A study of the effects of absorption on the nonlinear process of parametric down conversion is presented. Absorption within the nonlinear medium is accounted for by employing the framework of macroscopic QED and the Green tensor quantization of the electromagnetic field. An effective interaction Hamiltonian, which describes the nonlinear interaction of the electric field and the linear noise polarization field, is used to derive the quantum state of the light leaving a nonlinear crystal. The signal and idler modes of this quantum state are found to be a superpositions of the electric and noise polarization fields. Using this state, the expression for the coincident count rates for both Type I and Type II conversion are found. The nonlinear interaction with the noise polarization field were shown to cause an increase in the rate on the order of 10^{-12} for absorption of 10% per cm. This astonishingly small effect is found to be negligible compared to the decay caused by linear absorption of the propagating modes. From the expressions for the biphoton amplitude it can be seen the maximally entangled states can still be produced even in the presence of strong absorption.
Using a recently developed formalism of quantization of radiation in the presence of absorbing dielectric bodies, the problem of photon tunneling through absorbing barriers is studied. The multilayer barriers are described in terms of multistep complex permittivities in the frequency domain which satisfy the Kramers--Kronig relations. From the resulting input--output relations it is shown that losses in the layers may considerably change the photon tunneling times observed in two-photon interference experiments. It is further shown that for sufficiently large numbers of layers interference fri…
The eletromagnetic field in a linear absorptive dielectric medium, is quantized in the framework of the damped polarization model. A Hamiltonian containing a reservoir with continuous degrees of freedom, is proposed. The reservoir minimally interacts with the dielectric polarization and the electromagnetic field. The Lagevin-Schrodinger equation is obtained as the equation of motion of the polarization field. The radiation reaction electromagnetic field is considered. For a homogeneous medium, the equations of motion are solved using the Laplace transformation method.
The theory developed by Gruner and Welsch [Phys. Rev. A 54, 1661 (1996)] for calculating the 1D input-output relations of the quantized electromagnetic field at dispersing and absorbing dielectric (multilayer) plates is generalized to the three-dimensional case. First a general recipe for the derivation of the reflection and transmission coefficients at an arbitrary body that separates two half spaces from each other is presented. The general theory is then applied to the case of planar multilayer structures, for which the Green tensor is well-known.
Recently two methods have been developed for the quantization of the electromagnetic field in general dispersing and absorbing linear dielectrics. The first is based upon the introduction of a quantum Langevin current in Maxwell's equations [T. Gruner and D.-G. Welsch, Phys. Rev. A 53, 1818 (1996); Ho Trung Dung, L. Knöll, and D.-G. Welsch, Phys. Rev. A 57, 3931 (1998); S. Scheel, L. Knöll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)], whereas the second makes use of a set of auxiliary fields, followed by a canonical quantization procedure [A. Tip, Phys. Rev. A 57, 4818 (1998)]. We show that…
Starting from the quantized version of Maxwell's equations for the electromagnetic field in an arbitrary linear Kramers-Kronig dielectric, spontaneous decay of the excited state of a two-level atom embedded in a dispersive and absorbing medium is studied and the decay rate is calculated. The calculations are performed for both the (Clausius-Mosotti) virtual cavity model and the (Glauber-Lewenstein) real cavity model. It is shown that owing to nonradiative decay associated with absorption the rate of spontaneous decay sensitively depends on the cavity radius when the atomic transition frequency…
A quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive and absorbing dielectric medium is developed. The classical Maxwell equations with spatially varying and Kramers-Kronig consistent permittivity are regarded as operator-valued field equations, introducing additional current- and charge-density operator fields in order to take into account the noise associated with the dissipation in the medium. It is shown that the equal-time commutation relations between the fundamental electromagnetic fields $\hat …
We present a formalism for studying the influence of dispersive and absorbing dielectric bodies on a radiating atom in the framework of quantization of the phenomenological Maxwell equations for given complex permittivities of the bodies. In Markov approximation, the rate of spontaneous decay and the line shift associated with it can then be related to the complex permittivities and geometries of the bodies via the dyadic Green function of the classical boundary value problem of electrodynamics -- a result which is in agreement with second-order calculations for microscopic model systems. The …
