We develop a theoretical description of intravalley scattering of quasiparticles in graphene from multiple short-range scatterers of size much greater than the carbon-carbon bond length. Our theory provides a method to rapidly calculate the Green's function in graphene for arbitrary configurations of scatterers. We demonstrate that non-collinear multiple scattering trajectories generate pseudospin rotations that alter quasiparticle interference, resulting in significant modifications to the shape, intensity, and pattern of the interference fringes in the local density of states (LDOS). We illustrate these effects via theoretical calculations of the LDOS for a variety of scattering configurations in single layer graphene. A clear understanding of impurity scattering in graphene is a step towards exploiting graphene's unique properties to build future devices.
The pseudo-magnetic field generated by mechanical strain in graphene can have dramatic consequences on the behavior of electrons and holes. Here we show that pseudo-magnetic field fluctuations present in crumpled graphene can induce significant intravalley scattering of charge carriers. We detect this by measuring the confocal Raman spectra of crumpled areas, where we observe an increase of the D'/D peak intensity ratio by up to a factor of 300. We reproduce our observations by numerical calculation of the double resonant Raman spectra and interpret the results as experimental evidence of the …
The magnetic-field dependence of the energy spectrum, wave function, binding energy and oscillator strength of exciton states confined in a circular graphene quantum dot (CGQD) are obtained within the configuration interaction (CI) method. We predict that: (1) excitonic effects are very significant in the CGQD as a consequence of a combination of geometric confinement, magnetic confinement and reduced screening; (2) two types of excitons (intravalley and intervalley excitons) are present in the CGQD because of the valley degree of freedom in graphene; (3) the intravalley and intervalley excito…
Electron-hole generation and recombination rates for intravalley and intervalley phonon scattering in Graphene are presented. The transverse and the longitudinal optical phonon modes ($E_{2g}$-modes) near the zone center ($Γ$-point) contribute to intravalley interband carrier scattering. At the zone edge ($K(K')$-point), only the transverse optical phonon mode ($A'_{1}$-mode) contributes significantly to intervalley interband scattering with recombination rates faster than those due to zone center phonons. The calculated recombination times range from less than a picosecond to more than hundre…
A Kubo formalism is used to calculate the electronic and optical conductivity of a graphene superlattice with Y-shaped kekulé bond texture, similar to that visualized in recent experiments. We show that new conduction channels between the valleys in graphene are opened by the kekulé distortion. This intervalley contribution to the electronic transport is not present in pristine graphene and here appears due to the folding of the Dirac cones $K$, $K'$ on top of each other. The contribution of intervalley transport to the conductivity of graphene, as well as the modification of the intravalley t…
By considering analytical expressions for the self-energies of intervalley and intravalley phonons in graphene, we describe the behavior of D, 2D, and D$'$ Raman bands with changes in doping ($μ$) and light excitation energy ($E_L$). Comparing the self-energy with the observed $μ$ dependence of the 2D bandwidth, we estimate the wavevector $q$ of the constituent intervalley phonon at $\hbar vq\simeq E_L/1.6$ ($v$ is electron's Fermi velocity) and conclude that the self-energy makes a major contribution (60%) to the dispersive behavior of the D and 2D bands. The estimation of $q$ is based on an …
Band gap engineering in graphene may open the routes towards transistor devices in which electric current can be switched off and on at will. One may, however, ask if a semiconducting band gap alone is sufficient to quench the current in graphene. In this paper we demonstrate that despite a bulk band gap graphene can still have metallic conductance along the sample edges (provided that they are shorter than the localization length). We find this for single-layer graphene with a zigzag-type boundary which hosts gapless propagating edge states even in the presence of a bulk band gap. By generati…
Confinement and edge structures are known to play significant roles in electronic and transport properties of two-dimensional materials. Here, we report on low-temperature magnetotransport measurements of lithographically patterned graphene cavity nanodevices. It is found that the evolution of the low-field magnetoconductance characteristics with varying carrier density exhibits different behaviors in graphene cavity and bulk graphene devices. In the graphene cavity devices, we have observed that intravalley scattering becomes dominant as the Fermi level gets close to the Dirac point. We assoc…
