The feasibility of high-fidelity single-qubit operations of a hole spin in a quantum dot molecule by electric g tensor control is demonstrated. Apart from a constant external magnetic field the proposed scheme allows for an exclusively electric control of the hole spin. Realistic electric gate bias profiles are identified for various qubit operations using process-tomography-based optimal control. They are shown to be remarkably robust against decoherence and dissipation arising from the interaction of the hole with host-lattice nuclear spins and phonons, with a fidelity loss of $\approx$ 1 percent for gate operation times of $\approx 10$ ns. Spin-echo experiments for the hole spin are modeled to explore dephasing mechanisms and the role of pulse-timing imperfections on the gate fidelity loss is discussed.
The temperature dependence of the coherence time of hole spins confined in self-assembled (In,Ga)As/GaAs quantum dots is studied by spin mode-locking and spin echo techniques. Coherence times limited to about a μs are measured for temperatures below 8 K. For higher temperatures a fast drop occurs down to a few ns over a 10 K range. The hole-nuclear hyperfine interaction appears too weak to account for these limitations. We suggest that spin-orbit related interactions are the decisive sources for hole spin decoherence.
An ensemble of quantum dot excitons may be used for coherent information manipulation. Due to the ensemble inhomogeneity any optical information retrieval occurs in form of a photon echo. We show that the inhomogeneity can lead to a significant deviation from the conventional echo timing sequence. Variation of the area of the initial rotation pulse, which generates excitons in a dot sub-ensemble only, reveals this complex picture of photon echo formation. We observe a retarded echo for π/2 pulses, while for 3π/2 the echo is advanced in time as evidenced through monitoring the Rabi oscillations…
We report a measurement of the spin-echo decay of a single electron spin confined in a semiconductor quantum dot. When we tip the spin in the transverse plane via a magnetic field burst, it dephases in 37 ns due to the Larmor precession around a random effective field from the nuclear spins in the host material. We reverse this dephasing to a large extent via a spin-echo pulse, and find a spin-echo decay time of about 0.5 microseconds at 70 mT. These results are in the range of theoretical predictions of the electron spin coherence time governed by the dynamics of the electron-nuclear system.
The model considered in the paper is used nowadays to describe spin dynamics of quantum dots after optical excitation. Based on the exact diagonalization of a model Hamiltonian, we solve the problems of the electron spin polarization decay and magnetic field dependence of the steady state polarization. The important role of the nuclear state is shown and methods of its calculation for different regimes of optical excitation are proposed. The effect of spin echo observed after application of the magnetic field $π$-pulse is predicted.
We study the localization of dressed Dirac electrons in a cylindrical quantum dot (QD) formed on monolayer and bilayer graphene by spatially different potential profiles. Short lived excitonic states which are too broad to be resolved in linear spectroscopy are revealed by cross peaks in the photon-echo nonlinear technique. Signatures of the dynamic gap in the two-dimensional spectra are discussed. The effect of the Coulomb induced exciton-exciton scattering and the formation of biexciton molecules are demonstrated.
We develop a theory for the spin-echo dynamics of a heavy hole in a quantum dot, accounting for both hyperfine- and electric-field-induced fluctuations. We show that a moderate applied magnetic field can drive this system to a motional-averaging regime, making the hyperfine interaction ineffective as a decoherence source. Furthermore, we show that decay of the spin-echo envelope is highly sensitive to the geometry. In particular, we find a specific choice of initialization and π-pulse axes which can be used to study intrinsic hyperfine-induced hole-spin dynamics, even in systems with substanti…
Semiconductor quantum dots are excellent candidates for ultrafast coherent manipulation of qubits by laser pulses on picosecond timescales or even faster. In inhomogeneous ensembles a macroscopic optical polarization decays rapidly due to dephasing, which, however, is reversible in photon echoes carrying complete information about the coherent ensemble dynamics. Control of the echo emission time is mandatory for applications. Here, we propose a novel concept to reach this goal. In a two-pulse photon echo sequence, we apply an additional resonant control pulse with multiple of 2pi area. Dependi…
We study Rabi rotations arising in intensity-dependent photon echoes from an ensemble of self-assembled InGaAs quantum dots. To achieve a uniform distribution of intensities within the excited ensemble, we introduce flattop intensity profiles of picosecond laser pulses. This allows us to overcome the damping of Rabi rotations imposed by the spatial inhomogeneity of Rabi frequencies by a Gaussian laser profile. Using photon echo polarimetry, we distinguish between the coherent optical responses from exciton and trion ensembles. Here, we demonstrate that a photo-induced charging of the quantum d…
We report on the coherent optical response from an ensemble of (In,Ga)As quantum dots (QDs) embedded in a planar Tamm-plasmon microcavity with a quality factor of approx. 100. Significant enhancement of the light-matter interaction is demonstrated under selective laser excitation of those quantum dots which are in resonance with the cavity mode. The enhancement is manifested through Rabi oscillations of the photon echo, demonstrating coherent control of excitons with picosecond pulses at intensity levels more than an order of magnitude smaller as compared with bare quantum dots. The decay of t…
We propose a two-qubit optically controlled phase gate in quantum dot molecules via adiabatic passage and hole tunneling. Our proposal combines the merits of the current generation of vertically stacked self-assembled InAs quantum dots and adiabatic passage. The simulation shows an implementation of the gate with a fidelity exceeding 0.98.
