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arXiv 1302.3258cond-mat.dis-nncond-mat.soft
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无序系统中非线性电导率的频率依赖性:一个可解析解的模型

The frequency-dependence of nonlinear conductivity in disordered systems: an analytically solvable model

Clara Mattner, Bernhard Roling, Andreas Heuer

摘要:

对于包含能量和势垒无序的一维模型中的跳跃动力学,我们确定了任意外部频率下对外部场的线性和非线性响应。计算是以分析术语进行的。我们系统地分析了参数空间,并找到三个不同的制度,对应于定性不同的频率依赖性的非线性响应。两个政权同意最近的无机离子导体和离子液体的电导率实验的结果,分别。在直流区的非线性和线性电导率的比例可以明确地表示在无序参数。作为一个通用的功能,非线性电导率显示最小值作为频率的函数,可以确定与双势阱中的前向后动力学。最小值附近的非线性电导率的大小和符号是该模型中固有的无序的度量。令人惊讶的是,最小值的频率几乎不受无序的影响。

英文摘要:

For the hopping dynamics in a one-dimensional model, containing energy and barrier disorder, we determine the linear and nonlinear response to an external field for arbitrary external frequencies. The calculation is performed in analytical terms. We systematically analyze the parameter space and find three different regimes, corresponding to qualitatively different frequency dependencies of the nonlinear response. Two regimes agree with the results of recent conductivity experiments on inorganic ion conductors and ionic liquids, respectively. The ratio of the nonlinear and linear conductivity in the dc-regime can be explicitly expressed in terms of the disorder parameters. As a generic feature the nonlinear conductivity displays a minimum as a function of frequency which can be identified with forward-backward dynamics in a double-well potential. The magnitude and sign of the nonlinear conductivity around the minimum is a measure of the disorder, inherent in this model. Surprisingly, the frequency of the minimum is hardly influenced by the disorder.

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