy (NV) centers in diamond have become an important tool for quantum technologies. All of these applications rely on long coherence times of electron and nuclear spins associated with these centers. Here, we study the energy level anti-crossings of an NV center in diamond coupled to a first-shell 13C nuclear spin in a small static magnetic field. These level anti-crossings occur for specific orientations of the static magnetic field due to the strong non-secular components of the Hamiltonian. At these orientations we observe decoherence-free subspaces, where the electron spin coh…
Taming decoherence is essential in realizing quantum computation and quantum communication. Here we experimentally demonstrate that decoherence due to amplitude damping can be suppressed by exploiting quantum measurement reversal in which a weak measurement and the reversing measurement are introduced before and after the decoherence channel, respectively. We have also investigated the trade-off relation between the degree of decoherence suppression and the channel transmittance.
In this paper, we provide a mechanism of decoherence suppression for open quantum systems in general, and that for "Schrodinger cat-like" state in particular, through the strong couplings to non-Markovian reservoirs. Different from the usual strategies of suppressing decoherence by decoupling the system from the environment in the literatures, here the decoherence suppression employs the strong back-reaction from non-Markovian reservoirs. The mechanism relies on the existence of the singularities (bound states) of the nonequilibrium retarded Green function which completely determines the dissi…
The coherent behavior of the single electron and single nuclear spins of a defect center in diamond and a 13C nucleus in its vicinity, respectively, are investigated. The energy levels associated with the hyperfine coupling of the electron spin of the defect center to the 13C nuclear spin are analyzed. Methods of magnetic resonance together with optical readout of single defect centers have been applied in order to observe the coherent dynamics of the electron and nuclear spins. Long coherence times, in the order of microseconds for electron spins and tens of microseconds for nuclear spins, re…
We theoretically investigate spin decoherence of a single nitrogen-vacancy (NV) center in diamond. Using the spin coherent state P-representation method, coherence evolution of the NV center surrounded by nitrogen electron spins (N) is simulated. We find that spin decoherence time as well as free-induction decay of the NV center depend on the spatial configuration of N spins. Both the spin decoherence rate (1/T2) and dephasing rate (1/T2*) of the NV center increase linearly with the concentration of the N spins. Using the P-representation method, we also demonstrate extracting noise spectrum o…
Since there are many examples in which no decoherence-free subsystems exist (among them all cases where the error generators act irreducibly on the system Hilbert space), it is of interest to search for novel mechanisms which suppress decoherence in these more general cases. Drawing on recent work (quant-ph/0502153) we present three results which indicate decoherence suppression without the need for noiseless subsystems. There is a certain trade-off; our results do not necessarily apply to an arbitrary initial density matrix, or for completely generic noise parameters. On the other hand, our c…
The works on decoherence due to spin baths usually agree in studying a one-spin system in interaction with a large spin bath. In this paper we generalize those models by analyzing a many-spin system and by studying decoherence or its suppression in function of the relation between the numbers of spins of the system and the bath. This model may help to identify clusters of particles unaffected by decoherence, which, as a consequence, can be used to store quantum information.
We study the suppression of noise-induced phase decoherence in a single atomic qubit by employing pulse sequences. The atomic qubit is composed of a single neutral atom in a far-detuned optical dipole trap and the phase decoherence may originate from the laser intensity and beam pointing fluctuations as well as magnetic field fluctuations. We show that suitable pulse sequences may prolongate the qubit coherence time substantially as comparing to the conventional spin echo pulse.
A First-principles Computational Framework for Quantum Decoherence in Complex Diamond Spin Environments
Sungkyunkwan University（成均馆大学）；Ajou University（亚洲大学）；University of Chicago（芝加哥大学）；Korea Institute of Science and Technology（韩国科学技术院）；Korean Research Institute of Standards and Science（韩国计量科学研究院）；Ulm University（乌尔姆大学）；Korea University of Science and Technology（韩国科学技术院）；Argonne National Laboratory（阿贡国家实验室）
To protect a quantum system from decoherence due to interaction with its environment, we investigate the existence of initial states of the environment allowing for decoherence-free evolution of the system. For models in which a two-state system interacts with a dynamical environment, we prove that such states exist if and only if the interaction and self-evolution Hamiltonians share an eigenstate. If decoherence by state preparation is not possible, we show that initial states minimizing decoherence result from a delicate compromise between the environment and interaction dynamics.