We demonstrate the effects of cavity quantum electrodynamics for a quantum dot coupled to a photonic molecule, consisting of a pair of coupled photonic crystal cavities. We show anti-crossing between the quantum dot and the two super-modes of the photonic molecule, signifying achievement of the strong coupling regime. From the anti-crossing data, we estimate the contributions of both mode-coupling and intrinsic detuning to the total detuning between the super-modes. Finally, we also show signatures of off-resonant cavity-cavity interaction in the photonic molecule.
The puzzling behavior of the transition phase through a quantum dot can be understood in a natural way via a formation of the electron molecule in the quantum dot. In this case the resonance tunneling takes place through the quasi-stationary (doorway) state, which emerges when the number of electrons occupying the dot reaches a certain ``critical'' value, $N_{cr}$. Our estimation of this quantity agrees with the experimental data. The dependence of $N_{cr}$ on the dot's size is predicted as well.
We use photoluminescence spectroscopy to investigate the ground state of single self-assembled InGaAs lateral quantum dot molecules. We apply a voltage along the growth direction that allows us to control the total charge occupancy of the quantum dot molecule. Using a combination of computational modeling and experimental analysis, we assign the observed discrete spectral lines to specific charge distributions. We explain the dynamic processes that lead to these charge configurations through electrical injection and optical generation. Our systemic analysis provides evidence of inter-dot tunne…
We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and non-rephasing four-wave mixing (FWM) configurations. We emphasize the non-rephasing case, allowing to monitor two-photon coherence dynamics. Respective Fourier transform yields a double quantum 2D FWM map, which is corroborated with its single quantum counterpart, originating from the rephasing sequence. We introduce referencing of the FWM phase with the one…
A slanting magnetic field is usually used to realize a slight hybridization between the spin and orbital degrees of freedom in a semiconductor quantum dot, such that the spin is manipulable by an external oscillating electric field. Here we show that, the longitudinal slanting field mediates a longitudinal driving term in the electric-dipole spin resonance, such that the spin population inversion exhibits a modulated Rabi oscillation. Fortunately, we can reduce this modulation by increasing the static magnetic field. The longitudinal slanting field also mediates a spin-1/f-charge noise interac…
We discuss the optical response of a quantum molecule under the action of two lasers fields. Using a realistic model and parameters, we map the physical conditions to find three different phenomena reported in the literature: the tunneling induced transparency, the formation of Autler-Townes doublets, and the creation of a Mollow-like triplet. We found that the electron tunneling between quantum dots is the responsible for the different optical regime. Our results not only explain the experimental results in the literature but also give insights for future experiments and applications in optic…
In this work, it is investigated the behavior of the efficiency at maximum power of a quantum dot molecule, acting as a device for photovoltaic conversion. A theoretical approach using a master equation, considering the effect of the energy offsets, and the width of the quantum barrier, identifies realistic physical conditions that enhance the photovoltaic response of the photocell. The results show the potentiality of increasing the gain in 30\% of maximum power delivered per molecule if compared with a single quantum dot. Also, the system exhibits gain when compared to the Chambadal-Novikov …
We investigate theoretically the spin echo signal of an electron localized in a quantum dot and interacting with a bath of nuclear spins. We consider the regime of very low magnetic fields (corresponding to fields as low as a militesla in realistic GaAs and InGaAs dots). We use both the exact numerical simulations and the analytical theory employing the effective pure dephasing Hamiltonian. The comparison shows that the latter approach describes very well the spin echo decay at magnetic fields larger than the typical Overhauser field, and that the timescale at which this theory works is larger…
