The alpha decay half-lives of recently synthesized superheavy nuclei (SHN) are calculated by applying a new approach which estimates them with the help of their neighbors based on some simple formulas. The estimated half-life values are in very good agreement with the experimental ones, indicating the reliability of the experimental observations and measurements to a large extent as well as the predictive power of our approach. The second part of this work is to test the applicability of the Wentzel-Kramers-Brillouin (WKB) approximation for the quantum mechanical tunneling probability. We calculated the accurate barrier penetrability for alpha decay along with proton and cluster radioactivity by numerically solving Schrödinger equation. The calculated results are compared with those of the WKB method to find that WKB approximation works well for the three physically analogical decay modes.
The alpha decay half-lives of the recently produced isotopes of the 112, 114, 116 and 118 nuclei and decay products have been calculated in the quasi-molecular shape path using the experimental Qalpha value and a Generalized Liquid Drop Model including the proximity effects between nucleons in the neck or the gap between the nascent fragments. Reasonable estimates are obtained for the observed alpha decay half-lives. The results are compared with calculations using the Density-Dependent M3Y effective interaction and the Viola-Seaborg-Sobiczewski formulae. Generalized Liquid Drop Model predicti…
The alpha-decay half-lives of recently synthesized superheavy nuclei (SHN) are investigated based on a unified fission model (UFM) where a new method to calculate the assault frequency of alpha-emission is used. The excellent agreement with the experimental data indicates the UFM is a useful tool to investigate these alpha-decays. It is found that the half-lives become more and more insensitive to the Q_alpha values as the atomic number increases on the whole, which is favorable for us to predict the half-lives of SHN. In addition, a formula is suggested to compute the Q_alpha values for the n…
Recently, experimental researches on the $α$ decay with long lifetime are one of hot topics in the contemporary nuclear physics [e.g. N. Kinoshita {\sl et al.} (2012) and J. W. Beeman {\sl et al.} (2012) ]. In this study, we have systematically investigated the extremely long-lived $α$-decaying nuclei within a generalized density-dependent cluster model involving the experimental nuclear charge radii. In detail, the important density distribution of daughter nuclei is deduced from the corresponding experimental charge radii, leading to an improved $α$-core potential in the quantum tunneling ca…
Recent microscopic calculation based on the density functional theory predicts long-lived superheavy elements in a variety of shapes, including spherical, axial and triaxial configurations. Only when N=184 is approached one expects superheavy nuclei that are spherical in their ground states. Magic islands of extra-stability have been predicted to be around Z=114, 124 or, 126 with N=184, and Z=120, with N=172. However, the question of whether the fission-survived superheavy nuclei with high Z and N would live long enough for detection or, undergo alpha-decay in a very short time remains open. I…
We have constructed new proximity function particularly for interaction between two superheavy nuclei based on the experimental alpha decay half-lives. The new proximity function is used to produce the alpha decay half-lives of superheavy nuclei whose experimental values are known. The new proximity function produces the alpha decay half-lives close to the experiments. Hence we can conclude that the new proximity function can be used to study the interaction between two superheavy nuclei.