The power loss $P$ of hot Dirac fermions through the coupling to the intrinsic intravalley and intervalley acoustic and optical phonons is analytically investigated in silicene as a function of electron temperature $T_e$ and density $n_s$. At very low $T_e$, the power dissipation is found to follow the Bloch-Grüneisen power-law $\propto T_e^4$ and $n_s^{-0.5}$, as in graphene, and for $T_e \lesssim20-30$ K, the power loss is predominantly due to the intravalley acoustic phonon scattering. On the other hand, dispersionless low energy intervalley acoustic phonons begin to dominate the power tran…
We study quasiparticle dynamics in graphene exposed to a linearly-polarized electromagnetic wave of very large intensity. Low-energy transport in such system can be described by an effective time-independent Hamiltonian, characterized by multiple Dirac points in the first Brillouin zone. Around each Dirac point the spectrum is anisotropic: the velocity along the polarization of the radiation significantly exceeds the velocity in the perpendicular direction. Moreover, in some of the points the transverse velocity oscillates as a function of the radiation intensity. We find that the conductance …
We have carried out scanning tunneling spectroscopy measurements on exfoliated monolayer graphene on SiO$_2$ to probe the correlation between its electronic and structural properties. Maps of the local density of states are characterized by electron and hole puddles that arise due to long range intravalley scattering from intrinsic ripples in graphene and random charged impurities. At low energy, we observe short range intervalley scattering which we attribute to lattice defects. Our results demonstrate that the electronic properties of graphene are influenced by intrinsic ripples, defects and…
Tunneling of quasiparticles between two nearly-aligned graphene sheets produces resonant current-voltage characteristics because of the quasi-exact conservation of in-plane momentum. We claim that, in this regime, vertical transport in graphene/boron nitride/graphene heterostructures carries precious information on electron-electron interactions and the quasiparticle spectral function of the two-dimensional electron system in graphene. We present extensive microscopic calculations of the tunneling spectra with the inclusion of quasiparticle lifetime effects and elucidate the range of parameter…
We report localization of fractional quantum Hall (QH) quasiparticles on graphene antidots. By studying coherent tunneling through the localized QH edge modes on the antidot, we measured the QH quasiparticle charges to be approximately $\pm e/3$ at fractional fillings of $ν= \pm 1/3$. The Dirac spectrum in graphene allows large energy scales and robust quasiparticle localization against thermal excitation. The capability of localizing fractional quasiparticles on QH antidots brings promising opportunities for realizing anyon braiding and novel quantum electronics.
By using Fourier-transform scanning tunneling spectroscopy we measure the interference patterns produced by the impurity scattering of confined Dirac quasiparticles in epitaxial graphene nanoflakes. Upon comparison of the experimental results with tight-binding calculations of realistic model flakes, we show that the characteristic features observed in the Fourier-transformed local density of states are related to scattering between different transverse modes (sub-bands) of a graphene nanoflake and allow direct insight into the electronic spectrum of graphene. We also observe a strong reductio…
The electronic properties of twisted bilayer graphene on SiC substrate were studied via combination of transport measurements and scanning tunneling microscopy. We report the observation of enhanced intervalley scattering from one Dirac cone to the other, which contributes to weak localization, of the twisted bilayer graphene by increasing the interlayer coupling strength. Our experiment and analysis demonstrate that the enhanced intervalley scattering is closely related to the periodic AB stacked atoms (the A atom of layer 1 and the B atom of layer 2 that have the same horizontal positions) t…
Here we report a facile method to generate a high density of point defects in graphene on metal foil and show how the point defects affect the electronic structures of graphene layers. Our scanning tunneling microscopy (STM) measurements, complemented by first principle calculations, reveal that the point defects result in both the intervalley and intravalley scattering of graphene. The Fermi velocity is reduced in the vicinity area of the defect due to the enhanced scattering. Additionally, our analysis further points out that periodic point defects can tailor the electronic properties of gra…
We present a calculation of the quasiparticle decay rate due to electron-electron interactions in a doped graphene sheet. In particular, we emphasize subtle differences between the perturbative calculation of this quantity in a doped graphene sheet and the corresponding one in ordinary parabolic-band two-dimensional (2D) electron liquids. In the random phase approximation, dynamical overscreening near the light cone yields a universal quasiparticle lifetime, which is independent of the dielectric environment surrounding the 2D massless Dirac fermion fluid.