We model the decoherence and dephasing of nitrogen vacancy (NV) centers in diamond due to a noisy paramagnetic bath, with and without the presence of a rf field that couples levels of the ground electronic state manifold, using a simple quantum mechanical model that allows for analytical solutions. The model treats the NV three-level ground state system in the presence of fluctuating magnetic fields that arise from the environment, and that result in decoherence, dephasing and dissipation. We show that all 9 eigenmodes of the three-level system are coupled to each other due to interaction with…
We employ a continuous dynamical decoupling scheme to suppress the decoherence induced by elastic collisions of cold atoms. Using a continuous echo pulse we achieve a thirty-fold increase in the coherence time of Rb87 atoms trapped in a dipole trap. Coherence times of more than 100ms are demonstrated for an ensemble with an optical depth of 120.
We propose a novel symmetrization procedure to beat decoherence for oscillator-assisted quantum gate operations. The enacted symmetry is related to the global geometric features of qubits transformation based on ancillary oscillator modes, e.g. phonons in an ion-trap system. It is shown that the devised multi-circuit symmetrized evolution endows the system with a two-fold resilience against decoherence: insensitivity to thermal fluctuations and quantum dissipation.
We consider a cavity optomechanical cooling configuration consisting of a mechanical resonator (denoted as resonator b) and an electromagnetic resonator (denoted as resonator a), which are coupled in such a way that the effective resonance frequency of resonator a depends linearly on the displacement of resonator b. We study whether back-reaction effects in such a configuration can be efficiently employed for suppression of decoherence. To that end, we consider the case where the mechanical resonator is prepared in a superposition of two coherent states and evaluate the rate of decoherence. We…
We report on room-temperature coherent manipulation of the spin of a single nitrogen-vacancy center in diamond and a study of its coherence as a function of magnetic field. We use magnetic resonance to induce Rabi nutations, and apply a Hahn spin echo to remove the effect of low-frequency dephasing. A sharp rise in the decoherence rate is observed at magnetic fields where the nitrogen-vacancy center spin couples resonantly to substitutional nitrogen spins via the magnetic dipolar coupling. Finally, we find evidence that away from these energy resonances spin flips of nitrogen electrons are the…
It is discussed the decoherence problems in ensemble large-scale solid state NMR quantum computer based on the array of P donor atoms having nuclear spin I = 1/2. It is considered here, as main mechanisms of decoherence for low temperature (< 0.1 K), the adiabatic processes of random modulation of qubit resonance frequency determined by secular part of nuclear spin interaction with electron spin of the basic atoms, with impurity paramagnetic atoms and also with nuclear spins of impurity diamagnetic atoms. It was made estimations of allowed concentrations of magnetic impurities and of spin temp…
We measure and characterize anomalous motional decoherence of an atomic ion confined in the lowest quantum levels of a novel rf ion trap that features moveable electrodes. The scaling of decoherence rate with electrode proximity is measured, and when the electrodes are cooled from 300 K to 150 K, the decoherence rate is suppressed by an order of magnitude. This provides direct evidence that anomalous motional decoherence of trapped ions stems from microscopic noisy potentials on the electrodes. These observations are relevant to quantum information processing schemes using trapped ions or othe…
Liquid-state NMR quantum computer has demonstrated the possibility of quantum computation and supported its development. Using NMR quantum computer techniques, we observed phase decoherence under two kinds of artificial noise fields; one a noise with a long period, and the other with shorter random period. The first one models decoherence in a quantum channel while the second one models transverse relaxation. We demonstrated that the bang-bang control suppresses decoherence in both cases.