The spontaneous emission rate of a radiating atom reaches its time-independent equilibrium value after an initial transient regime. In this paper we consider the associated relaxation effects of the spontaneous decay rate of atoms in dispersive and absorbing dielectric media for atomic transition frequencies near material resonances. A quantum mechanical description of such media is furnished by a damped-polariton model, in which absorption is taken into account through coupling to a bath. We show how all field and matter operators in this theory can be expressed in terms of the bath operators…
Spontaneous emission and Lamb shift of atoms in absorbing dielectrics are discussed. A Green's-function approach is used based on the multipolar interaction Hamiltonian of a collection of atomic dipoles with the quantised radiation field. The rate of decay and level shifts are determined by the retarded Green's-function of the interacting electric displacement field, which is calculated from a Dyson equation describing multiple scattering. The positions of the atomic dipoles forming the dielectrics are assumed to be uncorrelated and a continuum approximation is used. The associated unphysical …
Within the framework of exact quantum electrodynamics in dielectric, we study the topological Berry phase of a classically pumped $Λ$-type three-level atom, prepared initially in a superposition of its two pumped levels and located near a planar dielectric half-space with model permittivity of Lorentz type, interacts with a vacuum field. The effects of material losses, expressed in terms of the Green tensor of the dielectric-matter formation including dispersion and absorption, on the topological Berry phase of the photon transition between the pumped levels have been studied. The outcomes are…
Recently the influence of dielectric and geometrical properties on the Casimir force between dispersing and absorbing multilayered plates in the zero-temperature limit has been studied within a 1D quantization scheme for the electromagnetic field in the presence of causal media [R. Esquivel-Sirvent, C. Villarreal, and G.H. Cocoletzi, Phys. Rev. Lett. 64, 052108 (2001)]. In the present paper a rigorous 3D analysis is given, which shows that for complex heterostructures the 1D theory only roughly reflects the dependence of the Casimir force on the plate separation in general. Further, an extensi…
A general theory of the interaction of the quantized electromagnetic field with atoms in the presence of dispersing and absorbing dielectric bodies of given Kramers--Kronig consistent permittivities is developed. It is based on a source-quantity representation of the electromagnetic field, in which the electromagnetic-field operators are expressed in terms of a continuous set of fundamental bosonic fields via the Green tensor of the classical problem. Introducing scalar and vector potentials, the formalism is extended in order to include in the theory the interaction of the quantized electroma…
The phenomenological Maxwell field is quantized for arbitrarily space- and frequency-dependent complex permittivity. The formalism takes account of the Kramers--Kronig relation and the dissipation-fluctuation theorem and yields the fundamental equal-time commutation relations of QED. Applications to the quantum-state transformation at absorbing and amplifying four-port devices and to the spontaneous decay of an excited atom in the presence of absorbing dielectric bodies are discussed.
Dielectric four-port devices play an important role in optical quantum information processing. Since for causality reasons the permittivity is a complex function of frequency, dielectrics are typical examples of noisy quantum channels, which cannot preserve quantum coherence. To study the effects of quantum decoherence, we start from the quantized electromagnetic field in an arbitrary Kramers--Kronig dielectric of given complex permittivity and construct the transformation relating the output quantum state to the input quantum state, without placing restrictions on the frequency. We apply the …
A formalism for studying spontaneous decay of an excited two-level atom in the presence of dispersing and absorbing dielectric bodies is developed. An integral equation, which is suitable for numerical solution, is derived for the atomic upper-state-probability amplitude. The emission pattern and the power spectrum of the emitted light are expressed in terms of the Green tensor of the dielectric-matter formation including absorption and dispersion. The theory is applied to the spontaneous decay of an excited atom at the center of a three-layered spherical cavity, with the cavity wall being mod…
After giving an outline of the quantization scheme based on the microscopic Hopfield model of a dielectric bulk material, we show how the classical phenomenological Maxwell equations of the electromagnetic field in the presence of dielectric matter of given space- and frequency-dependent complex permittivity can be transferred to quantum theory. Including in the theory the interaction of the medium-assisted field with atomic systems, we present both the minimal-coupling Hamiltonian and the multipolar-coupling Hamiltonian in the Coulomb gauge. To illustrate the concept, we discuss the input--ou…
