Compression of CEP-stable multi-mJ laser pulses down to 4 fs in long hollow fibers
Frederik Bohle, Martin Kretschmar, Aurelie Jullien, Mate Kovacs, Miguel Miranda, Rosa Romero, Helder Crespo, Uwe Morgner, Peter Simon, Rodrigo Lopez-Martens, Tamas Nagy
Carrier envelope phase stable 4 fs near-IR pulses with 3 mJ energy were generated by spectral broadening of circularly polarized 8 mJ pulses in a differentially pumped 2 m long composite stretched exible hollow ber. The pulses were characterized using both second-harmonic generation frequency-resolved optical gating (SHG-FROG) and SHG d-scan methods
A carrier envelope phase stable near-single cycle mid-infrared laser based on optical parametric chirped pulse amplification and hollow-core-fiber compression is demonstrated. 4 μm laser pulses with 11.8 mJ energy are delivered from a KTA based OPCPA with 100 Hz repetition rate, and compressed to be ~105 fs by a two-grating compressor with efficiency over 50%. Subsequently, the pulse spectrum is broadened by employing a krypton gas-filled hollow-core-fiber (HCF). Then, the pulse duration is further compressed to 21.5 fs through a CaF2 bulk material with energy of 2.6 mJ and stability of 0.9% R…
The ultimate limit on fiber loss is set by the intrinsic Rayleigh scattering of silica glass material. Here, we challenge this limit in the visible region by using a hollow-core fiber approach. Two visible-guiding hollow-core conjoined-tube negative-curvature fibers are successfully fabricated and exhibit the overall losses of 3.8 dB/km at 680 nm and 4.9 dB/km at 558 nm respectively. The loss of the latter fiber surpasses the Rayleigh scattering limit of silica glass fiber in the green spectral region by 2 dB. Numerical simulation indicates that this loss level is still much higher than the fu…
We report a high performance nodeless hollow-core anti-resonant fiber with a broadband guidance from 1050 nm to >1900 nm, a transmission attenuation of 200 dB/km, and a low bending loss of 0.25 dB/m for a 5 cm radius at wavelength of 1550 nm.
Hollow core fibers are considered as promising candidates to deliver intense temporally overlapping picosecond pulses in applications such as stimulated Raman scattering (SRS) microscopy and endoscopy because of their inherent low nonlinearity compared to solid-core silica fibers. Here we demonstrate that, contrary to prior assumptions, parasitic signals are generated in Kagomé lattice hollow core fibers. We identify the origin of the parasitic signals as an interplay between the Kerr nonlinearity of air and frequency-dependent fiber losses. Importantly, we identify the special cases of experi…
We demonstrate a new class of hollow-core Bragg fibers that are composed of concentric cylindrical silica rings separated by nanoscale support bridges. We theoretically predict and experimentally observe hollow-core confinement over an octave frequency range. The bandwidth of bandgap guiding in this new class of Bragg fibers exceeds that of other hollow-core fibers reported in the literature. With only three rings of silica cladding layers, these Bragg fibers achieve propagation loss of the order of 1 dB/m.
We investigated the carrier-envelope phase (CEP) stability of a hollow-fiber setup used for high-energy, few-cycle pulse generation. Saturation of the output pulse energy is observed at 0.6 mJ for a 260 um inner-diameter, 1 m long fiber, statically filled with neon, with the pressure adjusted to achieve an output spectrum capable of supporting sub-4fs pulses. The maximum output pulse energy can be increased to 0.8mJ by using either differential pumping, or circularly polarized input pulses. We observe the onset of an ionization-induced CEP instability, which does not increase beyond an input p…
Hollow core antiresonant fibers offer new possibilities in the near infrared and visible spectral range. I show here that the great flexibility of this technology can allow the design and fabrication of hollow core optical fibers with an extended transmission bandwidth in the near infrared and with very low optical attenuation in the visible wavelength regime. A very low attenuation of 175dB/km at 480nm is reported. A modification of the design of the studied fibers is proposed in order to achieve fast-responding gas detection.
