Correlated signal and idler photon pairs with small detuning in the telecom band can be generated through spontaneous four-wave mixing in dispersion shift fibers. However, photons originated from other nonlinear processes in optical fibers, such as Raman scattering and self-phase modulation, may contaminate the photon pairs. It has been proved that photons produced by Raman scattering are the background noise of photon pairs. Here we show that photons induced by self-phase modulation of pump pulses are another origin of background noise. After studying the dependence of self-phase modulation induced photons in signal and idler bands, we demonstrate that the quantum correlation of photon pairs can be degraded by the self-phase modulation effect. The investigations are useful for characterizing and optimizing an all fiber source of photon pairs.
We present an experimental proposal for the generation of photon triplets based on third-order spontaneous para- metric downconversion in thin optical fibers. Our analysis includes expressions for the quantum state, which de- scribes the photon triplets and for the generation rate in terms of all experimental parameters. We also present, for a specific source design, numerically calculated generation rates.
This paper reports 1.5-um band time-bin entanglement generation. We employed a spontaneous four-wave mixing process in a dispersion shifted fiber, with which correlated photon pairs with very narrow bandwidths were generated efficiently. To observe two-photon interference, we used planar lightwave circuit based interferometers that were operated stably without feedback control. As a result, we obtained coincidence fringes with 99 % visibilities after subtracting accidental coincidences, and successfully distributed entangled photons over 20-km standard single-mode fiber without any deteriorati…
We report the generation of polarization entangled photon pairs in the 1550-nm wavelength band using spontaneous four-wave mixing in a dispersion-shifted fiber loop. The use of the fiber-loop configuration made it possible to generate polarization entangled states very stably. With accidental coincidences subtracted, we obtained coincidence fringes with >90 % visibilities, and observed a violation of Bell's inequality by seven standard deviations. We also confirmed the preservation of the quantum correlation between the photons even after they had been separated by 20 km of optical fiber.
We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered photon-pair-generation scheme utilizes pump-pulse walk-off to produce pure heralded photons and phase matching is achieved through the dispersion properties of distinct spatial modes in a few-mode silica step-index fiber. We show that fiber-core-radius fluctuations in general severely impact the single-photon purity. Furthermore, by optimizing the fiber desig…
We study the third order spontaneous parametric down conversion (TOSPDC) process, as a means to generate entangled photon triplets. Specifically, we consider thin optical fibers as the nonlinear medium to be used as the basis for TOSPDC in configurations where phase matching is attained through the use of more than one fiber transverse modes. Our analysis in this paper, which follows from our earlier paper Optics Letters 36, 190 (2011), aims to supply experimentalists with the details required in order to design a TOSPDC photon-triplet source. Specifically, our analysis focuses on the photon t…
We study theoretically the generation of photon pairs by spontaneous four-wave mixing (SFWM) in photonic crystal optical fiber. We show that it is possible to engineer two-photon states with specific spectral correlation (``entanglement'') properties suitable for quantum information processing applications. We focus on the case exhibiting no spectral correlations in the two-photon component of the state, which we call factorability, and which allows heralding of single-photon pure-state wave packets without the need for spectral post filtering. We show that spontaneous four wave mixing exhibit…
We present a study of the spectral properties of photon pairs generated through the process of spontaneous four wave mixing (SFWM) in single mode fiber. Our analysis assumes narrowband pumps, which are allowed to be frequency-degenerate or non-degenerate. Based on this analysis, we derive conditions on the pump frequencies and on the fiber dispersion parameters which guarantee the generation of ultra-broadband photon pairs. Such photon pairs are characterized by: i) a very large degree of entanglement, and ii) a very high degree of temporal synchronization between the signal and idler photons.…
A novel time-domain approach using the momentum operator is used to model spontaneous four-wave mixing in a lossless nonlinear waveguide. The effects of self- and cross-phase modulation on the photon-pair production rate and heralded photon purity are investigated. We show that in the special case where only one half of the photon-pair state is filtered that the generation rate and purity of the heralded photons are unmodified by the presence of self- and cross-phase modulation. The significance of this special case arises when we consider heralded single-photon sources, where future schemes a…
We study scalar and vector modulation instabilities induced by the vacuum fluctuations in birefringent optical fibers. To this end, stochastic coupled nonlinear Schrodinger equations are derived. The stochastic model is equivalent to the quantum field operators equations and allow for dispersion, nonlinearity, and arbitrary level of birefringence. Numerical integration of the stochastic equations is compared to analytical formulas in the case of scalar modulation instability and non depleted pump approximation. The effect of classical noise and its competition with vacuum fluctuations for indu…
We study spontaneous emission from a rubidium atom into the fundamental and higher-order modes of a vacuum-clad ultrathin optical fiber. We show that the spontaneous emission rate depends on the magnetic sublevel, the type of modes, the orientation of the quantization axis, and the fiber radius. We find that the rate of spontaneous emission into the TE modes is always symmetric with respect to the propagation directions. Directional asymmetry of spontaneous emission into other modes may appear when the quantization axis does not lie in the meridional plane containing the position of the atom. …
This paper reports the first demonstration of the generation and distribution of entangled photon pairs in the 1.5-um band using spontaneous four-wave mixing in a cooled fiber. Noise photons induced by spontaneous Raman scattering were suppressed by cooling a dispersion shifted fiber with liquid nitrogen, which resulted in a significant improvement in the visibility of two-photon interference. By using this scheme, time-bin entangled qubits were successfully distributed over 60 km of optical fiber with a visibility of 76%, which was obtained without removing accidental coincidences.