In this work study on alpha decay chains emerging from isotopes of Z = 122 superheavy nuclei is carried out with emphasize on nuclear deformations and Langer modification. The interest in this particular superheavy nuclei is due to the recent experimental efforts to synthesize the isotope ^{299}120 in a fusion reaction at the velocity filter SHIP (GSI Darmstadt), which makes synthesis of Z = 122 nuclei to occur in the near future, and in turn will give the experimentalist the chance observe the decays associated with the isotopes of this nuclei. We perform our calculations by choosing the Wood…
Weak decays in superheavy nuclei with proton numbers Z = 118 - 120 and neutron numbers N = 175 - 184 are studied within a microscopic formalism based on deformed self-consistent Skyrme Hartree-Fock mean-field calculations with pairing correlations. The half-lives of beta+ decay and electron capture are compared with alpha-decay half-lives obtained from phenomenological formulas. The sensitivity of the half-lives to the unknown Q-energies is studied by comparing the results obtained from different approaches for the masses. It is shown that alpha-decay is always dominant in this mass region. Th…
A systematic study on the alpha decay half lives of various isotopes of superheavy element \textit{Z} = 121 within the range 290 $\leq$ A $\leq$ 339 is presented for the first time using Coulomb and proximity potential model for deformed nuclei (CPPMDN). The calculated $α$ decay half lives of the isotopes within our formalism match well with the values computed using Viola-Seaborg systematic, Universal curve of Poenaru et al., and the analytical formula of Royer. In our study by comparing the $α$ decay half lives with the spontaneous fission half lives, we have predicted $2α$ chain from $^{309…
The experimentally available data on the alpha decay half lives and Q? values for 96 superheavy nuclei are used to fix the parameters for a modified version of the Brown empirical formula through two fitting procedures which enables its comparison with similar fits using Viola-Seaborg and Royer formulas. The new expressions provide very good agreement with experimental data having fewer or the same number of parameters. All formulas with the obtained parameters are then extrapolated to generate half lives predictions for 125 unknown superheavy alpha emitters. The nuclei where the employed empi…
Potential energy surfaces of even-even superheavy nuclei are evaluated within the macroscopic-microscopic approximation. A very rapidly converging analytical Fourier-type shape parametrization is used to describe nuclear shapes throughout the periodic table, including those of fissioning nuclei. The Lublin Strasbourg Drop and another effective liquid-drop type mass formula are used to determine the macroscopic part of nuclear energy. The Yukawa-folded single-particle potential, the Strutinsky shell-correction method, and the BCS approximation for including pairing correlations are used to obta…
We systematically calculate the spontaneous fission half-lives for heavy and superheavy nuclei between U and Fl isotopes. The spontaneous fission process is studied within the semi-empirical WKB approximation. The potential barrier is obtained using a generalized liquid drop model, taking into account the nuclear proximity, the mass asymmetry, the phenomenological pairing correction, and the microscopic shell correction. Macroscopic inertial-mass function has been employed for the calculation of the fission half-life. The results reproduce rather well the experimental data. Relatively long hal…
Systematic alpha-nucleus folding potentials are used to analyze alpha-decay half-lives of superheavy nuclei. Preformation factors of about several per cent are found for all nuclei under study. The systematic behavior of the preformation factors and the volume integrals of the potentials allows to predict alpha-decay energies and half-lives for unknown nuclei. Shell closures can be determined from measured alpha-decay energies using the discontinuity of the volume integral at shell closures. For the first time a double shell closure is predicted for Z_magic = 132, N_magic = 194, and A_magic = …
Half-lives of beta+ decay and electron capture are studied in some selected superheavy nuclei produced in hot fusion reactions, namely, 290Fl, 293Mc, 294Lv, and 295Ts. The nuclear structure is described microscopically from deformed self-consistent Skyrme Hartree-Fock mean-field calculations that include pairing correlations. The sensitivity of the half-lives to deformation and to the QEC energies, which are still not determined experimentally, are studied. The results are compared with phenomenological alpha-decay half-lives, showing that the latter decay mode is dominant in this mass region.
