We experimentally and theoretically study self-phase modulation by Kerr effect in a liquid filled hollow core photonic crystal fiber. We perform a complete characterization of the linear optical properties of the hollow core photonic band gap fiber filled with deuterated acetone to determine all the characteristics of the propagation mode. The nonlinear coefficient of the fiber is determined by fitting the output spectra broadened by self-phase modulation with a new analytical expression giving the spectra of a secant hyperbolic pulse transmitted through a Kerr media. The experiment allows a precise determination of the nonlinear index change of acetone-d6 equal to (1.15$\pm$0.17)x10-19 m2W-1.
We found the self-similar solitary solutions of a recently proposed model for propagation of pulses in gas filled hollow-core photonic crystal fibers that includes a plasma induced nonlinearity. As anticipated for a simpler model and using a perturbation analysis, there are indeed stationary solitary waves that accelerate and self-shift to higher frequencies. However, if the plasma nonlinearity strength is large or the pulse amplitudes are small, the solutions have distinguished long tails and decay as they propagate.
We study theoretically the propagation of relatively long pulses with ionizing intensities in a hollow-core photonic crystal fiber filled with a Raman-inactive gas. Due to photoionization, previously unknown types of asymmetric self-phase modulation and `universal' modulational instabilities existing in both normal and anomalous dispersion regions appear. We also show that it is possible to spontaneously generate a plasma-induced continuum of blueshifting solitons, opening up new possibilities for pushing supercontinuum generation towards shorter and shorter wavelengths.
Frequency blueshifting was recently observed in light pulses propagating on gas filled hollow-core photonic crystal fibers where a plasma has been produced due to photoionization of the gas. One of the propagation models that is adequate to describe the actual experimental observations is here investigated. It is a nonlinear Schrödinger equation with an extra term, to which we applied a self-similar change of variables and found its accelerating solitons. As in other NLS related models possessing accelerating solitons, there exist asymmetrical pulses that decay as they propagate in some parame…
We demonstrate a route to supercontinuum generation in gas-filled hollow-core anti-resonant fibers through the creation of a broad vibrational Raman frequency comb followed by continuous broadening and merging of the comb lines through either rotational Raman scattering or the optical Kerr effect. Our demonstration experiments, utilizing a single pump pulse with 20 ps duration at 532 nm in a nitrogen-filled fiber, produce a supercontinuum spanning from 440 nm to 1200 nm, with an additional deep ultraviolet continuum from 250 nm to 360 nm. Numerical results suggest that this approach can produc…
We report a study of soliton self-frequency shifting in hydrogen-filled hollow-core fiber. The combination of hydrogen and short 40-fs input pulses underlies clean and efficient generation of Raman solitons between 1080 and 1600 nm. With 240-nJ input pulses, the Raman soliton energy ranges from 110 to 20 nJ over that wavelength range, and the pulse duration is approximately 45 fs. In particular, 70-nJ and 42-fs pulses are generated at 1300 nm. Numerical simulations agree reasonably well with experiments and predict that microjoule-energy tunable pulses should be possible with higher-energy inp…
Supercritical Xe at 293 K offers a Kerr nonlinearity that can exceed that of fused silica while being free of Raman scattering. It also has a much higher optical damage threshold and a transparency window that extends from the UV to the infrared. We report the observation of nonlinear phenomena, such as self-phase modulation, in hollow-core photonic crystal fiber filled with supercritical Xe. In the subcritical regime, intermodal four-wave-mixing resulted in the generation of UV light in the HE12 mode. The normal dispersion of the fiber at high pressures means that spectral broadening can clea…