We analyze the impact of geometrical parameters on such important optical characteristics of negative curvature hollow-core fibers (NCHCFs) as waveguide dispersion, waveguide losses and the structure of transmission bands. We consider both theoretically and experimentally the resonance effects and formation of band edges under bending in NCHCFs.
Hollow-core negative curvature fibers can confine light within air core and have small nonlinearity and dispersion and high damage threshold, thereby attracting a great deal of interest in the field of hollow core fibers. However, reducing the loss of hollow-core negative curvature fibers is a serious problem. On this basis, three new types of fibers with different nested tube structures are proposed in the near-infrared spectral regions and compared in detail with a previously proposed hollow-core negative curvature fiber. We used finite-element method for numerical simulation studies of thei…
Flying particle sensors in hollow-core photonic crystal fibers require accurate localization of the optically trapped microparticles. We report position measurement to micrometer-resolution, using optical frequency domain reflectometry, of two 1.65-$μ$m-diameter polystyrene particles.
We investigate various methods for extending the simple analytical capillary model to describe the dispersion and loss of anti-resonant hollow-core fibers without the need of detailed finite-element simulations across the desired wavelength range. This poor-man's model can with a single fitting parameter quite accurately mimic dispersion and loss resonances and anti-resonances from full finite-element simulations. Due to the analytical basis of the model it is easy to explore variations in core size and cladding wall thickness, and should therefore provide a valuable tool for numerical simulat…
In this paper we present a theoretical and numerical analysis of light localization in hollow core microstructured fibers (HCMFs) with a complicated shape of the core cladding boundary. The analysis is based on well established models (for example, the ARROW model) and also on the models proposed for the first time. In particular, we consider local and nonlocal mechanisms of light localization in the waveguide structures with a determined type of discrete rotational symmetry of the core cladding boundary. We interpret and analyze mechanisms of light localization in negative curvature hollow co…
We present empirical formulae that can provide dispersion and average effective area of the fundamental mode in hollow-core antiresonant fibers. The formulae draw on the structural parameters of the fiber, and allow one to obtain the guiding properties over a wide spectral bandwidth, without the need for time consuming numerical simulations. The formulae are validated by comparing their results with those obtained using a finite-element method. We also analyze the effects of changing the number of antiresonant tubes, as well as adding nested elements in the antiresonant tubes on the guiding pr…
We report on hollow-core fibers displaying rms core roughness under the surface capillary waves thermodynamic limit and record loss in the short-wavelength range (50.0 dB/km at 290 nm, 9.7 dB/km at 369 nm, 5.0 dB/km at 480 nm, 0.9 dB/km at 558 nm, 1.8 dB/km at 719 nm).
We found the self-similar solitary solutions of a recently proposed model for propagation of pulses in gas filled hollow-core photonic crystal fibers that includes a plasma induced nonlinearity. As anticipated for a simpler model and using a perturbation analysis, there are indeed stationary solitary waves that accelerate and self-shift to higher frequencies. However, if the plasma nonlinearity strength is large or the pulse amplitudes are small, the solutions have distinguished long tails and decay as they propagate.
We show how to apply tiling and pattern theory in the design of hollow-core photonic crystal fibers and guide light in multiple bandgaps. By combining two different glass apexes in a single [$3^6$;$3^2$.$4.3.4$] 2-uniform tiling, transmission regions with fundamental, second and third harmonic wavelengths are supported. This cladding design may also be an excellent candidate for high power beam delivery of Er/Yb, Nd:YAG and Ti:Sapphire laser sources.
