Quenching Factor for Low Energy Nuclear Recoils in a Plastic Scintillator
L. Reichhart, D. Yu. Akimov, H. M. Araujo, E. J. Barnes, V. A. Belov, A. A. Burenkov, V. Chepel, A. Currie, L. DeViveiros, B. Edwards, V. Francis, C. Ghag, A. H… 展开作者
L. Reichhart, D. Yu. Akimov, H. M. Araujo, E. J. Barnes, V. A. Belov, A. A. Burenkov, V. Chepel, A. Currie, L. DeViveiros, B. Edwards, V. Francis, C. Ghag, A. Hollingsworth, M. Horn, G. E. Kalmus, A. S. Kobyakin, A. G. Kovalenko, V. N. Lebedenko, A. Lindote, M. I. Lopes, R. Luscher, P. Majewski, A. St J. Murphy, F. Neves, S. M. Paling, J. Pinto da Cunha, R. Preece, J. J. Quenby, P. R. Scovell, C. Silva, V. N. Solovov, N. J. T. Smith, P. F. Smith, V. N. Stekhanov, T. J. Sumner, C. Thorne, R. J. Walker
Plastic scintillators are widely used in industry, medicine and scientific research, including nuclear and particle physics. Although one of their most common applications is in neutron detection, experimental data on their response to low-energy nuclear recoils are scarce. Here, the relative scintillation efficiency for neutron-induced nuclear recoils in a polystyrene-based plastic scintillator (UPS-923A) is presented, exploring recoil energies between 125 keV and 850 keV. Monte Carlo simulations, incorporating light collection efficiency and energy resolution effects, are used to generate neutron scattering spectra which are matched to observed distributions of scintillation signals to parameterise the energy-dependent quenching factor. At energies above 300 keV the dependence is reasonably described using the semi-empirical formulation of Birks and a kB factor of (0.014+/-0.002) g/MeVcm^2 has been determined. Below that energy the measured quenching factor falls more steeply than predicted by the Birks formalism.
We study the response of EJ-301 liquid scintillator to monochromatic 244.6 $\pm$ 8.4 keV neutrons, targeting the 10-100 keV proton recoil energy interval. Limited experimental information exists for proton light yield in this range, for this or any other organic scintillator. Our results confirm the adequacy of a modified Birks' model, common to all organic scintillator formulations, predicting a marked increase in quenching factor as proton energy approaches the few keV regime. The relevance of this behavior within the context of searches for low-mass particle dark matter is mentioned.
Detailed characterization of the newly available plastic scintillator (EJ-299-33A) having the pulse shape discrimination (PSD) property has been carried out in case of a large-sized detector (5 in.$\times$5 in.). The pulse height response of the scintillator for nearly mono-energetic neutrons has been reported in case of neutron energies E$_n$ =3, 6 and 9 MeV. Important properties (figure-of-merit (FOM), time resolution, detection efficiency) of the detector has been compared with a commonly used liquid organic scintillator based detector of the same size coupled to the same PMT for uniformity…
The Plastic Scintillator Detector (PSD) is one of the main sub-detectors in the DArk Matter Particle Explorer (DAMPE) project. It will be operated over a large temperature range from -$10$ to $30^{\circ}$C, so the temperature effect of the whole detection system should be studied in detail. The temperature dependence of the PSD system is mainly contributed by the three parts: the plastic scintillator bar, the photomultiplier tube (PMT), and the Front End Electronics (FEE). These three parts have been studied in detail and the contribution of each part has been obtained and discussed. The tempe…
Organic liquid scintillators are used in a wide variety of applications in experimental nuclear and particle physics. Boron-loaded scintillators are particularly useful for detecting neutron captures, due to the high thermal neutron capture cross section of $^{10}$B. These scintillators are commonly used in neutron detectors, including the DarkSide-50 neutron veto, where the neutron may produce a signal when it scatters off protons in the scintillator or when it captures on $^{10}$B. Reconstructing the energy of these recoils is complicated by scintillation quenching. Understanding how nuclear…
A large area plastic scintillator detector array(~ 1 m x1m) has been set up for fast neutron spectroscopy at the BARC-TIFR Pelletron laboratory, Mumbai. The energy, time and position response has been measured for electrons using radioactive sources and for mono-energetic neutrons using the 7Li(p,n1)7Be*(0.429 MeV) reaction at proton energies between 6.3 and 19 MeV. A Monte Carlo simulation of the energy dependent efficiency of the array for neutron detection is in agreement with the 7Li(p,n1) measurements. The array has been used to measure the neutron spectrum, in the energy range of 4-12 Me…
Semi-empirical method of calculation of quenching factors for scintillators is described. It is based on classical Birks formula with the total stopping powers for electrons and ions which are calculated with the ESTAR and SRIM codes, respectively. Method has only one fitting parameter (the Birks factor kB) which can have different values for the same material in different conditions of measurements and data treatment. A hypothesis is used that, once the kB value is obtained by fitting data for particles of one kind and in some energy region (e.g. for a few MeV alpha particles from internal co…
For the first time a molecule of 2-(4-styrylphenyl)benzoxazole containing benzoxazole and stilbene groups is applied as a scintillator dopant acting as a wavelength shifter. In this article a light yield of the plastic scintillator, prepared from styrene doped with 2 wt% of 2,5-diphenylbenzoxazole and 0.03 wt% of 2-(4-styrylphenyl)benzoxazole, is determined to be as large as 60% $\pm$ 2% of the anthracene light output. There is a potential to improve this value in the future by the optimization of the additives concentrations.
