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arXiv 1306.1474cond-mat.mtrl-sci
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稀磁半导体(Ga,Mn)As中磁性杂质态的电子激发

Electronic excitations of magnetic impurity state in diluted magnetic semiconductor (Ga,Mn)As

M. Kobayashi, H. Niwa, Y. Takeda, A. Fujimori, Y. Senba, H. Ohashi, A. Tanaka, S. Ohya, P. N. Hai, M. Tanaka, Y. Harada, M. Oshima

摘要:

用共振非弹性X射线散射(RIXS)研究了(Ga,Mn)As中Mn掺杂的电子结构。从组态相互作用簇模型计算,Mn $L_3$ RIXS光谱的线形可以解释为从Mn $^{3+}$基态的$d$ - $d$激发,主要由电荷转移态,而不是Mn $^{2+}$基态。与典型的$d$ - $d$激发不同,峰宽比实验能量分辨率宽。我们将加宽归因于$d$ - $d$激发的有限寿命,其通过Mn $3d$轨道与配体带的杂化而快速衰减为主体价带和导带中的电子-空穴对。

英文摘要:

The electronic structure of doped Mn in (Ga,Mn)As is studied by resonant inelastic X-ray scattering (RIXS). From configuration-interaction cluster-model calculations, the line shapes of the Mn $L_3$ RIXS spectra can be explained by $d$-$d$ excitations from the Mn$^{3+}$ ground state, dominated by charge-transferred states, rather than a Mn$^{2+}$ ground state. Unlike archetypical $d$-$d$ excitation, the peak widths are broader than the experimental energy resolution. We attribute the broadening to a finite lifetime of the $d$-$d$ excitations, which decay rapidly to electron-hole pairs in the host valence and conduction bands through hybridization of the Mn $3d$ orbital with the ligand band.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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