We experimentally and theoretically study self-phase modulation by Kerr effect in a liquid filled hollow core photonic crystal fiber. We perform a complete characterization of the linear optical properties of the hollow core photonic band gap fiber filled with deuterated acetone to determine all the characteristics of the propagation mode. The nonlinear coefficient of the fiber is determined by fitting the output spectra broadened by self-phase modulation with a new analytical expression giving the spectra of a secant hyperbolic pulse transmitted through a Kerr media. The experiment allows a p…
Gas-filled hollow-core photonic crystal fiber (PCF) is used for efficient nonlinear temporal compression of femtosecond laser pulses, two main schemes being direct soliton-effect self-compression, and spectral broadening followed by phase compensation. To obtain stable compressed pulses, it is crucial to avoid decoherence through modulational instability (MI) during spectral broadening. Here we show that changes in dispersion due to spectral anti-crossings between the fundamental core mode and core wall resonances in anti-resonant-guiding hollow-core PCF can strongly alter the MI gain spectrum…
We study coherent anti-Stokes Raman spectroscopy in air-filled anti-resonance hollow-core photonic crystal fiber, otherwise known as 'revolver' fiber. We compare the vibrational coherent anti-Stokes Raman signal of N$_2$, at 2331 cm$^{-1}$, generated in ambient air (no fiber present), with the one generated in a 2.96 cm of a revolver fiber. We show a 170 times enhancement for the signal produced in the fiber, due to an increased interaction path. Remarkably, the N$_2$ signal obtained in the revolver fiber shows near-zero non-resonant background, due to near-zero overlap between the laser field…
In this paper we consider mid-infrared Raman lasers based on gas-filled hollow-core silica fibers and provide theoretical and experimental analysis of factors that limit the efficiency and output power of these lasers. As a result, we realized an efficient ns-pulsed 4.42 μm Raman laser based on an 1H2-filled revolver silica fiber. Quantum efficiency as high as 36 % is achieved, and output average power as high as 250 mW is demonstrated. The possibilities of further improving the laser efficiency are discussed.
We present two novel hybrid photonic structures made of silica that possess two well-separated frequency bandgaps. The addition of interstitial air holes in a precise location and size allows these bandgaps to open up with a ratio of ${\sim3}$ between their central frequencies at the air line ${ck_z/w=1}$, thus fulfilling the basic guidance condition for third harmonic generation in hollow-core fibers. In addition, these designs may serve as high-power laser delivery of two well-separated wavelengths, such as visible and near infrared.
We build ring resonators to assess the potentialities of Kagome Hollow-Core Photonic Crystal Fibers for future applications to resonant rotation sensing. The large mode diameter of Kagome fibers permits to reduce the free space fiber-to-fiber coupling losses, leading to cavities with finesses of about 30 for a diameter equal to 15 cm. Resonance linewidths of 3.2~MHz with contrasts as large as 89\% are obtained. Comparison with 7-cell photonic band gap (PBG) fiber leads to better finesse and contrast with Kagome fiber. Resonators based on such fibers are compatible with the angular random walk …
In this paper we consider an interaction between the air core modes of hollow core waveguide microstructures and core cladding boundary walls in various shapes. The analysis is based on well established models such as the anti-resonant reflecting optical waveguide model and on the models proposed for the first time. In particular, we consider the dynamics of light localization in the polygonalcore cladding boundary wall as dependant on the type of its discrete rotational symmetry. Based on our findings we analyze the mechanisms of light localization in the core cladding boundary walls of negat…
We report on the generation of 6.1 mJ, 3.8 fs pulses by the compression of a kHz Ti:sapphire laser in a large-aperture long hollow fiber. In order to find optimal conditions for spectral broadening at high pulse energies, we explore different parameter ranges where ionization or the Kerr effect dominates. After identifying the optimum parameter settings, large spectral broadening at high waveguide transmission is obtained. The intense 1.5-cycle pulses are used for high-harmonic generation in argon and neon.
We study theoretically the propagation of relatively long pulses with ionizing intensities in a hollow-core photonic crystal fiber filled with a Raman-inactive gas. Due to photoionization, previously unknown types of asymmetric self-phase modulation and `universal' modulational instabilities existing in both normal and anomalous dispersion regions appear. We also show that it is possible to spontaneously generate a plasma-induced continuum of blueshifting solitons, opening up new possibilities for pushing supercontinuum generation towards shorter and shorter wavelengths.