Digital pulse shape discrimination has become readily available to distinguish nuclear recoil and electronic recoil events in scintillation detectors. We evaluate digital implementations of pulse shape discrimination algorithms discussed in the literature, namely the Charge Comparison Method, Pulse-Gradient Analysis, Fourier Series and Standard Event fitting. In addition, we present a novel algorithm based on a Laplace Transform. Instead of reducing the performance of these algorithms to a single Figure of Merit, we evaluate them as function of recoil energy. Specifically, using commercial EJ-…
We report on the development of a fast neutron detector using a liquid scintillator doped with enriched Li-6. The lithium was introduced in the form of an aqueous LiCl micro-emulsion with a di-isopropylnaphthalene-based liquid scintillator. A Li-6 concentration of 0.15 % by weight was obtained. A 125 mL glass cell was filled with the scintillator and irradiated with fission-source neutrons. Fast neutrons may produce recoil protons in the scintillator, and those neutrons that thermalize within the detector volume can be captured on the Li-6. The energy of the neutron may be determined by the li…
Anisotropic scintillators can offer a unique possibility to exploit the so-called directionality approach in order to investigate the presence of those Dark Matter (DM) candidates inducing nuclear recoils. In fact, their use can overcome the difficulty of detecting extremely short nuclear recoil traces. In this paper we present recent measurements performed on the anisotropic response of a ZnWO$_4$ crystal scintillator to nuclear recoils, in the framework of the ADAMO project. The anisotropic features of the ZnWO$_4$ crystal scintillators were initially measured with $α$ particles; those resul…
The polystyrene dopped with 2,5-diphenyloxazole as a primary fluor and 2-(4-styrylphenyl)benzoxazole as a wavelength shifter, prepared as a plastic scintillator was investigated using positronium probe in wide range of temperatures from 123 to 423 K. Three structural transitions at 260 K, 283 K and 370 K were found in the material. In the o-Ps intensity dependence on temperature, the significant hysteresis is observed. Heated to 370 K, the material exhibits the o-Ps intensity variations in time.
We report the first clear observation of neutron/gamma-ray pulse-shape sensitivity of a fully-instrumented 8 $\times$ 8 array of plastic scintillator segments coupled to two 5 cm $\times$ 5 cm 64-channel SiPM arrays as part of a study of the key metrics of a prototype antineutrino detector module designed for directional sensitivity. SANDD (a Segmented AntiNeutrino Directional Detector) will eventually comprise a central module of 64 elongated segments of $^{6}$Li-doped pulse-shape-sensitive scintillator rods, each with a square cross section of 5.4 mm $\times$ 5.4 mm, surrounded by larger cro…
We have constructed and tested a novel plastic-scintillator-based solid-state active proton target for use in nuclear spectroscopic studies with nuclear reactions induced by an ion beam in inverse kinematics. The active target system, named Stack Structure Solid organic Scintillator Active Target (S4AT), consists of five layers of plastic scintillators, each with a 1-mm thickness. To determine the reaction point in the thickness direction, we exploit the difference in the energy losses due to the beam particle and the charged reaction product(s) in the scintillator material. S4AT offers the pr…
AMoRE-II is the second phase of the Advanced Molybdenum-based Rare process Experiment aiming to search for the neutrino-less double beta decay of 100Mo isotopes using ~ 200 kg of molybdenum-containing cryogenic detectors. The AMoRE-II needs to keep the background level below 10-5 counts/keV/kg/year with various methods to maximize the sensitivity. One of the methods is to have the experiment be carried out deep underground free from the cosmic ray backgrounds. The AMoRE-II will run at Yemilab with ~ 1,000 m depth. However, even in such a deep underground environment, there are still survived c…
