We have measured the isotope shift of the narrow quadrupole-allowed 5 2S1/2 - 4 2D5/2 transition in 86Sr+ relative to the most abundant isotope 88Sr+. This was accomplished using high-resolution laser spectroscopy of individual trapped ions, and the measured shift is Delta-nu_meas^(88,86) = 570.281(4) MHz. We have also tested a recently developed and successful method for ab-initio calculation of isotope shifts in alkali-like atomic systems against this measurement, and our initial result of Delta-nu_calc^(88,86) = 457(28) MHz is also presented. To our knowledge, this is the first high precision measurement and calculation of that isotope shift. While the measurement and the calculation are in broad agreement, there is a clear discrepancy between them, and we believe that the specific mass shift was underestimated in our calculation. Our measurement provides a stringent test for further refinements of theoretical isotope shift calculation methods for atomic systems with a single valence electron.
Part-per-billion measurement of the $4^2S_{1/2} \rightarrow 3^2D_{5/2}$ electric quadrupole transition isotope shifts between $^{42,44,48}$Ca$^+$ and $^{40}$Ca$^+$
Oscillating quadrupole effects in high precision metrology
从理论上研究了振荡四极场对原子能级的影响,给出了四极矩阵元的一般表达式。结果是相关的任何基于离子的时钟,其中一个时钟状态支持四极矩。估计$^{176}$ Lu $^+$的时钟偏移,并表明耦合到四极场不会限制时钟精度在$\lesssim10^{-19}$水平。然而,建议一种方法,将允许这种转变进行校准。这种方法利用共振四极耦合,使四极矩的原子被测量。使用$^{138}$ Ba $^+$给出了原理证明,其中$D_{5/2}$态的四极矩估计为$Θ=3.229(89) e a_0^2$。
Precise Determination of Electric Quadrupole Moments and Isotope Shift Constants of Yb$^+$ in Pursuance of Probing Fundamental Physics and Nuclear Radii
Reliability test for the experimental results of electric quadrupole hyperfine structure constants and new assessment of nuclear quadrupole moments in $^{135,137}$Ba
我们调查电四极超精细结构常数($B$)的结果在$^{135}$ Ba $^+$和$^{137}$ Ba $^+$和比较它们的比率与报告的测量的比率之间的核四极矩($Q$)值的这些同位素。我们进行了置信度测试报告的实验$B$值和计算的$B/Q$从目前的工作。在来自使用相同技术进行的不同实验的两种同位素中观察到实验$B$值的增加。本文的计算是用全阶相对论多体理论进行的,只考虑了耦合团簇中的单激发和双激发。在对结果进行详细分析后,我们获得的$^{135}$ Ba和$^{137}$ Ba的$Q$值分别为0.153(2)$b$和0.236(3)$b$,与目前引用的精确值相差约4%。
Precision isotope shift measurements in Ca$^+$ using highly sensitive detection schemes
我们展示了一种有效的高精度光谱技术,为单囚禁离子与非封闭的过渡。在双搁置技术中,单个光子的吸收首先被放大到与不同种类的共捕获冷却离子共享的正常运动模式的几个声子,然后使用标准电子搁置技术被进一步放大到由冷却离子发射的数千个荧光光子。我们采用这种扩展的光子反冲光谱技术进行第一次高精度的绝对频率测量的$^{2}$ D $_{3/2}$ $\rightarrow$ $^{2}$ P $_{1/2}$过渡的$^{40}$钙$^{+}$,导致在$f=346\, 000\, 234\, 867(96)$ kHz的过渡频率。此外,我们确定了该跃迁的同位素位移和$^{2}$ S $_{1/2}$ $\rightarrow$ $^{2}$ P $_{1/2}$跃迁的$^{42}$ Ca $^{+}$,$^{44}$ Ca $^{+}$和$^{48}$ Ca $^{+}$离子相对于$^{40}$ Ca $^{+}$的精确度低于100 kHz。改进的场和质量移动常数的这些过渡,以及在均方核电荷半径的变化提取从这个高分辨率的数据。
Accurate long-range coefficients for two excited like isotope He atoms: He($2 ^1P$)--He($2 ^1P$), He($2 ^1P$)--He($2 ^3P$), and He($2 ^3P$)--He($2 ^3P$)
Theoretical study on the hyperfine interaction constants and the isotope shift factors for the $3s^2~^1 S_{ 0} ~-~ 3s3p~^{3,1}P^o_1$ transitions in Al$^+$
用多组态Dirac-Hartree-Fock方法计算了Al $^+$离子3s 3 p $^{3,1}P^o_1$态的磁偶极和电四极超精细相互作用常数,以及从这两个态到基态3s $^2~^1S_0$跃迁的同位素位移因子,包括质量和场位移因子.基于活性空间方法,详细研究了电子关联和Breit相互作用对这些物理量的影响。计算结果表明,CC和高阶关联对于评价原子参数的不确定度是相当重要的。超精细相互作用常数的不确定度小于1.5%.虽然同位素位移因子对电子关联高度敏感,但通过探索电子关联的影响,获得了合理的不确定性。此外,我们还发现Al $^{+}$的质量移动因子的相对论核反冲修正很小,对电子关联不敏感。这些原子参数对提取Al同位素的核电四极矩和均方电荷半径具有重要的参考价值。
Magneto-optical trapping of bosonic and fermionic neon isotopes and their mixtures: isotope shift of the ^3P_2 to ^3D_3 transition and hyperfine constants of the ^3D_3 state of Ne-21
Nuclear moments, charge radii, and magnetization distribution parameters of Ag isotopes from laser spectroscopy and \textit{ab initio} electronic-structure calculations
Petersburg Nuclear Physics Institute named by B.P. Konstantinov of National Research Centre “Kurchatov Institute”(以B.P.康斯坦丁诺夫命名的国家研究中心“库尔恰托夫研究所”圣彼得堡核物理研究所);Saint Petersburg State University(圣彼得堡国立大学);KU Leuven, Instituut voor Kern- en Stralingsfysica(荷语鲁汶大学核与辐射物理研究所);Centre for Cold Matter, Imperial College London(伦敦帝国理工学院冷物质中心);State Key Laboratory of Low-Dimensional Quantum Physics, Department of Physics, Tsinghua University(清华大学物理系低维量子物理国家重点实验室)