We demonstrate efficient generation of coherent super-octave pulses via a single-stage spectral broadening of a Yb:KGW laser in a single, pressurized, Ne-filled, hollow-core fiber capillary. Emerging pulses spectrally spanning over more than $\sim$1 PHz (250 nm- 1600 nm) at a dynamic range of $\sim$60 dB, and an excellent beam quality open the door to combining Yb:KGW lasers with modern light field synthesis techniques. Compression of a fraction of the generated supercontinuum to intense (8 fs, $\sim$2.4 cycle, $\sim$650 $μ$J) pulses allows convenient use of these novel laser sources in strong…
The ultimate limit on fiber loss is set by the intrinsic Rayleigh scattering of silica glass material. Here, we challenge this limit in the visible region by using a hollow-core fiber approach. Two visible-guiding hollow-core conjoined-tube negative-curvature fibers are successfully fabricated and exhibit the overall losses of 3.8 dB/km at 680 nm and 4.9 dB/km at 558 nm respectively. The loss of the latter fiber surpasses the Rayleigh scattering limit of silica glass fiber in the green spectral region by 2 dB. Numerical simulation indicates that this loss level is still much higher than the fu…
In this letter, an energetic and highly efficient dispersive wave (DW) generation at 200 nm has been numerically demonstrated by selectively exciting LP$_{02}$-like mode in a 10 bar Ar-filled hollow-core anti-resonant fiber pumping in the anomalous dispersion regime at 1030 nm with pulses of 30 fs duration and 7 $μ$J energy. Our calculations indicate high conversion efficiency of $>$35\% (2.5 $μ$J) after propagating 3.6 cm fiber length which is due to the strong shock effect and plasma induced blue-shifted soliton. It is observed that the efficiency of fundamental LP$_{01}$-mode is about 15\% …
Resonant dispersive wave (RDW) emission in gas-filled hollow waveguides is a powerful technique for the generation of bright few-femtosecond laser pulses from the vacuum ultraviolet to the near infrared. Here we investigate deep-ultraviolet RDW emission in a hollow capillary fibre filled with a longitudinal gas pressure gradient. We obtain broadly similar emission to the constant-pressure case by applying a surprisingly simple scaling rule for the gas pressure and study the energy-dependent dispersive-wave spectrum in detail using simulations. We further find that in addition to enabling dispe…
We report a high performance nodeless hollow-core anti-resonant fiber with a broadband guidance from 1050 nm to >1900 nm, a transmission attenuation of 200 dB/km, and a low bending loss of 0.25 dB/m for a 5 cm radius at wavelength of 1550 nm.
We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagomé-style photonic crystal fiber. By pumping with ultrashort, few $μ$J, pulses centered at 400 nm, we generate an idler pulse at 266 nm, and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%. Although the pump and seed pulse durations are ~100 fs, the generated ultraviolet spectral bandwidths support sub-15 fs pulses. These can be further extended to support few-cycle puls…
Based on the interplay between photoionization and Raman effect in gas-filled photonic crystal fibers, we propose a new optical device to control frequency-conversion of ultrashort pulses. By tuning the input-pulse energy, the output spectrum can be either down-converted, up-converted, or even frequency-shift compensated. For low input energies, Raman effect is dominant and leads to a redshift that increases linearly during propagation. For larger pulse energies, photoionization starts to take over the frequency conversion process, and induces a strong blueshift. We have found also that the fi…
Hollow core fibers are considered as promising candidates to deliver intense temporally overlapping picosecond pulses in applications such as stimulated Raman scattering (SRS) microscopy and endoscopy because of their inherent low nonlinearity compared to solid-core silica fibers. Here we demonstrate that, contrary to prior assumptions, parasitic signals are generated in Kagomé lattice hollow core fibers. We identify the origin of the parasitic signals as an interplay between the Kerr nonlinearity of air and frequency-dependent fiber losses. Importantly, we identify the special cases of experi…
We demonstrate a new class of hollow-core Bragg fibers that are composed of concentric cylindrical silica rings separated by nanoscale support bridges. We theoretically predict and experimentally observe hollow-core confinement over an octave frequency range. The bandwidth of bandgap guiding in this new class of Bragg fibers exceeds that of other hollow-core fibers reported in the literature. With only three rings of silica cladding layers, these Bragg fibers achieve propagation loss of the order of 1 dB/m.