Moiré superlattice created by twist stacking has multiple physical properties. These physical properties depend on the twist angle, hence investigation of the twist angle dependency is important for the deep understanding of physical phenomena in moiré superlattice. In this work, negative magnetoresistance owing to weak localization (WL) was investigated in twisted double bilayer graphene (TDBG) as a function of the twist angle. The ratio of the intervalley scattering time to the intravalley scattering time, estimated using the WL formula for bilayer graphene, tended to decrease as the twist a…
Thermodynamic properties of quasiparticles in a graphene-based structures are investigated. Two graphene superconducting layers (one superconducting component is placed on the top layeredgraphene structure and the other component in the bottom) separated by oxide dielectric layers and one normal graphene layer in the middle. The quasiparticle flow emerged due to external gate voltage, we considered it as a gas of electron-hole pairs whose components belong to different layers. This is a striking result in view of the complexity of these systems: we have established that specific heat exhibits …
We present a calculation of the modulation in the Local Density Of electronic States (LDOS) caused by an impurity in graphene in the presence of external magnetic field. We focus on the spatial Fourier Transform (FT) of this modulation around the impurity. The FT due to the low energy quasiparticles are found to be nonzero over the reciprocal lattice corresponding to graphene. At these lattice spots the FT exhibits well-defined features at wavevectors that are multiples of the inverse cyclotron orbit diameter (see Figure 2) and is cut off at the wavevector corresponding to the energy of observ…
We present calculations of the quasiparticle energies and band gaps of graphene nanoribbons (GNRs) carried out using a first-principles many-electron Green's function approach within the GW approximation. Because of the quasi-one-dimension nature of a GNR, electron-electron interaction effects due to the enhanced screened Coulomb interaction and confinement geometry greatly influence the quasiparticle band gap. Compared with previous tight-binding and density functional theory studies, our calculated quasiparticle band gaps show significant self-energy corrections for both armchair and zigzag …
The effects of substrate on electronic and optical properties of triangular and hexagonal graphene nanoflakes with armchair edges are investigated by using a configuration interaction approach beyond double excitation scheme. The quasiparticle correction to the energy gap and exciton binding energy are found to be dominated by the long-range Coulomb interactions and exhibit similar dependence on the dielectric constant of the substrate, which leads to a cancellation of their contributions to the optical gap. As a result, the optical gaps are shown to be insensitive to the dielectric environmen…
Pseudospin, an additional degree of freedom related to the honeycomb structure of graphene, is responsible of many of the outstanding electronic properties found in this material. This article provides a clear understanding of how such pseudospin impacts the quasiparticle interferences of monolayer (ML) and bilayer (BL) graphene measured by low temperature scanning tunneling microscopy and spectroscopy. We have used this technique to map, with very high energy and space resolution, the spatial modulations of the local density of states of ML and BL graphene epitaxialy grown on SiC(0001), in pr…
We use the non-interacting tight-binding model to study the effect of isolated hydrogen adsorbates on the quasiparticle spectra of single-layer graphene. Using the Green's function approach, we obtain analytic expressions for the local density of states and the spectral function of hydrogen-doped graphene, which are also numerically evaluated and plotted. Our results are relevant for the interpretation of scanning tunneling microscopy and angle-resolved photoemission spectroscopy data of functionalized graphene.