Frequency blueshifting was recently observed in light pulses propagating on gas filled hollow-core photonic crystal fibers where a plasma has been produced due to photoionization of the gas. One of the propagation models that is adequate to describe the actual experimental observations is here investigated. It is a nonlinear Schrödinger equation with an extra term, to which we applied a self-similar change of variables and found its accelerating solitons. As in other NLS related models possessing accelerating solitons, there exist asymmetrical pulses that decay as they propagate in some parame…
Soliton self-compression is demonstrated during the propagation of high spatial modes in hollow core fibers in the near-infrared spectral region, taking advantage of their negative dispersion response. We have found that there is always an optimum spatial mode to observe this phenomenon, compressing the pulses down to the single-cycle regime without needing any external compression device and with a consequent increase in the output peak power. Our result is relevant for any ultrashort laser application in which few- or single-cycle pulses are crucial.
We demonstrate a route to supercontinuum generation in gas-filled hollow-core anti-resonant fibers through the creation of a broad vibrational Raman frequency comb followed by continuous broadening and merging of the comb lines through either rotational Raman scattering or the optical Kerr effect. Our demonstration experiments, utilizing a single pump pulse with 20 ps duration at 532 nm in a nitrogen-filled fiber, produce a supercontinuum spanning from 440 nm to 1200 nm, with an additional deep ultraviolet continuum from 250 nm to 360 nm. Numerical results suggest that this approach can produc…
We theoretically study chirped four-wave mixing for VUV pulse generation in hollow-core photonic crystal fibers. We predict the generation of sub-10-fs VUV pulses with energy of up to hundreds of microjoule by broad-band chirped idler pulses at 830 nm and MW pump pulses with narrow-band at 277 nm. MW pump could be desirable to reduce the complexity of the laser system or use a high repetition rate-laser system. The energy conversion efficiency from pump pulse to VUV pulse reaches to 30%. This generation can be realized in kagome-lattice hollow-core PCF filled with noble gas of high pressure wi…
Simple structures are always a pursuit but sometimes not easily attainable. It took researchers nearly two decades for conceiving the structure of single-ring hollow-core negative curvature fiber (NCF). Recently NCF eventually approaches to the centre of intense study in fiber optics. The reason behind this slow-pace development is, undoubtfully, its inexplicit guidance mechanism. This paper aims at gaining a clear physical insight into the optical guidance mechanism in NCF. To clarify the origins of light confinement, we boldly disassemble the NCF structure into several layers and develop a m…
We report a study of soliton self-frequency shifting in hydrogen-filled hollow-core fiber. The combination of hydrogen and short 40-fs input pulses underlies clean and efficient generation of Raman solitons between 1080 and 1600 nm. With 240-nJ input pulses, the Raman soliton energy ranges from 110 to 20 nJ over that wavelength range, and the pulse duration is approximately 45 fs. In particular, 70-nJ and 42-fs pulses are generated at 1300 nm. Numerical simulations agree reasonably well with experiments and predict that microjoule-energy tunable pulses should be possible with higher-energy inp…
In this letter, an energetic and highly efficient dispersive wave (DW) generation at 200 nm has been numerically demonstrated by selectively exciting LP$_{02}$-like mode in a 10 bar Ar-filled hollow-core anti-resonant fiber pumping in the anomalous dispersion regime at 1030 nm with pulses of 30 fs duration and 7 $μ$J energy. Our calculations indicate high conversion efficiency of $>$35\% (2.5 $μ$J) after propagating 3.6 cm fiber length which is due to the strong shock effect and plasma induced blue-shifted soliton. It is observed that the efficiency of fundamental LP$_{01}$-mode is about 15\% …
Emission at 4.6 um was observed from an N2O filled hollow core fiber laser. 8-ns pump pulses at 1.517 um excited a vibrational overtone resulting in lasing on an R and P branch fundamental transition from the upper pump state. At optimum gas pressure of 80 Torr a photon conversion efficiency of 9% and a slope efficiency of 3% was observed from a mirrorless laser. The laser threshold occurred at an absorbed pump energy of 150 nJ in a 45-cm long fiber with 85 μm core diameter. The observed dependence of the laser output on gas pressure is shown to be a result of line broadening and relaxation ra…