In this work, two experimentally feasible methods of decoherence engineering-one based on the application of stochastic classical kicks and the other based on temporally randomized pulse sequences are combined. A different coupling interaction is proposed, which leads to amplitude damping as compared to existing methods which model phase damping, utilizing the $zz$ coupling interaction. The decoherence process on combining the stochastic kick method and the randomized pulse sequence method and the effectiveness of dynamical decoupling under these coupling interactions are analyzed. Finally, a …
Nitrogen vacancy (NV-) color centers in diamond are a prime candidate for use in quantum information devices, owing to their spin-1 ground state, straightforward optical initialization and readout, and long intrinsic coherence times in a room-temperature solid. While the 13C nuclear spin is often a dominant source of magnetic noise, we observe transitions between electron-nuclear hyperfine states of NV- centers in 99% 13C diamond that are robust to decoherence. At magnetic field strengths ranging from 550 - 900 G, these transitions are observable by optically detected magnetic resonance (ODMR)…
It is known that a quantum system with finite degrees of freedom can simulate a composite of a system and an environment if the state of the hypothetical environment is randomized by external manipulation. We show theoretically that any phase decoherence phenomena of a single qubit can be simulated with a two-qubit system and demonstrate experimentally two examples: one is phase decoherence of a single qubit in a transmission line, and the other is that in a quantum memory. We perform NMR experiments employing a two-spin molecule and clearly measure decoherence for both cases. We also prove ex…
The no-knowledge quantum feedback was proposed by Szigeti et al., Phys. Rev. Lett. 113, 020407 (2014), as a measurement-based feedback protocol for decoherence suppression for an open quantum system. By continuously measuring environmental noises and feeding back controls on the system, the protocol can completely reverse the measurement backaction and therefore suppress the system's decoherence. However, the complete decoherence cancellation was shown only for the instantaneous feedback, which is impractical in real experiments. Therefore, in this work, we generalize the original work and inv…
Due to omnipresent environmental interferences, quantum coherences inevitably undergo irreversible transformations over certain time-scales, thus leading to the loss of encoded information. This process, known as decoherence, has been a major obstacle in realizing efficient quantum information processors. Understanding the mechanism of decoherence is crucial in developing tools to inhibit it. Here we utilize a method proposed by Cory and co-workers [Phys. Rev. A 67, 062316 (2003)] to engineer artificial decoherence in the system qubits by randomly perturbing their surrounding ancilla qubits. U…
We evaluate exactly the non-Markovian effect on the decoherence dynamics of a qubit interacting with a dissipative vacuum reservoir and find that the coherence of the qubit can be partially trapped in the steady state when the memory effect of the reservoir is considered. Our analysis shows that it is the formation of a bound state between the qubit and its reservoir that results in this residual coherence in the steady state under the non-Markovian dynamics. A physical condition for the decoherence suppression is given explicitly. Our results suggest a potential way to decoherence control by …
We examine the effects of intra-environmental coupling on decoherence by constructing a low temperature spin--spin-bath model of an atomic impurity in a Debye crystal. The impurity interacts with phonons of the crystal through anti-ferromagnetic spin-spin interactions. The reduced density matrix of the central spin representing the impurity is calculated by dynamically integrating the full Schroedinger equation for the spin--spin-bath model for different thermally weighted eigenstates of the spin-bath. Exact numerical results show that increasing the intra-environmental coupling results in sup…
Universal quantum computation requiring only the Heisenberg exchange interaction and suppressing decoherence via an energy gap is presented. The combination of an always-on exchange interaction between the three physical qubits comprising the encoded qubit and a global magnetic field generates an energy gap between the subspace of interest and all other states. This energy gap suppresses decoherence. Always-on exchange couplings greatly simplify hardware specifications and the implementation of inter-logical-qubit gates. A controlled phase gate can be implemented using only three Heisenberg ex…
We experimentally demonstrate that the decoherence of a spin by a spin bath can be completely eliminated by fully polarizing the spin bath. We use electron paramagnetic resonance at 240 gigahertz and 8 Tesla to study the spin coherence time $T_2$ of nitrogen-vacancy centers and nitrogen impurities in diamond from room temperature down to 1.3 K. A sharp increase of $T_2$ is observed below the Zeeman energy (11.5 K). The data are well described by a suppression of the flip-flop induced spin bath fluctuations due to thermal spin polarization. $T_2$ saturates at $\sim 250 μs$ below 2 K, where the …
We study the application of decoupling techniques to the case of a damped vibrational mode of a chain of trapped ions, which can be used as a quantum bus in linear ion trap quantum computers. We show that vibrational heating could be efficiently suppressed using appropriate ``parity kicks''. We also show that vibrational decoherence can be suppressed by this decoupling procedure, even though this is generally more difficult because the rate at which the parity kicks have to applied increases with the effective bath temperature.