On the basis of systematic calculations for 1364 heavy and superheavy nuclei, including odd-systems, we have found a few candidates for high-K ground states in superheavy nuclei. The macroscopic-microscopic model based on the deformed Woods-Saxon single particle potential which we use offers a reasonable description of SH systems, including known: nuclear masses, $Q_α$-values, fission barriers, ground state deformations, super- and hyper-deformed minima in the heaviest nuclei. %For odd and odd-odd systems, both ways of including pairing correlations, % blocking and the quasi-particle method, h…
The lifetimes of the consecutive $α$ decay chains of recently synthesized new element 115, $^{287}115$ and $^{288}115$, have been calculated theoretically within the WKB approximation using microscopic $α$-nucleus interaction potentials obtained by folding in the densities of the $α$ and the daughter nuclei with a realistic effective interaction. M3Y effective interaction, supplemented by a zero-range pseudo-potential for exchange along with the density dependence, has been used for calculating the nuclear interaction potentials. Spherical charge distributions have been used for calculating th…
Theoretical estimates for the lifetimes of several isotopes of heavy elements with Z=102-120 are presented by calculating the quantum mechanical tunneling probability in a WKB framework and using microscopic nucleus-nucleus potential obtained by folding the densities of interacting nuclei with the DDM3Y effective nuclear interaction. The $α$-decay half lives calculated in this formalism using the experimental $Q$-values are in good agreement over a wide range of experimental data. Half lives are also calculated using $Q$-values extracted from two mass formulae. The Viola-Seaborg-Sobiczewski (V…
Relativistic energy density functionals (REDF) provide a complete and accurate, global description of nuclear structure phenomena. A modern semi-empirical functional, adjusted to the nuclear matter equation of state and to empirical masses of deformed nuclei, is applied to studies of shapes of superheavy nuclei. The theoretical framework is tested in a comparison of calculated masses, quadrupole deformations, and potential energy barriers to available data on actinide isotopes. Self-consistent mean-field calculations predict a variety of spherical, axial and triaxial shapes of long-lived super…
Recently synthesis of superheavy nuclei has been achieved in hot fusion reactions. A systematic theoretical calculation of alpha decay half-lives in this region of the periodic system, may be useful in the identification of new nuclei in these type of reactions. Alpha decay half-lives are obtained in the framework of the barrier penetration theory, built with the use of proximity and Coulomb forces. It is estimated from a classical viewpoint, a possible angular momentum maximum value for odd and odd-odd nuclei alpha particles. The masses of the nuclei are obtained from a macro-microscopic mode…
The lifetimes of $α$ decays of the recently produced isotopes of the elements 112, 114, 116 and the element $^{294}118$ and of some decay products have been calculated theoretically within the WKB approximation using microscopic $α$-nucleus interaction potentials. These nuclear potentials have been obtained by folding the densities of the $α$ and the daughter nuclei with the M3Y effective interaction, supplemented by a zero-range pseudo-potential for exchange along with the density dependence. Spherical charge distributions have been used for calculating the Coulomb interaction potentials. The…
For $α$ decay half-life calculations in this work, the Coulomb and proximity potential model with a new semiempirical formula for diffuseness parameter developed in previous work [Phys. Rev. C 100, 024601 (2019)] is used. The present model in this work is compared with the generalized liquid-drop model (GLDM), universal decay law (UDL), and experimental half-lives in the region $Z=104-118$. Next, the predicted half-lives of 51 superheavy nuclei (SHN) with $Z=122-125$ by the present model are compared with those of GLDM, and UDL. The present model is revealed to be more accurate in reproducing …