Understanding bend-loss in single-ring hollow-core photonic crystal fibers is becoming of increasing importance as the fibers enter practical applications. While purely numerical approaches are useful, there is a need for a simpler analytical formalism that provides physical insight and can be directly used in the design of PCFs with low bend-loss. We show theoretically and experimentally that a wavelength-dependent critical bend radius exists below which the bend-loss reaches a maximum, and that this can be calculated from the structural parameters of a fiber using a simple analytical formula…
While optical fibers display excellent performances in the infrared, visible and ultraviolet ranges remain poorly addressed by them. Obtaining better fibers for the short-wavelength range has been restricted, in all fiber optics, by scattering processes. In hollow-core fibers, the scattering loss arises from the core roughness and represents the limiting factor in reducing their loss regardless of the fiber cladding confinement power. To attain fibers performing at short wavelengths, it is paramount developing means to minimize the height variations on the fiber microstructure boundaries. Here…
We demonstrate efficient generation of coherent super-octave pulses via a single-stage spectral broadening of a Yb:KGW laser in a single, pressurized, Ne-filled, hollow-core fiber capillary. Emerging pulses spectrally spanning over more than $\sim$1 PHz (250 nm- 1600 nm) at a dynamic range of $\sim$60 dB, and an excellent beam quality open the door to combining Yb:KGW lasers with modern light field synthesis techniques. Compression of a fraction of the generated supercontinuum to intense (8 fs, $\sim$2.4 cycle, $\sim$650 $μ$J) pulses allows convenient use of these novel laser sources in strong…
We propose supercritical xenon in a hollow-core photonic bandgap fiber as a highly nonlinear medium, and demonstrate 200 nm control over the guidance window of the fiber as the xenon goes through its supercritical phase transition. The large optical polarizability and monoatomic nature of xenon are predicted to allow large optical nonlinearity, on the same order as that of fused silica, while maintaining greatly reduced Raman scattering, offering benefits for nonlinear and quantum optics.
We demonstrate an efficient scheme for the generation of broadband, high-energy, circularly polarized femtosecond laser pulses in the deep ultraviolet through seeded degenerate four-wave mixing in stretched gas-filled hollow capillary fibers. Pumping and seeding with circularly polarized 35 fs pulses centered at 400 nm and 800 nm, respectively, we generate idler pulses centered at 266 nm with more than 25 microjoule of energy and over 95% spectrally averaged ellipticity. Even higher idler energies and broad spectra (27 nm bandwidth) can be obtained at the cost of reduced ellipticity. Our syste…
Based on the interplay between photoionization and Raman effect in gas-filled photonic crystal fibers, we propose a new optical device to control frequency-conversion of ultrashort pulses. By tuning the input-pulse energy, the output spectrum can be either down-converted, up-converted, or even frequency-shift compensated. For low input energies, Raman effect is dominant and leads to a redshift that increases linearly during propagation. For larger pulse energies, photoionization starts to take over the frequency conversion process, and induces a strong blueshift. We have found also that the fi…
We demonstrate sensitive high-resolution stimulated Raman measurements of hydrogen using a hollow-core photonic crystal fiber (HC-PCF). The Raman transition is pumped by a narrow linewidth (<50 kHz) 1064 nm continuous-wave (CW) fiber laser. The probe light is produced by a homebuilt CW optical parametric oscillator (OPO), tunable from around 800 nm to 1300 nm (linewidth ~ 5 MHz). These narrow linewidth lasers allow for an excellent spectral resolution of approximately 10^-4 cm^(-1). The setup employs a differential measurement technique for noise rejection in the probe beam, which also elimina…
Infrared (IR) light is considered important for short-range wireless communication, thermal sensing, spectroscopy, material processing, medical surgery, astronomy etc. However, IR light is in general much harder to transport than optical light or microwave radiation. Existing hollow-core IR waveguides usually use a layer of metallic coating on the inner wall of the waveguide. Such a metallic layer, though reflective, still absorbs guided light significantly due to its finite Ohmic loss, especially for transverse-magnetic (TM) light. In this paper, we show that metal-wire based metamaterials ma…