The photonic hook, a beam that can propagate along a curved path, has attracted wide attention since its inception and experimental confirmation. In this paper, we propose a new type of structure, which was made by a hollow microcylinder and a Janus-shaped liquid column of two insoluble filling liquids, for producing photonic hook of easily tunable properties and long length. The E^2 field intensity distribution characteristics and formation mechanism of the photonic hook are studied by analyzing the energy flow using the finite element method. The profile and properties of the photonic hook c…
We report generation of an ultrafast supercontinuum extending into the mid- infrared in gas-filled single-ring hollow-core photonic crystal fiber (SR-PCF) pumped by 1.7 $μ$m light from an optical parametric amplifier. The simple fiber structure offers shallow dispersion and flat transmission in the near and mid-infrared, enabling the generation of broadband spectra extending from 300 nm to 3.1 $μ$m, with a total energy of a few $μ$J. In addition, we report the emission of ultraviolet dispersive waves whose frequency can be tuned simply by adjusting the pump wavelength. SR-PCF also provides an …
A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet (VUV) radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi2Se3 with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promi…
Hollow core antiresonant fibers offer new possibilities in the near infrared and visible spectral range. I show here that the great flexibility of this technology can allow the design and fabrication of hollow core optical fibers with an extended transmission bandwidth in the near infrared and with very low optical attenuation in the visible wavelength regime. A very low attenuation of 175dB/km at 480nm is reported. A modification of the design of the studied fibers is proposed in order to achieve fast-responding gas detection.
We analyze the impact of geometrical parameters on such important optical characteristics of negative curvature hollow-core fibers (NCHCFs) as waveguide dispersion, waveguide losses and the structure of transmission bands. We consider both theoretically and experimentally the resonance effects and formation of band edges under bending in NCHCFs.
We present a technique that uses noisy broadband pulse bursts generated by modulational instability to probe nonlinear processes, including infrared-inactive Raman transitions, in molecular gases. These processes imprint correlations between different regions of the noisy spectrum, which can be detected by acquiring single shot spectra and calculating the Pearson correlation coefficient between the different frequency components. Numerical simulations verify the experimental measurements and are used to further understand the system and discuss methods to improve the signal strength and the sp…
Hollow-core negative curvature fibers can confine light within air core and have small nonlinearity and dispersion and high damage threshold, thereby attracting a great deal of interest in the field of hollow core fibers. However, reducing the loss of hollow-core negative curvature fibers is a serious problem. On this basis, three new types of fibers with different nested tube structures are proposed in the near-infrared spectral regions and compared in detail with a previously proposed hollow-core negative curvature fiber. We used finite-element method for numerical simulation studies of thei…
We study coherent anti-Stokes Raman spectroscopy in air-filled anti-resonance hollow-core photonic crystal fiber, otherwise known as 'revolver' fiber. We compare the vibrational coherent anti-Stokes Raman signal of N$_2$, at 2331 cm$^{-1}$, generated in ambient air (no fiber present), with the one generated in a 2.96 cm of a revolver fiber. We show a 170 times enhancement for the signal produced in the fiber, due to an increased interaction path. Remarkably, the N$_2$ signal obtained in the revolver fiber shows near-zero non-resonant background, due to near-zero overlap between the laser field…
We numerically investigate the energy and arrival-time noise of ultrashort laser pulses produced via resonant dispersive wave emission in gas-filled hollow-core waveguides under the influence of pump-laser instability. We find that for low pump energy, fluctuations in the pump energy are strongly amplified. However, when the generation process is saturated, the energy of the resonant dispersive wave can be significantly less noisy than that of the pump pulse. This holds for a variety of generation conditions and while still producing few-femtosecond pulses. We further find that the arrival-tim…
We propose supercritical xenon in a hollow-core photonic bandgap fiber as a highly nonlinear medium, and demonstrate 200 nm control over the guidance window of the fiber as the xenon goes through its supercritical phase transition. The large optical polarizability and monoatomic nature of xenon are predicted to allow large optical nonlinearity, on the same order as that of fused silica, while maintaining greatly reduced Raman scattering, offering benefits for nonlinear and quantum optics.