Pauli spin blockade in quantum dot systems occurs when the charge transport is allowed only for some spin states, and it has been an efficient tool in spin-based qubit devices in semiconductors. We theoretically investigate a Pauli spin blockade in a triple quantum dot molecule consisting of three identical quantum dots in a semiconductor in the presence of an external magnetic field through the molecule. When the three-electron state is on resonance with two- or four-electron states, the Aharonov-Bohm oscillation and the Zeeman splitting lead to a periodic spin blockade effect. We focus on th…
Two main mechanisms dictate the tunneling process in a double quantum dot: overlap of excited wave functions, effectively described as a tunneling rate, and phonon-assisted tunneling. In this paper, we study different regimes of tunneling that arise from the competition between these two mechanisms in a double quantum dot molecule immersed in a unimodal optical cavity. We show how such regimes affect the mean number of excitations in each quantum dot and in the cavity, the spectroscopic resolution and emission peaks of the photoluminescence spectrum, and the second-order coherence function whi…
The spin of an electron in a self-assembled InAs/GaAs quantum dot molecule is optically prepared and measured through the trion triplet states. A longitudinal magnetic field is used to tune two of the trion states into resonance, forming a superposition state through asymmetric spin exchange. As a result, spin-flip Raman transitions can be used for optical spin initialization, while separate trion states enable cycling transitions for non-destructive measurement. With two-laser transmission spectroscopy we demonstrate both operations simultaneously, something not previously accomplished in a s…
We report on a single photon and spin storage device based on a semiconductor quantum dot molecule. Optically excited single electron-hole pairs are trapped within the molecule and their recombination rate is electrically controlled over three orders of magnitude. Single photons are stored up to 1 microsecond and read out on a sub-nanosecond timescale. Using resonant excitation, the circular polarisation of individual photons is transferred into the spin state of electron-hole pairs with a fidelity above 80%, which does not degrade for storage times up to the 12.5ns repetition period of the ex…
The nuclear spin bath (NSB) dynamics and its quantum control are of importance for the storage and processing of quantum information within a semiconductor environment. In the presence of a carrier spin, primarily it is the hyperfine interaction that rules the high frequency NSB characteristics. Here, we first study the overall coherence decay and rephasings in a hyperfine-driven NSB through the temporal and spectral behaviors of the so-called Loschmidt echo (LE). Its dependence on the NSB size, initial polarization, and coupling inhomogeneity are separately investigated, which leads to a simp…
We study phonon-assisted electron tunneling in semiconductor quantum dot molecules. In particular, singlet-singlet relaxation in a two-electron doped structure is considered. The influence of Coulomb interaction is discussed via comparison with a single electron system. We find that the relaxation rate reaches similar values in the two cases but the Coulomb interaction shifts the maximum rates towards larger separations between the dots. The difference in electron-phonon interaction between deformation potential and piezoelectric coupling is investigated. We show that the phonon-induced tunnel…
We investigate the generation of entanglement through a quantum dot molecule under the influence of vibrational phonon modes in a bias voltage junction. The molecular quantum dot system is realized by coupled quantum dots inside a suspended carbon nanotube. We consider the dynamical entanglement as a function of bias voltage and temperature by taking into account the electron-phonon interaction. In order to generate the robust entanglement between quantum dots and preserve it to reach the maximal achievable amount steadily, we introduce an asymmetric coupling protocol and apply the easy tunabl…
We propose an all-optical scheme to perform a non-demolition measurement of a single hole spin localized in a quantum-dot molecule. The latter is embedded in a microcavity and driven by two lasers. This allows to induce Raman transitions which entangle the spin state with the polarization of the emitted photons. We find that the measurement can be completed with high fidelity on a timescale of 100 ps, shorter than the typical T2. Furthermore, we show that the scheme can be used to induce and observe spin oscillations without the need of time-dependent magnetic fields.