We suggest the generation of photon pairs in a thermally induced nonlinear periodically-poled silica fiber by spontaneous parametric down-conversion. Photons are generated directly in eigenstates of optical angular momentum. Photons in a pair can be entangled in these states as well as in frequencies. We identify suitable spatial and polarization modes giving an efficient nonlinear interaction. By changing the pump field properties both narrow- and broad-band down-converted fields can be obtained.
We study the processes of spontaneous four wave mixing and of third-order spontaneous parametric downconversion in optical fibers, as the basis for the implementation of photon-pair and photon-triplet sources. We present a comparative analysis of the two processes including expressions for the respective quantum states and plots of the joint spectral intensity, a discussion of phasematching characteristics, and expressions for the conversion efficiency. We have also included a comparative study based on numerical results for the conversion efficiency for the two sources, as a function of sever…
We investigate (a) spontaneous Raman scattering of classical signals in long optical fiber links leading to significant Raman noise in quantum channels propagating in the same fiber and (b) impact of chromatic dispersion on the performance of high quantum bit rate QKD systems. One way of decreasing Raman noise is to decrease the classical signal power. This may be achieved by the use of coherent modulation formats and the deployment of Forward Error Correction technology. Additionally, low loss fiber with small Raman gain at telecom wavelengths enables the simultaneous transmission of multiple…
We put forth an approach to obtain a quantum master equation for the propagation of light in nonlinear fiber optics by relying on simple quantum pictures of the processes (linear and nonlinear) occurring along propagation in an optical fiber. This equation is shown to be in excellent agreement with the classical Generalized Nonlinear Schrodinger Equation and predicts the effects of self-steepening and spontaneous Raman scattering. Last, we apply these results to the analysis of two cases of relevance in quantum technologies: single-photon frequency translation and spontaneous four-wave mixing.
We study the generation of correlated photon pairs and heralded single photons via strongly non-degenerate spontaneous four-wave mixing (SFWM) in a series of identical micro-/nano fibers (MNF). Joint spectral intensity of the biphoton field generated at the wavelength of about 880 nm and 1310 nm has been measured under excitation by 100 ps laser pulses demonstrating good agreement with the theoretical prediction. The measured zero-time second-order autocorrelation function was about 0.2 when the emission rate of the heralded photons was of 4 Hz. The MNF-based source perfectly matches standard …
We study a novel scheme named spontaneous parametric fiber loop (SPFL), configured by deliberately intro- ducing dispersive elements into the nonlinear Sagnac loop, and show it can function as a passive switch of photon pairs. The two-photon state coming out of SPFL highly depends on the dispersion induced phase difference of photon pairs counter-propagating in the loop. By properly managing the dispersive elements, the signal and idler photons of a pair with a certain detuning and bandwidth can be directed to the desired spatial modes of SPFL. If the photon pairs are used to generate heralded…
We study both experimentally and theoretically the generation of photon pairs by spontaneous four-wave mixing (SFWM) in standard birefringent optical fibers. The ability to produce a range of two-photon spectral states, from highly correlated (entangled) to completely factorable, by means of cross-polarized birefringent phase matching, is explored. A simple model is developed to predict the spectral state of the photon pair which shows how this can be adjusted by choosing the appropriate pump bandwidth, fiber length and birefringence. Spontaneous Raman scattering is modeled to determine the tr…
The binary (one-bit-per-photon) encoding that most existing quantum key distribution (QKD) protocols employ puts a fundamental limit on their achievable key rates, especially under high channel loss conditions associated with long-distance fiber-optic or satellite-to-ground links. Inspired by the pulse-position-modulation (PPM) approach to photon-starved classical communications, we design and demonstrate the first PPM-QKD, whose security against collective attacks is established through continuous-variable entanglement measurements that also enable a novel decoy-state protocol performed conve…
The photonic crystal fiber (PCF) is one of the excellent media for generating photon pairs via spontaneous four wave mixing. Here we study how the inhomogeneity of PCFs affect the spectral properties of photon pairs from both the theoretical and experimental aspects. The theoretical model shows that the photon pairs born in different place of the inhomogeneous PCF are coherently superposed, and a modulation in the broadened spectrum of phase matching function will appear, which prevents the realization of spectral factorable photon pairs. In particular, the inhomogeneity induced modulation can…
We present a theoretical and experimental study of the generation of photon pairs through the process of spontaneous four wave mixing (SFWM) in a few-mode, birefringent fiber. Under these conditions, multiple SFWM processes are in fact possible, each associated with a different combination of transverse modes for the four waves involved. We show that in the weakly guiding regime, for which the propagation modes may be well approximated by linearly polarized modes, the departure from circular symmetry due to the fiber birefringence translates into conservation rules which retain elements from a…
We experimentally demonstrate the generation of a three-photon discrete-energy-entangled W state using multi-photon-pair generation by spontaneous four-wave mixing in an optical fiber. We show that by making use of prior information on the photon source we can verify the state produced by this source without resorting to frequency conversion.