Mesoscopic conductance fluctuations in graphene samples at energies not very close to the Dirac point are studied analytically. We demonstrate that the conductance variance $<[δG]^2>$ is very sensitive to the elastic scattering breaking the valley symmetry. In the absence of such scattering (disorder potential smooth at atomic scales, trigonal warping negligible), the variance $<[δG]^2 > = 4 < [δG]^2 >_\text{metal}$ is four times greater than that in conventional metals, which is due to the two-fold valley degeneracy. In the absence of intervalley scattering, but for strong intravalley scatter…
We calculate the real and imaginary electron self-energy as well as the quasiparticle spectral function in doped graphene taking into account electron-electron interaction in the leading order dynamically screened Coulomb coupling. Our theory provides the basis for calculating {\it all} one-electron properties of extrinsic graphene. Comparison with existing ARPES measurements shows broad qualitative agreement between theory and experiment. We also calculate the renormalized graphene momentum distribution function, finding a typical Fermi liquid discontinuity at k_F. We also provide a critical …
Early experiments on alkali-doped graphene demonstrated that the dopant adatoms modify the conductivity of graphene significantly, as extra carriers enhance conductivity while Coulomb scattering off the adatoms suppresses it. However, conductivity probes the overall scattering rate, so a dominant channel associated with long-range Coulomb scattering will mask weaker short-range channels. We present weak localization measurements of epitaxial graphene with lithium adatoms that separately quantify intra- and intervalley scattering rates, then compare the measurements to tight-binding calculation…
We address the question of how small can the quasiparticle decay rate be at low energies in undoped graphene, where kinematical constraints are known to prevent the decay into particle-hole excitations. For this purpose, we study the renormalization of the phonon dispersion by many-body effects, which turns out to be very strong in the case of the out-of-plane phonons at the K point of the spectrum. We show that these evolve into a branch of very soft modes that provide the relevant channel for quasiparticle decay, at energies below the scale of the optical phonon modes. In this regime, we fin…
Graphene, a monolayer of carbon atoms arranged in a hexagonal pattern, provides a unique two-dimensional (2D) system exhibiting exotic phenomena such as quantum Hall effects, massless Dirac quasiparticle excitations and universal absorption & conductivity. The linear energy-momentum dispersion relation in graphene also offers the opportunity to mimic the physics of far-away relativistic particles like neutron stars and white dwarfs. In this letter, we perform a counterintuitive ultrafast pump-probe experiment with high photon energies to isolate the Drude-like intraband dynamics of photoexcite…
Using many-body diagrammatic perturbation theory we consider carrier density- and substrate-dependent many-body renormalization of doped or gated graphene induced by Coulombic electron-electron interaction effects. We quantitatively calculate the many-body spectral function, the renormalized quasiparticle energy dispersion, and the renormalized graphene velocity using the leading-order self-energy in the dynamically screened Coulomb interaction within the ring diagram approximation. We predict experimentally detectable many-body signatures, which are enhanced as the carrier density and the sub…
We calculate the quasiparticle properties of chiral two-dimensional Dirac electrons in graphene within the Landau Fermi Liquid scheme based on $GW$ approximation in the presence of disorder. Disorder effects due to charged impurity scattering plays a crucial role in density dependence of quasiparticle quantities. Mode-coupling approach to scattering rate and self-energy in $GW$ approximation for quasiparticle renormalized Fermi velocity and spin-antisymmetric Landau Fermi parameter incorporating the many-body interactions and the disorder effects show reduction of these quantities by 5-15 perc…
We investigate the creation of massless quasiparticle pairs from the vacuum state in graphene by the space homogeneous time-dependent electric field. For this purpose the formalism of (2+1)-dimensional quantum electrodynamics is applied to the case of a nonstationary background with arbitrary time dependence allowing the S-matrix formulation of the problem. The number of created pairs per unit graphene area is expressed via the asymptotic solution at $t\to\infty$ of the second-order differential equation of an oscillator type with complex frequency satisfying some initial conditions at $t\to-\…