Flying particle sensors in hollow-core photonic crystal fibers require accurate localization of the optically trapped microparticles. We report position measurement to micrometer-resolution, using optical frequency domain reflectometry, of two 1.65-$μ$m-diameter polystyrene particles.
We investigate various methods for extending the simple analytical capillary model to describe the dispersion and loss of anti-resonant hollow-core fibers without the need of detailed finite-element simulations across the desired wavelength range. This poor-man's model can with a single fitting parameter quite accurately mimic dispersion and loss resonances and anti-resonances from full finite-element simulations. Due to the analytical basis of the model it is easy to explore variations in core size and cladding wall thickness, and should therefore provide a valuable tool for numerical simulat…
We investigate numerically soliton-plasma interaction in a noble-gas-filled silica hollow-core anti-resonant fiber pumped in the mid-IR at 3.0 μm. We observe multiple soliton self-compression stages due to distinct stages where either the self-focusing or the self-defocusing nonlinearity dominates. Specifically, the parameters may be tuned so the competing plasma self-defocusing nonlinearity only dominates over the Kerr self-focusing nonlinearity around the soliton self-compression stage, where the increasing peak intensity on the leading pulse edge initiates a competing self-defocusing plasma…
We report on the generation of a three-octave-wide supercontinuum extending from the vacuum ultraviolet (VUV) to the near-infrared, spanning at least 113 to 1000 nm (i.e., 11 to 1.2 eV), in He-filled hollow-core kagome-style photonic crystal fiber. Numerical simulations confirm that the main mechanism is a novel and previously undiscovered interaction between dispersive-wave emission and plasma-induced blueshifted soliton recompression around the fiber zero dispersion frequency. The VUV part of the supercontinuum, which modeling shows to be coherent and possess a simple phase structure, has su…
In this paper we present a theoretical and numerical analysis of light localization in hollow core microstructured fibers (HCMFs) with a complicated shape of the core cladding boundary. The analysis is based on well established models (for example, the ARROW model) and also on the models proposed for the first time. In particular, we consider local and nonlocal mechanisms of light localization in the waveguide structures with a determined type of discrete rotational symmetry of the core cladding boundary. We interpret and analyze mechanisms of light localization in negative curvature hollow co…
We present empirical formulae that can provide dispersion and average effective area of the fundamental mode in hollow-core antiresonant fibers. The formulae draw on the structural parameters of the fiber, and allow one to obtain the guiding properties over a wide spectral bandwidth, without the need for time consuming numerical simulations. The formulae are validated by comparing their results with those obtained using a finite-element method. We also analyze the effects of changing the number of antiresonant tubes, as well as adding nested elements in the antiresonant tubes on the guiding pr…
We report on hollow-core fibers displaying rms core roughness under the surface capillary waves thermodynamic limit and record loss in the short-wavelength range (50.0 dB/km at 290 nm, 9.7 dB/km at 369 nm, 5.0 dB/km at 480 nm, 0.9 dB/km at 558 nm, 1.8 dB/km at 719 nm).
Gas-filled hollow-core photonic crystal fibers offer unprecedented opportunities to observe novel nonlinear phenomena. The various properties of gases that can be used to fill these fibers give additional degrees of freedom for investigating nonlinear pulse propagation in a wide range of different media. In this review, we will consider some of the the new nonlinear interactions that have been discovered in recent years, in particular those which are based on soliton dynamics.
Broadband-tunable sources of circularly-polarized light are crucial in fields such as laser science, biomedicine and spectroscopy. Conventional sources rely on nonlinear wavelength conversion and polarization control using standard optical components, and are limited by the availability of suitably transparent crystals and glasses. Although gas-filled hollow-core photonic crystal fiber provides pressure-tunable dispersion, long well-controlled optical path-lengths, and high Raman conversion efficiency, it is unable to preserve circular polarization state, typically exhibiting weak linear biref…
We show how to apply tiling and pattern theory in the design of hollow-core photonic crystal fibers and guide light in multiple bandgaps. By combining two different glass apexes in a single [$3^6$;$3^2$.$4.3.4$] 2-uniform tiling, transmission regions with fundamental, second and third harmonic wavelengths are supported. This cladding design may also be an excellent candidate for high power beam delivery of Er/Yb, Nd:YAG and Ti:Sapphire laser sources.