Solid-state quantum registers are exceptional for storing quantum information at room temperature with long coherence time. Nevertheless, practical applications toward quantum supremacy require even longer coherence time to allow for more complex algorithms. In this work we propose a quantum register that lies in a decoherence-free subspace to be implemented with color centers in diamond. The quantum information is encoded in two logical states composed of two nearby nuclear spins, while an electron spin is used as ancilla for initialization and control. Moreover, by tuning an off-axis magneti…
The dynamics of a decohering two-level system driven by a suitable control Hamiltonian is studied. The control procedure is implemented as a sequence of radiofrequency pulses that repetitively flip the state of the system, a technique that can be termed quantum "bang-bang" control after its classical analog. Decoherence introduced by the system's interaction with a quantum environment is shown to be washed out completely in the limit of continuous flipping and greatly suppressed provided the interval between the pulses is made comparable to the correlation time of the environment. The model su…
The dynamics of two coupled spins-1/2 coupled to a spin-bath is studied as an extended model of the Tessieri-Wilkie Hamiltonian \cite{TWmodel}. The pair of spins served as an open subsystem were prepared in one of the Bell states and the bath consisted of some spins-1/2 is in a thermal equilibrium state from the very beginning. It is found that with the increasing the coupling strength of the bath spins, the bath forms a resonant antiferromagnetic order. The polarization correlation between the two spins of the subsystem and the concurrence are recovered in some extent to the isolated subsyste…
We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen vacancy (NV) color centers in diamond and the associated substitutional nitrogen spin bath. We perform measurements of NV spin free induction decay times $T_2^*$ and spin-echo coherence times $T_2$ in 25 diamond samples with nitrogen concentrations [N] ranging from 0.01 to 300\,ppm. We introduce a microscopic model and perform numerical simulations to quantitatively explain the degradation of both $T_2^*$ and $T_2$ over four orders …
It is shown that the magnetic state decoherence produced by collisions in a thermal vapor can be suppressed by the application of a train of ultrafast optical pulses.
We investigate cat codes that can correct multiple excitation losses and identify two types of logical errors: bit-flip errors due to excessive excitation loss and dephasing errors due to quantum back-action from the environment. We show that selected choices of logical subspace and coherent amplitude can efficiently reduce dephasing errors. The trade-off between the two major errors enables optimized performance of cat codes in terms of minimized decoherence. With high coupling efficiency, we show that one-way quantum repeaters with cat codes feature drastically boosted secure communication r…
Entanglement and quantum squeezing have wide applications in quantum technologies due to their non-classical characteristics. Here we study entanglement and quantum squeezing in an open spin-optomechanical system, in which a Rabi model (a spin coupled to the mechanical oscillator) is coupled to an ancillary cavity field via a quadratic optomechanical coupling. We find that their performances can be significantly modulated via the photon of the ancillary cavity, which comes from photon-dependent spin-oscillator coupling and detuning. Specifically, a fully switchable spin-oscillator entanglement…
In this paper, we study the suppression of adiabatic decoherence in a three-level atom with $Λ$ configuration using bang-bang control technique. We have given the decoupling bang-bang operation group, and programmed a sequence of periodic radio frequency twinborn pulses to realize the control process. Moreover, we have studied the process with non-ideal situation and established the condition for efficient suppression of adiabatic decoherence.
Projective measurements are an essential element of quantum mechanics. In most cases, they cause an irreversible change of the quantum system on which they act. However, measurements can also be used to stabilize quantum states from decay processes, which is known as the quantum Zeno effect (QZE). Here, we demonstrate this effect for the case of a superposition state of a nuclear spin qubit, using an ancilla to perform the measurement. As a result, the quantum state of the qubit is protected against dephasing without relying on an ensemble nature of NMR experiments. We also propose a scheme to…
We describe a method allowing transient suppression of decoherence effects on the atom-optics realization of the kicked rotor. The system is prepared in an initial state with a momentum distribution concentrated in an interval much sharper than the Brillouin zone; the measure of the momentum distribution is restricted to this interval of quasimomenta: As most of the atoms undergoing decoherence processes fall outside this detection range and thus are not detected, the measured signal is effectively decoherence-free.