We calculate the density-density response function and electron self-energy for undoped bilayer graphene, within the Random Phase Approximation (RPA). We show that the quasiparticle decay rate scales linearly with the quasiparticle energy, and quasiparticle weight vanishes logarithmically in the low-energy limit, indicating non-Fermi liquid behavior. This is a consequence of the absence of a Fermi surface for neutral bilayer graphene and corresponding larger phase space available for scattering processes. Experimental consequences of our results as well as their differences from those of singl…
We obtain the quasiparticle band structure of ABA and ABC-stacked graphene trilayers through ab initio density functional theory (DFT) and many-body quasiparticle calculations within the GW approximation. To interpret our results, we fit the DFT and GW $π$ bands to a low energy tight-binding model, which is found to reproduce very well the observed features near the K point. The values of the extracted hopping parameters are reported and compared with available theoretical and experimental data. For both stackings, the self energy corrections lead to a renormalization of the Fermi velocity, an…
We investigate the effect of electron-electron interactions in ABC stacked graphene trilayers. In the gapless regime, we show that the self-energy corrections lead to the renormalization of the dynamical exponent $z=3+α_{1}/N$, with $α_{1}\approx0.52$ and $N$ is the number of fermionic species. Although the quasiparticle residue is suppressed near the neutrality point, the lifetime has a sublinear scaling with the energy and the quasiparticles are well defined even at zero energy. We calculate the renormalization of different physical observables, which can be directly measured in experiments.
Graphene is considered to be a promising material for future electronics. The envisaged transistor applications often rely on precision cutting of graphene sheets with nanometer accuracy. In this letter we demonstrate graphene-based quantum dots created by using atomic force microscopy (AFM) with tip-assisted electrochemical etching. This lithography technique provides resolution of about 20 nm, which can probably be further improved by employing sharper tips and better humidity control. The behavior of our smallest dots in magnetic field has allowed us to identify the charge neutrality point …
Quantum confinement of graphene Dirac-like electrons in artificially crafted nanometer structures is a long sought goal that would provide a strategy to selectively tune the electronic properties of graphene, including bandgap opening or quantization of energy levels However, creating confining structures with nanometer precision in shape, size and location, remains as an experimental challenge, both for top-down and bottom-up approaches. Moreover, Klein tunneling, offering an escape route to graphene electrons, limits the efficiency of electrostatic confinement. Here, a scanning tunneling mic…
We calculate the form of quasiparticle interference patterns in bilayer graphene within a low-energy description, taking into account perturbatively the trigonal warping terms. We introduce four different types of impurities localized on the A and B sublattices of the first and the second layer, and we obtain closed-form analytical expressions both in real and Fourier spaces for the oscillatory corrections to the local density of states generated by the impurities. Finally, we compare our findings with recent experimental and semi-analytical T-matrix results from arXiv:2104.10620 and we show t…
Two-dimensional Dirac fermions are used to discuss quasiparticles in graphene in the presence of impurity scattering. Transport properties are completely dominated by diffusion. This may explain why recent experiments did not find weak localization in graphene. The diffusion coefficient of the quasiparticles decreases strongly with increasing strength of disorder. Using the Kubo formalism, however, we find a robust minimal conductivity that is independent of disorder. This is a consequence of the fact that the change of the diffusion coefficient is fully compensated by a change of the number o…
We adopt the GW approximation and random phase approximation to study finite temperature effects on the inelastic mean free path and quasiparticle lifetime by directly calculating the imaginary part of the finite temperature self-energy induced by electron-electron interaction in extrinsic and intrinsic graphene. In particular, we provide the density-dependent leading order temperature correction to the inelastic scattering rate for both single-layer and double-layer graphene systems. We find that the inelastic mean free path is strongly influenced by finite-temperature effects. We present the…