Spontaneous decay of an excited atom near a dispersing and absorbing microsphere of given complex permittivity that satisfies the Kramers-Kronig relations is studied, with special emphasis on a Drude-Lorentz permittivity. Both the whispering gallery field resonances below the band gap (for a dielectric sphere) and the surface-guided field resonances inside the gap (for a dielectric or a metallic sphere) are considered. Since the decay rate mimics the spectral density of the sphere-assisted ground-state fluctuation of the radiation field, the strengths and widths of the field resonances essenti…
The decay rate and the classical radiation power of an excited molecule (atom) located in the center of a dispersive and absorbing dielectric sphere taken as a simple model of a cavity are calculated adopting the Onsager model for the local field. The local-field correction factor to the external (radiation and absorption) power loss of the molecule is found to be $|3ε(ω)/[3ε(ω)+1]|^2$, with $ε(ω)$ being the dielectric function of the sphere. However, local-field corrections to the total decay rate (power loss) of the molecule are found to be much more complex, including those to the decay rat…
We build up a consistent theory of quantum electrodynamics in the presence of macroscopic polarizable media. We use the Huttner-Barnett model of a dispersive and absorbing dielectric medium and formulate the theory in terms of interacting quantum fields. We integrate out the damped polaritons by using diagrammatic techniques and find an exact expression for the displacement field (photon) propagator in the presence of a dispersive and absorbing dielectric half-space. This opens a new route to traceable perturbative calculations of the same kind as in free-space quantum electrodynamics. As a wo…
By using the Green-function concept of quantization of the electromagnetic field in dispersing and absorbing media, the quantized field in the presence of a dispersing and absorbing dielectric multilayer plate is studied. Three-dimensional input-output relations are derived for both amplitude operators in the ${\bf k}$-space and the field operators in the coordinate space. The conditions are discussed, under which the input-output relations can be expressed in terms of bosonic operators. The theory applies to both (effectively) free fields and fields, created by active atomic sources inside an…
The derivation of Casimir forces between dielectrics can be simplified by ignoring absorption, calculating energy changes due to displacements of the dielectrics, and only then admitting absorption by allowing permittivities to be complex. As a first step towards a better understanding of this situation we consider in this paper the model of a dielectric as a collection of oscillators, each of which is coupled to a reservoir giving rise to damping and Langevin forces on the oscillators and a noise polarization acting as a source of a fluctuating electromagnetic (EM) field in the dielectric. Th…
The Casimir effect in a dispersive and absorbing multilayered system is considered adopting the (net) vacuum-field pressure point of view to the Casimir force. Using the properties of the macroscopic field operators appropriate for absorbing systems and a convenient compact form of the Green function for a multilayer, a straightforward and transparent derivation of the Casimir force in a lossless layer of an otherwise absorbing multilayer is presented. The resulting expression in terms of the reflection coefficients of the surrounding stacks of layers is of the same form as that obtained by Zh…
Recently a quantization scheme for the phenomenological Maxwell theory of the full electromagnetic field in an inhomogeneous three-dimensional, dispersive, and absorbing dielectric medium has been developed and applied to a system consisting of two infinite half-spaces with a common planar interface (H.T. Dung, L. Knoell, and D.-G. Welsch, Phys. Rev. A 57, in press). Here we show that the scheme, which is based on the classical Green-tensor integral representation of the electromagnetic field, applies to any inhomogeneous medium. For this purpose we prove that the fundamental equal-time commut…
Within leading-order perturbation theory, the Casimir-Polder potential of a ground-state atom placed within an arbitrary arrangement of dispersing and absorbing linear bodies can be expressed in terms of the polarizability of the atom and the scattering Green tensor of the body-assisted electromagnetic field. Based on a Born series of the Green tensor, a systematic expansion of the Casimir-Polder potential in powers of the susceptibilities of the bodies is presented. The Born expansion is used to show how and under which conditions the Casimir-Polder force can be related to microscopic many-at…
We derive an effective Hamiltonian for the nonlinear process of parametric down conversion in the presence of absorption. Based upon the Green function method for quantizing the electromagnetic field, we first set up Heisenberg's equations of motion for a single atom driven by an external electric field and in the presence of an absorbing dielectric material. The equations of motion are then solved to second order in perturbation theory which, in rotating-wave approximation, yields the standard effective interaction Hamiltonian known from free-space nonlinear optics. In a second step, we deriv…