It is shown that a nonequilibrium environment can be instrumental in suppressing decoherence between distinct decoherence free subspaces in quantum registers. The effect is found in the framework of exact coherent-product solutions for model registers decohering in a bath of degenerate harmonic modes, through couplings linear in bath coordinates. These solutions represent a natural nonequilibrium extension of the standard solution for a decoupled initial register state and a thermal environment. Under appropriate conditions, the corresponding reduced register distribution can propagate in an u…
We show that the qubit decoherence due to zero-temperature energy relaxation can be almost completely suppressed by using the quantum uncollapsing procedure. To protect a qubit state, a partial quantum measurement moves it towards the ground state, where it is kept during the storage period, while the second partial measurement restores the initial state. This procedure preferentially selects the cases without energy decay events. Stronger decoherence suppression requires smaller selection probability; a desired point in this trade-off can be chosen by varying the measurement strength. The exp…
Understanding and mitigating decoherence is a key challenge for quantum science and technology. The main source of decoherence for solid-state spin systems is the uncontrolled spin bath environment. Here, we demonstrate quantum control of a mesoscopic spin bath in diamond at room temperature that is composed of electron spins of substitutional nitrogen impurities. The resulting spin bath dynamics are probed using a single nitrogen-vacancy (NV) centre electron spin as a magnetic field sensor. We exploit the spin bath control to dynamically suppress dephasing of the NV spin by the spin bath. Fur…
In quantum mechanics an incoming particle wave packet with sufficient energy will undergo both transmission and reflection when encountering a barrier of lower energy, but in classical mechanics there is no reflection, only transmission. In this paper we seek to explain the disappearance of quantum-mechanical reflection in the quasi-classical limit, using standard methods of decoherence through environmental interaction. We consider two models. In the first, the incoming particle is classicalized by coupling it to an environment described by a standard Lindblad master equation diagonalizing in…
The silicon-vacancy center in diamond offers attractive opportunities in quantum photonics due to its favorable optical properties and optically addressable electronic spin. Here, we combine both to achieve all-optical coherent control of its spin states. We utilize this method to explore spin dephasing effects in an impurity-rich sample beyond the limit of phonon-induced decoherence: Employing Ramsey and Hahn-echo techniques at 12mK base temperature we identify resonant coupling to a substitutional nitrogen spin bath as the limiting decoherence source for the electron spin.
Coherent interaction of a quantum system with environment usually induces quantum decoherence. However, remarkably, in certain configurations the coherent system-environment coupling can be simultaneously explored to engineer a specific dark state of the environment that eliminates the decoherence. Here we report on experimental demonstration of such protocol for suppression of quantum decoherence by quantum decoherence itself. The protocol is based on indirect control of the environment via quantum measurements on quantum probes interacting with the environment prior to the system that should…
We present an experimental method to perform dual-channel lock-in magnetometry of time-dependent magnetic fields using a single spin associated with a nitrogen-vacancy (NV) color center in diamond. We incorporate multi-pulse quantum sensing sequences with phase estimation algorithms to achieve linearized field readout and constant, nearly decoherence-limited sensitivity over a wide dynamic range. Furthermore, we demonstrate unambiguous reconstruction of the amplitude and phase of the magnetic field. We show that our technique can be applied to measure random phase jumps in the magnetic field, …
We examine the role of interactions for a Bose gas trapped in a double-well potential ("Bose-Josephson junction") when external noise is applied and the system is initially delocalized with equal probability amplitudes in both sites. The noise may have two kinds of effects: loss of atoms from the trap, and random shifts in the relative phase or number difference between the two wells. The effects of phase noise are mitigated by atom-atom interactions and tunneling, such that the dephasing rate may be reduced to half its single-atom value. Decoherence due to number noise (which induces fluctuat…
Charge fluctuations from gate bias and background traps severely limit the performance of a charge qubit in a Cooper-pair box (CPB). Here we present an experimentally realizable method to control the decoherence effects of these charge fluctuations using two strongly capacitively coupled CPBs. This coupled-box system has a low-decoherence subspace of two states. Our results show that the inter-box Coulomb correlation can help significantly suppress decoherence of this two-level system, making it a promising candidate as a logical qubit, encoded using two CPBs.
Methods of optimal control are applied to a model system of interacting two-level particles (e.g., spin-half atomic nuclei or electrons or two-level atoms) to produce high-fidelity quantum gates while simultaneously negating the detrimental effect of decoherence. One set of particles functions as the quantum information processor, whose evolution is controlled by a time-dependent external field. The other particles are not directly controlled and serve as an effective environment, coupling to which is the source of decoherence. The control objective is to generate target one- and two-qubit uni…
In the propagation of optical pulses through dispersive media, the frequency degree of freedom acts as an effective decohering environment on the polarization state of the pulse. Here we discuss the application of open-loop dynamical-decoupling techniques for suppressing such a polarization decoherence in one-way communication channels. We describe in detail the experimental proof of principle of the "bang-bang" protection technique recently applied to flying qubits in [Damodarakurup et al., Phys. Rev. Lett. 103, 040502]. Bang-bang operations are implemented through appropriately oriented wave…