Research achievements in hollow-core photonic crystal fibers technology allow ascertaining such fibers as outstanding platforms for delivering high-power laser beams. Indeed, the key property underlying the success of this family of optical fibers for high-power beam delivery is their capability of efficiently transmitting light through empty space with minimal interaction with the fiber microstructure. In this context, here we widen the framework of hollow-core fiber-based beam delivery applications by demonstrating their utilization as promising platforms for Power-over-Fiber systems. Thus, …
We report trapping and propagation of photonic Dirac mode in a helically twisted hollow core photonic crystal fiber (HC-PCF) where the trapped light in the hollow (air) defect can preserve the orbital angular momentum (OAM). We show that a photonic Dirac point can emerge even in a twisted system for a suitable choice of curvilinear coordinate and the related waveguide defect modes defined in the new basis can preserve the associated OAM during axial translation. The effect of twist rate, defect geometry and crystal dimension on the propagation of OAM carrying trapped Dirac modes is critically …
We report a series of experimental, analytical and numerical studies demonstrating strong circular dichroism in helically twisted hollow-core single-ring photonic crystal fiber (SR-PCF), formed by spinning the preform during fiber drawing. In the SR-PCFs studied, the hollow core is surrounded by a single ring of non-touching capillaries. Coupling between these capillaries results in the formation of helical Bloch modes carrying orbital angular momentum. In the twisted fiber, strong circular birefringence appears in the ring, so that when a core mode with a certain circular polarization state (…
In this letter, we present a high pulse energy Raman laser at 1946 nm wavelength directly pumped with a 1533 nm custom-made fiber laser. The Raman laser is based on the stimulated Raman scattering (SRS) in an 8-meter carbon dioxide (CO2) filled nested anti-resonant hollow-core fiber (ARHCF). The low energy phonon emission combined with the inherent SRS process along the low-loss fiber allows the generation of high pulse energy up to 15.4 μJ at atmospheric CO2 pressure. The Raman laser exhibits good long-term stability and low relative intensity noise (RIN) of less than 4%. We also investigate …
Broadband-tunable sources of circularly-polarized light are crucial in fields such as laser science, biomedicine and spectroscopy. Conventional sources rely on nonlinear wavelength conversion and polarization control using standard optical components, and are limited by the availability of suitably transparent crystals and glasses. Although gas-filled hollow-core photonic crystal fiber provides pressure-tunable dispersion, long well-controlled optical path-lengths, and high Raman conversion efficiency, it is unable to preserve circular polarization state, typically exhibiting weak linear biref…
In this letter, to the best of our knowledge, a new type of hollow-core anti-resonant fiber (HC-ARF) design using hybrid silica/chalcogenide cladding is presented for single-polarization, high-birefringence, and endlessly single-mode operation at 2 $μ$m wavelength. We show that the inclusion of a chalcogenide layer in the cladding allows strong suppression of $x$-polarization, while maintaining low propagation loss and single-mode propagation for $y$-polarization. The optimized HC-ARF design includes a combination of low propagation loss, high-birefringence, and polarization-extinction ratio (…
High-Resolution Coherent DFS Over 20km Ultra-Low-Loss Anti-Resonant Hollow-Core Fiber with Live Traffic
Nokia Bell Labs(诺基亚贝尔实验室);State Key Laboratory of Optical Fiber and Cable Manufacture Technology, Yangtze Optical Fibre and Cable Joint Stock Limited Company (YOFC)(光纤和光缆制造技术国家重点实验室,长飞光纤光缆股份有限公司);Silentsys;Nokia Networks France, Optics division(诺基亚法国网络公司,光学部门)
Optimum suppression of higher order modes in single-ring hollow-core photonic crystal fibers (SR-PCFs) occurs when the capillary-to-core diameter ratio d/D = 0.68. Here we report that, in SR-PCFs with sub-optimal values of d/D, higher-order mode suppression can be recovered by spinning the preform during fiber drawing, thus introducing a continuous helical twist. This geometrically increases the effective axial propagation constant (initially too low) of the LP01-like modes of the capillaries surrounding the core, enabling robust single-mode operation. The effect is explored by means of extens…
A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet (VUV) radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi2Se3 with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promi…