Nuclei with $A>282$ have been studied in the Relativistic Mean Field approach using the force FSU Gold and a zero range pairing interaction. The Euler-Lagrange equations have been solved in the co-ordinate space. Alpha nucleus potential has been constructed with the DDM3Y1 interaction, which has an exponential density dependence, in the double folding model using the nucleon densities in the daughter nucleus and the $α$ particle. Half lives of $α$ decay have been calculated for tunneling of the $α$ particle through the potential barrier in the WKB approximation and assuming a constant preforma…
Cold reaction valleys in the radioactive decay of superheavy nuclei {286}^112, {292}^114 and {296}^116 are studied taking Coulomb and Proximity Potential as the interacting barrier. It is found that in addition to alpha particle, 8^Be, 14^C, 28^Mg, 34^Si, 50^Ca, etc. are optimal cases of cluster radioactivity since they lie in the cold valleys. Two other regions of deep minima centered on 208^Pb and 132^Sn are also found. Within our Coulomb and Proximity Potential Model half-life times and other characteristics such as barrier penetrability, decay constant for clusters ranging from alpha parti…
The $α$- decay half-lives of the superheavy nuclei are systematically studied using different versions of proximity potential and a exact method to calculate Coulomb potential between spherical and deformed nuclei in the framework of the double folding model. To reproduce the $α$-decay half-life, the experimental $α$-decay energy and Wentzel-Kramers-Brillouin approximation have been used. It is found that the computed values by the Ng$\hat{o}$ 80 are in good compromise with the experimental half-lives in comparison with other versions. Also, by using this version and within $Q_{WS4}$ for deter…
An intense study of the alpha decay properties of the isotopes of superheavy element Z=113 have been performed within the Coulomb and proximity potential model for deformed nuclei (CPPMDN) within the wide range 255 l.e. A l.e. 314. The predicted alpha decay half lives of $^{278}$113 and $^{282}$113 and the alpha half lives of their decay products are in good agreement with the experimental data. 6{α) chains and 4α chains predicted respectively for $^{278}$113 and $^{282}$113 are in agreement with the experimental observation. Our study shows that the isotopes in the mass range 278 l.e. A l.e. …
Spontaneous fission and alpha decay are the main decay modes for superheavy nuclei. The superheavy nuclei which have small alpha decay half-life compared to spontaneous fission half-life will survive fission and can be detected in the laboratory through alpha decay. We have studied the alpha decay half-life and spontaneous half-life of some superheavy elements in the atomic range Z = 100-130. Spontaneous fission half-lives of superheavy nuclei have been calculated using the phenomenological formula and the alpha decay half-lives using Viola-Seaborg-Sobiczewski formula (Sobiczewski et al. 1989)…
In this work, the $β$-stable region for Z $\geq$ 90 is proposed. The calculated $β$-stable nuclei in the $β$-stable region are in good agreement with the ones obtained by Möller \emph{et al}.. The half-lives of the nuclei close to the $β$-stable region are calculated and the competition between $α$-decay and $β$-decay is systematically investigated. The calculated half-lives and the suggested decay modes are well in line with the experimental results. The predictions for half-lives and decay modes of the nuclei with Z = 107$-$110 are presented.
We have investigated properties of $α$-decay chains of recently produced superheavy elements Z=115 and Z=113 using the new Lagrangian model NL-SV1 with inclusion of the vector self-coupling of $ω$ meson in the framework of the relativistic mean-field theory. It is shown that the experimentally observed alpha-decay energies and half-lives are reproduced well by this Lagrangian model. Further calculations for the heavier elements with Z=117-125 show that these nuclei are superdeformed with a prolate shape in the ground state. A superdeformed shell-closure at Z=118 lends an additional binding and…
The concept of heavy particle radioactivity (HPR) is changed to allow emitted particles with Z_e>28 from parents with Z>110 and daughter around 208Pb. Calculations for superheavy (SH) nuclei with Z=104-124 are showing a trend toward shorter half-lives and larger branching ratio relative to alpha decay for heavier SHs. It is possible to find regions in which HPR is stronger than alpha decay. The new mass table AME11 and the theoretical KTUY05 and FRDM95 masses are used to determine the released energy. For 124 we found isotopes with half-lives in the range of ns to ps.
