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arXiv 1109.0384cond-mat.str-el
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角分辨NMR:BaFe2As2中~(75)As T1弛豫速率的定量理论

Angle-resolved NMR: quantitative theory of 75As T1 relaxation rate in BaFe2As2

Andrew Smerald, Nic Shannon

摘要:

虽然核能谱的NMR测量通常用于表征量子磁体的静态性质,但是锁定在NMR 1/T1弛豫速率中的动态信息仍然非常难以解释。困难来自于这样一个事实,即关于电子所有可能的低能自旋激发及其与核磁矩的耦合的信息被折叠成一个单一的数字1/T1。在这里,我们开发了共线反铁磁体的NMR 1/T1弛豫速率的定量理论,专注于BaFe 2As 2的具体例子。BaFe_2As_2最显著的磁性特征之一是1/T_1与外加磁场的方向有很强的依赖性。通过仔细分析的核和电子的时刻之间的耦合,我们展示了这种各向异性如何产生的“过滤”的自旋波动的形状因子转移超精细相互作用。这使我们能够使令人信服的,定量的,适合BaFe 2As 2的实验1/T1数据,对于不同的磁场方向。我们继续展示如何定量的,角度依赖的弛豫率理论导致新的方法来测量磁系统的动力学参数,特别是自旋波的速度。

英文摘要:

While NMR measurements of nuclear energy spectra are routinely used to characterize the static properties of quantum magnets, the dynamical information locked in NMR 1/T1 relaxation rates remains notoriously difficult to interpret. The difficulty arises from the fact that information about all possible low-energy spin excitations of the electrons, and their coupling to the nuclear moments, is folded into a single number, 1/T1. Here we develop a quantitative theory of the NMR 1/T1 relaxation rate in a collinear antiferromagnet, focusing on the specific example of BaFe2As2. One of the most striking features of magnetism in BaFe2As2 is a strong dependence of 1/T1 on the orientation of the applied magnetic field. By careful analysis of the coupling between the nuclear and electronic moments, we show how this anisotropy arises from the "filtering" of spin fluctuations by the form-factor for transferred hyperfine interactions. This allows us to make convincing, quantitative, fits to experimental 1/T1 data for BaFe2As2, for different field orientations. We go on to show how a quantitative, angle-dependent theory for the relaxation rate leads to new ways of measuring the dynamical parameters of magnetic systems, in particular the spin wave velocities.

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