We report measurement of reactor based electron anti-neutrinos from a prototype array of plastic scintillator bars ( mini-ISMRAN ) located inside Dhruva research reactor hall, BARC. The detector setup took data for 128 days for reactor on (RON) and 51 days for reactor off (ROFF) condition. A detailed analysis procedure is developed to select the anti-neutrino candidate events based on the energy deposition, number of bars hit as well as topological event selection criteria in position and time. Each of these selection criteria are compared with Monte Carlo based simulations and further an embe…
Pixelated Plastic Scintillator Array Manufacturing using Fast-, Photo-Curable Resin
Air Force Institute of Technology（空军理工学院）；Oak Ridge National Laboratory（橡树岭国家实验室）；Defense Threat Reduction Agency Nuclear Science and Engineering Research Center（国防威胁降低局核科学与工程研究中心）
We report results of fast neutron response in plastic scintillator (PS) bars from deuterium-deuterium (D-D) and deuterium-tritium (D-T) reactions using Purnima Neutron Generator Facility, BARC, Mumbai. These measurements are useful in context of Indian Scintillator Matrix for Reactor Anti-Neutrino (ISMRAN) detection, an array of 10x10 PS bars, used to measure reactor anti-neutrinos through inverse beta decay (IBD) signal. ISMRAN detector, an above-ground experiment close to the reactor core (~13m), deals with an active fast neutron background inside the reactor hall. A good understanding of fa…
The detection of 200-1000 MeV neutrons requires large amounts, $\sim$100 cm, of detector material because of the long nuclear interaction length of these particles. In the example of the NeuLAND neutron time-of-flight detector at FAIR, this is accomplished by using 3000 monolithic scintillator bars of 270$\times$5$\times$5 cm$^3$ size made of a fast plastic. Each bar is read out on the two long ends, and the needed time resolution of $σ_t$ $<$ 150 ps is reached with fast timing photomultipliers. In the present work, it is investigated whether silicon photomultiplier (SiPM) photosensors can be …
Time of Flight Positron Emission Tomography scanner based on plastic scintillators is being developed at the Jagiellonian University by the J-PET collaboration. The main challenge of the conducted research lies in the elaboration of a method allowing application of plastic scintillators for the detection of low energy gamma quanta. In this article we report on tests of a single detection module built out from BC-420 plastic scintillator strip (with dimensions of 5x19x300mm^3) read out at two ends by Hamamatsu R5320 photomultipliers. The measurements were performed using collimated beam of anni…
A comparative study of the neutron-$γ$ Pulse Shape Discrimination (PSD) with seven organic scintillators is performed using an identical setup and digital electronics. The scintillators include plastics (EJ-299-33 and a plastic prototype), single crystals (stilbene and the recent doped $p$-terphenyl) and liquids (BC501A, NE213 and the deuterated liquid BC537). First, the overall PSD performance of the different scintillators is compared and threshold neutron energies for a given discrimination quality are determined. Then, using statistical arguments, two intrinsic contributions to the PSD cap…
A new type of neutron detector, named Stack Structure Solid organic Scintillator (S$^4$), consisting of multi-layer plastic scintillators with capability to suppress low-energy $γ$ rays under high-counting rate has been constructed and tested. To achieve $\it{n}$-$γ$ discrimination, we exploit the difference in the ranges of the secondary charged particles produced by the interactions of neutrons and $γ$ rays in the scintillator material. The thickness of a plastic scintillator layer was determined based on the results of Monte Carlo simulations using the Geant4 toolkit. With layer thicknesses…
The timing characteristics of scintillators must be understood in order to determine which applications they are appropriate for. Polyethylene naphthalate (PEN) and polyethylene teraphthalate (PET) are common plastics with uncommon scintillation properties. Here, we report the timing characteristics of PEN and PET, determined by exciting them with 120 GeV protons. The test beam was provided by Fermi National Accelerator Laboratory, and the scintillators were tested at the Fermilab Test Beam Facility. PEN and PET are found to have dominant decay constants of 34.91 ns and 6.78 ns, respectively.