The probability of $α$ particle emission for some recently observed superheavy nuclei (SHN) are investigated. The $α$-decay half lives of SHN are calculated in a quantum tunneling model with density dependent M3Y (DDM3Y) effective nuclear interaction using theoretical and measured $Q_α$ values. We determine the density distribution of $α$ and daughter nuclei from the relativistic mean field theory (RMF) using FSUGold force, NL3 and TM1 parameter sets. The double folded nuclear potential is numerically calculated in a more microscopic manner using these density distributions. The estimated valu…
Magic islands for extra-stable nuclei in the midst of the sea of fission-instability were predicted to be around Z=114, 124 or, 126 with N=184, and Z=120, with N=172. Whether these fission-survived superheavy nuclei with high Z and N would live long enough for detection or, undergo alpha-decay in a very short time remains an open question. Alpha-decay half lives of nuclei with 130 < Z < 100 have been calculated in a WKB framework using density-dependent M3Y interaction with Q-values from different mass formulae. The results are in excellent agreement with the experimental data. Fission survive…
In this paper, we have calculated the $α$-decay half-lives of superheavy nuclei with $106 \leq Z \leq 126$ and a neutron number of $150 \leq N \leq 200$ within proximity potentials and deformed-spherical Coulomb potentials by using $WS4$ $α$-decay energy and the semi-classical Wentzel-Kramers-Brillouin approximation for penetration probability. Besides, we have included the preformation factor within the cluster-formation model. We have investigated magic numbers and submagic numbers in the mentioned region; with high probability 162, 178, and 184 are predicted as neutron magic numbers. We als…
The feasibility for the alpha decay and the heavy particle decay from the even-even superheavy (SH) nuclei with Z = 116-124 have been studied within the Coulomb and proximity potential model (CPPM). The Universal formula for cluster decay (UNIV) of Poenaru et al., the Universal Decay Law (UDL) and the Scaling Law of Horoi et al., has also been used for the evaluation of the decay half lives. A comparison of our predicted half lives with the values evaluated using these empirical formulas are in agreement with each other and hence CPPM could be considered as a unified model for alpha and cluste…
The cluster decay process in $^{270-318}$118 superheavy nuclei has been studied extensively within the Coulomb and proximity potential model (CPPM), thereby investigating the probable cluster decays from the various isotopes of $Z = 118$. On comparing the predicted decay half lives with the values evaluated using the Universal formula for cluster decay (UNIV) of Poenaru et al., the Universal Decay Law (UDL) of Qi et al., and the Scaling Law of Horoi et al., it was seen that, our values matches well with these theoretical values. A comparison of the predicted alpha decay half life of the experi…
The connection of synthesis of long-lived superheavy nuclei and existence of the island of stability with the choice of realistic nuclear potential is discussed: the behaviour of the average field of nuclei is an important element of nuclear models. It is also shown that it is just Dubna that possesses the priority both in the recent synthesis of a superheavy nucleus with charge Z=114 and in its theoretical prediction made 35 years ago. Possible sizes of the island of stability of superheavy nuclei are considered.
We study stability of superdeformed oblate (SDO) superheavy $Z\geq 120$ nuclei predicted by systematic macroscopic-microscopic calculations in 12D deformation space and confirmed by the Hartree-Fock calculations with the realistic SLy6 force. We include into consideration high-$K$ isomers that very likely form at the SDO shape. Although half-lives $T_{1/2}\lesssim10^{-5}$ s are calclulated or estimated for even-even spin zero systems, decay hindrances known for high-$K$ isomers suggest that some SDO superheavy nuclei may be detectable by the present experimental technique.