Multi-electron semiconductor quantum dots have found wide application in qubits, where they enable readout and enhance polarizability. However, coherent control in such dots has typically been restricted to only the lowest two levels, and such control in the strongly interacting regime has not been realized. Here we report quantum control of eight different resonances in a silicon-based quantum dot. We use qubit readout to perform spectroscopy, revealing a dense set of energy levels with characteristic spacing far smaller than the single-particle energy. By comparing with full configuration in…
The wide set of control parameters and reduced size scale make semiconductor quantum dots attractive candidates to implement solid-state quantum computation. Considering an asymmetric double quantum dot coupled by tunneling, we combine the action of a laser field and the spontaneous emission of the excitonic state to protect an arbitrary superposition state of the indirect exciton and ground state. As a by-product we show how to use the protected state to solve the Deutsch problem.
We demonstrate the extension of coherence between all four two-electron spin ground states of an InAs quantum dot molecule (QDM) via non-local suppression of nuclear spin fluctuations in both constituent quantum dots (QDs), while optically addressing only the upper QD transitions. Long coherence times are revealed through dark-state spectroscopy as resulting from nuclear spin locking mediated by the exchange interaction between the QDs. Lineshape analysis provides the first measurement of the quieting of the Overhauser field distribution correlating with reduced nuclear spin fluctuations.
The spin states of electrons and holes confined in InAs quantum dot molecules have recently come to fore as a promising system for the storage or manipulation of quantum information. We describe here a feasible scheme for complete quantum optical control of two electron spin qubits in two vertically-stacked singly-charged InAs quantum dots coupled by coherent electron tunneling. With an applied magnetic field transverse to the growth direction, we construct a universal set of gates that corresponds to the possible Raman transitions between the spin states. We detail the procedure to decompose …
The effects caused by phonon-assisted tunnelling (PhAT) in a double quantum dot (QD) molecule immersed in a cavity were studied under the quantum Markovian master equation formalism in order to account for dissipation phenomena. We explain how for higher PhAT rates, a stronger interaction between a QD and the cavity at off-resonance takes place through the resonant interaction of another QD and the cavity, where the QDs interact through tunnelling. A closer look at the system's allowed optical transitions as a function of PhAT rates showed coalescence of the transition energies, leading to a l…
Two-electron charged self-assembled quantum dot molecules exhibit a decoherence-avoiding singlet-triplet qubit subspace and an efficient spin-photon interface. We demonstrate quantum entanglement between emitted photons and the spin-qubit after the emission event. We measure the overlap with a fully entangled state to be $69.5\pm2.7\,\%$, exceeding the threshold of $50\,\%$ required to prove the non-separability of the density matrix of the system. The photonic qubit is encoded in two photon states with an energy difference larger than the timing resolution of existing detectors. We devise a n…
Self-assembled optically active quantum dot molecules (QDMs) allow the creation of protected qubits via singlet-triplet spin states. The qubit energy splitting of these states is defined by the tunnel coupling strength and is, therefore, determined by the potential landscape and thus fixed during growth. Applying an in-plane magnetic field increases the confinement of the hybridized wave functions within the quantum dots, leading to a decrease of the tunnel coupling strength. We achieve a tuning of the coupling strength by $(53.4\pm1.7)$ %. The ability to fine-tune this coupling is essential f…
Laterally coupled quantum dot molecules are studied using exact diagonalization techniques. We examine the two-electron singlet-triplet energy difference as a function of magnetic field strength and investigate the magnetization and vortex formation of two- and four-minima lateral quantum dot molecules. Special attention is paid to the analysis of how the distorted symmetry affects the properties of quantum-dot molecules.
Full counting statistics of electron transport is a powerful diagnostic tool for probing the nature of quantum transport beyond what is obtainable from the average current or conductance measurement alone. In particular, the non-Markovian dynamics of quantum dot molecule plays an important role in the nonequilibrium electron tunneling processes. It is thus necessary to understand the non-Markovian full counting statistics in a quantum dot molecule. Here we study the non-Markovian full counting statistics in two typical quantum dot molecules, namely, serially coupled and side-coupled double qua…
We study theoretically the nonlinear four wave mixing (FWM) response of an ensemble of coupled pairs of quantum dots (quantum dot molecules). We discuss the shape of the FWM echo signal depending on the parameters of the ensemble: the statistics of transition energies and the degree of size correlations between the dots forming the molecules.
In this theoretical work, we study a double quantum dot interacting strongly with a microcavity, while undergoing resonant tunneling. Effects of interdot tunneling on the light-matter hybridized states are determined, and tunability of their brightness degrees and associated dipole moments is demonstrated. These results predict dipolariton generation in artificial molecules coupled to optical resonators, and provide a promising scenario for control of emission efficiency and coherence times of exciton polaritons.