The NeuLAND (New Large-Area Neutron Detector) plastic-scintillator-based time-of-flight detector for 0.1-1.6 GeV neutrons is currently under construction at the Facility for Antiproton and Ion Research (FAIR), Darmstadt, Germany. In its final configuration, NeuLAND will consist of 3000 2.7 m $\times$ 5 cm $\times$ 5 cm big plastic scintillator bars that are read out on each end by fast timing photomultipliers. Here, data from a comprehensive study of an alternative light readout scheme using silicon photomultipliers (SiPM) are reported. For this purpose, a NeuLAND bar was instrumented on each …
We present a detailed study on detector response to different radioactive sources and the measurements of non-reactor environmental backgrounds with the Indian Scintillator Matrix for Reactor Anti-Neutrinos (ISMRAN) detector setup consisting of 9$\times$10 Plastic Scintillator Bars (PSBs) array at BARC, Mumbai. These measurements are useful in the context of the ISMRAN detector setup, which will be used to detect the reactor anti-neutrinos (${\bar{\ensuremathν}}_{e}$) and measure its energy spectra, through the inverse beta decay (IBD) process. A GEANT4 based Monte Carlo (MC) simulation is use…
A 3-D position sensitive neutron detector is being developed based on a plastic scintillator array. A double side SiPM readout is used to determine the depth of interaction (DOI) in each scintillator unit. In the preliminary test, the DOI in a 254 x 6 x 6 mm3 SP101 plastic scintillator is measured at different positions using a collimated Co-60 source. The SiPM (KETEK PM6660) signals are recorded by a 2.5 GS/s digital oscilloscope. The DOI results are calculated using both the amplitude and the temporal information. Position resolutions (FWHM) of 2.5 cm and 6.6 cm are realized, respectively. A…
Fast timing detectors are an essential element in the experimental setup for time-of-flight (ToF) mass measurements of unstable nuclei. We have upgraded the scintillator detectors used in experiments at the National Superconducting Cyclotron Laboratory (NSCL) by increasing the number of photomultiplier tubes that read out their light signals to four per detector, and characterized them in a test experiment with $^{48}$Ca beam at the NSCL. The new detectors achieved a time resolution ($σ$) of 7.5 ps. We systematically investigated different factors that affect their timing performance. In addit…
The scintillation light output response of stilbene crystals has been measured for protons recoiling along the \textit{a}, \textit{b}, and \textit{c'} crystalline axes with energies between 1.3 and 10 MeV using neutrons produced with the tandem Van de Graaff accelerator at Triangle Universities Nuclear Laboratory. The proton recoil energy and direction were measured using the coincident detection of neutrons between a stilbene scintillator and an array of EJ-309 liquid scintillators spanning arranged neutron recoil angles. The maximum light output was found to coincide with proton recoils alon…
Plastic scintillator detectors are widely used in particle physics thanks to the very good particle identification, tracking capabilities and time resolution. However, new experimental challenges and the need for enhanced performance require the construction of detector geometries that are complicated using the current production techniques. In this article we propose a new production technique based on additive manufacturing that aims to 3D print polystyrene-based scintillator. The production process and the results of the scintillation light output measurement of the 3D-printed scintillator …
We describe a beta electron spectrometer for use in an upcoming experiment that will measure the beta-antineutrino correlation coefficient (a-coefficient) in neutron beta decay. Electron energy is measured by a thick plastic scintillator detector. A conical array of plastic scintillator veto detectors is used to suppress events where the electron backscattered. A Monte Carlo simulation of this device in the configuration of the a-coefficient experiment is presented. The design, construction, and testing of a full-scale prototype device is described. We discuss the performance of this spectrome…
We report on the prototyping of a plastic scintillator hodoscope with wavelength-shifting fibre read-out by a multi-anode photomultiplier as part of the development of a detector for cosmic ray muons to be carried aboard an aircraft. Light yield and light attenuation measurements on single- and double-clad wavelength-shifting fibres were performed. Low power, low-threshold, discriminators were designed. A prototype 16-channel hodoscope with two planes was built and tested with cosmic rays. After correcting for geometrical factors a global intrinsic efficiency of $ε> 98$ % was obtained in both …
As part of an experimental effort to demonstrate sensitivity in a large-mass detector to the ultra-low energy recoils expected from coherent neutrino-nucleus elastic scattering, we have designed and built a highly monochromatic 24 keV neutron beam at the Kansas State University Triga Mark-II reactor. The beam characteristics were chosen so as to mimic the soft recoil energies expected from reactor antineutrinos in a variety of targets, allowing to understand the response of dedicated detector technologies in this yet unexplored sub-keV recoil range. A full characterization of the beam properti…
We study the possibility of using CsI[Na] scintillators as an advantageous target for the detection of coherent elastic neutrino-nucleus scattering (CENNS), using the neutrino emissions from the SNS spallation source at Oak Ridge National Laboratory. The response of this material to low-energy nuclear recoils like those expected from this process is characterized. Backgrounds are studied using a 2 kg low-background prototype crystal in a dedicated radiation shield. The conclusion is that a planned 14 kg detector should measure approximately 550 CENNS events per year above a demonstrated $\sim7…
J-PET is a photon detector built of plastic scintillators, which already has been commissioned for CPT studies in the decays of positronium. In the first experiment, J-PET has achieved a sensitivity to CPT violation at a level of 10^{-4}, and now it aims to reach a level of 10^{-5}. This will be done by enhancing the three-photon registration efficiency for ortho-positronium decays using a new layer of densely packed plastic scintillators termed Modular J-PET. We present the simulation studies performed for different experimental detection setups to be used for the next CPT test with the Modul…