In 1964 Bloembergen and Shen predicted that Raman gain could be suppressed if the rates of phonon creation and annihilation (by inelastic scattering) exactly balance. This is only possible if the momentum required for each process is identical, i.e., phonon coherence waves created by pump-to-Stokes scattering are identical to those annihilated in pump-to-anti-Stokes scattering. In bulk gas cells, this can only be achieved over limited interaction lengths at an oblique angle to the pump axis. Here we report a simple system that provides dramatic Raman gain suppression over long collinear path-l…
Gas-filled hollow-core photonic crystal fiber (PCF) is used for efficient nonlinear temporal compression of femtosecond laser pulses, two main schemes being direct soliton-effect self-compression, and spectral broadening followed by phase compensation. To obtain stable compressed pulses, it is crucial to avoid decoherence through modulational instability (MI) during spectral broadening. Here we show that changes in dispersion due to spectral anti-crossings between the fundamental core mode and core wall resonances in anti-resonant-guiding hollow-core PCF can strongly alter the MI gain spectrum…
In this paper we consider mid-infrared Raman lasers based on gas-filled hollow-core silica fibers and provide theoretical and experimental analysis of factors that limit the efficiency and output power of these lasers. As a result, we realized an efficient ns-pulsed 4.42 μm Raman laser based on an 1H2-filled revolver silica fiber. Quantum efficiency as high as 36 % is achieved, and output average power as high as 250 mW is demonstrated. The possibilities of further improving the laser efficiency are discussed.
We present two novel hybrid photonic structures made of silica that possess two well-separated frequency bandgaps. The addition of interstitial air holes in a precise location and size allows these bandgaps to open up with a ratio of ${\sim3}$ between their central frequencies at the air line ${ck_z/w=1}$, thus fulfilling the basic guidance condition for third harmonic generation in hollow-core fibers. In addition, these designs may serve as high-power laser delivery of two well-separated wavelengths, such as visible and near infrared.
We build ring resonators to assess the potentialities of Kagome Hollow-Core Photonic Crystal Fibers for future applications to resonant rotation sensing. The large mode diameter of Kagome fibers permits to reduce the free space fiber-to-fiber coupling losses, leading to cavities with finesses of about 30 for a diameter equal to 15 cm. Resonance linewidths of 3.2~MHz with contrasts as large as 89\% are obtained. Comparison with 7-cell photonic band gap (PBG) fiber leads to better finesse and contrast with Kagome fiber. Resonators based on such fibers are compatible with the angular random walk …
In this paper we consider an interaction between the air core modes of hollow core waveguide microstructures and core cladding boundary walls in various shapes. The analysis is based on well established models such as the anti-resonant reflecting optical waveguide model and on the models proposed for the first time. In particular, we consider the dynamics of light localization in the polygonalcore cladding boundary wall as dependant on the type of its discrete rotational symmetry. Based on our findings we analyze the mechanisms of light localization in the core cladding boundary walls of negat…
We report on the generation of 6.1 mJ, 3.8 fs pulses by the compression of a kHz Ti:sapphire laser in a large-aperture long hollow fiber. In order to find optimal conditions for spectral broadening at high pulse energies, we explore different parameter ranges where ionization or the Kerr effect dominates. After identifying the optimum parameter settings, large spectral broadening at high waveguide transmission is obtained. The intense 1.5-cycle pulses are used for high-harmonic generation in argon and neon.