In present work, we systematically study the $α$ decay half-lives of 170 even-even nuclei with $60 \leqslant Z \leqslant 118$ within the two-potential approach while the $α$ decay preformation factor $P_α$ is obtained by the cluster-formation model. The calculated results can well reproduce the experimental data. In addition, we extend this model to predict the $α$ decay half-lives of 64 even-even nuclei with $104 \leqslant Z \leqslant 128$ whose $α$ decay is energetically allowed or observed but not yet quantified. For comparing, the two famous models i.e. SemFIS proposed by D. Poenaru ${et\ …
The $α$-decay half-lives of 204 superheavy nuclei covering the range $114 \leq Z \leq 126$ have been investigated using the relativistic mean-field model (RMF) for NL3$^*$ parameter set. The ground state bulk properties such as binding energy, quadrupole deformation parameter ($β_2$ ), and root-mean-square charge radii for these nuclei are analyzed. Four different semi-empirical formulae, namely, the universal decay law (UDL), the Viola-Seaborg (VSS) formula, the modified universal decay law (MUDL), and the modified Brown formula (MBrown), are used to obtain the $α$-decay half-lives for the co…
The constrained Hartree-Fock-Bogoliubov approximation, based on the recent parametrization D1M$^{*}$ of the Gogny energy density functional, is used to describe fission in 435 superheavy nuclei. The Gogny-D1M$^{*}$ parametrization is benchmarked against available experimental data on inner and second barrier heights, excitation energies of the fission isomers and half-lives in a selected set of Pu, Cm, Cf, Fm, No, Rf, Sg, Hs and Fl nuclei. Results are also compared with those obtained with the Gogny-D1M energy density functional. A detailed study of the minimal energy fission paths is carried …
The competition between alpha- and beta+/EC-decay modes is studied systematically in nuclei along the alpha-decay chains following the synthesis of superheavy nuclei with Z = 119 and Z = 120. A microscopic approach based on deformed self-consistent Hartree-Fock mean-field calculations with Skyrme forces and pairing correlations is used to describe the beta+ and electron capture weak decays, whereas the alpha-decay is estimated from existing phenomenological expressions. It is shown that alpha-decay is in most cases the dominant decay mode, but interesting instances are identified where the hal…
Configuration-constrained calculations of potential-energy surfaces in even-even superheavy nuclei reveal systematically the existence at low excitation energies of multi-quasiparticle states with deformed axially symmetric shapes and large angular momenta. These results indicate the prevalence of long-lived, multi-quasiparticle isomers. In a quantal system, the ground state is usually more stable than the excited states. In contrast, in superheavy nuclei the multi-qausiparticle excitations decrease the probability for both fission and $α$ decay, implying enhanced stability. Hence, the systema…
The barriers standing against the formation of superheavy elements and their consecutive $α$ decay have been determined in the quasimolecular shape path within a Generalized Liquid Drop Model including the proximity effects between nucleons in a neck, the mass and charge asymmetry, a precise nuclear radius and the shell effects given by the Droplet Model. For moderately asymmetric reactions double-hump potential barriers stand and fast fission of compact shapes in the outer well is possible. Very asymmetric reactions lead to one hump barriers which can be passed only with a high energy relativ…
Taking the Coulomb and proximity potential model for deformed nuclei (CPPMDN) as the interacting potential for the post-scission region, the alpha decay properties of 34 isotopes of the superheavy nuclei with Z = 128 within the range 306 $\leq$ A $\leq$ 339 have been studied, considering both the parent and daughter nuclei to be deformed. The manuscript also deals with the decay properties of the isotopes of Z = 126 (within 288 $\leq$ A $\leq$ 339), Z = 124 (within 284 $\leq$A $\leq$ 339) and Z = 122 (within 280 $\leq$ A $\leq$ 339). The alpha decay half lives thus evaluated has been compared …
Starting from the WKB approximation, a new barrier penetration formula is proposed for potential barriers containing a long-range Coulomb interaction. This formula is especially proper for the barrier penetration with penetration energy much lower than the Coulomb barrier. The penetrabilities calculated from the new formula agree well with the results from the WKB method. As a first attempt, this new formula is used to evaluate alpha decay half-lives of atomic nuclei and a good agreement with the experiment is obtained.
Mathematical model of heavy and superheavy nuclei production in intensive pulsed neutron fluxes of explosive process is developed. The pulse character of the process allows dividing it in time into two stages: very short rapid process of multiple neutron captures with higher temperature and very intensive neutron fluxes, and relatively slower process with lower temperature and neutron fluxes. The model was also extended for calculation of the transuranium yields in nuclear explosions takes into account the adiabatic character of the process, the probabilities of delayed fission, and the emissi…