A monolayer of graphene irradiated with circularly polarized light suggests a unique platform for surface electromagnetic wave (plasmon-polariton) manipulation. In fact, the time periodicity of the Hamiltonian leads to a geometric Aharonov-Anandan phase and results in a photovoltaic Hall effect in graphene, creating off-diagonal components of the conductivity tensor. The latter drastically changes the dispersion relation of surface plasmon-polaritons, leading to hybrid wave generation. In this paper we present a systematic and self-contained analysis of the hybrid surface waves obtained from M…
The analytical expressions for both diagonal and off-diagonal ac and dc conductivities of graphene placed in an external magnetic field are derived. These conductivities exhibit rather unusual behavior as functions of frequency, chemical potential and applied field which is caused by the fact that the quasiparticle excitations in graphene are Dirac-like. One of the most striking effects observed in graphene is the odd integer quantum Hall effect. We argue that it is caused by the anomalous properties of the Dirac quasiparticles from the lowest Landau level. Other quantities such as Hall angle …
We present numerical calculations of the impact of charge carriers-carriers interactions on the dynamical properties of quasiparticles such as renormalized velocity and quasiparticle inelastic scattering lifetime in a gapped graphene sheet. Our formalism is based on the many-body $G_0W$-approximation for the self-energy. We present results for the many-body renormalized velocity suppression and the renormalization constant over a broad range of energy gap values. We find that the renormalized velocity is almost independence of the carrier densities at large density regime. We also show that th…
Here we show, with simultaneous transport and photoemission measurements, that the graphene terminated SiC(0001) surface undergoes a metal-insulator transition (MIT) upon dosingwith small amounts of atomic hydrogen. We find the room temperature resistance increases by about 4 orders of magnitude, a transition accompanied by anomalies in the momentum-resolved spectral function including a non-Fermi Liquid behaviour and a breakdown of the quasiparticle picture. These effects are discussed in terms of a possible transition to a strongly (Anderson) localized ground state.
Electrons in graphene with heavy adatoms (such as In or Tl) have been predicted to form a 2D topological insulator phase with a substantial spectral gap potentially suitable for future practical applications. In order to facilitate the ongoing experimental efforts to identify this phase we perform a theoretical study of its spectral properties in a model graphene system with randomly distributed adatoms. Our extensive modeling shows that random heavy adatoms produce a full spectral gap (as opposed to a mobility gap) accompanied by distinctive quasiparticle interference patterns observable by m…
We present an alternative methodology for calculating the quasi-particle energy, energy loss, and optical spectra of a molecule deposited on graphene or a metallic substrate. To test the accuracy of the method it is first applied to the isolated benzene (C6H6) molecule. The quasiparticle energy levels and especially the energies of the benzene excitons (triplet, singlet, optically active and inactive) are in very good agreement with available experimental results. It is shown that the vicinity of the various substrates (pristine/doped graphene or (jellium) metal surface) reduces the quasiparti…
We investigate the electronic structure of terraces of single layer graphene (SLG) by scanning tunneling microscopy (STM) on samples grown by thermal decomposition of 6H-SiC(0001) crystals in ultra-high vacuum. We focus on the perturbations of the local density of states (LDOS) in the vicinity of edges of SLG terraces. Armchair edges are found to favour intervalley quasiparticle scattering, leading to the (\surd3\times\surd3)R30° LDOS superstructure already reported for graphite edges and more recently for SLG on SiC(0001). Using Fourier transform of LDOS images, we demonstrate that the intrin…
A perpendicular electric field breaks the layer symmetry of Bernal-stacked bilayer graphene, resulting in the opening of a band gap and a modification of the effective mass of the charge carriers. Using scanning tunneling microscopy and spectroscopy, we examine standing waves in the local density of states of bilayer graphene formed by scattering from a bilayer/trilayer boundary. The quasiparticle interference properties are controlled by the bilayer graphene band structure, allowing a direct local probe of the evolution of the band structure of bilayer graphene as a function of electric field…
Trilayer graphene (TLG) exhibits rich novel electronic properties and extraordinary quantum Hall phenomena owning to enhanced electronic interactions and tunable chirality of its quasiparticles. Here, we report direct observation of chirality transition of quasiparticles at stacking solitons of TLG via spatial-resolved Landau level spectroscopy. The one-dimensional stacking solitons with width of the order of 10 nm separate adjacent Bernal-stacked TLG and rhombohedral-stacked TLG. By using high field tunneling spectra of scanning tunneling microscopy, we measured Landau quantization in both th…