We derive a quantum-kinetic description of phonon-assisted F{ö}rster transfer between two coupled quantum dots (a quantum dot molecule). We show that the exciton state decays to the ground state of the QDM via a combination of the Rabi rotation and exponential decay. For moderately spaced dots this process takes place on a picosecond time scale.
In this work, we have investigated conduction through an artificial molecule comprising two coupled quantum dots. The question addressed is the role of inter-dot coupling on electronic transport. We find that the current through the molecule exhibits step-like features as a function of the voltage between the leads, where the step size increases as the inter-dot coupling is increased. These step-like features disappear with increasing tunneling rate from the leads, but we find that in the presence of coupling, this smooth behavior is not observed rather two kinks are seen in the current voltag…
Atomistic electronic structure calculations are performed to study the coherent inter-dot couplings of the electronic states in a single InGaAs quantum dot molecule. The experimentally observed excitonic spectrum [12] is quantitatively reproduced, and the correct energy states are identified based on a previously validated atomistic tight binding model. The extended devices are represented explicitly in space with 15 million atom structures. An excited state spectroscopy technique is presented in which the externally applied electric field is swept to probe the ladder of the electronic energy …
We investigate theoretically the slowdown of optical pulses due to quantum-coherence effects in InGaAs-based quantum dots and quantum dot molecules. Simple models for the electronic structure of quantum dots and, in particular, quantum-dot molecules are described and calibrated using numerical simulations. It is shown how these models can be used to design optimized quantum-dot molecules for quantum coherence applications. The wave functions and energies obtained from the optimizations are used as input for a microscopic calculation of the quantum-dot material dynamics including carrier scatte…
We study two-dimensional quantum dots using the variational quantum Monte Carlo technique in the weak-confinement limit where the system approaches the Wigner molecule, i.e., the classical solution of point charges in an external potential. We observe the spin-polarization of electrons followed by a smooth transition to a Wigner-molecule-like state as the confining potential is made weaker.
We introduce an integrability-based method enabling the study of semiconductor quantum dot models incorporating both the full hyperfine interaction as well as a mean-field treatment of dipole-dipole interactions in the nuclear spin bath. By performing free induction decay and spin echo simulations we characterize the combined effect of both types of interactions on the decoherence of the electron spin, for external fields ranging from low to high values. We show that for spin echo simulations the hyperfine interaction is the dominant source of decoherence at short times for low fields, and com…
We report electron transport measurements of a silicon double dot formed in multi-gated metal-oxide-semiconductor structures with a 15-nm-thick silicon-on-insulator layer. Tunable tunnel coupling enables us to observe an excitation spectrum in weakly coupled dots and an energy level anticrossing in strongly coupled ones. Such a quantum dot molecule with both charge and energy quantization provides the essential prerequisite for future implementation of silicon-based quantum computations.
Motivated by recent experiments on electric transport through single molecules and quantum dots, we investigate a model for transport that allows for significant coupling between the electrons and a boson mode isolated on the molecule or dot. We focus our attention on the temperature dependent properties of the transport. In the Holstein picture for polaronic transport in molecular crystals the temperature dependence of the conductivity exhibits a crossover from coherent (band) to incoherent (hopping) transport. Here, the temperature dependence of the differential conductance on resonance does…
We report on the observation of Kondo and split Kondo peaks in single-molecule transistors containing a single spin transition molecule with a Fe2+ ion. Coulomb blockade characteristics reveal a double quantum dot behavior in a parallel configuration, making our system a molecular equivalent to a semiconducting double-quantum-dot system. As the gate voltage is increased the charging of the second dot by an additional electron induces a splitting of the Kondo peak. We discuss possible origins of this effect including a spin transition into a high-spin state.
We discuss pure dephasing of singlet-triplet superpositions in two-electron double quantum dots due to elastic phonon scattering. We generalize our previous results to a system built of two non-identical dots. We show that the asymmetry must be very strong in order to considerably affect the dephasing rate.
