The symmetry and structure of the superconducting gap in the Fe-based superconductors are the central issue for understanding these novel materials. So far the experimental data and theoretical models have been highly controversial. Some experiments favor two or more constant or nearly-constant gaps, others indicate strong anisotropy and yet others suggest gap zeros ("nodes"). Theoretical models also vary, suggesting that the absence or presence of the nodes depends quantitatively on the model parameters. An opinion that has gained substantial currency is that the gap structure, unlike all other known superconductors, including cuprates, may be different in different compounds within the same family. A unique method for addressing this issue, one of the very few methods that are bulk and angle-resolved, calls for measuring the electronic specific heat in a rotating magnetic field, as a function of field orientation with respect to the crystallographic axes. In this Communication we present the first such measurement for an Fe-based high-Tc superconductor (FeBSC). We observed a fourfold oscillation of the specific heat as a function of the in-plane magnetic field direction, which allowed us to identify the locations of the gap minima (or nodes) on the Fermi surface. Our results are consistent with the expectations of an extended s-wave model with a significant gap anisotropy on the electron pockets and the gap minima along the ΓM (or Fe-Fe bond) direction.
Angle-Resolved Photoemission Spectroscopy of the Antiferromagnetic Superconductor Nd1.87Ce0.13CuO4: Anisotropic Spin-Correlation Gap, Pseudogap, and the Induced Quasiparticle Mass Enhancement
Relaxation timescales and electron-phonon coupling in optically-pumped YBa$_2$Cu$_3$O$_{6+x}$ revealed by time-resolved Raman scattering
时间分辨测量提供了一种新的方法来解开量子材料中复杂的相互作用,由于它们的不同的时间尺度。利用泵浦-探测喇曼散射研究了非平衡条件下$_2$ O $_{6+x}$中氧的顶面振动。声子布居的时间依赖性表现出强烈的电子-声子耦合。最重要的是,声子转移到一个更高的能量,由于瞬态涂抹的费米表面在一个显着的协议与图解理论。我们还讨论了新的见解光致超导报道在较低的掺杂,遵循这些结果。
Fermi surfaces and orbital polarization in superconducting CeO$_{0.5}$F$_{0.5}$BiS$_{2}$ revealed by angle-resolved photoemission spectroscopy
利用偏振相关角分辨光电子能谱(ARPES)研究了BiSPDMATHABMM基CeO $_{0.5}$ F $_{0.5}$ BiS $_2$超导体的电子结构,并成功地阐明了费米面上的轨道特征.在X点周围的矩形费米口袋中,平行于$k_y$方向的直线部分由Bi $6p_x$特征主导。轨道极化表明BiS $_2$系统的准一维电子结构。此外,四边形排列的Bi上的扭曲可以引起带Jahn-Teller效应。
Anisotropic dressing of charge-carriers in the electron-doped cuprate superconductor Sm(1.85)Ce(0.15)CuO(4) from angle-resolved photoemission measurements
Theoretical study on the anisotropic electronic structure of antiferromagnetic BaFe$_2$As$_2$ and Co-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ seen by angle-resolved photoemission
用一步模型计算方法研究了铁磷属元素化物原型化合物BaFe $_2$ As $_2$和Ba(Fe $_{1-x}$ Co $_x$)$_2$ As $_2$在低温反铁磁相中的角分辨光电发射中所表现出的强面内各向异性.完全相对论计算是基于Korringa-Kohn-Rostoker-Green函数方法结合相干势近似合金理论,以一种可靠的方式来解释Co取代Fe位引起的无序。计算的结果可以直接与实验光谱的解孪晶单晶。人们发现非常好的协议与实验,可以揭示所有的电子结构的功能,有助于在平面各向异性。特别是局域密度近似可以捕捉到大多数的相关效应的调查系统,而不需要更先进的技术。此外,可以几乎连续地跟踪Ba(Fe $x$ Co $_x$)$_2$ As $_2$中随Co浓度增加的各向异性的演变。结果也被用来讨论表面效应,它是可能的,以确定明确的签名,以得出不同类型的表面终止。
Nematicity in the pseudogap state of cuprate superconductors revealed by angle-resolved photoemission spectroscopy
赝能隙的性质及其与超导电性的关系是铜氧化物超导体的核心问题之一。最近,一种可能的情况已经提出,赝能隙状态是一个独特的阶段,其特征在于自发的旋转对称性破缺称为“向列性”的基础上的运输和磁化率测量,其中的对称性破缺被观察到低于赝能隙温度$T^*$。在这里,我们报告了一个温度依赖的ARPES研究的向列性在轻微过掺杂的Bi ${}_{1.7}$ Pb ${}_{0.5}$ Sr ${}_{1.9}$ CaCu ${}_2$ O ${}_{8+δ}$沿Cu-O键方向施加的单轴应变触发。虽然向列性增强的赝隙状态,在以前的研究中,它被抑制在超导状态。这些结果表明赝能隙态具有自发旋转对称破缺的特征,向列性可能与超导性竞争。这些新的实验发现可能为赝能隙的性质及其与超导电性的关系提供线索。