We propose an effective scheme for realizing a long-range quantum state phase-covariant cloning between two qubits in fiber-nanocavity system via an adiabatic passage. Since no cavity (fiber) photons or excited levels of the nitrogen-vacancy (NV) center are populated during the whole process, the scheme is immune to the decay of cavity (fiber) and spontaneous emission of the NV center. The strictly numerical simulation shows that the fidelity is high even in the presence of realistic imperfections.
We report on theoretical and experimental demonstration of high-efficiency coupling of two-photon entangled states produced in the nonlinear process of spontaneous parametric down conversion into a single-mode fiber. We determine constraints for the optimal coupling parameters. This result is crucial for practical implementation of quantum key distribution protocols with entangled states.
We report on the experimental characterization of a novel nonlinear liquid-filled hollow-core photonic-crystal fiber for the generation of photon pairs at telecommunication wavelength through spontaneous four-wave-mixing. We show that the optimization procedure in view of this application links the choice of the nonlinear liquid to the design parameters of the fiber, and we give an example of such an optimization at telecom wavelengths. Combining the modeling of the fiber and classical characterization techniques at these wavelengths, we identify, for the chosen fiber and liquid combination, s…
We study the force of light on a two-level atom near an ultrathin optical fiber using the mode function method and the Green tensor technique. We show that the total force consists of the driving-field force, the spontaneous-emission recoil force, and the fiber-induced van der Waals potential force. Due to the existence of a nonzero axial component of the field in a guided mode, the Rabi frequency and, hence, the magnitude of the force of the guided driving field may depend on the propagation direction. When the atomic dipole rotates in the meridional plane, the spontaneous-emission recoil for…
Preservation of photon statistics upon selective molecular modulation in hollow-core fibers
University of the Basque Country (EHU)（巴斯克大学）；University of Limoges（利摩日大学）；CNRS UMR 7252（法国国家科学研究中心）；University of Erlangen-Nürnberg（埃尔朗根-纽伦堡大学）；Max Planck Institute for the Science of Light（马克斯·普朗克光科学研究所）；IKERBASQUE, Basque Foundation for Science（伊克尔巴斯基奎，巴斯克科学基金会）
High coherent frequency-entangled photons at telecom band are critical in quantum information protocols and quantum tele-communication. While photon pairs generated by spontaneous parametric down-conversion in nonlinear crystal or modulation instability in optical fiber exhibit random fluctuations, making the photons distinguishable among consecutive roundtrips. Here, we demonstrate a frequency-entangled photons based on parametric instability in an active fiber ring cavity, where periodic modulation of dispersion excites parametric resonance. The characteristic wave number in parametric insta…
Photons occupying multiple spatial modes hold a great promise for implementing high-dimensional quantum communication. We use spontaneous four-wave mixing to generate multimode photon pairs in a few mode fiber. We show the photons are correlated in the fiber mode basis using an all-fiber mode sorter. Our demonstration offers an essential building block for realizing high-dimensional quantum protocols based on standard, commercially available fibers, in an all-fiber configuration.
We report on a series of experiments on the dynamics of spontaneous emission controlled nanolasers. The laser cavity is a photonic crystal slab cavity, embedding self-assembled quantum dots as gain material. The implementation of cavity electrodynamics effects increases significantly the large signal modulation bandwidth, with measured modulation speeds of the order of 10 GHz while keeping an extinction ratio of 19 dB. A linear transient wavelength shift is reported, corresponding to a chirp of less than 100 pm for a 35-ps laser pulse. We observe that the chirp characteristics are independent …