Carrier envelope phase stable 4 fs near-IR pulses with 3 mJ energy were generated by spectral broadening of circularly polarized 8 mJ pulses in a differentially pumped 2 m long composite stretched exible hollow ber. The pulses were characterized using both second-harmonic generation frequency-resolved optical gating (SHG-FROG) and SHG d-scan methods
Soliton self-compression is demonstrated during the propagation of high spatial modes in hollow core fibers in the near-infrared spectral region, taking advantage of their negative dispersion response. We have found that there is always an optimum spatial mode to observe this phenomenon, compressing the pulses down to the single-cycle regime without needing any external compression device and with a consequent increase in the output peak power. Our result is relevant for any ultrashort laser application in which few- or single-cycle pulses are crucial.
We theoretically study chirped four-wave mixing for VUV pulse generation in hollow-core photonic crystal fibers. We predict the generation of sub-10-fs VUV pulses with energy of up to hundreds of microjoule by broad-band chirped idler pulses at 830 nm and MW pump pulses with narrow-band at 277 nm. MW pump could be desirable to reduce the complexity of the laser system or use a high repetition rate-laser system. The energy conversion efficiency from pump pulse to VUV pulse reaches to 30%. This generation can be realized in kagome-lattice hollow-core PCF filled with noble gas of high pressure wi…
Simple structures are always a pursuit but sometimes not easily attainable. It took researchers nearly two decades for conceiving the structure of single-ring hollow-core negative curvature fiber (NCF). Recently NCF eventually approaches to the centre of intense study in fiber optics. The reason behind this slow-pace development is, undoubtfully, its inexplicit guidance mechanism. This paper aims at gaining a clear physical insight into the optical guidance mechanism in NCF. To clarify the origins of light confinement, we boldly disassemble the NCF structure into several layers and develop a m…
Emission at 4.6 um was observed from an N2O filled hollow core fiber laser. 8-ns pump pulses at 1.517 um excited a vibrational overtone resulting in lasing on an R and P branch fundamental transition from the upper pump state. At optimum gas pressure of 80 Torr a photon conversion efficiency of 9% and a slope efficiency of 3% was observed from a mirrorless laser. The laser threshold occurred at an absorbed pump energy of 150 nJ in a 45-cm long fiber with 85 μm core diameter. The observed dependence of the laser output on gas pressure is shown to be a result of line broadening and relaxation ra…
In this work, we numerically investigate an experimentally feasible design of a tapered Ne-filled hollow-core anti-resonant fiber and we report the generation of multiple dispersive waves (DWs) in the range 90-120 nm, well into the extreme ultraviolet (UV) region. The simulations assume an 800 nm pump pulse with 30 fs 10 $μ$J pulse energy, launched into a 9 bar Ne-filled fiber with $34~μ$m initial core diameter that is then tapered to a $10~μ$m core diameter. The simulations were performed using a new model that provides a realistic description of both loss and dispersion of the resonant and a…
Understanding bend-loss in single-ring hollow-core photonic crystal fibers is becoming of increasing importance as the fibers enter practical applications. While purely numerical approaches are useful, there is a need for a simpler analytical formalism that provides physical insight and can be directly used in the design of PCFs with low bend-loss. We show theoretically and experimentally that a wavelength-dependent critical bend radius exists below which the bend-loss reaches a maximum, and that this can be calculated from the structural parameters of a fiber using a simple analytical formula…
The generation of THz radiation from ionizing two-color femtosecond pulses propagating in metallic hollow waveguides filled with Ar is numerically studied. We observe a strong reshaping of the low-frequency part of the spectrum. Namely, after several millimeters of propagation the spectrum is extended from hundreds of GHz up to ~150 THz. For longer propagation distances, nearly single-cycle near-infrared pulses with wavelengths around 4.5 um are obtained by appropriate spectral filtering, with an efficiency of up to 0.25%.
While optical fibers display excellent performances in the infrared, visible and ultraviolet ranges remain poorly addressed by them. Obtaining better fibers for the short-wavelength range has been restricted, in all fiber optics, by scattering processes. In hollow-core fibers, the scattering loss arises from the core roughness and represents the limiting factor in reducing their loss regardless of the fiber cladding confinement power. To attain fibers performing at short wavelengths, it is paramount developing means to minimize the height variations on the fiber microstructure boundaries. Here…