Relativistic fermionic systems have physical quantities calculated by well stablished quantum electrodynamic prescriptions. In the last few years there has been an enormous interest in condensed matter systems in which the fermions exhibit relativistic dispersion, as Dirac fermions in graphene. We employ a non-perturbative method in order to obtain a non-perturbative correction to the quasiparticle velocity in graphene, and compare with the experimental data. We find a better agreement between the quasiparticle velocity corrected with non-perturbative corrections and measurements, when compare…
Advances in infrared nanoscopy have enabled access to the finite momentum optical conductivity $σ(\vec{q},ω)$. The finite momentum optical conductivity in graphene has a peak at the Dirac fermion quasiparticle energy $ε(k_F-q)$, i.e. at the Fermi momentum minus the incident photon momentum. We find that the peak remains robust even at finite temperature as well as with residual scattering. It can be used to trace out the fermion dispersion curves. However, this effect depends strongly on the linearity of the Dirac dispersion. Should the Dirac fermions acquire a mass, the peak in $σ(q,w)$ shift…
The scattering of two-dimensional massless Dirac fermions from local spin-orbit interactions with an origin in dilute concentrations of physisorbed atomic species on graphene is theoretically investigated. The hybridization between graphene and the adatoms' orbitals lifts spin and valley degeneracies of the pristine host material, giving rise to rich spin-orbit coupling mechanisms with features determined by the exact adsorption position on the honeycomb lattice - bridge, hollow or top position - and the adatoms' outer-shell orbital type. Effective graphene-only Hamiltonians are derived from s…
Graphite crystals used to prepare graphene-based heterostructures are generally assumed to be defect free. We report here scanning tunneling microscopy results that show graphite commonly used to prepare graphene devices can contain a significant amount of native defects. Extensive scanning of the surface allows us to determine the concentration of native defects to be 6.6$\times$10$^8$ cm$^{-2}$. We further study the effects of these native defects on the electronic properties of Bernal-stacked bilayer graphene. We observe gate-dependent intravalley scattering and successfully compare our exp…
We address spin polarization dependence of graphene's Fermi liquid properties quantitatively using a microscopic Random Phase Approximation theory in an interacting spin-polarized Dirac electron system. We show an enhancement of the minority-spin many-body velocity renormalization at fully spin polarization due to reduction in the electron density and consequently increase in the interaction between electrons near the Fermi surface. We also show that the spin dependence of the Fermi velocity in the chiral Fermi systems is different than that in a conventional two-dimensional electron liquid. I…
Spectroscopic studies of electronic phenomena in graphene are reviewed. A variety of methods and techniques are surveyed, from quasiparticle spectroscopies (tunneling, photoemission) to methods probing density and current response (infrared optics, Raman) to scanning probe nanoscopy and ultrafast pump-probe experiments. Vast complimentary information derived from these investigations is shown to highlight unusual properties of Dirac quasiparticles and many-body interaction effects in the physics of graphene.
We study the spectral function and quasiparticle scattering in Li-decorated graphene (Li@graphene) with an atomistic $T$-matrix formalism and uncover adatom-induced spectral effects which shed light on experimentally observed angle-resolved photoemission spectroscopy (ARPES) features. From transport studies, alkali adatoms are known to introduce charged-impurity scattering limiting the carrier mobility. Here, we demonstrate that Li adatoms furthermore give rise to a low-energy impurity band centered at the $Γ$ point which originates from the hybridization between the atomic 2s state of the Li …
The collective properties of different quasiparticles in various graphene based structures in high magnetic field have been studied. We predict Bose-Einstein condensation (BEC) and superfluidity of 2D spatially indirect magnetoexcitons in two-layer graphene. The superfluid density and the temperature of the Kosterlitz-Thouless phase transition are shown to be increasing functions of the excitonic density but decreasing functions of magnetic field and the interlayer separation. The instability of the ground state of the interacting 2D indirect magnetoexcitons in a slab of superlattice with alte…