Two component dynamics of the superconducting order parameter revealed by time-resolved Raman scattering
利用时间分辨抽运-探测喇曼实验研究了高$T_c$铜氧化物Bi $_2$ Sr $_2$ CaCu $_2$ O $_{8-δ}$的超导序参量动力学.我们发现两种不同的耦合机制,同样有助于对破峰。一个耦合在2 ps时非常快地开始并且缓慢地松弛,而另一个耦合被延迟并且大约在5 ps时开始并且快速地松弛。通过声子耦合空穴的模型能够再现凝聚动力学的一部分,因此,我们认为空穴-自旋相互作用也是重要的。
Nematic fluctuations mediated superconductivity revealed by anisotropic strain in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$
各向异性应变是一种能够选择性地解决超导涨落在促进超导性中的作用的外部场。我们证明了这一点,使用偏振分辨的弹性拉曼散射探测下的正常和超导状态的典型的铁基超导体Ba(Fe $_{1-x}$ Co $_x$)$_2$ As $_2$的应变下的电子涨落的演变。在非超导的母体化合物BaFe $_2$ As $_2$中,我们观察到了应变引起的超导磁化率的抑制,它遵循了对称破缺场下伊辛序参量的预期行为。对于超导化合物,超导磁化率的抑制与超导临界温度$T_c$的降低有关。我们的研究结果表明,一个显着的贡献,电子配对和增强$T_c$附近的一个量子临界点的理论方案验证的涨落。
Unusual Fermi surface nesting in parent compounds of iron arsenic high temperature superconductors revealed by Angle Resolved Photoemission Spectroscopy
Disappearance of Superconductivity and a Concomitant Lifshitz Transition in Heavily-Overdoped Bi2Sr2CuO6 Superconductor Revealed by Angle-Resolved Photoemission Spectroscopy
Signatures of superconductivity and pseudogap formation in non-equilibrium nodal quasiparticles revealed by ultrafast angle-resolved photoemission
我们用时间分辨和角分辨光电子能谱测量了$_2$ $_2$ O $_2$的各种掺杂的节非平衡电子态。我们发现,这些ungapped状态的初始泵浦诱导的瞬态信号的强烈影响的超导能隙在$T_c$,超导配对波动在$T_p$,和赝能隙在$T^*$的发病。此外,$T_p$标记了通量依赖性瞬态信号中的一个提示性阈值,出现了低于$T_p$的临界通量,该临界通量对应于使所有库珀对断裂所需的能量。这些结果挑战了铜氧化物超导体中结-反结二分法的概念,在结准粒子和铜氧化物相图之间建立了一个新的联系。
Inhomogeneous reduction-annealing effects on the electron-doped cuprate superconductor revealed by micro-focused angle-resolved photoemission spectroscopy
Anomalous contribution to the nematic electronic states from the structural transition in FeSe revealed by time- and angle-resolved photoemission spectroscopy
Electronic Structure and Superconducting Gap of HgBa$_2$Ca$_2$Cu$_3$O$_{8+δ}$ Revealed by Laser-Based Angle-Resolved Photoemission Spectroscopy
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所凝聚态物理国家实验室);University of Chinese Academy of Sciences(中国科学院大学);Technical Institute of Physics and Chemistry, Chinese Academy of Sciences(中国科学院化学物理研究所);Songshan Lake Materials Laboratory(松山湖材料实验室)
Hidden itinerant-spin phase in heavily-overdoped La2-xSrxCuO4 revealed by dilute Fe doping: A combined neutron scattering and angle-resolved photoemission study
Coexistence of Two Sharp-Mode Couplings and Their Unusual Momentum Dependence in the Superconducting State of Bi2Sr2CaCu2O8+d Superconductor Revealed by Laser-Based Angle-Resolved Photoemission
Common Fermi Surface Topology and Nodeless Superconducting Gap in K0.68Fe1.79Se2 and (Tl0.45K0.34)Fe1.84Se2 Superconductors Revealed from Angle-Resolved Photoemission Spectroscopy
Orbital-dependent electron correlation effect on the two- and three-dimensional Fermi surfaces in KFe2As2 revealed by angle-resolved photoemission spectroscopy
Detailed Electronic Structure of the Three-Dimensional Fermi Surface and its Sensitivity to Charge Density Wave Transition in ZrTe3 Revealed by High Resolution Laser-Based Angle-Resolved Photoemission Spectroscopy
Explicit Turn Resolution with Anisotropic Homogenisation for Efficient 3D Magneto-Thermal Finite-Element Simulation of Large-Scale No-Insulation HTS Magnets
Doping Evolution of Nodal Electron Dynamics in Trilayer Cuprate Superconductor Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ Revealed by Laser-Based Angle-Resolved Photoemission Spectroscopy