The decay of an excited atom in the presence of a medium that both scatters and absorbs radiation is studied with the help of a quantum-electrodynamical model. The medium is represented by a half space filled with a randomly distributed set of non-overlapping spheres, which consist of a linear absorptive dielectric material. The absorption effects are described by means of a quantized damped-polariton theory. It is found that the effective susceptibility of the bulk does not fully account for the medium-induced change in the atomic decay rate. In fact, surface effects contribute to the modific…
The influence of the size and shape of a dispersing and absorbing dielectric body on the local-field corrected spontaneous-decay of an excited atom embedded in the body is studied on the basis of the real-cavity model. By means of a Born expansion of the Green tensor of the system it is shown that to linear order in the susceptibility of the body the decay rate exactly follows Tomas's formula found for the special case of an atom at the center of a homogeneous dielectric sphere [Phys. Rev. A 63, 053811 (2001)]. It is further shown that for an atom situated at the interior of an arbitrary diele…
We extend our approach to the Casimir effect between absorbing dielectric multilayers [M. S. Tomas, Phys. Rev. A 66, 052103 (2002)] to magnetodielectric systems. The resulting expression for the force is used to numerically explore the effect of the medium dispersion on the attractive/repulsive force in a metal-magnetodielectric system described by the Drude-Lorentz permittivities and permeabilities.
A general, exact formula is derived for the expectation value of the electromagnetic energy density of an inhomogeneous absorbing and dispersive dielectric medium in thermal equilibrium, assuming that the medium is well approximated as a continuum. From this formula we obtain the formal expression for the Casimir force density. Unlike most previous approaches to Casimir effects in which absorption is either ignored or admitted implicitly through the required analytic properties of the permittivity, we include dissipation explicitly via the coupling of each dipole oscillator of the medium to a …
The retarded dispersion interaction (Casimir interaction) between two dilute dielectric media at high temperatures is considered. The excited atoms are taken into account. It is shown that the perturbation technique can not be applied to this problem due to the divergence of integrals. A non-perturbative approach based on kinetic Green functions is implemented. We consider interaction between two atoms (one of them is excited0 embedded in an absorbing dielectric medium. We take into account possible absorption of photons in the medium, which solves the problem of divergence. The force between …
We compare the behavior of propagating and evanescent light waves in absorbing media with that of electrons in the presence of inelastic scattering. The imaginary part of the dielectric constant results primarily in an exponential decay of a propagating wave, but a phase shift for an evanescent wave. We then describe how the scattering of quantum particles out of a particular coherent channel can be modeled by introducing an imaginary part to the potential in analogy with the optical case. The imaginary part of the potential causes additional scattering which can dominate and actually prevent …
Heat radiation and near-field radiative heat transfer can be strongly manipulated by adjusting geometrical shapes, optical properties, or the relative positions of the objects involved. Typically these objects are considered as embedded in vacuum. By applying the methods of fluctuational electrodynamics, we derive general closed-form expressions for heat radiation and heat transfer in a system of $N$ arbitrary objects embedded in a passive non-absorbing background medium. Taking into account the principle of reciprocity, we explicitly prove the symmetry and positivity of transfer in any such s…
In this article we compute the Casimir force between two finite-width mirrors at finite temperature, working in a simplified model in 1+1 dimensions. The mirrors, considered as dissipative media, are modeled by a continuous set of harmonic oscillators which in turn are coupled to an external environment at thermal equilibrium. The calculation of the Casimir force is performed in the framework of the theory of quantum open systems. It is shown that the Casimir interaction has two different contributions: the usual radiation pressure from vacuum, which is obtained for ideal mirrors without dissi…
A recently developed scheme [S. Scheel, L. Knoll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)] for quantizing the macroscopic electromagnetic field in linear dispersive and absorbing dielectrics satisfying the Kramers-Kronig relations is used to derive the quantum local-field correction for the standard virtual-sphere-cavity model. The electric and magnetic local-field operators are shown to be consistent with QED only if the polarization noise is fully taken into account. It is shown that the polarization fluctuations in the local field can dramatically change the spontaneous decay rate, co…