Exciton levels and fine-structure splitting in laterally-coupled quantum dot molecules are studied. The electron and hole tunneling energies as well as the direct Coulomb interaction are essential for the exciton levels. It is found that fine-structure splitting of the two-lowest exciton levels is contributed from the intra- and inter-dot exchange interactions, both of which are largely influenced by the symmetry and tunnel-coupling between the two dots. As the inter-dot separation is reduced, fine-structure splitting of the exciton ground state is largely increased while those of the excited …
The theory of exciton coupling to photons and LO phonons in quantum dots (QDs) and quantum-dot molecules (QDMs) is presented. Resonant-round trips of the exciton between the ground (bright) and excited (dark or bright) states mediated by the LO-phonon alter the decay time and yield the Rabi oscillation. The initial distributions of the population in the ground and the excited states dominate the oscillating amplitude and frequency. This property provides a detectable signature to the information stored in a qubit made from QD or QDM for a wide range of temperature T. Our results presented here…
We demonstrate theoretically that it is possible to use Rabi oscillations to coherently control the electron tunneling in an asymmetric double quantum dot system, a quantum dot molecule. By applying an optical pump pulse we can excite an electron in one of the dots, which can in turn tunnel to the second dot, as controlled by an external voltage. Varying the intensity of the pulse one can suppress or enhance the tunneling between the dots for given level resonance conditions. This approach allows substantial flexibility in the control of the quantum mechanical state of the system.
We theoretically study the effects of bias-controlled interdot tunneling in vertically coupled quantum dots on the emission properties of spin excitons in various bias-controlled tunneling regimes. As a main result, for strongly coupled dots we predict substantial reduction of optical fine structure splitting without any drop in the optical oscillator strength. This special reduction diminishes the distinguibility of polarized decay paths in cascade emission processes suggesting the use of stacked quantum dot molecules as entangled photon-pair sources.
The conductance through a serial double dot structure for which the inter-dot tunneling is stronger than the tunneling to the leads is studied using the numerical density matrix renormalization group method and analytic arguments. When the dots are occupied by 1 or 3 electrons the usual Kondo peak is obtained. For the case in which 2 electrons occupy the molecule a singlet is formed. Nevertheless, the conductance in that case has a constant non-zero value, and might even be equal to the maximum conductance of $2 e^2/h$ for certain values of the molecule parameters. We show that this is the res…
Resonant electron transport through a mesoscopic region (quantum dot or single molecule) with electron-phonon interaction is considered at finite voltage. In this case the standard Landauer-Büttiker approach cannot be applied. Using the nonequilibrium Green function method we show that due to a nonequilibrium distribution function of electrons in the mesoscopic region, the inelastic scattering rate and spectral function of the dot become functions of the voltage and have to be calculated self-consistently.
The exciton lifetimes $T_1$ in arrays of InAs/GaAs vertically coupled quantum dot pairs have been measured by time-resolved photoluminescence. A considerable reduction of $T_1$ by up to a factor of $\sim$ 2 has been observed as compared to a quantum dots reference, reflecting the inter-dot coherence. Increase of the molecular coupling strength leads to a systematic decrease of $T_1$ with decreasing barrier width, as for wide barriers a fraction of structures shows reduced coupling while for narrow barriers all molecules appear to be well coupled. The coherent excitons in the molecules gain the…
The electronic transport through a parallel double quantum-dot molecule attached asymmetrically to leads is studied under a magnetic field. We model the system by means of a non interacting two-impurity Anderson Hamiltonian. We find that the conductance shows Fano and Dicke effects that can be controlled by the magnetic flux.
Transmission and reflection of an electromagnetic pulse through a dielectric slab doped with the quantum dot molecules is investigated. It is shown that the transmitted and reflected pulses depend on the inter-dot tunneling effect and can be controlled by applying a gate voltage.
Electron tunneling through a double quantum dot molecule side attached to a quantum wire, in the Kondo regime, is studied. The mean-field finite-U slave-boson formalism is used to obtain the solution of the problem. We found conductance cancelations when the molecular energies of the side attached double quantum-dot cross the Fermi energy. We investigate the many body molecular Kondo states as a function of the parameters of the system.
We study the influence of the phonon environment on the electron dynamics in a doped quantum dot molecule. A non-perturbative quantum kinetic theory based on correlation expansion is used in order to describe both diagonal and off-diagonal electron-phonon couplings representing real and virtual processes with relevant acoustic phonons. We show that the relaxation is dominated by phonon-assisted electron tunneling between constituent quantum dots and occurs on a picosecond time scale. The dependence of the time evolution of the quantum dot occupation probabilities on the energy mismatch between…
